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Coherence and entanglement are both the fundamental properties which quantify the degree of nonclassicality possessed in a quantum state. Recently coherence and entanglement are considered as a dynamical resource where the nonclassicality is strongly related to the amount of the static resources which can be generated in a quantum process. In [Phys. Rev. Lett. 125, 130401 (2020)10.1103/PhysRevLett.125.130401], for the first time, the authors study the interconvertability of these two kinds of dynamical resources. Here, we demonstrate this resource conversion in an all optical setup, and successfully observe the dynamical resource conversion. The experimental observation prove the ability of manipulating dynamical resource within current quantum photonic technologies.

The resource theory of coherence studies the operational value of superpositions in quantum technologies. A key question in this theory concerns the efficiency of manipulation and inter-conversion of the resource. Here we solve this question completely for qubit states by determining the optimal probabilities for mixed state conversions via stochastic incoherent operations. Extending the discussion to distributed scenarios, we introduce and address the task of assisted incoherent state conversion where the process is enhanced by making use of correlations with a second party. Building on these results, we demonstrate experimentally that the optimal state conversion probabilities can be achieved in a linear optics set-up. This paves the way towards real world applications of coherence transformations in current quantum technologies., Comment: 7+14 pages, 4+2 figures, article supersedes arXiv:1804.09467

Wave-particle duality is one of the basic features of quantum mechanics, giving rise to the use of complex numbers in describing states of quantum systems, their dynamics, and interaction. Since the inception of quantum theory, it has been debated whether complex numbers are actually essential, or whether an alternative consistent formulation is possible using real numbers only. Here, we attack this long-standing problem both theoretically and experimentally, using the powerful tools of quantum resource theories. We show that - under reasonable assumptions - quantum states are easier to create and manipulate if they only have real elements. This gives an operational meaning to the resource theory of imaginarity. We identify and answer several important questions which include the state-conversion problem for all qubit states and all pure states of any dimension, and the approximate imaginarity distillation for all quantum states. As an application, we show that imaginarity plays a crucial role for state discrimination: there exist real quantum states which can be perfectly distinguished via local operations and classical communication, but which cannot be distinguished with any nonzero probability if one of the parties has no access to imaginarity. We confirm this phenomenon experimentally with linear optics, performing discrimination of different two-photon quantum states by local projective measurements. These results prove that complex numbers are an indispensable part of quantum mechanics., 6+2 pages, 2 figures

Complex numbers are widely used in both classical and quantum physics, and are indispensable components for describing quantum systems and their dynamical behavior. Recently, the resource theory of imaginarity has been introduced, allowing for a systematic study of complex numbers in quantum mechanics and quantum information theory. In this work we develop theoretical methods for the resource theory of imaginarity, motivated by recent progress within theories of entanglement and coherence. We investigate imaginarity quantification, focusing on the geometric imaginarity and the robustness of imaginarity, and apply these tools to the state conversion problem in imaginarity theory. Moreover, we analyze the complexity of real and general operations in optical experiments, focusing on the number of unfixed wave plates for their implementation. We also discuss the role of imaginarity for local state discrimination, proving that any pair of real orthogonal pure states can be discriminated via local real operations and classical communication. Our study reveals the significance of complex numbers in quantum physics, and proves that imaginarity is a resource in optical experiments., 13 pages, 2 figures. Accompanying article for arXiv:2007.14847

The low-activity cationic monomer tert-butyl-dime1hyl-(4-methyl-pent-4-enyloxy)-silane was synthesized by Grignard reaction and hydroxyl-protection reaction. Living polyisobutylene chains were initially synthesized by controlled cationic polymerization and then capped with tert-butyl-dimethyl-(4-methyl-pent-4-enyloxy)-silane. The hydrolysis of these polyisobutylenes end capped with tert-butyl-dimethyl-(4-methyl-pent-4-enyloxy)-silane gave rise to hydroxytelechelic polyisobutylene. NMR analysis confirmed that the hydrolysis was complete. Results also showed that a low polymerization temperature favored the participation of tert-butyl-dimethyl-(4-methyl-pent-4-enyloxy)-silane in the end-capping reaction. Moreover, polyisobutylene-based polyurethane exhibited greater acid resistance than commercial polyurethane.

