Search

The existence of cosmic dark matter and neutrino properties are long-standing problems in cosmology and particle physics. These problems have been investigated by using radiation detectors. We will discuss the application of inorganic crystal scintillators to studies on dark matter and neutrino properties. A large volume and high-purity inorganic crystal is a promising detector for investigating dark matter and neutrino.

The dark matter observation claim by the DAMA/LIBRA collaboration has been a long-standing puzzle within the particle physics community. Efforts of other research groups to verify the claim have been insufficient by significant radioactivity of present NaI(Tl) crystals. PICOLON (Pure Inorganic Crystal Observatory for LOw-energy Neut(ra)lino) experiment conducts independent search for Weakly Interacting Massive Particles (WIMPs) using NaI(Tl) crystals. Our NaI(Tl) crystal manufactured in 2020 (Ingot #85) reached the same purity level as DAMA/LIBRA crystals. In this report, we describe the radiopurity of the new Ingot #94 crystal produced using the same purification technique as Ingot #85. The $\alpha$-ray events were selected by pulse-shape discrimination method. The impurities in the Ingot #94, $^{232}$Th, $^{226}$Ra and $^{210}$Po radioactivity were $4.6\pm 1.2~\mathrm{\mu Bq/kg}$, $7.9\pm 4.4~\mathrm{\mu Bq/kg}$, and $19\pm 6~\mathrm{\mu Bq/kg}$, which are equivalent to those of the DAMA/LIBRA crystals. The background rate in the energy region of 2-6 keV , was 2-5 events/d/kg/keV without applying a veto trigger., Comment: We have found duplicate contents in Fig.6 to Fig.8 that overlap with the KEK proceedings(page. 154-155 in https://lib-extopc.kek.jp/preprints/PDF/2023/2325/2325001.pdf), so the data analysis needs to be redone. In addition, we are withdrawing this paper because removing these contents would significantly reduce the quality of the paper

PICOLON (Pure Inorganic Crystal Observatory for LOw-energy Neutr(al)ino) aims to search for cosmic dark matter by high purity NaI(Tl) scintillator. We developed extremely pure NaI(Tl) crystal by hybrid purification method. The recent result of $^{210}$Pb in our NaI(Tl) is less than 5.7 $\mu$Bq/kg. We will report the test experiment in the low-background measurement at Kamioka Underground Laboratory. The sensitivity for annual modulating signals and finding dark matter particles will be discussed., Comment: To be published in the Proceedings of TAUP2021. (Journal of Physics: Conference Series (JPCS),)

A dark matter search project needs and extremely low background radiation detector since the expected event rate of dark matter is less than a few events in one year in one tonne of the detector mass. The authors developed a highly radiopure NaI(Tl) crystal to search for dark matter. The best combination of the purification methods was developed, resulting $^{\mathrm{nat}}$K and $^{210}$Pb were less than 20 ppb and 5.7 $\mu$Bq/kg, respectively. The authors will construct a large volume detector system with high-purity NaI(Tl) crystals. The design and the performance of the prototype detector module will be reported in this article., Comment: 12 pages, 7 figures, RADIATION DETECTORS AND THEIR USES Proceedings of the 35th Workshop on Radiation Detectors and Their Uses in KEK

The highly radiopure NaI(Tl) was developed to search for particle candidates of dark matter. The optimized methods were combined to reduce various radioactive impurities. The $^{40}$K was effectively reduced by the re-crystallization method. The progenies of the decay chains of uranium and thorium were reduced by appropriate resins. The concentration of natural potassium in NaI(Tl) crystal was reduced down to 20 ppb. Concentrations of alpha-ray emitters were successfully reduced by appropriate selection of resin. The present concentration of thorium series and 226Ra were $1.2 \pm1.4$ $\mu$Bq/kg and $13\pm4$ $\mu$Bq/kg, respectively. No significant excess in the concentration of $^{210}$Pb was obtained, and the upper limit was 5.7 $\mu$Bq/kg at 90% C. L. The achieved level of radiopurity of NaI(Tl) crystals makes construction of a dark matter detector possible., Comment: 11 pages, 6 figures, accepted to Progress of Theoretical and Experimental Physics

