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In several processes of stellar nucleosynthesis, like the astrophysical gamma-process, nuclear reactions involving alpha particles play an important role. The description of these reactions necessitates the knowledge of the alpha-nucleus optical model potential (AOMP) which is highly ambiguous at low, astrophysical energies. This ambiguity introduces a substantial uncertainty in the stellar models for predicting elemental and isotopic abundances. The experimental study of the AOMP is thus necessary which can be implemented by measuring the cross section of alpha-induced nuclear reactions. At low energies, (a,n) reactions are suitable for such a purpose. Therefore, in the present work, the (a,n) cross sections of four Te isotopes have been measured, mostly for the first time, and compared with theoretical predictions. The (a,n) cross sections of 120,122,124,130Te have been measured in the energy range between about 10 and 17 MeV using the activation method. The detection of the gamma radiation following the decay of the radioactive reaction products were used to determine the cross sections. The measured cross sections are compared with statistical model calculations obtained from the widely used TALYS nuclear reaction simulation code. Predictions using various available AOMPs are investigated. It is found that the recently developed Atomki-V2 AOMP provides the best description for all studied reactions and this potential also reproduces well the total reaction cross sections from elastic scattering experiments, when they are available in literature. We recommend therefore to use the astrophysical reaction rates based on this potential for nucleosynthesis models of heavy elements., Comment: Accepted for publication in Phys. Rev. C

Isomer spectroscopy of heavy neutron-rich nuclei beyond the N=126 closed shell has been performed for the first time at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. New millisecond isomers have been identified at low excitation energies, 985.3(19) keV in 213Tl and 874(5) keV in 215Tl. The measured half-lives of 1.34(5) ms in 213Tl and 3.0(3) ms in 215Tl suggest spins and parities 11/2- with the single proton-hole configuration h11/2 as leading component. They are populated via E1 transitions by the decay of higher-lying isomeric states with proposed spin and parity 17/2+, interpreted as arising from a single s1/2 proton hole coupled to the 8+ seniority isomer in the (A+1)Pb cores. The lowering of the 11/2- states is ascribed to an increase of the h11/2 proton effective single-particle energy as the second g9/2 orbital is filled by neutrons, owing to a significant reduction of the proton-neutron monopole interaction between the h11/2 and g9/2 orbitals. The new ms-isomers provide the first experimental observation of shell evolution in the almost unexplored N>126 nuclear region below doubly-magic 208Pb., Comment: 9 pages, 3 figures, 1 table

The $^3$He($\alpha$,$\gamma$)$^7$Be reaction plays a major role both in the BBN producing the majority of the primordial $^7$Li, and in the pp-chain, where it is the branching point. As a few-nucleon system, this reaction is often used to validate ab-initio theoretical calculations and/or test R-matrix theory and code implementations. For the latter, experimental data in an extended energy range is of crucial importance to test the fit and extrapolation capabilities of the different codes. The $^3$He($\alpha$,$\gamma$)$^7$Be reaction cross section has been measured by several groups up to the first resonance ($E_{c.m.} \approx 3$ MeV) in the reaction. However, only one dataset exists above the $^7$Be proton separation threshold measured in a narrow energy range ($E_{c.m.} = 4.0-4.4$ MeV). In this work we extend the available experimental capture cross section database to the energy range of known $^7$Be levels. The activation method was used. The experiment was performed using a thin-window gas cell with two high-purity Al foils as entrance and exit windows. The activity of the $^7$Be nuclei implanted in the exit/catcher foil was measured by detecting the yield of the emitted $\gamma$~rays using shielded high-purity germanium detectors. New experimental $^3$He($\alpha$,$\gamma$)$^7$Be reaction cross section data were obtained for the first time in the $E_{c.m.}=4.3-8.3$ MeV energy region. The new dataset with about 0.2 MeV step covers the energy range of known levels and particle separation thresholds. No prominent structures are observer around the $^7$Be levels. The reaction cross section is slowly increasing with increasing energy. Above the $^6$Li$+p_1$ threshold, a decrease starts in the cross section trend. The overall structure of the cross section suggest a broad resonance peaking around $E_x=7.5$ MeV $^7$Be excitation energy, with a width of 8 MeV., Comment: Typos are corrected, mainly in Table II., second column where the numerical values were incorrectly entered before

This work describes a silicon tracker system developed for experiments with proton-rich radioactive ion beams at the SAMURAI superconducting spectrometer of RIBF at RIKEN. The system is designed for accurate angular reconstruction and atomic number identification of relativistic heavy ions and protons which are simultaneously produced in reactions motivated by studies of proton capture reactions of interest for nuclear astrophysics. The technical characteristics of the tracking array are described in detail as are its performance in two pilot experiments. The physics justification for such a system is also presented.