Quantum uncertainty is a well-known property of quantum mechanics that states the impossibility of predicting measurement outcomes of multiple incompatible observables simultaneously. In contrast, the uncertainty in the classical domain comes from the lack of information about the exact state of the system. One may naturally ask, whether the quantum uncertainty is indeed a fully intrinsic property of the quantum theory, or whether similarly to the classical domain lack of knowledge about specific parts of the physical system might be the source of this uncertainty. This question has been addressed in the previous literature where the authors argue that in the entropic formulation of the uncertainty principle that can be illustrated using the, so-called, guessing games, indeed such lack of information has a significant contribution to the arising quantum uncertainty. Here we investigate this issue experimentally by implementing the corresponding two-dimensional and three-dimensional guessing games. Our results confirm that within the guessing-game framework, the quantum uncertainty to a large extent relies on the fact that quantum information determining the key properties of the game is stored in the degrees of freedom that remain inaccessible to the guessing party. Moreover, we offer an experimentally compact method to construct the high-dimensional Fourier gate which is a major building block for various tasks in quantum computation, quantum communication, and quantum metrology., Comment: close to the version published in npj quantum information

When an observable is measured on an evolving coherent quantum system twice, the first measurement generally alters the statistics of the second one, which is known as measurement back-action. We introduce, and push to its theoretical and experimental limits, a novel method of back-action evasion, whereby entangled collective measurements are performed on several copies of the system. This method is inspired by a similar idea designed for the problem of measuring quantum work [Perarnau-Llobet \textit{et al}., (https://doi.org/10.1103/PhysRevLett.118.070601) Phys. Rev. Lett. \textbf{118}, 070601 (2017)]. By utilizing entanglement as a resource, we show that the back-action can be extremely suppressed compared to all previous schemes. Importantly, the back-action can be eliminated in highly coherent processes.

We investigate whether paradigmatic measurements for quantum state tomography, namely mutually unbiased bases and symmetric informationally complete measurements, can be employed to certify quantum correlations. For this purpose, we identify a simple and noise-robust correlation witness for entanglement detection, steering and nonlocality that can be evaluated based on the outcome statistics obtained in the tomography experiment. This allows us to perform state tomography on entangled qutrits, a test of Einstein-Podolsky-Rosen steering and a Bell inequality test, all within a single experiment. We also investigate the trade-off between quantum correlations and subsets of tomographically complete measurements as well as the quantification of entanglement in the different scenarios. Finally, we perform a photonics experiment in which we demonstrate quantum correlations under these flexible assumptions, namely with both parties trusted, one party untrusted and both parties untrusted., See also the communication game of arXiv:2007.15643 to which our nonlocal game is strongly related

Quantum coherence is a fundamental property of quantum systems, separating quantum from classical physics. Recently, there has been significant interest in the characterization of quantum coherence as a resource, investigating how coherence can be extracted and used for quantum technological applications. In this work we review the progress of this research, focusing in particular on recent experimental efforts. After a brief review of the underlying theory we discuss the main platforms for realizing the experiments: linear optics, nuclear magnetic resonance, and superconducting systems. We then consider experimental detection and quantification of coherence, experimental state conversion and coherence distillation, and experiments investigating the dynamics of quantum coherence. We also review experiments exploring the connections between coherence and uncertainty relations, path information, and coherence of operations and measurements. Experimental efforts on multipartite and multilevel coherence are also discussed.

In quantum thermodynamics, the standard approach to estimate work fluctuations in unitary processes is based on two projective measurements, one performed at the beginning of the process and one at the end. The first measurement destroys any initial coherence in the energy basis, thus preventing later interference effects. In order to decrease this back-action, a scheme based on collective measurements has been proposed in~[PRL 118, 070601 (2017)]. Here, we report its experimental implementation in an optical system. The experiment consists of a deterministic collective measurement on identically prepared two qubits, encoded in the polarisation and path degree of a single photon. The standard two projective measurement approach is also experimentally realized for comparison. Our results show the potential of collective schemes to decrease the back-action of projective measurements, and capture subtle effects arising from quantum coherence., Comment: 9 pages, 4 figures

The dynamics of open quantum systems and manipulation of quantum resources are both of fundamental interest in quantum physics. Here, we investigate the relation between quantum Markovianity and coherence, providing an effective way for detecting non-Markovianity based on the \textit{quantum-incoherent relative entropy of coherence} ($\mathcal{QI}$ REC). We theoretically show the relation between completely positive (CP) divisibility and the monotonic behavior of the $\mathcal{QI}$ REC. Also we implement an all-optical experiment to demonstrate that the behavior of the $\mathcal{QI}$ REC is coincident with the entanglement shared between the system and the ancilla for both Markovian and non-Markovian evolution; while other coherence-based non-Markovian information carriers violate monotonicity, even in Markovian processes. Moreover, we experimentally observe that non-Markovianity enhances the ability of creating coherence on an ancilla. This is the first experimental study of the relation between dynamical behavior of the $\mathcal{QI}$ REC and the phenomenon of information backflow. Moreover, our method for detecting non-Markovianity is applicable to general quantum evolutions., Comment: 6+14 pages, 9 figures

