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Pair-breaking edges of $d$-wave superconductors feature Andreev bound states at the Fermi energy. Since these states are energetically highly unfavorable they are susceptible to effects that shift them to finite energy. We investigate the free energy of two different mechanisms: spontaneous phase gradients in the superconducting order parameter and surface ferromagnetism caused by Fermi liquid interaction effects. We find that the surface magnetization appears at lower temperatures than the spontaneous current flow of the phase-crystal state. The magnetic state can, however, be energetically favorable at lower temperatures for sufficiently strong Fermi liquid effects. As a result, first-order transitions between the two states are possible, suggesting a rich low-temperature phase diagram in $d$-wave superconductors., Comment: 10 pages, 6 figures

We present results for the steady-state nonlinear response of a $d_{x^2-y^2}$ superconducting film connected to normal-metal reservoirs under voltage bias, allowing for a subdominant $s$-wave component appearing near the interfaces. Our investigation is based on a current-conserving theory that self-consistently includes the non-equilibrium distribution functions, charge imbalance, and the voltage-dependencies of order parameters and scalar impurity self-energies. For a pure $d$-wave superconductor with [110] orientation of the interfaces to the contacts, the conductance contains a zero-bias peak reflecting the large density of zero-energy interface Andreev bound states. Including a subdominant $s$-wave pairing channel, it is in equilibrium energetically favorable for an $s$-wave order parameter component $\Delta_\mathrm{s}$ to appear near the interfaces in the time-reversal symmetry breaking combination $d+is$. The Andreev states then shift to finite energies in the density of states. Under voltage bias, we find that the non-equilibrium distribution in the contact area causes a rapid suppression of the $s$-wave component to zero as the voltage $eV\rightarrow\Delta_\mathrm{s}$. The resulting spectral rearrangements and voltage-dependent scattering amplitudes lead to a pronounced non-thermally broadened split of the zero-bias conductance peak that is not seen in a non-selfconsistent Landauer-B\"uttiker scattering approach., Comment: 15 pages, 11 figures

We show that epitaxial graphene on silicon carbide (epigraphene) grown at high temperatures (T > 1850 {\deg}C) readily acts as material for implementing solar-blind ultraviolet (UV) detectors with outstanding performance. We present centimeter-sized epigraphene metal-semiconductor-metal (MSM) detectors with peak external quantum efficiency of ~ 85% for wavelengths 250-280 nm, corresponding to nearly 100% internal quantum efficiency when accounting for reflection losses. Zero bias operation is possible in asymmetric devices, with the responsivity to UV remaining as high as R = 134 mA/W, making this a self-powered detector. The low dark currents Io ~50 fA translate into an estimated record high specific detectivity D = 3.5 x 10^15 Jones. The performance that we demonstrate, together with material reproducibility, renders epigraphene technologically attractive to implement high-performance planar MSM devices with a low processing effort, including multi-pixel UV sensor arrays, suitable for a number of practical applications.

In an unconventional superconductor, the interplay of scattering off impurities and Andreev processes may lead to different scattering times for electronlike and holelike quasiparticles. Such electron-hole asymmetry appears when the impurity scattering phase shift is intermediate between the Born and unitary limits and leads to an expectation for large thermoelectric effects. Here, we examine the thermoelectric response of a $d$-wave superconductor connected to normal-metal reservoirs under a temperature bias using a fully self-consistent quasiclassical theory. The thermoelectrically induced quasiparticle current is cancelled by superflow in an open circuit setup, but at the cost of a charge imbalance induced at the contacts and extending across the structure. We investigate the resulting thermopower and thermophase and their dependencies on scattering phase shift, mean free path, and interface transparency. For crystal-axis orientations such that surface-bound zero-energy Andreev states are formed, the thermoelectric effect is reduced as a result of locally reduced electron-hole asymmetry. For a semiballistic superconductor with good contacts, we find thermopowers of order several ${\mu}V/K$, suggesting a thermovoltage measurement as a promising path to investigate thermoelectricity in unconventional superconductors., Comment: 11 pages, 6 figures

