Search

Single-crystal europium iron garnet (EuIG) thin films epitaxially strain-grown on gadolinium gallium garnet (GGG)(100) substrates using off-axis sputtering have strain-induced perpendicular magnetic anisotropy (PMA). By varying the sputtering conditions, we have tuned the europium/iron (Eu/Fe) composition ratios in the films to tailor the film strains. The films exhibited an extremely smooth, particle-free surface with roughness as low as 0.1 nm as observed using atomic force microscopy. High-resolution x-ray diffraction analysis and reciprocal space maps showed in-plane epitaxial film growth, very smooth film/substrate interface, excellent film crystallinity with a small full width at half maximum of 0.012$^{\circ}$ in the rocking curve scans, and an in-plane compressive strain without relaxation. In addition, spherical aberration-corrected scanning transmission electron microscopy showed an atomically abrupt interface between the EuIG film and GGG. The measured squarish out-of-plane magnetization-field hysteresis loops by vibrating sample magnetometry in conjunction with the measurements from angle-dependent x-ray magnetic dichroism demonstrated the PMA in the films. We have tailored the magnetic properties of the EuIG thin films, including saturation magnetization ranging from 71.91 to 124.51 emu/c.c. (increase with the (Eu/Fe) ratios), coercive field from 27 to 157.64 Oe, and the strength of PMA field ($H_\bot$) increasing from 4.21 to 18.87 kOe with the in-plane compressive strain from -0.774 to -1.044%. We have also investigated spin transport in Pt/EuIG bi-layer structure and evaluated the real part of spin mixing conductance to be $3.48\times10^{14} {\Omega}^{-1}m^{-2}$. We demonstrated the current-induced magnetization switching with a low critical switching current density of $3.5\times10^6 A/cm^2$, showing excellent potential for low-dissipation spintronic devices., Comment: 29 pages, 9 figures, 1 table

Transport signatures of exchange gap opening because of magnetic proximity effect (MPE) are reported for bilayer structures of Bi2Se3 thin films on yttrium iron garnet (YIG) and thulium iron garnet (TmIG) of perpendicular magnetic anisotropy (PMA). Pronounced negative magnetoresistance (MR) was detected, and attributed to an emergent weak localization (WL) effect superimposing on a weak antilocalization (WAL). Thickness-dependent study shows that the WL originates from the time-reversal-symmetry breaking of topological surface states by interfacial exchange coupling. The weight of WL declined when the interfacial magnetization was aligned toward the in-plane direction, which is understood as the effect of tuning the exchange gap size by varying the perpendicular magnetization component. Importantly, magnetotransport study revealed anomalous Hall effect (AHE) of square loops and anisotropic magnetoresistance (AMR) characteristic, typifying a ferromagnetic conductor in Bi2Se3/TmIG, and the presence of an interfacial ferromagnetism driven by MPE. Coexistence of MPE-induced ferromagnetism and the finite exchange gap provides an opportunity of realizing zero magnetic-field dissipation-less transport in topological insulator/ferromagnetic insulator heterostructures., Comment: 31 pages, 9 figures

The integration of quantum materials like topological insulators (TIs) with magnetic insulators (MIs) has important technological implications for spintronics and quantum computing. Here we report excellent crystallinity of c-axis oriented epitaxial TI films Bi2Se3 grown on MI films, a rare earth iron garnet (ReIG), such as thulium iron garnet (Tm3Fe5O12, TmIG) by molecular beam epitaxy (MBE) with a Se-buffered low-temperature (SBLT) growth technique. We demonstrated a streaky reflection high-energy electron diffraction pattern starting from the very first quintuple layer of Bi2Se3, indicating the high-quality interface between TmIG and Bi2Se3, a prerequisite for studying interfacial exchange coupling effects. The strong interfacial exchange interaction was manifested by observations of anomalous Hall effect in the Bi2Se3/TmIG bilayer and a shift of ferromagnetic resonance field of TmIG induced by Bi2Se3. We have reproducibly grown high-quality Bi2Se3/ReIG and interfaces using this new TI growth method, which may be applied to grow other types of van der Waals (vdW) hetero-structures., Comment: 17 pages, 4 figures

We report strong interfacial exchange coupling in Bi2Se3/yttrium iron garnet (YIG) bilayers manifested as large in-plane interfacial magnetic anisotropy (IMA) and enhancement of damping probed by ferromagnetic resonance (FMR). The IMA and spin mixing conductance reached a maximum when Bi2Se3 was around 6 quintuple-layer (QL) thick. The unconventional Bi2Se3 thickness dependence of the IMA and spin mixing conductance are correlated with the evolution of surface band structure of Bi2Se3, indicating that topological surface states play an important role in the magnetization dynamics of YIG. Temperature-dependent FMR of Bi2Se3/YIG revealed signatures of magnetic proximity effect of $T_c$ as high as 180 K, and an effective field parallel to the YIG magnetization direction at low temperature. Our study sheds light on the effects of topological insulators on magnetization dynamics, essential for development of TI-based spintronic devices., Comment: 16 pages, 4 figures, supplemental material