A random copolymer of isobutylene (IB) and 4-vinylbenzenecyclobutylene (4-VBCB) was synthesized by cationic polymerization at &minus, 80 &deg, C using 2-chloro-2,4,4-trimethylpentane (TMPCl) as initiator. The laws of copolymerization were investigated by changing the feed quantities of 4-VBCB. The molecular weight of the copolymer decreased, and its molecular weight distribution (MWD) increased with increasing 4-VBCB content. We proposed a possible copolymerization mechanism behind the increase in the chain transfer reaction to 4-VBCB with increasing of feed quantities of 4-VBCB. The thermal properties of the copolymers were studied by solid-phase heating and crosslinking. After crosslinking, the decomposition and glass transition temperatures (Tg) of the copolymer increased, the network structure that formed did not break when reheated, and the mechanical properties remarkably improved.

When a photon passes through an interferometer, quantum mechanics does not provide a clear answer as to its past. Quantum retrodiction is a quantitative theory, which endeavors to make statements about the past of a system based on present knowledge. Quantum retrodiction may be used to analyze the past of a photon, that is, its trajectory. Here we experimentally retrodict the trajectories of single photons in double interferometers by measuring the final state of the photon. A sequence of measurements is made on a photon to determine which path the photon followed, so a series of retrodiction of measurement results can be regarded as a photon trajectory. We obtain information about the partial trajectory and the entire trajectory of the photon. Furthermore, we also observe the effect of different measurements in the extraction of trajectory information. Our experiment highlights the application of retrodiction theory to the study of the photon's past, and provides potential application in quantum communications.

Collective measurements on identically prepared quantum systems can extract more information than local measurements, thereby enhancing information-processing efficiency. Although this nonclassical phenomenon has been known for two decades, it has remained a challenging task to demonstrate the advantage of collective measurements in experiments. Here, we introduce a general recipe for performing deterministic collective measurements on two identically prepared qubits based on quantum walks. Using photonic quantum walks, we realize experimentally an optimized collective measurement with fidelity 0.9946 without post selection. As an application, we achieve the highest tomographic efficiency in qubit state tomography to date. Our work offers an effective recipe for beating the precision limit of local measurements in quantum state tomography and metrology. In addition, our study opens an avenue for harvesting the power of collective measurements in quantum information-processing and for exploring the intriguing physics behind this power., Demonstrating the advantage of collective measurements in experiments remains a daunting task. Here the authors introduce a general recipe for performing deterministic collective measurements on two identically prepared qubits based on quantum walks.

Quantum resource theories seek to quantify sources of non-classicality that bestow quantum technologies their operational advantage. Chief among these are studies of quantum correlations and quantum coherence. The former to isolate non-classicality in the correlations between systems, the latter to capture non-classicality of quantum superpositions within a single physical system. Here we present a scheme that cyclically inter-converts between these resources without loss. The first stage converts coherence present in an input system into correlations with an ancilla. The second stage harnesses these correlations to restore coherence on the input system by measurement of the ancilla. We experimentally demonstrate this inter-conversion process using linear optics. Our experiment highlights the connection between non-classicality of correlations and non-classicality within local quantum systems, and provides potential flexibilities in exploiting one resource to perform tasks normally associated with the other., 8 pages, 4 figures, comments welcome

Quantum coherence, which quantifies the superposition properties of a quantum state, plays an indispensable role in quantum resource theory. A recent theoretical work [Phys. Rev. Lett. \textbf{116}, 070402 (2016)] studied the manipulation of quantum coherence in bipartite or multipartite systems under the protocol Local Incoherent Operation and Classical Communication (LQICC). Here we present the first experimental realization of obtaining maximal coherence in assisted distillation protocol based on linear optical system. The results of our work show that the optimal distillable coherence rate can be reached even in one-copy scenario when the overall bipartite qubit state is pure. Moreover, the experiments for mixed states showed that distillable coherence can be increased with less demand than entanglement distillation. Our work might be helpful in the remote quantum information processing and quantum control., Comment: 7 pages, 5 figures