Search

The correspondence principle bridges the quantum and classical worlds by establishing a direct link between their dynamics. This well-accepted tenant of quantum physics has been explored in quantum systems wherein the number of particles is increased to macroscopic scales. However, theoretical investigations of nanoscale structures have revealed discrepancies when attempting to bridge classical and quantum physics. Here, we report on the experimental observation of anomalous classical-to-quantum transitions in open many-body optical systems. We demonstrate, for the first time, the lack of classical-to-quantum correspondence between a macroscopic optical system and its constituent quantum multiphoton subsystems. In contrast to common belief, we demonstrate that the coherence dynamics of many-body quantum subsystems with up to forty particles can indeed be opposite to that exhibited by the hosting macroscopic system. By employing complex-Gaussian statistics, we show that these effects are universal for open many-body systems. Consequently, our work can have important implications for other fields of physics ranging from condensed matter to nuclear physics.

Excitation energy transfer is a photophysical process upon which many chemical and biological phenomena are built. From natural small systems to synthetic multichromophoric macromolecules, energy transfer deals with the process of migration of electronic excitation energy from an excited donor to an acceptor. Although this phenomenon has been extensively studied in the past, the rapid evolution of quantum-enabled technologies has motivated the question on whether nonclassical sources of light, such as entangled photon pairs, may provide us with a better control (or enhancement) of energy transfer at the nanoscale. In this work, we provide a comprehensive study of the joint excitation of two non-interacting two-level atoms by time-frequency correlated photon pairs -- whose central frequencies are not resonant with the individual particles -- generated by means of spontaneous parametric down conversion (SPDC). We demonstrate that while strong frequency anti-correlation between photons guarantees a large two-photon excitation (TPE) probability, photons bearing a sine cardinal spectral shape exhibit a $\sim$3.8 times larger TPE signal than photons with a Gaussian spectrum. More importantly, we find that suppression of time-ordered excitation pathways does not substantially modify the TPE probability for two-photon states with a Gaussian spectral shape; whereas photons with a sine cardinal spectrum exhibit the strongest TPE signals when two-photon excitation pathways are not suppressed. Our results not only help elucidating the role of time-frequency correlations in resonance energy transfer with SPDC photons, but also provide valuable information regarding the optimal source to be used in its experimental implementation.

It is thought that schemes for quantum imaging are fragile against realistic environments in which the background noise is often stronger than the nonclassical signal of the imaging photons. Unfortunately, it is unfeasible to produce brighter quantum light sources to alleviate this problem. Here, we overcome this paradigmatic limitation by developing a quantum imaging scheme that relies on the use of natural sources of light. This is achieved by performing conditional detection on the photon number of the thermal light field scattered by a remote object. Specifically, the conditional measurements in our scheme enable us to extract quantum features of the detected thermal photons to produce quantum images with improved signal-to-noise ratios. This technique shows a remarkable exponential enhancement in the contrast of quantum images. Surprisingly, this measurement scheme enables the possibility of producing images from the vacuum fluctuations of the light field. This is experimentally demonstrated through the implementation of a single-pixel camera with photon-number-resolving capabilities. As such, we believe that our scheme opens a new paradigm in the field of quantum imaging. It also unveils the potential of combining natural light sources with nonclassical detection schemes for the development of robust quantum technologies.

The identification of nonclassical features of multiphoton quantum states represents a task of the utmost importance in the development of many quantum photonic technologies. Under realistic experimental conditions, a photonic quantum state gets affected by its interaction with several nonideal opto-electronic devices, including those used to guide, detect or characterize it. The result of such noisy interaction is that the nonclassical features of the original quantum state get considerably reduced or are completely absent in the detected, final state. In this work, the self-learning features of artificial neural networks are exploited to experimentally show that the nonclassicality of multiphoton quantum states can be assessed and fully characterized, even in the cases in which the nonclassical features are concealed by the measuring devices. Our work paves the way toward artificial-intelligence-assisted experimental-setup characterization, as well as smart quantum-state nonclassicality identification., Comment: 10 pages, 6 figures

The modification of the quantum properties of coherence of photons through their interaction with matter lies at the heart of the quantum theory of light. Indeed, the absorption and emission of photons by atoms can lead to different kinds of light with characteristic quantum statistical properties. As such, different types of light are typically associated with distinct sources. Here, we report on the observation of the modification of quantum coherence of multiphoton systems in free space. This surprising effect is produced by the scattering of thermal multiphoton wavepackets upon propagation. The modification of the excitation mode of a photonic system and its associated quantum fluctuations result in the formation of different light fields with distinct quantum coherence properties. Remarkably, we show that these processes of scattering can lead to multiphoton systems with sub-shot-noise quantum properties. Our observations are validated through the nonclassical formulation of the emblematic van Cittert-Zernike theorem. We believe that the possibility of producing quantum systems with modified properties of coherence, through linear propagation, can have dramatic implications for diverse quantum technologies.