We consider the steady-state nonequilibrium behavior of mesoscopic superconducting wires connected to normal-metal reservoirs. Going beyond the diffusive limit, we utilize the quasiclassical theory and perform a self-consistent calculation that guarantees current conservation through the entire system. Going from the ballistic to the diffusive limit, we investigate several crucial phenomena such as charge imbalance, momentum-resolved nonequilbrium distributions, and the current-to-superflow conversion. Connecting to earlier results for the diffusive case, we find that superconductivity can break down at a critical bias voltage $V_\mathrm{c}$. We find that $V_\mathrm{c}$ generally increases as the interface transparency is reduced, while the dependence on the mean-free path is non-monotonous. We discussthe key differences of the ballistic and semi-ballistic regimes to the fully diffusive case., Comment: 17 pages, 14 figures

The simultaneous interplay of strong electron-electron correlations, topological zero-energy states, and disorder is yet an unexplored territory but of immense interest due to their inevitable presence in many materials. Copper oxide high-temperature superconductors (cuprates) with pair breaking edges host a flat band of topological zero-energy states, making them an ideal playground where strong correlations, topology, and disorder are strongly intertwined. Here we show that this interplay in cuprates generates a new phase of matter: a fully gapped ``phase crystal" state that breaks both translational and time-reversal invariance, characterized by a modulation of the $d$-wave superconducting phase co-existing with a modulating extended $s$-wave superconducting order. In contrast to conventional wisdom, we find that this phase crystal state is remarkably robust to omnipresent disorder, but only in the presence of strong correlations, thus giving a clear route to its experimental realization., Comment: Added discussion and analysis on comparison with experiments

We theoretically study the electronic and transport properties of two graphene layers vertically coupled by an insulating layer under the influence of a time-periodic external light field. The non-adiabatic driving induces excitations of electrons and a redistribution of the occupied states which is manifested in the opening of gaps in the quasienergy spectrum of graphene. When a voltage is applied between the top and bottom graphene layers, the photo-induced nonequilibrium occupation modifies the transport properties of the contact. We investigate the electronic and transport properties of the contact by using the nonequilibrium Green's function formalism. To illustrate the behavior of the differential conductance of the vertical contact under the light illumination, we consider two cases. First, we assume that both the bottom and top layers consist of graphene and second we consider a finite mass term in the bottom layer. We obtain that the differential conductance is strongly suppressed due to the opening of gaps in the quasienergy spectrum in graphene. Additionally, the conductance shows features corresponding to the tunneling of photoexcited electrons at energies of the van Hove singularity for both the top and bottom layers. In the case of a finite mass term in the bottom layer, the differential conductance can be directly related to the tunneling of photoexcited electrons.

Unconventional d-wave superconductors with pair-breaking edges are predicted to have ground states with spontaneously broken time-reversal and translational symmetries. We use the quasiclassical theory of superconductivity to demonstrate that such phases can exist at any single pair-breaking facet. This implies that a greater variety of systems, not necessarily mesoscopic in size, should be unstable to such symmetry breaking. The density of states averaged over the facet displays a broad peak centered at zero energy, which is consistent with experimental findings of a broad zero-bias conductance peak with a temperature-independent width at low temperatures., Comment: Accepted for the Proceedings of LT28 - The 28th International Conference on Low Temperature Physics

By using Fourier-transform scanning tunneling spectroscopy we measure the interference patterns produced by the impurity scattering of confined Dirac quasiparticles in epitaxial graphene nanoflakes. Upon comparison of the experimental results with tight-binding calculations of realistic model flakes, we show that the characteristic features observed in the Fourier-transformed local density of states are related to scattering between different transverse modes (sub-bands) of a graphene nanoflake and allow direct insight into the electronic spectrum of graphene. We also observe a strong reduction of quasiparticle lifetime which is attributed to the interaction with the underlying substrate. In addition, we show that the distribution of the onsite energies at flower defects leads to an effectively broken pseudospin selection rule, where intravalley back-scattering is allowed., Comment: 11 pages, 3 figures