The CNO cycle is one of the fundamental processes of hydrogen burning in stars. The first reaction of the cycle is the radiative proton capture on 12C and the rate of this 12C(p,gamma)13N reaction is related to the 12C/13C ratio observed e.g. in the Solar System. The low-energy cross section of this reaction was measured several times in the past, however, the experimental data are scarce in a wide energy range especially around the resonance at 1.7 MeV. In the present work the 12C(p,gamma)13N cross section was measured between 300 and 1900 keV using the activation method. This method was only used several decades ago in the low-energy region. As the activation method provides the total cross section and has uncertainties different from those of the in-beam gamma-spectroscopy technique, the present results provide a largely independent data set for future low-energy extrapolations and thus for astrophysical reaction rate calculations., Comment: Accepted for publication in European Physical Journal A

Nuclear reactions involving alpha particles play an important role in various astrophysical processes such as the gamma-process of heavy element nucleosynthesis. The poorly known low-energy alpha-nucleus optical (AOMP) potential is a key parameter to estimate the rates of these reactions. The AOMP can be tested by measuring the cross section of alpha-scattering as well as alpha-induced reactions. Low energy elastic alpha-scattering on 144Sm has recently been measured with high precision. The aim of the present work was to complement that work by measuring the (a,n) cross sections on 144Sm at low energies. The experimental data shall be used to constrain the AOMP. From this potential the 144Sm(a,g)148Gd reaction rate can be derived with reduced uncertainties. The 144Sm(a,n)147Gd reaction was studied by bombarding Sm targets with alpha-beams provided by the cyclotron accelerator of Atomki. The cross section was determined using the activation method. The gamma-radiation following the decay of the 147Gd reaction product was measured with a HPGe detector. The experimental data are analyzed within the statistical model. The cross section was measured in the alpha-energy range between 13 and 20 MeV in 1 MeV steps, i.e., from close above the (a,n) threshold. The results were compared with statistical model calculations using various approaches and parametrizations for the AOMP, and excellent agreement was obtained for two recent potentials. However, these potentials cannot reproduce literature data for the 144Sm(a,g)148Gd reaction with the same accuracy. Constraints for the AOMP were derived from an analysis of the new 144Sm(a,n)147Gd data and literature data for 144Sm(a,g)148Gd. These constraints enable a determination of the reaction rate of the 144Sm(a,g)148Gd reaction with significantly reduced uncertainties of less than a factor of two., Comment: Accepted for publication in Phys. Rev. C

Nuclear Astrophysics is a field at the intersection of nuclear physics and astrophysics, which seeks to understand the nuclear engines of astronomical objects and the origin of the chemical elements. This white paper summarizes progress and status of the field, the new open questions that have emerged, and the tremendous scientific opportunities that have opened up with major advances in capabilities across an ever growing number of disciplines and subfields that need to be integrated. We take a holistic view of the field discussing the unique challenges and opportunities in nuclear astrophysics in regards to science, diversity, education, and the interdisciplinarity and breadth of the field. Clearly nuclear astrophysics is a dynamic field with a bright future that is entering a new era of discovery opportunities., Comment: 96 pages. Submitted to Journal of Physics G

14N(p,gamma)15O is one of the key reactions of nuclear astrophysics playing a role in various stellar processes and influencing energy generation of stars, stellar evolution and nucleosynthesis. For a reliable reaction rate calculation the low energy cross section of 14N(p,gamma)15O must be known with high accuracy. Owing to the unmeasurable low cross sections, theoretical calculations are unavoidable. High precision experimental cross section data are needed in a wide energy range in order to provide the necessary basis for low energy extrapolations. In the present work the total 14N(p,gamma)15O cross section was measured with a method complementary to the available data sets. The cross section was measured with activation, based on the detection of the annihilation radiation following the beta+ decay of the reaction product 15O. This method, which provides directly the astrophysically important total cross section, was never used for the 14N(p,gamma)15O cross section measurement in the studied energy range. The non-resonant cross section was measured between 550 keV and 1400 keV center-of-mass energies with total uncertainty of about 10%. The results were compared with literature data using an R-matrix analysis. It is found that the cross sections measured in this work are in acceptable agreement with the two recent measurements only if the weak transitions - not measured in those works - are included. The present data set, being largely independent from the other available data, can be used to constrain the extrapolated cross sections to astrophysical energies and helps to make the astrophysical model calculations more reliable., Comment: Accepted for publication in Phys. Rev. C as a letter

The synthesis of heavy, proton rich isotopes is a poorly understood astrophysical process. Thermonuclear (type Ia) supernova explosions are among the suggested sites and the abundance of some isotopes present in the early solar system may be used to test the models. 92Nb is such an isotope and one of the reactions playing a role in its synthesis is 91Zr(p,gamma)92Nb. As no experimental cross sections were available for this reaction so far, nucleosynthesis models had to solely rely on theoretical calculations. In the present work the cross section of 91Zr(p,gamma)92mNb has been measured at astrophysical energies by activation. The results excellently confirm the predictions of cross sections and reaction rates for 91Zr(p,gamma)92Nb, as used in astrophysical simulations., Comment: Accepted for publication in Journal of Physics G

The precise knowledge of the half-life of the reaction product is of crucial importance for a nuclear reaction cross section measurement carried out with the activation technique. The cross section of the $^{92}$Mo($\alpha$,n)$^{95}$Ru reaction was measured recently using this experimental approach. The preliminary results indicated that the literature half-life of $^{95}$Ru, derived about half a century ago, is overestimated. Therefore, the half-lives of $^{95}$Ru and its daughter isotope $^{95}$Tc and $^{95m}$Tc have been measured with high precision using $\gamma$-spectroscopy. The results are t$_{1/2}$=1.6033 $\pm$ 0.0044 h for $^{95}$Ru, t$_{1/2}$ = 19.258 $\pm$ 0.026 h for $^{95}$Tc and t$_{1/2}$ = 61.96 $\pm$ 0.24 d for $^{95m}$Tc. The precision of the half-life values has been increased, consequently the recently measured $^{92}$Mo($\alpha$,n)$^{95}$Ru activation cross section will become more precise.