Entanglement is a quintessential quantum mechanical phenomenon with no classical equivalent. First discussed by Einstein, Podolsky, and Rosen and formally introduced by Schr\"odinger in 1935, entanglement has grown from a scientific debate to a radically new resource that sparks a technological revolution. This review focuses on the fundamentals and recent advances in entanglement-based quantum information technology (QIT), specifically in photonic systems. Photons are unique quantum information carriers with several advantages, such as their ability to operate at room temperature, their compatibility with existing communication and sensing infrastructures, and the availability of readily accessible optical components. Photons also interface well with other solid-state quantum platforms. We will first provide an overview on entanglement, starting with an introduction to its development from a historical perspective followed by the theory for entanglement generation and the associated representative experiments. We will then dive into the applications of entanglement-based QIT for sensing, imaging, spectroscopy, data processing, and communication. Before closing, we will present an outlook for the architecture of the next-generation entanglement-based QIT and its prospective applications., Comment: 87 pages, 40 figures. Comments are welcome

Structured light beams, in particular those carrying orbital angular momentum (OAM), have gained a lot of attention due to their potential for enlarging the transmission capabilities of communication systems. However, the use of OAM-carrying light in communications faces two major problems, namely distortions introduced during propagation in disordered media, such as the atmosphere or optical fibers, and the large divergence that high-order OAM modes experience. While the use of non-orthogonal modes may offer a way to circumvent the divergence of high-order OAM fields, artificial intelligence (AI) algorithms have shown promise for solving the mode-distortion issue. Unfortunately, current AI-based algorithms make use of large-amount data-handling protocols that generally lead to large processing time and high power consumption. Here we show that a low-power, low-cost image sensor can itself act as an artificial neural network that simultaneously detects and reconstructs distorted OAM-carrying beams. We demonstrate the capabilities of our device by reconstructing (with a 95$\%$ efficiency) individual Vortex, Laguerre-Gaussian (LG) and Bessel modes, as well as hybrid (non-orthogonal) coherent superpositions of such modes. Our work provides a potentially useful basis for the development of low-power-consumption, light-based communication devices.

We experimentally study the infinite-size limit of the Dicke model of quantum optics with a parity-breaking deformation strength that couples the system to an external bosonic reservoir. We focus on the dynamical consequences of such symmetry-breaking, which makes the classical phase space asymmetric with non-equivalent energy wells. We present an experimental implementation of the classical version of the deformed Dicke model using a state-of-the-art bi-parametric electronic platform. Our platform constitutes a playground for studying representative phenomena of the deformed Dicke model in electrical circuits with the possibility of externally controlling parameters and initial conditions. In particular, we investigate the dynamics of the ground state, various phase transitions, and the asymmetry of the energy wells as a function of the coupling strength $\gamma$ and the deformation strength $\alpha$ in the resonant case. Additionally, to characterize the various behavior regimes, we present a two-dimensional phase diagram as a function of the two intrinsic system parameters. The onset of chaos is also analyzed experimentally. Our findings provide a clear connection between theoretical predictions and experimental observations, demonstrating the usefulness of our bi-parametric electronic setup.

Exceptional points (EPs) are degeneracies of non-Hermitian systems, where both eigenvalues and eigenvectors coalesce. Classical and quantum systems exhibiting high-order EPs have recently been identified as fundamental building blocks for the development of novel, ultra-sensitive opto-electronic devices. However, arguably one of their major drawbacks is that they rely on non-linear amplification processes that could limit their potential applications, particularly in the quantum realm. In this work, we show that high-order EPs can be designed by means of linear, time-modulated, chain of inductively coupled RLC (where R stands for resistance, L for inductance, and C for capacitance) electronic circuits. With a general theory, we show that $N$ coupled circuits with $2N$ dynamical variables and time-dependent parameters can be mapped onto an $N$-site, time-dependent, non-Hermitian Hamiltonian, and obtain constraints for $\mathcal{PT}$-symmetry in such models. With numerical calculations, we obtain the Floquet exceptional contours of order $N$ by studying the energy dynamics in the circuit. Our results pave the way toward realizing robust, arbitrary-order EPs by means of synthetic gauge fields, with important implications for sensing, energy transfer, and topology.

