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We report the Stark deceleration of CaF molecules in the strong-field seeking ground state and in a weak-field seeking component of a rotationally-excited state. We use two types of decelerator, a conventional Stark decelerator for the weak-field seekers, and an alternating gradient decelerator for the strong-field seekers, and we compare their relative merits. We also consider the application of laser cooling to increase the phase-space density of decelerated molecules., Comment: 10 pages, 8 figures

We describe a method for determining the radiative decay properties of a molecule by studying the saturation of laser-induced fluorescence and the associated power broadening of spectral lines. The fluorescence saturates because the molecules decay to states that are not resonant with the laser. The amplitudes and widths of two hyperfine components of a spectral line are measured over a range of laser intensities and the results compared to a model of the laser-molecule interaction. Using this method we measure the lifetime of the A(v'=0) state of CaF to be tau=19.2 \pm 0.7 ns, and the Franck-Condon factor for the transition to the X(v=0) state to be Z=0.987 (+0.013 || -0.019). In addition, our analysis provides a measure of the hyperfine interval in the lowest-lying state of A(v'=0), Delta_e=4.8 \pm 1.1 MHz., Comment: 10 pages, 6 figures. Minor revisions following referee suggestions

Quantum resonances in the kicked rotor are characterized by a dramatically increased energy absorption rate, in stark contrast to the momentum localization generally observed. These resonances occur when the scaled Planck's constant hbar=(r/s)*4pi, for any integers r and s. However only the hbar=r*2pi resonances are easily observable. We have observed high-order quantum resonances (s>2) utilizing a sample of low temperature, non-condensed atoms and a pulsed optical standing wave. Resonances are observed for hbar=(r/16)*4pi r=2-6. Quantum numerical simulations suggest that our observation of high-order resonances indicates a larger coherence length than expected from an initially thermal atomic sample.

Atoms trapped in optical lattice have long been a system of interest in the AMO community, and in recent years much study has been devoted to both short- and long-range coherence in this system, as well as to its possible applications to quantum information processing. Here we demonstrate for the first time complete determination of the quantum phase space distributions for an ensemble of $^{85}Rb$ atoms in such a lattice, including a negative Wigner function for atoms in an inverted state., Comment: Submitted to Journal of Optics B: Quantum and Semiclassical Optics. Special issue in connection with the 9th International Conference on Squeezed States and Uncertainty Relations, to be held in Besancon, France, on 2-6 May 2005