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Spin angular momentum transfer in magnetic bilayers offers the possibility of ultrafast and low-loss operation for next-generation spintronic devices. We report the field- and temperature- dependent measurements on the magnetization precessions in Co$_2$FeAl/(Ga,Mn)As by time-resolved magneto-optical Kerr effect (TRMOKE). Analysis of the effective Gilbert damping and phase shift indicates a clear signature of an enhanced dynamic exchange coupling between the two ferromagnetic (FM) layers due to the reinforced spin pumping at resonance. The temperature dependence of the dynamic exchange-coupling reveals a primary contribution from the ferromagnetism in (Ga,Mn)As., Comment: arXiv admin note: text overlap with arXiv:2203.00293

Fast spin manipulation in magnetic heterostructures, where magnetic interactions between different materials often define the functionality of devices, is a key issue in the development of ultrafast spintronics. Although recently developed optical approaches such as ultrafast spin-transfer and spin-orbit torques open new pathways to fast spin manipulation, these processes do not fully utilize the unique possibilities offered by interfacial magnetic coupling effects in ferromagnetic multilayer systems. Here, we experimentally demonstrate ultrafast photo-enhanced interfacial exchange interactions in the ferromagnetic Co$_2$FeAl/(Ga,Mn)As system at low laser fluence levels. The excitation efficiency of Co$_2$FeAl with the (Ga,Mn)As layer is 30-40 times higher than the case with the GaAs layer at 5 K due to a photo-enhanced exchange coupling interaction via photoexcited charge transfer between the two ferromagnetic layers. In addition, the coherent spin precessions persist to room temperature, excluding the drive of photo-enhanced magnetization in the (Ga,Mn)As layer and indicating a proximity-effect-related optical excitation mechanism. The results highlight the importance of considering the range of interfacial exchange interactions in ferromagnetic heterostructures and how these magnetic coupling effects can be utilized for ultrafast, low-power spin manipulation.

We report structural and physical properties of the single crystalline ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$. The X-ray diffraction(XRD) results show that ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$ adopts the trigonal ${\mathrm{Ca}}{\mathrm{Al}}_{2}{\mathrm{Si}}_{2}$-type structure. Temperature dependent electrical resistivity $\rho(T)$ measurements indicate an insulating ground state for ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$ with activation energies of 40 meV and 0.64 meV for two distinct regions, respectively. Magnetization measurements show no apparent magnetic phase transition under 400 K. Different from other ${\mathrm{A}}{\mathrm{Mn}}_{2}{\mathrm{Pn}}_{2}$ (A = Ca, Sr, and Ba, and Pn = P, As, and Sb) compounds with the same structure, heat capacity $C_{\mathrm{p}}(T)$ and $\rho(T)$ reveal that ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$ has a first-order transition at $T$ = 69.5 K and the transition temperature shifts to high temperature upon increasing pressure. The emergence of plenty of new Raman modes below the transition, clearly suggests a change in symmetry accompanying the transition. The combination of the structural, transport, thermal and magnetic measurements, points to an unusual origin of the transition., Comment: 6 pages, 6 figures. Accepted by Europhysics Letters

We present a detailed analysis of the time series of time-stamped neutron counts obtained by single-neutron interferometry. The neutron counting statistics display the usual Poissonian behavior, but the variance of the neutron counts does not. Instead, the variance is found to exhibit a dependence on the phase-shifter setting which can be explained by a probabilistic model that accounts for fluctuations of the phase shift. The time series of the detection events exhibit long-time correlations with amplitudes that also depend on the phase-shifter setting. These correlations appear as damped oscillations with a period of about 2.8 s. By simulation, we show that the correlations of the time differences observed in the experiment can be reproduced by assuming that, for a fixed setting of the phase shifter, the phase shift experienced by the neutrons varies periodically in time with a period of 2.8 s. The same simulations also reproduce the behavior of the variance. Our analysis of the experimental data suggests that time-stamped data of singleparticle interference experiments may exhibit transient features that require a description in terms of non-stationary processes, going beyond the standard quantum model of independent random events.