The nature of light sources is defined by the statistical fluctuations of the electromagnetic field. As such, the photon statistics of light sources are typically associated with distinct emitters. Here, we demonstrate the possibility of producing light beams with various photon statistics through the spatial modulation of coherent light. This is achieved by the sequential encoding of controllable Kolmogorov phase screens in a digital micromirror device. Interestingly, the flexibility of our scheme allows for the arbitrary shaping of spatial light modes with engineered photon statistics at different spatial positions. The performance of our scheme is assessed through the photon-number-resolving characterization of different families of spatial light modes with engineered photon statistics. We believe that the possibility of controlling the photon fluctuations of the light field at arbitrary spatial locations has important implications for quantum spectroscopy, sensing, and imaging., Comment: 5 pages, 3 figures

Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of entangled two-photon absorption (eTPA), there is still a heated debate on whether eTPA has truly been observed. This interesting debate has arisen, mainly because it has been recently argued that single-photon-loss mechanisms, such as scattering or hot-band absorption may mimic the expected entangled-photon linear absorption behavior. In this work, we focus on transmission measurements of eTPA, and explore three different two-photon quantum interferometers in the context of assessing eTPA. We demonstrate that the so-called N00N-state configuration is the only one amongst those considered insensitive to linear (single-photon) losses. Remarkably, our results show that N00N states may become a potentially powerful tool for quantum spectroscopy, and place them as a strong candidate for the certification of eTPA in an arbitrary sample., Comment: 10 pages, 4 figures. Updated References

Recent progress on quantum state engineering has enabled the preparation of quantum photonic systems comprising multiple interacting particles. Interestingly, multiphoton quantum systems can host many complex forms of interference and scattering processes that are essential to perform operations that are intractable on classical systems. Unfortunately, the quantum coherence properties of multiphoton systems degrade upon propagation leading to undesired quantum-to-classical transitions. Furthermore, the manipulation of multiphoton quantum systems requires of nonlinear interactions at the few-photon level. Here, we introduce the quantum van Cittert-Zernike theorem to describe the scattering and interference effects of propagating multiphoton systems. This fundamental theorem demonstrates that the quantum statistical fluctuations, which define the nature of diverse light sources, can be modified upon propagation in the absence of light-matter interactions. The generality of our formalism unveils the conditions under which the evolution of multiphoton systems can lead to surprising classical-to-quantum transitions. Specifically, we show that the implementation of conditional measurements may enable the all-optical preparation of multiphoton systems with attenuated quantum statistics below the shot-noise limit. Remarkably, this effect had not been discussed before and cannot be explained through the classical theory of optical coherence. As such, our work opens new paradigms within the established field of quantum coherence., Comment: Updated version

Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy based on tunable classical light has been long established, quantum light provides an alternative way towards excitation spectroscopy with potential advantages in temporal and spectral resolution, as well as reduced photon fluxes. By using a quantum Fourier transform that connects the sum-frequency intensity and N00N-state temporal interference, we present an approach for quantum interferometric two-photon excitation spectroscopy. Our proposed protocol overcomes the difficulties of engineering two-photon joint spectral intensities and fine-tuned absorption-frequency selection. These results may significantly facilitate the use of quantum interferometric spectroscopy for extracting the information about the electronic structure of the two-photon excited-state manifold of atoms or molecules, in a "single-shot" measurement. This may be particularly relevant for photon-sensitive biological and chemical samples., Comment: 6 pages, 4 figures

