Search

We characterize the superconducting diode effect (SDE) in two-dimensional diffusive structures with Rashba spin-orbit coupling using the quasiclassical formalism. We consider both homogeneous superconductors and Josephson junctions. In the first case, the diode effect monotonically increases as the magnetic field is increased and the temperature is reduced, in contrast to the non-monotonic behavior found in clean structures. In Josephson junctions, SDE dramatically increases and changes its sign close to the $0-\pi$ transition of the junction, which occurs at specific junction lengths and strengths of the magnetic field. We show that the SDE is strongly suppressed in narrow junctions. Our results are relevant for understanding recent experiments that measure SDE in mesoscopic nanostructures, where significant disorder is unavoidable., Comment: 9 pages, 6 figures

In 1966, Pierre-Gilles de Gennes proposed a non-volatile mechanism for switching superconductivity on and off in a magnetic device. This involved a superconductor (S) sandwiched between ferromagnetic (F) insulators in which the net magnetic exchange field could be controlled through the magnetisation-orientation of the F layers. Because superconducting switches are attractive for a range of applications, extensive studies have been carried out on $F/S/F$ structures. Although these have demonstrated a sensitivity of the superconducting critical temperature ($T_{c}$) to parallel (P) and antiparallel (AP) magnetisation-orientations of the F layers, corresponding shifts in $T_c$ (i.e., ${\Delta}T_c = T_{c,AP} - T_{c,P}$) are lower than predicted with ${\Delta}T_c$ only a small fraction of $T_{c,AP}$, precluding the development of applications. Here, we report $EuS/Au/Nb/EuS$ structures where EuS is an insulating ferromagnet, Nb is a superconductor and Au is a heavy metal. For P magnetisations, the superconducting state in this structure is quenched down to the lowest measured temperature of 20 mK meaning that ${\Delta}T_c/T_{c,AP}$ is practically 1. The key to this so-called absolute switching effect is a sizable spin-mixing conductance at the $EuS/Au$ interface which ensures a robust magnetic proximity effect, unlocking the potential of $F/S/F$ switches for low power electronics.

We present a theory of weak localization (WL) in the presence of generic spin-dependent fields, including any type of spin-orbit coupling, Zeeman fields, and non-homogeneous magnetic textures. We go beyond the usual diffusive approximation, considering systems with short-range disorder of arbitrary strength, and obtain a compact expression for the weak localization (WL) correction to the conductivity in terms of the singlet-triplet polarization operator in momentum space. The latter can be directly related to the solution of the quasiclassical Eilenberger equation for superconducting systems. This formulation presents an intuitive framework to explore how the interplay of various spin-dependent fields drives weak (anti) localization. We apply our results to study in-plane magnetoconductivity in systems with spin-orbit coupling, and in newly discovered altermagnets. Our results enable straightforward calculation of the WL conductivity at arbitrary disorder strength, which can be particularly useful for interpreting experiments on high-mobility samples., Comment: 14 pages, 8 figures

We study the spectral properties of disordered superconductors with Ising spin-orbit coupling (ISOC) subjected to in-plane magnetic fields. In addition to the conventional singlet pairing, we also consider the recently proposed equal-spin triplet pairing, which couples to the singlet at finite in-plane magnetic fields. While both singlet and triplet order parameters are immune to intravalley scattering, they are significantly affected by intervalley scattering. In the realistic regime of strong ISOC, we find that the properties of the superconductor are well described by a simple formula reminiscent of the well-known Abrikosov-Gor'kov theory, but with a modified self-consistency condition. Our results enable straightforward self-consistent calculation of singlet and triplet order parameters and the density of states of disordered Ising superconductors, which can be particularly useful for interpreting recent tunneling spectroscopy experiments in these systems. We also investigate the high-energy features in the density of states, the so-called mirage gaps, and discuss how they are modified by triplet pairing., Comment: 9 pages, 5 figures

We review the use of hybrid thin films composed of superconductors and ferromagnets for creating non-reciprocal electronic components and self-biased detectors of electromagnetic radiation. We begin by introducing the theory behind these effects, as well as discussing various potential materials that can be used in the fabrication of these components. We then proceed with a detailed discussion on the fabrication and characterization of Al/EuS/Cu and EuS/Al/Co-based detectors, along with their noise analysis. Additionally, we suggest some approaches for multiplexing such self-biased detectors., Comment: 30 pages, 21 figures

We show that the amplitude, or Higgs mode of a superconductor with strong spin-orbit coupling and an exchange field, couples linearly to the electromagnetic field. Furthermore, by coupling such a superconductor to an LC resonator, we demonstrate that the Higgs resonance becomes a regular mode at frequencies smaller than the quasiparticle energy threshold $2\Delta$. We finally propose and discuss a possible experiment based on microwave spectroscopy for an unequivocal detection of the Higgs mode. Our approach may allow visualizing Higgs modes also in more complicated multiband superconductors with a coupling between the charge and other electronic degrees of freedom., Comment: 6+4 pages, 5 figures