Lighter heavy elements beyond iron and up to around silver can form in neutrino-driven ejecta in core-collapse supernovae and neutron star mergers. Slightly neutron-rich conditions favour a weak r-process that follows a path close to stability. Therefore, the beta decays are slow compared to the expansion time scales, and ($\alpha$,n) reactions become critical to move matter towards heavier nuclei. The rates of these reactions are calculated with the statistical model and their main uncertainty, at energies relevant for the weak r-process, is the $\alpha$+nucleus optical potential. There are several sets of parameters to calculate the $\alpha$+nucleus optical potential leading to large deviations for the reaction rates, exceeding even one order of magnitude. Recently the $^{96}$Zr($\alpha$,n)$^{99}$Mo reaction has been identified as a key reaction that impacts the production of elements from Ru to Cd. Here, we present the first cross section measurement of this reaction at energies (6.22 MeV $\leq$ E$_\mathrm{c.m.}$ $\leq$ 12.47 MeV) relevant for the weak r-process. The new data provide a stringent test of various model predictions which is necessary to improve the precision of the weak r-process network calculations. The strongly reduced reaction rate uncertainty leads to very well-constrained nucleosynthesis yields for $Z = 44 - 48$ isotopes under different neutrino-driven wind conditions.

The prediction of stellar ($\gamma$,$\alpha$) reaction rates for heavy nuclei is based on the calculation of ($\alpha$,$\gamma$) cross sections at sub-Coulomb energies. These rates are essential for modeling the nucleosynthesis of so-called $p$-nuclei. The standard calculations in the statistical model show a dramatic sensitivity to the chosen $\alpha$-nucleus potential. The present study explains the reason for this dramatic sensitivity which results from the tail of the imaginary $\alpha$-nucleus potential in the underlying optical model calculation of the total reaction cross section. As an alternative to the optical model, a simple barrier transmission model is suggested. It is shown that this simple model in combination with a well-chosen $\alpha$-nucleus potential is able to predict total $\alpha$-induced reaction cross sections for a wide range of heavy target nuclei above $A \gtrsim 150$ with uncertainties below a factor of two. The new predictions from the simple model do not require any adjustment of parameters to experimental reaction cross sections whereas in previous statistical model calculations all predictions remained very uncertain because the parameters of the $\alpha$-nucleus potential had to be adjusted to experimental data. The new model allows to predict the reaction rate of the astrophysically important $^{176}$W($\alpha$,$\gamma$)$^{180}$Os reaction with reduced uncertainties, leading to a significantly lower reaction rate at low temperatures. The new approach could also be validated for a broad range of target nuclei from $A \approx 60$ up to $A \gtrsim 200$., Comment: 6 pages, 3 figures; 6 pages supplement with 3 additional figures and 3 tables; Physical Review Letters, accepted for publication

Statistical model calculations have to be used for the determination of reaction rates in large-scale reaction networks for heavy-element nucleosynthesis. A basic ingredient of such a calculation is the a-nucleus optical model potential. Several different parameter sets are available in literature, but their predictions of a-induced reaction rates vary widely, sometimes even exceeding one order of magnitude. This paper presents the result of a-induced reaction cross-section measurements on gold which could be carried out for the first time very close to the astrophysically relevant energy region. The new experimental data are used to test statistical model predictions and to constrain the a-nucleus optical model potential. For the measurements the activation technique was used. The cross section of the (a,n) and (a,2n) reactions was determined from g-ray counting, while that of the radiative capture was determined via X-ray counting. The cross section of the reactions was measured below E$_a=20.0$~MeV. In the case of the $^{197}$Au(a,2n)$^{199}$Tl reaction down to 17.5~MeV with 0.5-MeV steps, reaching closer to the reaction threshold than ever before. The cross section of $^{197}$Au(a,n)$^{200}$Tl and $^{197}$Au(a,g)$^{201}$Tl was measured down to E$_a=13.6$ and 14.0~MeV, respectively, with 0.5-MeV steps above the (a,2n) reaction threshold and with 1.0-MeV steps below that. The new dataset is in agreement with the available values from the literature, but is more precise and extends towards lower energies. Two orders of magnitude lower cross sections were successfully measured than in previous experiments which used g-ray counting only, thus providing experimental data at lower energies than ever before. The new precision dataset allows us to find the best-fit a-nucleus optical model potential and to predict cross sections in the Gamow window with smaller uncertainties., Comment: Accepted for publication in Phys. Rev. C

The 14N(p,gamma)15O reaction plays a vital role in various astrophysical scenarios. Its reaction rate must be accurately known in the present era of high precision astrophysics. The cross section of the reaction is often measured relative to a low energy resonance, the strength of which must therefore be determined precisely. The activation method, based on the measurement of 15O decay, has not been used in modern measurements of the 14N(p,gamma)15O reaction. The aim of the present work is to provide strength data for two resonances in the 14N(p,gamma)15O reaction using the activation method. The obtained values are largely independent from previous data measured by in-beam gamma-spectroscopy and are free from some of their systematic uncertainties. Solid state TiN targets were irradiated with a proton beam provided by the Tandetron accelerator of Atomki using a cyclic activation. The decay of the produced 15O isotopes was measured by detecting the 511 keV positron annihilation gamma-rays. The strength of the Ep = 278 keV resonance was measured to be 13.4 +- 0.8 meV while for the Ep = 1058 keV resonance the strength is 442 +- 27 meV. The obtained Ep = 278 keV resonance strength is in fair agreement with the values recommended by two recent works. On the other hand, the Ep = 1058 keV resonance strength is about 20% higher than the previous value. The discrepancy may be caused in part by a previously neglected finite target thickness correction. As only the low energy resonance is used as a normalization point for cross section measurements, the calculated astrophysical reaction rate of the 14N(p,gamma)15O reaction and therefore the astrophysical consequences are not changed by the present results., Comment: Accepted for publication in Phys. Rev. C