The manifestation of the wave nature of light through diffraction imposes limits on the resolution of optical imaging. For over a century, the Abbe-Rayleigh criterion has been utilized to assess the spatial resolution limits of optical instruments. Recently, there has been an enormous impetus in overcoming the Abbe-Rayleigh resolution limit by projecting target light beams onto spatial modes. These conventional schemes for superresolution rely on a series of spatial projective measurements to pick up phase information that is used to boost the spatial resolution of optical systems. Unfortunately, these schemes require a priori information regarding the coherence properties of "unknown" light beams. Furthermore, they require stringent alignment and centering conditions that cannot be achieved in realistic scenarios. Here, we introduce a smart quantum camera for superresolving imaging. This camera exploits the self-learning features of artificial intelligence to identify the statistical fluctuations of unknown mixtures of light sources at each pixel. This is achieved through a universal quantum model that enables the design of artificial neural networks for the identification of quantum photon fluctuations. Our camera overcomes the inherent limitations of existing superresolution schemes based on spatial mode projection. Thus, our work provides a new perspective in the field of imaging with important implications for microscopy, remote sensing, and astronomy., Comment: 10 pages, 5 figures

What is the fate of an oscillator when its inductance and capacitance are varied while its frequency is kept constant? Inspired by this question, we propose a protocol to implement parity-time (PT) symmetry in a lone oscillator. Different forms of constrained variations lead to static, periodic, or arbitrary balanced gain and loss profiles, that can be interpreted as purely imaginary gauge fields. With a state-of-the-art, dynamically tunable LC oscillator comprising synthetic circuit elements, we demonstrate static and Floquet PT breaking transitions, including those at vanishingly small gain and loss, by tracking the circuit energy. Concurrently, we derive and observe conserved quantities in this open, balanced gain-loss system, both in the static and Floquet cases. Lastly, by measuring the circuit energy, we unveil a giant dynamical asymmetry along exceptional point (EP) contours that emerge symmetrically from the Hermitian degeneracies at Floquet resonances. Distinct from material or parametric gain and loss mechanisms, our protocol enables on-demand parity-time symmetry in a minimal classical system -- a single oscillator -- and may be ported to other realizations including metamaterials and optomechanical systems., Comment: 8 pages, 4 figures

The ability to engineer the spatial wavefunction of photons has enabled a variety of quantum protocols for communication, sensing, and information processing. These protocols exploit the high dimensionality of structured light enabling the encodinng of multiple bits of information in a single photon, the measurement of small physical parameters, and the achievement of unprecedented levels of security in schemes for cryptography. Unfortunately, the potential of structured light has been restrained to free-space platforms in which the spatial profile of photons is preserved. Here, we make an important step forward to using structured light for fiber optical communication. We introduce a smart high-dimensional encryption protocol in which the propagation of spatial modes in multimode fibers is used as a natural mechanism for encryption. This provides a secure communication channel for data transmission. The information encoded in spatial modes is retrieved using artificial neural networks, which are trained from the intensity distributions of experimentally detected spatial modes. Our on-fiber communication platform allows us to use spatial modes of light for high-dimensional bit-by-bit and byte-by-byte encoding. This protocol enables one to recover messages and images with almost perfect accuracy. Our smart protocol for high-dimensional optical encryption in optical fibers has key implications for quantum technologies relying on structured fields of light, particularly those that are challenged by free-space propagation., Comment: 7 pages, 3 figures

The concept of quantum discord aims at unveiling quantum correlations that go beyond those described by entanglement. Its original formulation [J. Phys. A 34, 6899 (2001); Phys. Rev. Lett 88, 017901 (2002)] is difficult to compute even for the simplest case of two-qubits systems. Alternative formulations have been developed to address this drawback, such as the geometric measure of quantum discord [Phys. Rev. A 87, 062303 (2013)] and the local quantum uncertainty [Phys. Rev. Lett 110, 240402 (2013)] that can be evaluated in closed form for some quantum systems, such as two-qubit systems. We show here that these two measures of quantum discord are equivalent for 2 x D dimensional bipartite quantum systems. By considering the relevant example of N00N states for phase estimation in lossy environments, we also show that both metrics of quantum discord quantify the decrease of quantum Fisher information of the phase estimation protocol. Given their ease of computation in 2 x D bipartite systems, the geometric measure of quantum discord and the local quantum uncertainty demonstrate their relevance as computable measures of quantum discord., Comment: 7 pages - 4 figures