The dark matter search project by means of ultra high purity NaI(Tl) scintillator is now underdevelopment. An array of large volume NaI(Tl) detectors whose volume is 12.7 cm$\phi\times$12.7 cm is applied to search for dark matter signal. To remove radioactive impurities in NaI(Tl) crystal is one of the most important task to find small number of dark matter signals. We have developed high purity NaI(Tl) crystal which contains small amounts of radioactive impurities, $<4$ ppb of $^{nat}$K, 0.3 ppt of Th chain, 58 $\mu$Bq/kg of $^{226}$Ra and 30 $\mu$Bq/kg of $^{210}$Pb. Future prospects to search for dark matter by means of a large volume and high purity NaI(Tl) scintillator is discussed., Comment: 8 pages, 5 figures. Proceedings of 31st Workshop on Radiation Detector and Their Uses, January 23-25, 2017. KEK, JAPAN

The PICO-LON project aims at search for cold dark matter by means of highly radio-pure and large volume NaI(Tl) scintillator. The NaI powder was purifed by chemical processing to remove lead isotopes and selecting a high purity graphite crucible. The concentrations of radioactive impurities of $^{226}$Ra and $^{228}$Th were effectively reduced to 58$\pm$4 $\mu$Bq/kg and 1.5$\pm$1.9 $\mu$Bq/kg, respectively. It should be remarked that the concentration of $^{210}$Pb, which is crucial for the sensitivity to dark matter, was reduced to 24$\pm$2 $\mu$Bq/kg. The total background rate at 10 keVee was as low as 8 keV$^{-1}$kg$^{-1}$day$^{-1}$, which was sufficiently low to search for dark matter. Further purification of NaI(Tl) ingot and future prospect of PICO-LON project is discussed., Comment: Submitted to Proceedings of TAUP 2015

KamLAND-PICO project aims to search for WIMPs dark matter by means of NaI(Tl) scintillator. To investigate the WIMPs candidate whose cross section is as small as $10^{-9}$ pb, a pure NaI(Tl) crystal was developed by chemical processing and taking care of surroundings. The concentration of U and Th chain was reduced to $5.4\pm0.9$ ppt and $3.3\pm2.2$ ppt, respectively. It should be remarked that the concentration of $^{210}$Pb which was difficult to reduce reached to the high purity as $58\pm26$ $\mu$Bq/kg., Comment: 6 pages 5 figures, Proceedings of the 26th Workshop on "Radiation Detectors and Their Uses" January 26-28 20214. KEK Tsukuba Japan. Accepted for publication

Thin and large area NaI(Tl) scintillator to search for WIMPs dark matter was developed. The performance of thin and wide area NaI(Tl) showed good enough to search for dark matter. The energy threshold was as low as 2keV and the energy resolution was about 24% in FWHM at 60keV., Comment: 7pages, 7figures, Proceedings of the 26th Workshop on Radiation Detectors and Their Uses, KEK-Proc1225008, (2012) p122

The WIMPs search project PICO-LON has been started with multilayer thin NaI(Tl) crystals. The thin (0.05cm) and wide area (5cmx5cm) NaI(Tl) crystals was successfully developed. The performances of thin NaI(Tl) scintillator was measured and they showed good energy resolution (20% at 60keV) and good position resolution (20% in 5cmx5cm wider area)., Comment: Proceeding of IDM2006

A thin (0.05cm) and wide area (5cmX5cm) NaI(Tl) scintillator was developed. The performance of the thin NaI(Tl) plate, energy resolution, single photoelectron energy and position sensitivity were tested. An excellent energy resolution of 20% (FWHM) at 60keV was obtained. The single photoelectron energy was calculated to be approximately 0.42 0.02keV. Position information in the 5cmx5cm area of the detector was also obtained by analyzing the ratio of the number of photons collected at opposite ends of the detector. The position resolution was obtained to be 1cm (FWHM) in the 5cmx5cm area., Comment: 10 pages. Accepted to Journal of Physical Society of Japan

A second quantised theory of electrons and positrons in a deep time-dependent potential well is discussed. It is shown that positron production from the well is a natural consequence of Dirac's hole theory when the strength of the well becomes supercritical. A formalism is developed whereby the amplitude for emission of a positron of a given momentum can be calculated. The difference between positron production and electron-positron pair production is demonstrated. Considerations of the vacuum charge and of Levinson's theorem are required for a full description of the problem., Comment: 31 pages; following macros/styles included; tcilatex.tex, thmsupp.tex, a4.sty,sw20jart.sty,jeep.sty,gnuindex.sty, thmsa.sty,thmsb.sty,thmsc.sty,thmsd.sty;paper.ps is postscript version of paper