The $^3$He($\alpha$,$\gamma$)$^7$Be reaction is a widely studied nuclear reaction; however, it is still not understood with the required precision. It has a great importance both in Big Bang nucleosynthesis and in solar hydrogen burning. The low mass number of the reaction partners makes it also suitable for testing microscopic calculations. Despite the high number of experimental studies, none of them addresses the $^3$He($\alpha$,$\gamma$)$^7$Be reaction cross sections above 3.1-MeV center-of-mass energy. Recently, a previously unobserved resonance in the $^6$Li(p,$\gamma$)$^7$Be reaction suggested a new level in $^7$Be, which would also have an impact on the $^3$He($\alpha$,$\gamma$)$^7$Be reaction in the energy range above 4.0 MeV. The aim of the present experiment is to measure the $^3$He($\alpha$,$\gamma$)$^7$Be reaction cross section in the energy range of the proposed level. For this investigation the activation technique was used. A thin window gas-cell target confining $^3$He gas was irradiated using an $\alpha$ beam. The $^7$Be produced was implanted into the exit foil. The $^7$Be activity was determined by counting the $\gamma$ rays following its decay by a well-shielded high-purity germanium detector. Reaction cross sections have been determined between $E_{cm} = 4.0 - 4.4$ MeV with 0.04-MeV steps covering the energy range of the proposed nuclear level. One lower-energy cross-section point was also determined to be able to compare the results with previous studies. A constant cross section of around 10.5 $\mu$barn was observed around the $^7$Be proton separation energy. An upper limit of 45 neV for the strength of a $^3$He($\alpha$,$\gamma$)$^7$Be resonance is derived., Comment: Accepted for publication in Physical Review C

In order to provide data for the simulation of the astrophysical $\gamma$-process, the cross section measurement of the $^{124}$Xe(p,$\gamma$)$^{125}$Cs reaction is in progress at MTA Atomki using the activation technique. Precise information on the decay characteristics of the reaction products is of crucial importance for measurements carried out using this method. The half-lives of the produced $^{125}$Cs and its daughter $^{125}$Xe are published in previous works, but with large uncertainties and ambiguous values. To make these nuclear parameters more precise, the half-lives have been re-measured with high precision using $\gamma$-spectroscopy. The obtained new half-life values are t$_{1/2}$ = 44.35 $\pm$ 0.29 minutes for $^{125}$Cs and t$_{1/2}$ = 16.87 $\pm$ 0.08 hours for $^{125}$Xe.

The literature half-life value of 65Ga is based on only one experiment carried out more than 60 years ago and it has a relatively large uncertainty. In the present work this half-life is determined based on the counting of the gamma-rays following the beta-decay of 65Ga. Our new recommended half-life is 15.133 +- 0.028 min which is in agreement with the literature value but almost one order of magnitude more precise.

The primary aim of experimental nuclear astrophysics is to determine the rates of nuclear reactions taking place in stars in various astrophysical conditions. These reaction rates are important ingredient for understanding the elemental abundance distribution in our solar system and the galaxy. The reaction rates are determined from the cross sections which need to be measured at energies as close to the astrophysically relevant ones as possible. In many cases the final nucleus of an astrophysically important reaction is radioactive which allows the cross section to be determined based on the off-line measurement of the number of produced isotopes. In general, this technique is referred to as the activation method, which often has substantial advantages over in-beam particle- or gamma-detection measurements. In this paper the activation method is reviewed from the viewpoint of nuclear astrophysics. Important aspects of the activation method are given through several reaction studies for charged particle, neutron and gamma-induced reactions. Various techniques for the measurement of the produced activity are detailed. As a special case of activation, the technique of Accelerator Mass Spectrometry in cross section measurements is also reviewed., Comment: Review paper accepted for publication in European Physical Journal A

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

Many choices are available in order to evaluate large radioactive decay networks. %multi-particle decay data. There are many parameters that influence the calculated $\beta$-decay delayed single and multi-neutron emission branching fractions. We describe assumptions about the decay model, background, and other parameters and their influence on $\beta$-decay delayed multi-neutron emission analysis. An analysis technique, the ORNL BRIKEN analysis procedure, for determining $\beta$-delayed multi-neutron branching ratios in $\beta$-neutron precursors produced by means of heavy-ion fragmentation is presented. The technique is based on estimating the initial activities of zero, one, and two neutrons occurring in coincidence with an ion-implant and $\beta$ trigger. The technique allows one to extract $\beta$-delayed multi-neutron decay branching ratios measured with the hybrid \textsuperscript{3}He BRIKEN neutron counter. As an example, two analyses of the $\beta$-neutron emitter \textsuperscript{77}Cu based on different {\it a priori} assumptions are presented along with comparisons to literature values., Comment: 21 pages, 10 figures

[Background] Alpha-nucleus optical potentials are basic ingredients of statistical model calculations used in nucleosynthesis simulations. While the nucleon+nucleus optical potential is fairly well known, for the alpha+nucleus optical potential several different parameter sets exist and large deviations, reaching sometimes even an order of magnitude, are found between the cross section predictions calculated using different parameter sets. [Purpose] A measurement of the radiative alpha-capture and the alpha-induced reaction cross sections on the nucleus 115In at low energies allows a stringent test of statistical model predictions. Since experimental data is scarce in this mass region, this measurement can be an important input to test the global applicability of alpha+nucleus optical model potentials and further ingredients of the statistical model. [Methods] The reaction cross sections were measured by means of the activation method. The produced activities were determined by off-line detection of the gamma-rays and characteristic x-rays emitted during the electron capture decay of the produced Sb isotopes. The 115In(alpha,gamma)119Sb and 115In(alpha,n)118Sbm reaction cross sections were measured between Ec.m. = 8.83 MeV - 15.58 MeV, and the 115In(alpha,n)118Sbg reaction was studied between Ec.m. = 11.10 MeV - 15.58 MeV. The theoretical analysis was performed within the statistical model.