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of entanglement and the delay time between the photons have been varied. This works well for simple systems but quickly becomes rather difficult when many intermediate states are involved. We propose and discuss an extension of entangled two-photon absorption spectroscopy that solves this problem by means of repeated measurements at different pump wavelengths. Specifically, we demonstrate that our extension works well for a variety of realistic experimental setups., Comment: 14 pages, 6 figures, currently in peer review in JOSA B

Transport phenomena in photosynthetic systems have attracted a great deal of attention due to their potential role in devising novel photovoltaic materials. In particular, energy transport in light-harvesting complexes is considered quite efficient due to the balance between coherent quantum evolution and decoherence, a phenomenon coined Environment-Assisted Quantum Transport (ENAQT). Although this effect has been extensively studied, its behavior is typically described in terms of the decoherence's strength, namely weak, moderate or strong. Here, we study the ENAQT in terms of quantum correlations that go beyond entanglement. Using a subsystem of the Fenna-Matthews-Olson complex, we find that discord-like correlations maximize when the subsystem's transport efficiency increases, while the entanglement between sites vanishes. Our results suggest that quantum discord is a manifestation of the ENAQT and highlight the importance of beyond-entanglement correlations in photosynthetic energy transport processes.

For almost two decades, it has been believed that the quantum statistical properties of bosons are preserved in plasmonic systems. This idea has been stimulated by experimental work reporting the possibility of preserving nonclassical correlations in light-matter interactions mediated by scattering among photons and plasmons. Furthermore, it has been assumed that similar dynamics underlies the conservation of the quantum fluctuations that define the nature of light sources. Here, we demonstrate that quantum statistics are not always preserved in plasmonic systems and report the first observation of their modification. Moreover, we show that multiparticle scattering effects induced by confined optical near fields can lead to the modification of the excitation mode of plasmonic systems. These observations are validated through the quantum theory of optical coherence for single- and multi-mode plasmonic systems. Our findings constitute a new paradigm in the understanding of the quantum properties of plasmonic systems and unveil new paths to perform exquisite control of quantum multiparticle systems., Comment: 12 pages, 5 figures

We theoretically show that the dynamics of a driven quantum harmonic oscillator subject to non-dissipative noise is formally equivalent to the single-particle dynamics propagating through an experimentally feasible dynamically-disordered photonic network. Using this correspondence, we find that noise assisted energy transport occurs in this network and, if the noise is Markovian or delta-correlated, we can obtain an analytical solution for the maximum amount of transferred energy between all network's sites at a fixed propagation distance. Beyond the Markovian limit, we further consider two different types of non-Markovian noise and show that it is possible to have efficient energy transport for larger values of the dephasing rate., Comment: 12 pages, 4 figures

Entangled two-photon absorption (ETPA) has recently become a topic of lively debate, mainly due to the apparent inconsistencies in the experimentally-reported ETPA cross sections of organic molecules. In this work, we provide a thorough experimental study of ETPA in the organic molecules Rhodamine B (RhB) and Zinc Tetraphenylporphirin (ZnTPP). The goal of this contribution is twofold: on one hand, it seeks to reproduce the results of previous experimental reports and, on the other, it aims to determine the effects of different temporal correlations -- introduced as a controllable time-delay between the photons to be absorbed -- on the strength of the ETPA signal. In our experiment, the samples are excited by entangled pairs produced by type-I SPDC, with a spectral distribution centered at 810 nm. Surprisingly, and contrary to what was expected, the time delay did not produce in our experiments any systematic change in the cross-sections when monitoring the ETPA signal using a transmission measurement scheme. As a plausible cause of this unexpected result, we argue that the photon-pair flux, typically-used in these experiments, is not sufficient to promote the two-photon absorption process in these molecules. This suggests that the actual absorption cross-section values are lower than those previously reported, and therefore do not lead to a measurable ETPA effect for the transmission method., Comment: 24 pages, 7 figures

We demonstrate a smart laser-diffraction analysis technique for particle mixture identification. We retrieve information about the size, geometry, and ratio concentration of two-component heterogeneous particle mixtures with an efficiency above 92%. In contrast to commonly-used laser diffraction schemes -- in which a large number of detectors is needed -- our machine-learning-assisted protocol makes use of a single far-field diffraction pattern, contained within a small angle ($\sim 0.26^{\circ}$) around the light propagation axis. Because of its reliability and ease of implementation, our work may pave the way towards the development of novel smart identification technologies for sample classification and particle contamination monitoring in industrial manufacturing processes., Comment: 7 pages, 4 figures

