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Spin ensembles play a pivotal role in various quantum applications such as metrology and simulating many-body physics. Recent research has proposed utilizing spin cat states to encode logical quantum information, with potentially logical lifetimes on the order of seconds via enhanced collective interactions that scale with system size. We investigate the dynamics of spin cat states under inhomogeneous broadening, revealing a phenomenon termed `parity-sensitive inhomogeneous dephasing': odd cat states are significantly more susceptible to inhomogeneous dephasing compared to even cat states due to parity symmetry. Additionally, from a mean-field analysis of the driven-dissipative dynamics, we identify a synchronization phase transition wherein the ensemble becomes completely dephased beyond a critical inhomogeneous linewidth. Our findings shed light on the stability of collective spin states, important for advancing quantum technologies., Comment: 10 pages, 4 figures

The optimization of system parameters is a ubiquitous problem in science and engineering. The traditional approach involves setting to zero the partial derivatives of the objective function with respect to each parameter, in order to extract the optimal solution. However, the system parameters often take the form of complex matrices. In such situations, conventional methods become unwieldy. The `Wirtinger Calculus' provides a relatively simple methodology for such optimization problems. In this tutorial, we provide a pedagogical introduction to Wirtinger Calculus. To illustrate the utility of this framework in quantum information theory, we also discuss a few example applications., Comment: Comments are most welcome

Amplification (mitigation) is the increase (decrease) in the change of thermodynamic quantities when an initial thermal state is thermalized to a different temperature in the presence of constraints, studied thus far only for permutationally invariant baths. In this manuscript, we generalize amplification and mitigation to accommodate generic strong symmetries of open quantum systems and connect the phenomenon to Landauer's erasure. We exemplify our general theory with a new bath-induced battery charging protocol that overcomes the passivity of KMS-preserving transitions., Comment: Harshank Shrotriya and Midhun Krishna contributed equally, 8 pages, comments welcome

Reducing noise in quantum systems is a major challenge towards the application of quantum technologies. Here, we propose and demonstrate a scheme to reduce noise using a quantum autoencoder with rigorous performance guarantees. The quantum autoencoder learns to compresses noisy quantum states into a latent subspace and removes noise via projective measurements. We find various noise models where we can perfectly reconstruct the original state even for high noise levels. We apply the autoencoder to cool thermal states to the ground state and reduce the cost of magic state distillation by several orders of magnitude. Our autoencoder can be implemented using only unitary transformations without ancillas, making it immediately compatible with the state of the art. We experimentally demonstrate our methods to reduce noise in a photonic integrated circuit. Our results can be directly applied to make quantum technologies more robust to noise.

In the modern financial industry system, the structure of products has become more and more complex, and the bottleneck constraint of classical computing power has already restricted the development of the financial industry. Here, we present a photonic chip that implements the unary approach to European option pricing, in combination with the quantum amplitude estimation algorithm, to achieve a quadratic speedup compared to classical Monte Carlo methods. The circuit consists of three modules: a module loading the distribution of asset prices, a module computing the expected payoff, and a module performing the quantum amplitude estimation algorithm to introduce speed-ups. In the distribution module, a generative adversarial network is embedded for efficient learning and loading of asset distributions, which precisely capture the market trends. This work is a step forward in the development of specialized photonic processors for applications in finance, with the potential to improve the efficiency and quality of financial services., Comment: 11 pages, 7 figures

Quantum Federated Learning (QFL) is an emerging interdisciplinary field that merges the principles of Quantum Computing (QC) and Federated Learning (FL), with the goal of leveraging quantum technologies to enhance privacy, security, and efficiency in the learning process. Currently, there is no comprehensive survey for this interdisciplinary field. This review offers a thorough, holistic examination of QFL. We aim to provide a comprehensive understanding of the principles, techniques, and emerging applications of QFL. We discuss the current state of research in this rapidly evolving field, identify challenges and opportunities associated with integrating these technologies, and outline future directions and open research questions. We propose a unique taxonomy of QFL techniques, categorized according to their characteristics and the quantum techniques employed. As the field of QFL continues to progress, we can anticipate further breakthroughs and applications across various industries, driving innovation and addressing challenges related to data privacy, security, and resource optimization. This review serves as a first-of-its-kind comprehensive guide for researchers and practitioners interested in understanding and advancing the field of QFL., Comment: Survey of quantum federated learning (QFL)