The aim of the present work is to measure the $^{121}$Sb($\alpha,\gamma$)$^{125}$I, $^{121}$Sb($\alpha$,n)$^{124}$I, and $^{123}$Sb($\alpha$,n)$^{126}$I reaction cross sections. The $\alpha$-induced reactions on natural and enriched antimony targets were investigated using the activation technique. The ($\alpha$,$\gamma$) cross sections of $^{121}$Sb were measured and are reported for first time. To determine the cross section of the $^{121}$Sb($\alpha$,$\gamma$)$^{125}$I, $^{121}$Sb($\alpha$,n)$^{124}$I, and $^{123}$Sb($\alpha$,n)$^{126}$I reactions, the yields of $\gamma$-rays following the $\beta$-decay of the reaction products were measured. For the measurement of the lowest cross sections, the characteristic X-rays were counted with a LEPS (Low Energy Photon Spectrometer) detector. The cross section of the $^{121}$Sb($\alpha$,$\gamma$)$^{125}$I, $^{121}$Sb($\alpha$,n)$^{124}$I and $^{123}$Sb($\alpha$,n)$^{126}$I reactions were measured with high precision in an energy range between 9.74 MeV to 15.48 MeV, close to the astrophysically relevant energy window. The results are compared with the predictions of statistical model calculations. The ($\alpha$,n) data show that the $\alpha$ widths are predicted well for these reactions. The ($\alpha$,$\gamma$) results are overestimated by the calculations but this is due to the applied neutron- and $\gamma$ widths. Relevant for the astrophysical reaction rate is the $\alpha$ width used in the calculations.While for other reactions the $\alpha$ widths seem to have been overestimated and their energy dependence was not described well in the measured energy range, this is not the case for the reactions studied here. The result is consistent with the proposal that additional reaction channels, such as Coulomb excitation, may have led to the discrepancies found in other reactions.

In a recent work, the cross section measurement of the 64Zn(p,alpha)61Cu reaction was used to prove that the standard alpha-nucleus optical potentials used in astrophysical network calculation fail to reproduce the experimental data at energies relevant for heavy element nucleosynthesis. In the present paper the analysis of the obtained experimental data is continued by comparing the results with the predictions using different parameters. It is shown that the recently suggested modification of the standard optical potential leads to a better description of the data., Comment: Proceedings of the Nuclear Physics in Astrophysics VII conference, York, UK, 2015

The stellar reaction rates of radiative $\alpha$-capture reactions on heavy isotopes are of crucial importance for the $\gamma$ process network calculations. These rates are usually derived from statistical model calculations, which need to be validated, but the experimental database is very scarce. This paper presents the results of $\alpha$-induced reaction cross section measurements on iridium isotopes carried out at first close to the astrophysically relevant energy region. Thick target yields of $^{191}$Ir($\alpha$,$\gamma$)$^{195}$Au, $^{191}$Ir($\alpha$,n)$^{194}$Au, $^{193}$Ir($\alpha$,n)$^{196m}$Au, $^{193}$Ir($\alpha$,n)$^{196}$Au reactions have been measured with the activation technique between E$_\alpha = 13.4$ MeV and 17 MeV. For the first time the thick target yield was determined with X-ray counting. This led to a previously unprecedented sensitivity. From the measured thick target yields, reaction cross sections are derived and compared with statistical model calculations. The recently suggested energy-dependent modification of the $\alpha$+nucleus optical potential gives a good description of the experimental data., Comment: Accepted for publication in Physics Letters B

The 17O(p,g)18F reaction plays an important role in hydrogen burning processes in different stages of stellar evolution. The rate of this reaction must therefore be known with high accuracy in order to provide the necessary input for astrophysical models. The cross section of 17O(p,g)18F is characterized by a complicated resonance structure at low energies. Experimental data, however, is scarce in a wide energy range which increases the uncertainty of the low energy extrapolations. The purpose of the present work is therefore to provide consistent and precise cross section values in a wide energy range. The cross section is measured using the activation method which provides directly the total cross section. With this technique some typical systematic uncertainties encountered in in-beam gamma-spectroscopy experiments can be avoided. The cross section was measured between 500 keV and 1.8 MeV proton energies with a total uncertainty of typically 10%. The results are compared with earlier measurements and it is found that the gross features of the 17O(p,g)18F excitation function is relatively well reproduced by the present data. Deviation of roughly a factor of 1.5 is found in the case of the total cross section when compared with the only one high energy dataset. At the lowest measured energy our result is in agreement with two recent datasets within one standard deviation and deviates by roughly two standard deviations from a third one. An R-matrix analysis of the present and previous data strengthen the reliability of the extrapolated zero energy astrophysical S-factor. Using an independent experimental technique, the literature cross section data of 17O(p,g)18F is confirmed in the energy region of the resonances while lower direct capture cross section is recommended at higher energies. The present dataset provides a constraint for the theoretical cross sections., Comment: Accepted for publication in Phys. Rev. C. Abstract shortened in order to comply with arxiv rules