Recently, we have demonstrated (Jin et al. 2020, J. Phys. B: At. Mol. Opt. Phys. 53, 075201) that a hybrid subconfiguration-average and level-to-level distorted wave treatment of electron-impact single ionisation (EISI) of W$^{14+}$ ions represents an accurate and manageable approach for the calculation of EISI cross sections of a complex ion. Here we demonstrate the more general validity of this approach by comparing hybrid cross sections for EISI of W$^{15+}$ and W$^{16+}$ with the recent experimental results of Schury et al. 2020, J. Phys. B: At. Mol. Opt. Phys. 53, 015201). Our calculations also account for the resonant-excitation double autoionisation (REDA) process which is important in the electron energy range 370-600 eV and for the possible presence of initially metastable ions in the experiment., Comment: 7 pages, 8 figures, 1 table

The ground state properties of correlated electron systems can be extraordinarily sensitive to external stimuli, such as temperature, strain, and electromagnetic fields, offering abundant platforms for functional materials. We present a metastable and reversible photoinduced ferromagnetic transition in strained films of the doped manganite La(2/3)Ca(1/3)MnO3. Using the novel multi-messenger combination of atomic force microscopy, cryogenic scanning near-field optical microscopy, magnetic force microscopy, and ultrafast laser excitation, we demonstrate both "writing" and "erasing" of a metastable ferromagnetic metal phase with nanometer-resolved finesse. By tracking both optical conductivity and magnetism at the nano-scale, we reveal how spontaneous strain underlies the thermal stability, persistence, and reversal of this photoinduced metal. Our first-principles electronic structure calculations reveal how an epitaxially engineered Jahn-Teller distortion can stabilize nearly degenerate antiferromagnetic insulator and ferromagnetic metal phases. We propose a Ginzburg-Landau description to rationalize the co-active interplay of strain, lattice distortion, and magnetism we resolve in strained LCMO, thus guiding future functional engineering of epitaxial oxides like manganites into the regime of phase-programmable materials., Comment: 18 pages, 5 figures, supplementary information

Absolute cross sections for electron-impact single ionisation (EISI) of multiply charged tungsten ions (W$^{q+}$) with charge states in the range $ 11 \leq q \leq 18$ in the electron-ion collision energy ranges from below the respective ionisation thresholds up to 1000~eV were measured employing the electron-ion crossed-beams method. In order to extend the results to higher energies, cross section calculations were performed using the subconfiguration-averaged distorted-wave (SCADW) method for electron-ion collision energies up to 150~keV. From the combined experimental and scaled theoretical cross sections rate coefficients were derived which are compared with the ones contained in the ADAS database and which are based on the configuration-averaged distorted wave (CADW) calculations of Loch et al. [Phys. Rev. A 72, 052716 (2005)]. Significant discrepancies were found at the temperatures where the ions investigated here are expected to form in collisionally ionised plasmas. These discrepancies are attributed to the limitations of the CADW approach and also the more detailed SCADW treatment which do not allow for a sufficiently accurate description of the EISI cross sections particularly at the ionisation thresholds., Comment: 14 pages, 4 figures, 4 tabels

We extensively test a recent protocol to demonstrate quantum fault tolerance on three systems: (1) a real-time simulation of five spin qubits coupled to an environment with two-level defects, (2) a real-time simulation of transmon quantum computers, and (3) the 16-qubit processor of the IBM Q Experience. In the simulations, the dynamics of the full system is obtained by numerically solving the time-dependent Schr\"odinger equation. We find that the fault-tolerant scheme provides a systematic way to improve the results when the errors are dominated by the inherent control and measurement errors present in transmon systems. However, the scheme fails to satisfy the criterion for fault tolerance when decoherence effects are dominant.

In the model of gate-based quantum computation, the qubits are controlled by a sequence of quantum gates. In superconducting qubit systems, these gates can be implemented by voltage pulses. The success of implementing a particular gate can be expressed by various metrics such as the average gate fidelity, the diamond distance, and the unitarity. We analyze these metrics of gate pulses for a system of two superconducting transmon qubits coupled by a resonator, a system inspired by the architecture of the IBM Quantum Experience. The metrics are obtained by numerical solution of the time-dependent Schr\"odinger equation of the transmon system. We find that the metrics reflect systematic errors that are most pronounced for echoed cross-resonance gates, but that none of the studied metrics can reliably predict the performance of a gate when used repeatedly in a quantum algorithm.