Quantum synchronization has emerged as a crucial phenomenon in quantum nonlinear dynamics with potential applications in quantum information processing. Multiple measures for quantifying quantum synchronization exist. However, there is currently no widely agreed metric that is universally adopted. In this paper, we propose using classical and quantum Fisher information (FI) as alternative metrics to detect and measure quantum synchronization. We establish the connection between FI and quantum synchronization, demonstrating that both classical and quantum FI can be deployed as more general indicators of quantum phase synchronization, in some regimes where all other existing measures fail to provide reliable results. We show advantages in FI-based measures, especially in 2-to-1 synchronization. Furthermore, we analyze the impact of noise on the synchronization measures, revealing the robustness and susceptibility of each method in the presence of dissipation and decoherence. Our results open up new avenues for understanding and exploiting quantum synchronization., Comment: 9 pages, 12 figures

Quantum entanglement serves as an important resource for quantum processing. In the original thought experiment of the Quantum Cheshire Cat, the physical properties of the cat (state) can be decoupled from its quantum entities. How do quantum entanglement and weak values affect such thought experiment? Here, we conceive a new thought experiment that exploits quantum entanglement with weak (value) measurement. Specifically, we ask: can two entangled particles exchange physical and quantum properties? We answer the question in the affirmative.

Quantum synchronization has been a central topic in quantum nonlinear dynamics. Despite rapid development in this field, very few have studied how to efficiently boost synchronization. Homodyne measurement emerges as one of the successful candidates for this task, but preferably in the semi-classical regime. In our work, we focus on the phase synchronization of a harmonic-driven quantum Stuart-Landau oscillator, and show that the enhancement induced by homodyne measurement persists into the quantum regime. Interestingly, optimal two-photon damping rates exist when the oscillator and driving are at resonance and with a small single-photon damping rate. We also report noise-induced enhancement in quantum synchronization when the single-photon damping rate is sufficiently large. Apart from these results, we discover that adding a squeezing Hamiltonian can further boost synchronization, especially in the semi-classical regime. Furthermore, the addition of squeezing causes the optimal two-photon pumping rates to shift and converge., Comment: 6 pages, 8 figures

We propose a natural application of Quantum Linear Systems Problem (QLSP) solvers such as the HHL algorithm to efficiently prepare highly excited interior eigenstates of physical Hamiltonians in a variational and targeted manner. This is enabled by the efficient computation of the expectation values of inverse Hamiltonians on quantum computers, in situations where Hamiltonian simulation and the representation of eigenstates on quantum computers are efficient. Importantly, the usage of the QLSP solver as a subroutine within our algorithm -- with its inputs and outputs corresponding to physically meaningful objects such as Hamiltonians and eigenstates arising from physical systems -- does not conceal exponentially costly pre/post-processing steps that usually accompanies it in generic linear algebraic applications. We detail implementations of this scheme for both fault-tolerant and near-term quantum computers, analyze their efficiency and implementability, and detail conditions under which the QLSP solvers' exponentially better scaling in problem size render it advantageous over existing classical and quantum approaches. Simulation results for applications in many-body physics and quantum chemistry further demonstrate its effectiveness and scalability over existing approaches., Comment: 16 pages, 6 figures

A paradigm for quantum synchronization is the quantum analog of the Stuart--Landau oscillator, which corresponds to a van der Pol oscillator in the limit of weak (i.e. vanishingly small) nonlinearity. Due to this limitation, the quantum Stuart--Landau oscillator fails to capture interesting nonlinearity-induced phenomena such as relaxation oscillations. To overcome this deficiency we propose an alternative model which approximates the van der Pol oscillator to finitely large nonlinearities while remaining numerically tractable. This allows us to uncover interesting phenomena in the deep-quantum strongly-nonlinear regime with no classical analog, such as the persistence of amplitude death on resonance. We also report nonlinearity-induced position correlations in reactively coupled quantum oscillators. Such coupled oscillations become more and more correlated with increasing nonlinearity before reaching some maximum. Again, this behavior is absent classically. We also show how strong nonlinearity can enlarge the synchronization bandwidth in both single and coupled oscillators. This effect can be harnessed to induce mutual synchronization between two oscillators initially in amplitude death., Comment: 13 pages, 8 figures

MNDO-based semiempirical methods in quantum chemistry have found widespread application in the modelling of large and complex systems. A method for the analytic evaluation of first and second derivatives of molecular properties against semiempirical parameters in MNDO-based NDDO-descendant models is presented, and the resultant parameter Hessian is compared against the approximant currently used in parameterization for the PMx models. As a proof of concept, the exact parameter Hessian is employed in a limited reparameterization of MNDO for the elements C, H, N, O and F using 1206 molecules for reference data., Comment: 18 pages; remainder is supplementary information