Conventional superconductors disordered by magnetic impurities demonstrate physical properties drastically different from their pristine counterparts. In our previous work [Phys. Rev. B 92, 245430 (2015)] we explored spectral and thermodynamic properties of such systems for two extreme cases: completely random and ferromagnetically aligned impurity magnetic moments. Here we consider transport properties of these systems, and show that they have a potential to be used in superconducting spintronic devices. Each magnetic impurity contributes a Yu-Shiba-Rusinov (YSR) bound state to the spectrum, residing at sub-gap energies. Provided the YSR states form metallic bands, we demonstrate that the tunneling current carried by these states can be highly spin-polarized when the impurities are ferromagnetically ordered. The spin polarization can be switched by simply tuning the bias voltage. Moreover, even when the impurity spins are completely uncorrelated, one can still achieve almost 100% spin polarization of the current, if the tunnel interface is spin-active. We compute electric current and noise, varying parameters of the interface between tunneling and fully transparent regimes, and analyze the relative role of single-particle and Andreev reflection processes., Comment: 14 pages, 10 figures

We present a comprehensive theoretical study of thermodynamic properties of superconductors with a dilute concentration of magnetic impurities, with focus on how the properties of the superconducting host change if the magnetic moments of the impurities order ferromagnetically. Scattering off the magnetic impurities leads to the formation of a band of Yu-Shiba-Rusinov states within the superconducting energy gap that drastically influences superconductivity. In the magnetically ordered system, the magnetization displays a sudden drop as function of impurity density or magnetic moment amplitude. The drop occurs as the spin-polarized impurity band crosses the Fermi level and is associated with a quantum phase transition first put forward by Sakurai for the single impurity case. Taking into account that the background magnetic field created by the ordered impurity moments enters as a Zeeman shift, we find that the superconducting phase transition changes from second order to first order for high enough impurity concentration., Comment: 16 pages, 13 figures

Conventional superconductors are strong diamagnets that through the Meissner effect expel magnetic fields. It would therefore be surprising if a superconducting ground state would support spontaneous magnetics fields. Such time-reversal symmetry broken states have been proposed for the high-temperature superconductors, but their identification remains experimentally controversial. Here we show a route to a low-temperature superconducting state with broken time-reversal symmetry that may accommodate currently conflicting experiments. This state is characterised by an unusual vortex pattern in the form of a necklace of fractional vortices around the perimeter of the material, where neighbouring vortices have opposite current circulation. This vortex pattern is a result of a spectral rearrangement of current carrying states near the surfaces.

We consider a heterostructure consisting of a normal metal and a superconductor separated by a spin-active interface. At finite-bias voltages, spin-filtering and spin-mixing effects at the interface allow for an induced magnetization (spin imbalance) on the superconducting side of the junction, which relaxes to zero in the bulk. Such interfaces are also known to host a pair of in-gap Andreev bound states which were recently observed experimentally. We show that these states are responsible for the dominant contribution to the induced spin imbalance close to the interface. Motivated by recent experiments on spin-charge density separation in superconducting aluminum wires, we propose an alternative way to observe spin imbalance without applying an external magnetic field. We also suggest that the peculiar dependence of the spin imbalance on the applied bias voltage permits an indirect bound-state spectroscopy., Comment: 7 pages, 4 figures

We study the pi phase in a superconductor-ferromagnet-superconductor Josephson junction, with a ferromagnet showing a cycloidal spiral spin modulation with in-plane propagation vector. Our results reveal a high sensitivity of the junction to the spiral order and indicate the presence of 0-pi quantum phase transitions as function of the spiral wave vector. We find that the chiral magnetic order introduces chiral superconducting triplet pairs that strongly influence the physics in such Josephson junctions, with potential applications in nanoelectronics and spintronics., Comment: 4 pages, 4 figures; the derivation part has been reorganized + added note and new references, published version