Spin-orbitronic devices can integrate memory and logic by exploiting spin-charge interconversion (SCI), which is optimized by design and materials selection. In these devices, such as the magnetoelectric spin-orbit (MESO) logic, interfaces are crucial elements as they can prohibit or promote spin flow in a device as well as possess spin-orbit coupling resulting in interfacial SCI. Here, we study the origin of SCI in a Py/Cu/W lateral spin valve and quantify its efficiency. An exhaustive characterization of the interface between Cu and W electrodes uncovers the presence of an oxidized layer (WO$_x$). We determine that the SCI occurs at the Cu/WO$_x$ interface with a temperature-independent interfacial spin-loss conductance of $G_{||} \approx$ 20 $\times$ 10$^{13} \Omega^{-1}m^{-2}$ and an interfacial spin-charge conductivity $\sigma_{SC}=-$1610 $\Omega^{-1}cm^{-1}$ at 10 K ($-$830 $\Omega^{-1}cm^{-1}$ at 300 K). This corresponds to an efficiency given by the inverse Edelstein length $\lambda_{IEE}=-$0.76 nm at 10 K ($-$0.4 nm at 300 K), which is remarkably larger than in metal/metal and metal/oxide interfaces and bulk heavy metals. The large SCI efficiency at such an oxidized interface is a promising candidate for the magnetic readout in MESO logic devices., Comment: 11 pages, 3 figures, and Supplemental Material

The macroscopic coherence in superconductors supports dissipationless supercurrents which could play a central role in emerging quantum technologies. Accomplishing unequal supercurrents in the forward and backward directions would enable unprecedented functionalities. This nonreciprocity of critical supercurrents is called superconducting (SC) diode effect. We demonstrate strong SC diode effect in conventional SC thin films, such as niobium and vanadium, employing external magnetic fields as small as 1 Oe. Interfacing the SC layer with a ferromagnetic semiconductor EuS, we further accomplish non-volatile SC diode effect reaching a giant efficiency of 65%. By careful control experiments and theoretical modeling, we demonstrate that the critical supercurrent nonreciprocity in SC thin films could be easily accomplished with asymmetrical vortex edge/surface barriers and the universal Meissner screening current governing the critical currents. Our engineering of the SC diode effect in simple systems opens door for novel technologies. Meanwhile, we reveal the ubiquity of Meissner screening effect induced SC diode effect in superconducting films, which should be eliminated with great care in the search of exotic superconducting states harboring finite-momentum Cooper pairing., Comment: 27 pages, 16 figures

Spin-split superconductors exhibit an electron-hole asymmetric spin-resolved density of states, but the symmetry is restored upon averaging over spin. On the other hand, asymmetry appears again in tunneling junctions of spin-split superconductors with a spin-polarized barrier. As demonstrated recently in both theory and experiment, this fact leads to a particularly strong thermoelectric effect in superconductor-ferromagnet structures. In this work we show another important effect stemming from the electron-hole asymmetry - current rectification. We calculate the charge current in spin-polarized tunnel junctions of normal metal and a spin-split superconductor with AC and DC voltage bias. In the DC case, the I-V curve is not fully antisymmetric and has a voltage-symmetric component due to spin polarization. This translates to the existence of a rectified current in the AC case, which is proportional to the spin polarization of the junction and strongly depends on the frequency of the applied bias. We discuss possible applications of the rectification effect, including a diode for superconducting electronics and radiation detectors. The analysis of the rectified charge current is supplemented by the discussion of heat current and relevant noise correlators, where electron-hole asymmetry also plays an important role, and which are useful for applications in detectors., Comment: 13 pages, 11 figures

We calculate the non-reciprocal critical current and quantify the supercurrent diode effect in Rashba superconductors with arbitrary disorder, using the quasiclassical Eilenberger equation. The non-reciprocity is caused by the helical superconducting state, which appears when both inversion and time-reversal symmetries are broken. In the absence of disorder, we find a very strong diode effect, with the non-reciprocity exceeding 40% at optimal temperatures, magnetic fields and spin-orbit coupling. We establish that the effect persists even in the presence of strong disorder. We show that the sign of the diode effect changes as magnetic field and disorder are increased, reflecting the changes in the nature of the helical state., Comment: 9 pages, 7 figures. Significantly revised