Photon-mediated interactions within an excited ensemble of emitters can result in Dicke superradiance, where the emission rate is greatly enhanced, manifesting as a high-intensity burst at short times. The superradiant burst is most commonly observed in systems with long-range interactions between the emitters, although the minimal interaction range remains unknown. Here, we put forward a new theoretical method to bound the maximum emission rate by upper bounding the spectral radius of an auxiliary Hamiltonian. We harness this tool to prove that for an arbitrary ordered array with only nearest-neighbor interactions in all dimensions, a superradiant burst is not physically observable. We show that Dicke superradiance requires minimally the inclusion of next-nearest-neighbor interactions. For exponentially decaying interactions, the critical coupling is found to be asymptotically independent of the number of emitters in all dimensions, thereby defining the threshold interaction range where the collective enhancement balances out the decoherence effects. Our findings provide key physical insights to the understanding of collective decay in many-body quantum systems, and the designing of superradiant emission in physical systems for applications such as energy harvesting and quantum sensing., Comment: 5 pages, 4 figures

Digital quantum computers have the potential to simulate complex quantum systems. The spin-boson model is one of such systems, used in disparate physical domains. Importantly, in a number of setups, the spin-boson model is open, i.e. the system is in contact with an external environment which can, for instance, cause the decay of the spin state. Here we study how to simulate such open quantum dynamics in a digital quantum computer, for which we use one of IBM's hardware. We consider in particular how accurate different implementations of the evolution result as a function of the level of noise in the hardware and of the parameters of the open dynamics. For the regimes studied, we show that the key aspect is to simulate the unitary portion of the dynamics, while the dissipative part can lead to a more noise-resistant simulation. We consider both a single spin coupled to a harmonic oscillator, and also two spins coupled to the oscillator. In the latter case, we show that it is possible to simulate the emergence of correlations between the spins via the oscillator.

It is known that the superposition of two bound states in the continuum (BIC) leads to the phenomenon of an oscillating bound state, where excitations mediated by the continuum modes oscillate persistently. We perform exact calculations for the oscillating BICs in a 1D photonic lattice coupled to a "giant atom" at multiple points. Our work is significantly distinct from previous proposals of oscillating BICs in continuous waveguide systems due to the presence of a finite energy band contributing band-edge effects. In particular, we show that the bound states outside the energy band are detrimental to the oscillating BIC phenomenon, and can be suppressed by increasing either the number of coupling points or the separation between each coupling point. Crucially, non-Markovianity is necessary for the existence of oscillating BIC, and the oscillation amplitude increases with the characteristic delay time of the giant atom interactions. We also propose a novel initialization scheme in the BIC subspace. Our work be experimentally implemented on current photonic waveguide array platforms and opens up new prospects in utilizing reservoir engineering for the storage of quantum information in photonic lattices., Comment: 20 pages, 8 figures

Periodic driving has the longstanding reputation for generating exotic phases of matter with no static counterparts. This work explores the interplay among periodic driving, interaction effects, and $\mathbb{Z}_2$ symmetry that leads to the emergence of Floquet symmetry protected second-order topological phases in a simple but insightful two-dimensional spin-1/2 lattice. Through a combination of analytical and numerical treatments, we verify the formation of 0 and $\pi$ modes, i.e., corner localized $\mathbb{Z}_2$ symmetry broken operators that respectively commute and anticommute with the one-period time evolution operator. We further verify the topological nature of these modes by demonstrating their presence over a wide range of parameter values and explicitly deriving their associated topological invariants under special conditions. Finally, we propose a means to detect the signature of such modes in experiments and discuss the effect of imperfections., Comment: 16 pages, 10 figures. Comments are most welcome

Self-testing has been established as a major approach for quantum device certification based on experimental statistics under minimal assumptions. However, despite more than 20 years of research effort most of the self-testing protocols are restricted to spatial scenarios (Bell scenarios), without any temporal generalisations known. Under the scenario of sequential measurements performed on a single quantum system, we build upon previous works which used semi-definite programming (SDP) based methods to bound sequential measurement inequalities. For such SDPs, we show that the optimiser matrix is unique and moreover this uniqueness is robust to small deviations from the quantum bound. Further, we consider a generalised scenario in presence of quantum channels and draw analogies in the structure of Bell and sequential inequalities using the pseudo-density matrix formalism. These analogies allow us to show a practical use of maximal violations of sequential inequalities in the form of certification of quantum channels up to isometries., Comment: 12 pages; comments welcome