Background: alpha-nucleus potentials play an essential role for the calculation of alpha-induced reaction cross sections at low energies in the statistical model... Purpose: The present work studies the total reaction cross section sigma_reac of alpha-induced reactions at low energies which can be determined from the elastic scattering angular distribution or from the sum over the cross sections of all open non-elastic channels. Method: Elastic and inelastic 64Zn(a,a)64Zn angular distributions were measured at two energies around the Coulomb barrier at 12.1 MeV and 16.1 MeV. Reaction cross sections of the (a,g), (a,n), and (a,p) reactions were measured at the same energies using the activation technique. The contributions of missing non-elastic channels were estimated from statistical model calculations. Results: The total reaction cross sections from elastic scattering and from the sum of the cross sections over all open non-elastic channels agree well within the uncertainties. This finding confirms the consistency of the experimental data. At the higher energy of 16.1 MeV, the predicted significant contribution of compound-inelastic scattering to the total reaction cross section is confirmed experimentally. As a by-product it is found that most recent global alpha-nucleus potentials are able to describe the reaction cross sections for 64Zn around the Coulomb barrier. Conclusions: Total reaction cross sections of alpha-induced reactions can be well determined from elastic scattering angular distributions. The present study proves experimentally that the total cross section from elastic scattering is identical to the sum of non-elastic reaction cross sections. Thus, the statistical model can reliably be used to distribute the total reaction cross section among the different open channels., Comment: 15 pages, 12 figures, accepted for publication in Phys. Rev. C; abstract shortened due to arXiv limitations; revised submission: typo in Table III corrected; references updated

The synthesis of heavy, proton rich isotopes in the astrophysical gamma-process proceeds through photodisintegration reactions. For the improved understanding of the process, the rates of the involved nuclear reactions must be known. The reaction 128Ba(g,a)124Xe was found to affect the abundance of the p nucleus 124Xe. Since the stellar rate for this reaction cannot be determined by a measurement directly, the aim of the present work was to measure the cross section of the inverse 124Xe(a,g)128Ba reaction and to compare the results with statistical model predictions. Of great importance is the fact that data below the (a,n) threshold was obtained. Studying simultaneously the 124Xe(a,n)127Ba reaction channel at higher energy allowed to further identify the source of a discrepancy between data and prediction. The 124Xe + alpha cross sections were measured with the activation method using a thin window 124Xe gas cell. The studied energy range was between E = 11 and 15 MeV close above the astrophysically relevant energy range. The obtained cross sections are compared with statistical model calculations. The experimental cross sections are smaller than standard predictions previously used in astrophysical calculations. As dominating source of the difference, the theoretical alpha width was identified. The experimental data suggest an alpha width lower by at least a factor of 0.125 in the astrophysical energy range. An upper limit for the 128Ba(g,a)124Xe stellar rate was inferred from our measurement. The impact of this rate was studied in two different models for core-collapse supernova explosions of 25 solar mass stars. A significant contribution to the 124Xe abundance via this reaction path would only be possible when the rate was increased above the previous standard value. Since the experimental data rule this out, they also demonstrate the closure of this production path., Comment: Accepted for publication in Phys. Rev. C

In 2008 a Starting Grant project supported by the European Research Council titled "Nuclear reaction studies relevant to the astrophysical p-process nucleosynthesis" was launched. After five years of successful research related to the experimental investigation of proton- and alpha-induced nuclear reaction for the astrophysical p-process, the project came to an end. In this paper a summary of the research and the most important achievements is given., Comment: To appear in Journal of Physics: Conference Series, the proceedings of the Nuclear Physics in Astrophysics VI conference, Lisbon, Portugal, 2013. The version posted here is slightly modified compared to the published one

Alpha elastic scattering angular distributions of the 106Cd(alpha,alpha)106Cd reaction were measured at three energies around the Coulomb barrier to provide a sensitive test for the alpha + nucleus optical potential parameter sets. Furthermore, the new high precision angular distributions, together with the data available from the literature were used to study the energy dependence of the locally optimized {\alpha}+nucleus optical potential in a wide energy region ranging from E_Lab = 27.0 MeV down to 16.1 MeV. The potentials under study are a basic prerequisite for the prediction of alpha-induced reaction cross sections and thus, for the calculation of stellar reaction rates used for the astrophysical gamma process. Therefore, statistical model predictions using as input the optical potentials discussed in the present work are compared to the available 106Cd + alpha cross section data.

