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2. alpha-Benzoin Oxime in Higher Oxidation State 3d Metal Cluster Chemistry: Structural and Magnetic Study of a New Mn-9(III) Complex

Author

Koumousi, E. S., Manos, M. J., Lampropoulos, C., Tasiopoulos, A. J., Wernsdorfer, W., Christou, G., and Stamatatos, T. C.

Subjects
carboxylate, manganese clusters, ligands, high-spin molecules, single-molecule magnets
Abstract

The initial employment of alpha-benzoin oxime (bzoxH(2)) in higher oxidation state 3d metal cluster chemistry has provided access to a new enneanuclear Mn-III complex with an unprecedented metal-core topology consisting of two triangular [Mn-3(mu(3)-O2-)(mu-ON)(3)](4+) fragments connected by a linear [Mn-3(mu-ON)(6)](3+) unit. The Mn-9(III) cluster is antiferromagnetically coupled and has an S=3 spin ground state. Inorg Chem

Published
2010

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