The calculation of off-diagonal matrix elements has various applications in fields such as nuclear physics and quantum chemistry. In this paper, we present a noisy intermediate scale quantum algorithm for estimating the diagonal and off-diagonal matrix elements of a generic observable in the energy eigenbasis of a given Hamiltonian. Several numerical simulations indicate that this approach can find many of the matrix elements even when the trial functions are randomly initialized across a wide range of parameter values without, at the same time, the need to prepare the energy eigenstates.

We study a multi-functional device for cold atoms consisting of a three-terminal ring circuit pierced by a synthetic magnetic flux, where the ring can be continuous or discretized. The flux controls the atomic current through the ring via the Aharonov-Bohm effect. Our device shows a flux-induced transition of reflections from an Andreev-like negative density to positive density. Further, the flux can direct the atomic current into specific output ports, realizing a flexible non-reciprocal switch to connect multiple atomic systems or sense rotations. By changing the flux linearly in time, we convert constant matter wave currents into an AC modulated current. This effect can be used to realize an atomic frequency generator and study fundamental problems related to the Aharonov-Bohm effect. We experimentally demonstrate Bose-Einstein condensation into the light-shaped optical potential of the three-terminal ring. Our work opens up the possibility of novel atomtronic devices for practical applications in quantum technologies., Comment: 17 pages, 11 figures

Finding the transient and steady state properties of open quantum systems is a central problem in various fields of quantum technologies. Here, we present a quantum-assisted algorithm to determine the steady states of open system dynamics. By reformulating the problem of finding the fixed point of Lindblad dynamics as a feasibility semidefinite program, we bypass several well-known issues with variational quantum approaches to solving for steady states. We demonstrate that our hybrid approach allows us to estimate the steady states of higher dimensional open quantum systems and discuss how our method can find multiple steady states for systems with symmetries., Comment: 14 pages, 4 figures

Certifying individual quantum devices with minimal assumptions is crucial for the development of quantum technologies. Here, we investigate how to leverage single-system contextuality to realize self-testing. We develop a robust self-testing protocol based on the simplest contextuality witness for the simplest contextual quantum system, the Klyachko-Can-Binicio\u{g}lu-Shumovsky (KCBS) inequality for the qutrit. We establish a lower bound on the fidelity of the state and the measurements (to an ideal configuration) as a function of the value of the witness under a pragmatic assumption on the measurements we call the KCBS orthogonality condition. We apply the method in an experiment with randomly chosen measurements on a single trapped $^{40}{\rm Ca}^+$ and near-perfect detection efficiency. The observed statistics allow us to self-test the system and provide the first experimental demonstration of quantum self-testing of a single system. Further, we quantify and report that deviations from our assumptions are minimal, an aspect previously overlooked by contextuality experiments., Comment: 19+6 pages, 2+1 figures

Machine learning methods have revolutionized the discovery process of new molecules and materials. However, the intensive training process of neural networks for molecules with ever-increasing complexity has resulted in exponential growth in computation cost, leading to long simulation time and high energy consumption. Photonic chip technology offers an alternative platform for implementing neural networks with faster data processing and lower energy usage compared to digital computers. Photonics technology is naturally capable of implementing complex-valued neural networks at no additional hardware cost. Here, we demonstrate the capability of photonic neural networks for predicting the quantum mechanical properties of molecules. To the best of our knowledge, this work is the first to harness photonic technology for machine learning applications in computational chemistry and molecular sciences, such as drug discovery and materials design. We further show that multiple properties can be learned simultaneously in a photonic chip via a multi-task regression learning algorithm, which is also the first of its kind as well, as most previous works focus on implementing a network in the classification task.

Uncertainty and disturbance are two most fundamental properties of a quantum measurement and they are usually separately studied in terms of the preparation and the measurement uncertainty relations. Here we shall establish an intimate connection between them that goes beyond the above mentioned two kinds of uncertainty relations. Our basic observation is that the disturbance of one measurement to a subsequent measurement, which can be quantified based on observed data, sets lower-bounds to uncertainty. This idea can be universally applied to various measures of uncertainty and disturbance, with the help of data processing inequality. The obtained relations, referred to as disturbance enhanced uncertainty relations, immediately find various applications in the field of quantum information. They ensure preparation uncertainty relation such as novel entropic uncertainty relations independent of the Maassen and Uffink relation. And they also result in a simple protocol to estimate coherence. We anticipate that this new twist on uncertainty principle may shed new light on quantum foundations and may also inspire further applications in the field of quantum information.