Astrophysical reaction rates, which are mostly derived from theoretical cross sections, are necessary input to nuclear reaction network simulations for studying the origin of $p$ nuclei. Past experiments have found a considerable difference between theoretical and experimental cross sections in some cases, especially for ($\alpha$,$\gamma$) reactions at low energy. Therefore, it is important to experimentally test theoretical cross section predictions at low, astrophysically relevant energies. The aim is to measure reaction cross sections of $^{107}$Ag($\alpha$,$\gamma$)$^{111}$In and $^{107}$Ag($\alpha$,n)$^{110}$In at low energies in order to extend the experimental database for astrophysical reactions involving $\alpha$ particles towards lower mass numbers. Reaction rate predictions are very sensitive to the optical model parameters and this introduces a large uncertainty into theoretical rates involving $\alpha$ particles at low energy. We have also used Hauser-Feshbach statistical model calculations to study the origin of possible discrepancies between prediction and data. An activation technique has been used to measure the reaction cross sections at effective center of mass energies between 7.79 MeV and 12.50 MeV. Isomeric and ground state cross sections of the ($\alpha$,n) reaction were determined separately. The measured cross sections were found to be lower than theoretical predictions for the ($\alpha$,$\gamma$) reaction. Varying the calculated averaged widths in the Hauser-Feshbach model, it became evident that the data for the ($\alpha$,$\gamma$) and ($\alpha$,n) reactions can only be simultaneously reproduced when rescaling the ratio of $\gamma$- to neutron width and using an energy-dependent imaginary part in the optical $\alpha$+$^{107}$Ag potential.......

The $\gamma$-process in core-collapse and/or type Ia supernova explosions is thought to explain the origin of the majority of the so-called $p$ nuclei (the 35 proton-rich isotopes between Se and Hg). Reaction rates for $\gamma$-process reaction network studies have to be predicted using Hauser-Feshbach statistical model calculations. Recent investigations have shown problems in the prediction of $\alpha$-widths at astrophysical energies which are an essential input for the statistical model. It has an impact on the reliability of abundance predictions in the upper mass range of the $p$ nuclei. With the measurement of the $^{164,166}$Er($\alpha$,n)$^{167,169}$Yb reaction cross sections at energies close to the astrophysically relevant energy range we tested the recently suggested low energy modification of the $\alpha$+nucleus optical potential in a mass region where $\gamma$-process calculations exhibit an underproduction of the $p$ nuclei. Using the same optical potential for the $\alpha$-width which was derived from combined $^{162}$Er($\alpha$,n) and $^{162}$Er($\alpha$,$\gamma$) measurement makes it plausible that a low-energy modification of the optical $\alpha$+nucleus potential is needed.

In the model calculations of heavy element nucleosynthesis processes the nuclear reaction rates are taken from statistical model calculations which utilize various nuclear input parameters. It is found that in the case of reactions involving alpha particles the calculations bear a high uncertainty owing to the largely unknown low energy alpha-nucleus optical potential. Experiments are typically restricted to higher energies and therefore no direct astrophysical consequences can be drawn. In the present work a (p,alpha) reaction is used for the first time to study the alpha-nucleus optical potential. The measured 64Zn(p,alpha)61Cu cross section is uniquely sensitive to the alpha-nucleus potential and the measurement covers the whole astrophysically relevant energy range. By the comparison to model calculations, direct evidence is provided for the incorrectness of global optical potentials used in astrophysical models., Comment: Accepted for publication in Physical Review C as a Rapid Communication

A measurement of total cross-section values of the $^{130}$Ba(p,$\gamma$)$^{131}$La reaction at low proton energies allows a stringent test of statistical model predictions with different proton+nucleus optical model potentials. Since no experimental data are available for proton-capture reactions in this mass region around A~$\approx$~130, this measurement can be an important input to test the global applicability of proton+nucleus optical model potentials. The total reaction cross-section values were measured by means of the activation method. After the irradiation with protons, the reaction yield was determined by use of $\gamma$-ray spectroscopy using two clover-type high-purity germanium detectors. In total, cross-section values for eight different proton energies could be determined in the energy range between 3.6 MeV $\leq E_p \leq$ 5.0 MeV, thus, inside the astrophysically relevant energy region. The measured cross-section values were compared to Hauser-Feshbach calculations using the statistical model codes TALYS and SMARAGD with different proton+nucleus optical model potentials. With the semi-microscopic JLM proton+nucleus optical model potential used in the SMARAGD code, the absolute cross-section values are reproduced well, but the energy dependence is too steep at the lowest energies. The best description is given by a TALYS calculation using the semi-microscopic Bauge proton+nucleus optical model potential using a constant renormalization factor., Comment: 7 pages, 6 figures

The cross sections of the 162Er(a,g,)166Yb and 162Er(a,n)165Yb reactions have been measured for the first time. The radiative alpha capture reaction cross section was measured from Ec.m. = 16.09 down to Ec.m. = 11.21 MeV, close to the astrophysically relevant region (which lies between 7.8 and 11.48 MeV at 3 GK stellar temperature). The 162Er(a,n)165Yb reaction was studied above the reaction threshold between Ec.m. = 12.19 and 16.09 MeV. The fact that the 162Er(a,g)166Yb cross sections were measured below the (a,n) threshold at first time in this mass region opens the opportunity to study directly the a-widths required for the determination of astrophysical reaction rates. The data clearly show that compound nucleus formation in this reaction proceeds differently than previously predicted.