We study the real-time and real-space dynamics of charge in the one-dimensional Hubbard model in the limit of high temperatures. To this end, we prepare pure initial states with sharply peaked density profiles and calculate the time evolution of these nonequilibrium states, by using numerical forward-propagation approaches to chains as long as 20 sites. For a class of typical states, we find excellent agreement with linear-response theory and unveil the existence of remarkably clean charge diffusion in the regime of strong particle-particle interactions. Moreover, we demonstrate that this diffusive behavior does not depend on certain details of our initial conditions, i.e., it occurs for five different realizations with random and nonrandom internal degrees of freedom, single and double occupation of the central site, and displacement of spin-up and spin-down particles., Comment: 5 pages, 4 figures (+ 3 pages, 5 figures)

The real-time broadening of density profiles starting from non-equilibrium states is at the center of transport in condensed-matter systems and dynamics in ultracold atomic gases. Initial profiles close to equilibrium are expected to evolve according to linear response, e.g., as given by the current correlator evaluated exactly at equilibrium. Significantly off equilibrium, linear response is expected to break down and even a description in terms of canonical ensembles is questionable. We unveil that single pure states with density profiles of maximum amplitude yield a broadening in perfect agreement with linear response, if the structure of these states involves randomness in terms of decoherent off-diagonal density-matrix elements. While these states allow for spin diffusion in the XXZ spin-1/2 chain at large exchange anisotropies, coherences yield entirely different behavior., Comment: 7 pages, 7 figures, accepted for publication in Phys. Rev. B

Data of the numerical solution of the time-dependent Schr\"odinger equation of a system containing one spin-1/2 particle interacting with a bath of up to 32 spin-1/2 particles is used to construct a Markovian quantum master equation describing the dynamics of the system spin. The procedure of obtaining this quantum master equation, which takes the form of a Bloch equation with time-independent coefficients, accounts for all non-Markovian effects in as much the general structure of the quantum master equation allows. Our simulation results show that, with a few rather exotic exceptions, the Bloch-type equation with time-independent coefficients provides a simple and accurate description of the dynamics of a spin-1/2 particle in contact with a thermal bath. A calculation of the coefficients that appear in the Redfield master equation in the Markovian limit shows that this perturbatively derived equation quantitatively differs from the numerically estimated Markovian master equation, the results of which agree very well with the solution of the time-dependent Schr\"odinger equation., Comment: Corrections + additional results, accepted for publication in Physical Review E

Since the first suggestion of the Jarzynski equality many derivations of this equality have been presented in both, the classical and the quantum context. While the approaches and settings greatly differ from one to another, they all appear to rely on the initial state being a thermal Gibbs state. Here, we present an investigation of work distributions in driven isolated quantum systems, starting off from pure states that are close to energy eigenstates of the initial Hamiltonian. We find that, for the nonintegrable system in quest, the Jarzynski equality is fulfilled to good accuracy., Comment: 9 pages, 7 figures

We study measures of decoherence and thermalization of a quantum system $S$ in the presence of a quantum environment (bath) $E$. The entirety $S$$+$$E$ is prepared in a canonical thermal state at a finite temperature, that is the entirety is in a steady state. Both our numerical results and theoretical predictions show that measures of the decoherence and the thermalization of $S$ are generally finite, even in the thermodynamic limit, when the entirety $S$$+$$E$ is at finite temperature. Notably, applying perturbation theory with respect to the system-environment coupling strength, we find that under common Hamiltonian symmetries, up to first order in the coupling strength it is sufficient to consider $S$ uncoupled from $E$, but entangled with $E$, to predict decoherence and thermalization measures of $S$. This decoupling allows closed form expressions for perturbative expansions for the measures of decoherence and thermalization in terms of the free energies of $S$ and of $E$. Large-scale numerical results for both coupled and uncoupled entireties with up to 40 quantum spins support these findings., Comment: 46 pages, 21 figures, long appendix includes the perturbation theory calculation details

We study the charge conductivity of the one-dimensional repulsive Hubbard model at finite temperature using the method of dynamical quantum typicality, focusing at half filling. This numerical approach allows us to obtain current autocorrelation functions from systems with as many as 18 sites, way beyond the range of standard exact diagonalization. Our data clearly suggest that the charge Drude weight vanishes with a power law as a function of system size. The low-frequency dependence of the conductivity is consistent with a finite dc value and thus with diffusion, despite large finite-size effects. Furthermore, we consider the mass-imbalanced Hubbard model for which the charge Drude weight decays exponentially with system size, as expected for a non-integrable model. We analyze the conductivity and diffusion constant as a function of the mass imbalance and we observe that the conductivity of the lighter component decreases exponentially fast with the mass-imbalance ratio. While in the extreme limit of immobile heavy particles, the Falicov-Kimball model, there is an effective Anderson-localization mechanism leading to a vanishing conductivity of the lighter species, we resolve finite conductivities for an inverse mass ratio of $\eta \gtrsim 0.25$., Comment: 13 pages, 11 figures