In 1981, Richard Feynman discussed the possibility of performing quantum mechanical simulations of nature. Ever since, there has been an enormous interest in using quantum mechanical systems, known as quantum simulators, to mimic specific physical systems. Hitherto, these controllable systems have been implemented on different platforms that rely on trapped atoms, superconducting circuits and photonic arrays. Unfortunately, these platforms do not seem to satisfy, at once, all desirable features of an universal simulator, namely long-lived coherence, full control of system parameters, low losses, and scalability. Here, we overcome these challenges and demonstrate robust simulation of quantum transport phenomena using a state-of-art reconfigurable electronic network. To test the robustness and precise control of our platform, we explore the ballistic propagation of a single-excitation wavefunction in an ordered lattice, and its localization due to disorder. We implement the Su-Schrieffer-Heeger model to directly observe the emergence of topologically-protected one-dimensional edge states. Furthermore, we present the realization of the so-called perfect transport protocol, a key milestone for the development of scalable quantum computing and communication. Finally, we show the first simulation of the exciton dynamics in the B800 ring of the purple bacteria LH2 complex. The high fidelity of our simulations together with the low decoherence of our device make it a robust, versatile and promising platform for the simulation of quantum transport phenomena.

Activating transitions between internal states of physical systems has emerged as an appealing approach to create lattices and complex networks. In such a scheme, the internal states or modes of a physical system are regarded as lattice sites or network nodes in an abstract space whose dimensionality may exceed the systems' apparent (geometric) dimensionality. This introduces the notion of synthetic dimensions, thus providing entirely novel pathways for fundamental research and applications. Here, we analytically show that the propagation of multi-photon states through multi-port waveguide arrays gives rise to synthetic dimensions where a single waveguide system generates a multitude of synthetic lattices. Since these synthetic lattices exist in photon-number space, we introduce the concept of pseudo-energy and demonstrate its utility for studying multi-photon interference processes. Specifically, the spectrum of the associated pseudo-energy operator generates a unique ordering of the relevant states. Together with generalized pseudo-energy ladder operators, this allows for representing the dynamics of multi-photon states by way of pseudo-energy term diagrams that are associated with a synthetic atom. As a result, the pseudo-energy representation leads to concise analytical expressions for the eigensystem of $N$ photons propagating through $M$ nearest-neighbor coupled waveguides. In the regime where $N>2$ and $M>2$, non-local coupling in Fock space gives rise to hitherto unknown all-optical dark states which display intriguing non-trivial dynamics., Comment: Two-column layout, 11 pages, 8 figures

Topological phenomena in non-Hermitian systems have recently become a subject of great interest in the photonics and condensed-matter communities. In particular, the possibility of observing topologically-protected edge states in non-Hermitian lattices has sparked an intensive search for systems where this kind of states are sustained. Here, we present the first study on the emergence of topological edge states in two-dimensional Haldane lattices exhibiting balanced gain and loss. In line with recent studies on other Chern insulator models, we show that edge states can be observed in the so-called broken $\mathcal{P}\mathcal{T}$-symmetric phase, that is, when the spectrum of the gain-loss-balanced system's Hamiltonian is not entirely real. More importantly, we find that such topologically protected edge states emerge irrespective of the lattice boundaries, namely zigzag, bearded or armchair.

We report the experimental implementation of the Dicke model in the semiclassical approximation, which describes a large number of two-level atoms interacting with a single-mode electromagnetic field in a perfectly reflecting cavity. This is managed by making use of two non-linearly coupled active, synthetic LC circuits, implemented by means of analog electrical components. The simplicity and versatility of our platform allows us not only to experimentally explore the coexistence of regular and chaotic trajectories in the Dicke model but also to directly observe the so-called ground-state and excited-state ``quantum'' phase transitions. In this analysis, the trajectories in phase space, Lyapunov exponents and the recently introduced Out-of-Time-Order-Correlator (OTOC) are used to identify the different operating regimes of our electronic device. Exhaustive numerical simulations are performed to show the quantitative and qualitative agreement between theory and experiment.