Geometric and holonomic quantum computation utilizes intrinsic geometric properties of quantum-mechanical state spaces to realize quantum logic gates. Since both geometric phases and quantum holonomies are global quantities depending only on the evolution paths of quantum systems, quantum gates based on them possess built-in resilience to certain kinds of errors. This review provides an introduction to the topic as well as gives an overview of the theoretical and experimental progress for constructing geometric and holonomic quantum gates and how to combine them with other error-resistant techniques., Comment: added a new section "experimental realizations and gates robustness", updated the section on "Combining GQC and HQC with other quantum technologies" with 80 more references

Atomtronics is an emerging field that aims to manipulate ultracold atom moving in matter wave circuits for both fundamental studies in quantum science and technological applications. In this colloquium, we review recent progress in matter-wave circuitry and atomtronics-based quantum technology. After a short introduction to the basic physical principles and the key experimental techniques needed to realize atomtronic systems, we describe the physics of matter-waves in simple circuits such as ring traps and two-terminal systems. The main experimental observations and outstanding questions are discussed. We also present possible applications to a broad range of quantum technologies, from quantum sensing with atom interferometry to future quantum simulation and quantum computation architectures., Comment: 33 revtex pages; 10 figs. To be published in Reviews of Modern Physics

It is known that strong disorder in closed quantum systems leads to many-body localization (MBL), and that this quantum phase can be destroyed by coupling to an infinitely large Markovian environment. However, the stability of the MBL phase is less clear when the system and environment are of finite and comparable size. Here, we study the stability and eventual localization properties of a disordered Heisenberg spin chain coupled to a finite environment, and extensively explore the effects of environment disorder, geometry, initial state and system-bath coupling strength. By studying the non-equilibrium dynamics and the eventual steady-state properties of different initial states, our numerical results indicate that in most cases, the system retains its localization properties despite the coupling to the finite environment, albeit to a reduced extent. However, in cases where the system and environment is strongly coupled in the ladder configuration, the eventual localization properties are highly dependent on the initial state, and could lead to either thermalization or localization.

Semidefinite programs (SDPs) are convex optimization programs with vast applications in control theory, quantum information, combinatorial optimization and operational research. Noisy intermediate-scale quantum (NISQ) algorithms aim to make an efficient use of the current generation of quantum hardware. However, optimizing variational quantum algorithms is a challenge as it is an NP-hard problem that in general requires an exponential time to solve and can contain many far from optimal local minima. Here, we present a current term NISQ algorithm for solving SDPs. The classical optimization program of our NISQ solver is another SDP over a lower dimensional ansatz space. We harness the SDP based formulation of the Hamiltonian ground state problem to design a NISQ eigensolver. Unlike variational quantum eigensolvers, the classical optimization program of our eigensolver is convex, can be solved in polynomial time with the number of ansatz parameters and every local minimum is a global minimum. We find numeric evidence that NISQ SDP can improve the estimation of ground state energies in a scalable manner. Further, we efficiently solve constrained problems to calculate the excited states of Hamiltonians, find the lowest energy of symmetry constrained Hamiltonians and determine the optimal measurements for quantum state discrimination. We demonstrate the potential of our approach by finding the largest eigenvalue of up to $2^{1000}$ dimensional matrices and solving graph problems related to quantum contextuality. We also discuss NISQ algorithms for rank-constrained SDPs. Our work extends the application of NISQ computers onto one of the most successful algorithmic frameworks of the past few decades., Comment: 16 pages, 9 figures

Universal quantum entangling gates are a crucial building block in the large-scale quantum computation and quantum communication, and it is an important task to find simple ways to implement them. Here an effective quantum circuit for the implementation of a controlled-NOT (CNOT) gate is constructed by introducing a non-computational quantum state in the auxiliary space. Furthermore, the method is extended to the construction of a general n-control-qubit Toffoli gate with (2n-1) qubit-qudit gates and (2n-2) single-qudit gates. Based on the presented quantum circuits, the polarization CNOT and Toffoli gates with linear optics are designed by operating on the spatial-mode degree of freedom of photons. The proposed optical schemes can be achieved with a higher success probability and no extra auxiliary photons are needed., Comment: 13 pages,7 figures,1 table