For the better understanding of the astrophysical gamma-process the experimental determination of low energy proton- and alpha-capture cross sections on heavy isotopes is required. The existing data for the 92Mo(p,gamma)93Tc reaction are contradictory and strong fluctuation of the cross section is observed which cannot be explained by the statistical model. In this paper a new determination of the 92Mo(p,gamma)93Tc and 98Mo(p,gamma)99mTc cross sections based on thick target yield measurements are presented and the results are compared with existing data and model calculations. Reaction rates of 92Mo(p,gamma)93Tc at temperatures relevant for the gamma-process are derived directly from the measured thick target yields. The obtained rates are a factor of 2 lower than the ones used in astrophysical network calculations. It is argued that in the case of fluctuating cross sections the thick target yield measurement can be more suited for a reliable reaction rate determination., Comment: Accepted for publication in Nuclear Physics A

The elastic scattering cross sections for the reactions $^{110,116}$Cd($\alpha,\alpha$)$^{110,116}$Cd at energies above and below the Coulomb barrier are presented to provide a sensitive test for the alpha-nucleus optical potential parameter sets. Additional constraints for the optical potential are taken from the analysis of elastic scattering excitation functions at backward angles which are available in literature. Moreover, the variation of the elastic alpha scattering cross sections along the $Z = 48$ isotopic and $N = 62$ isotonic chain is investigated by the study of the ratios of the of $^{106,110,116}$Cd($\alpha,\alpha$)$^{106,110,116}$Cd scattering cross sections at E$_{c.m.} \approx$ 15.6 and 18.8 MeV and the ratio of the $^{110}$Cd($\alpha,\alpha$)$^{110}$Cd and $^{112}$Sn($\alpha,\alpha$)$^{112}$Sn reaction cross sections at E$_{c.m.} \approx$ 18.8 MeV, respectively. These ratios are sensitive probes for the alpha-nucleus optical potential parameterizations. The potentials under study are a basic prerequisite for the prediction of $\alpha$-induced reaction cross sections, e.g.\ for the calculation of stellar reaction rates in the astrophysical $p$- or $\gamma$-process.

The $\gamma$ process in supernova explosions is thought to explain the origin of proton-rich isotopes between Se and Hg, the so-called $p$ nuclei. The majority of the reaction rates for $\gamma$ process reaction network studies has to be predicted in Hauser-Feshbach statistical model calculations using global optical potential parameterizations. While the nucleon+nucleus optical potential is fairly known, for the $\alpha$+nucleus optical potential several different parameterizations exist and large deviations are found between the predictions calculated using different parameter sets. By the measurement of elastic $\alpha$-scattering angular distributions at energies around the Coulomb barrier a comprehensive test for the different global $\alpha$+nucleus optical potential parameter sets is provided. Between 20$^{\circ}$ and 175$^{\circ}$ complete elastic alpha scattering angular distributions were measured on the $^{113}$In \textit{p} nucleus with high precision at E$_{c.m.}$ = 15.59 and 18.82 MeV. The elastic scattering cross sections of the $^{113}$In($\alpha$,$\alpha$)$^{113}$In reaction were measured for the first time at energies close to the astrophysically relevant energy region. The high precision experimental data were used to evaluate the predictions of the recent global and regional $\alpha$+nucleus optical potentials. Parameters for a local $\alpha$+nucleus optical potential were derived from the measured angular distributions. Predictions for the reaction cross sections of $^{113}$In($\alpha,\gamma$)$^{117}$Sb and $^{113}$In($\alpha$,n)$^{116}$Sb at astrophysically relevant energies were given using the global and local optical potential parameterizations.

Cross sections for the 168Yb(alpha,gamma)172Hf and 168Yb(alpha,n)171$Hf reactions were measured by means of the activation method using alpha particles with energies between 12.9 MeV and 15.1 MeV. The spectroscopy of the gamma rays emitted by the reaction products was performed using three different HPGe detector types, namely clover-type high-purity germanium detectors, a low-energy photon spectrometer detector, and a coaxial high-purity germanium detector. The results were compared to Hauser-Feshbach statistical model calculations. Within certain assumptions, astrophysical conclusions could be drawn concerning the production of the p nucleus 168Yb. The data in this work can serve as a contribution to the current very fragmentary experimental data base for charged-particle induced reactions. In addition, the absolute intensity for nine gamma-ray transitions following the electron capture decay of 171Hf could be derived., Comment: 21 pages, 9 figures, published in Nucl. Phys. A

The astrophysically important 3He(a,g)7Be reaction was studied at high energies where the available experimental data are in contradiction. A thin window 3He gas cell was used and the cross section was measured with the activation method. The obtained cross sections at energies between Ec.m. = 1.5 and 2.5 MeV are compared with the available data and theoretical calculations. The present results support the validity of the high energy cross section energy dependence observed by recent experiments., Comment: 16 pages, 5 figures

High precision angular distribution data of ($\alpha$,$\alpha$) elastic scattering are presented for the nuclei $^{89}$Y, $^{92}$Mo, $^{106,110,116}$Cd, $^{112,124}$Sn, and $^{144}$Sm at energies around the Coulomb barrier. Such data with small experimental uncertainties over the full angular range (20-170 degrees) are the indispensable prerequisite for the extraction of local optical potentials and for the determination of the total reaction cross section $\sigma_{\rm{reac}}$. A systematic fitting procedure was applied to the presented experimental scattering data to obtain comprehensive local potential parameter sets which are composed of a real folding potential and an imaginary potential of Woods-Saxon surface type. The obtained potential parameters were used in turn to construct a new systematic $\alpha$-nucleus potential with very few parameters. Although this new potential cannot reproduce the angular distributions with the same small deviations as the local potential, the new potential is able to predict the total reaction cross sections for all cases under study., Comment: 41 pages, 2+3 figures, 3+17 tables, At. Data Nucl. Data Tables, accepted for publication

The total reaction cross section is related to the elastic scattering angular distribution by a basic quantum-mechanical relation. We present new experimental data for alpha-induced reaction cross sections on 64Zn which allow for the first time the experimental verification of this simple relation at low energies by comparison of the new experimental reaction data to the result obtained from 64Zn(alpha,alpha)64Zn elastic scattering., Comment: Accepted for publication in Phys. Rev. C as Rapid Communication