Josephson junctions (JJs), where both time-reversal and inversion symmetry are broken, exhibit a phase shift $\phi_0$ in their current-phase relation. This allows for an anomalous supercurrent to flow in the junction even in the absence of a phase bias between the superconductors. We show that a finite phase shift also manifests in the so-called Andreev interferometers - a device that consists of a mesoscopic conductor coupled to the $\phi_0$-junction. Due to the proximity effect, the resistance of this conductor is phase-sensitive - it oscillates by varying the phase of the JJ. As a result, the quasiparticle current $I_{\mathrm{qp}}$ flowing through the conductor has an anomalous component, which exists only at finite $\phi_0$. Thus, the Andreev interferometry could be used to probe the $\phi_0$ effect. We consider two realizations of the $\phi_0$-junction and calculate $I_{\mathrm{qp}}$ in the interferometer: a superconducting structure with spin-orbit coupling and a system of spin-split superconductors with spin-polarized tunneling barriers., Comment: 11 pages, 2 figures

Ferromagnetic insulators can induce a strong exchange field in an adjacent superconductor via the magnetic proximity effect. This manifests as spin-splitting of the BCS density of states of the superconductor, an important ingredient for numerous superconducting spintronics applications and the realization of Majorana fermions. A crucial parameter that determines the magnitude of the induced spin-splitting in FI/S bilayers is the thickness of the S layer $d$: In very thin samples, the superconductivity is suppressed by the strong magnetism. By contrast, in very thick samples, the spin splitting is absent at distances away from the interface. In this work, we calculate the density of states and critical field of FI/S bilayers of arbitrary thickness. From here, we determine the range of parameters of interest for applications, where the exchange field and superconductivity coexist. We compare our theory with the tunneling spectroscopy measurements in several EuS/Al/AlO$_x$/Al samples. If the Al film in contact with the EuS is thinner than a certain critical value, we do not observe superconductivity, whereas, in thicker samples, we find evidence of a first-order phase transition induced by an external field. The complete transition is preceded by a regime in which normal and superconducting regions coexist. We attribute this mixed phase to inhomogeneities of the Al film thickness and the presence of superparamagnetic grains at the EuS/Al interface with different switching fields. Our results demonstrate on the one hand, the important role of the S layer thickness, which is particularly relevant for the fabrication of high-quality samples suitable for applications. On the other hand, the agreement between theory and experiment demonstrates the accuracy of our theory, which, originally developed for homogeneous situations, is generalized to highly inhomogeneous systems., Comment: 14 pages, 6 figures

The Eilenberger equation is a standard tool in the description of superconductors with an arbitrary degree of disorder. It can be generalized to systems with linear-in-momentum spin-orbit coupling (SOC), by exploiting the analogy of SOC with a non-abelian background field. Such field mixes singlet and triplet components and yields the rich physics of magnetoelectric phenomena. In this work we show that the application of this equation extends further, beyond superconductivity. In the normal state, the linearized Eilenberger equation describes the coupled spin-charge dynamics. Moreover, its resolvent corresponds to the so called Cooperons, and can be used to calculate the weak localization corrections. Specifically, we show how to solve this equation for any source term and provide a closed-form solution for the case of Rashba SOC. We use this solution to address several problems of interest for spintronics and superconductivity. Firstly, we study spin injection from ferromagnetic electrodes in the normal state, and describe the spatial evolution of spin density in the sample, and the complete crossover from the diffusive to the ballistic limit. Secondly, we address the so-called superconducting Edelstein effect, and generalize the previously known results to arbitrary disorder. Thirdly, we study weak localization correction beyond the diffusive limit, which can be a valuable tool in experimental characterization of materials with very strong SOC. We also address the so-called pure gauge case where the persistent spin helices form. Our work establishes the linearized Eilenberger equation as a powerful and a very versatile method for the study of materials with spin-orbit coupling, which often provides a simpler and more intuitive picture compared to alternative methods., Comment: 14 pages, 8 figures

We calculate the interference correction to the conductivity of doped transition metal dichalcogenide (TMDC) monolayers. Because of the interplay between valley structure and intrinsic spin-orbit coupling (SOC), these materials exhibit a rich weak localization (WL) behavior that is qualitatively different from conventional metals or similar two-dimensional materials such as graphene. Our results can also be used to describe graphene/TMDC heterostructures, where the SOC is induced in the graphene sheet. We discuss new parameter regimes that go beyond existing theories, and can be used to interpret recent experiments in order to assess the strength of SOC and disorder. Furthermore, we show that an in-plane Zeeman field can be used to distinguish the contributions of different kinds of SOC to the WL magnetoconductance., Comment: 15 pages, 6 figures

We calculate the effect of impurities on the superconducting phase diagram of transition metal dichalcogenide monolayers in the presence of an in-plane magnetic field. Due to strong intrinsic spin-orbit coupling, the upper critical field greatly surpasses the Pauli limit at low temperatures. We find that it is insensitive to intravalley scattering and, ultimately, limited by intervalley scattering., Comment: 10 pages, 8 figures