Transport phenomena in organic, self-assembled molecular J-aggregates have long attracted a great deal of attention due to its potential role in designing novel organic photovoltaic devices. A large number of theoretical and experimental studies have been carried out describing excitonic energy transfer in J-aggregates under the assumption that excitons are induced by a coherent laser-light source or initialized by a localized excitation on a particular chromophore. However, these assumptions may not provide an accurate description to assess the efficiency of J-aggregates, particularly as building blocks of organic solar cells. In natural conditions, J-aggregates would be subjected to an incoherent source of light (as is sunlight), which would illuminate the whole photosynthetic complex rather than a single molecule. In this work, we present the first study of the efficiency of photosynthetic energy transport in self-assembled molecular aggregates under incoherent sunlight illumination. By making use of a minimalistic model of a cyanine dye J-aggregate, we demonstrate that long-range transport efficiency is enhanced when exciting the aggregate with incoherent light. Our results thus support the conclusion that J-aggregates are indeed excellent candidates for devices where efficient long-range incoherently-induced exciton transport is desired, such as in highly efficient organic solar cells.

The identification of light sources represents a task of utmost importance for the development of multiple photonic technologies. Over the last decades, the identification of light sources as diverse as sunlight, laser radiation and molecule fluorescence has relied on the collection of photon statistics or the implementation of quantum state tomography. In general, this task requires an extensive number of measurements to unveil the characteristic statistical fluctuations and correlation properties of light, particularly in the low-photon flux regime. In this article, we exploit the self-learning features of artificial neural networks and naive Bayes classifier to dramatically reduce the number of measurements required to discriminate thermal light from coherent light at the single-photon level. We demonstrate robust light identification with tens of measurements at mean photon numbers below one. Our work demonstrates an improvement in terms of the number of measurements of several orders of magnitude with respect to conventional schemes for characterization of light sources. Our work has important implications for multiple photonic technologies such as LIDAR and microscopy., Comment: 8 pages, 10 figures

Exceptional points (EPs) are degeneracies of non-Hermitian operators where, in addition to the eigenvalues, corresponding eigenmodes become degenerate. Classical and quantum photonic systems with EPs have attracted tremendous attention due to their unusual properties, topological features, and an enhanced sensitivity that depends on the order of the EP, i.e. the number of degenerate eigenmodes. Yet, experimentally engineering higher-order EPs in classical or quantum domains remains an open challenge due to the stringent symmetry constraints that are required for the coalescence of multiple eigenmodes. Here we analytically show that the number-resolved dynamics of a single, lossy, waveguide beamsplitter, excited by $N$ indistinguishable photons and post-selected to the $N$-photon subspace, will exhibit an EP of order $N+1$. By using the well-established mapping between a beamsplitter Hamiltonian and the perfect state transfer model in the photon-number space, we analytically obtain the time evolution of a general $N$-photon state, and numerically simulate the system's evolution in the post-selected manifold. Our results pave the way towards realizing robust, arbitrary-order EPs on demand in a single device., Comment: 5 pages, 2 figures

In this work we demonstrate single microparticle transport in a symmetric noisy optical ratchet where each potential is a low power ($<2.5$ mW) three dimensional trap. The optical potentials consist of 20 symmetric optical traps arranged in a one-dimensional lattice produced by a spatial light modulator. The external periodic force of the ratchet system adds to zero over one period (symmetric) and is generated by the motion of a piezo-electric microscope stage. Transport is achieved by adding noise to the potentials by randomly varying the diffracted power into the traps at the same frequency of the external force. We show that the direction and speed of motion (current) is coupled to the phase difference between the noise in the optical potentials and the external periodic force.

Quantum walks in dynamically-disordered networks have become an invaluable tool for understanding the physics of open quantum systems. In this work, we introduce a novel approach to describe the dynamics of indistinguishable particles in noisy quantum networks. By making use of stochastic calculus, we derive a master equation for the propagation of two non-interacting correlated particles in tight-binding networks affected by off-diagonal dynamical disorder. We show that the presence of noise in the couplings of a quantum network creates a pure-dephasing-like process that destroys all coherences in the single-particle Hilbert subspace. Remarkably, we find that when two or more correlated particles propagate in the network, coherences accounting for particle indistinguishability are robust against the impact of noise, thus showing that it is possible, in principle, to find specific conditions for which many indistinguishable particles can traverse dynamically-disordered systems without losing their ability to interfere. These results shed light on the role of particle indistinguishability in the preservation of quantum coherence in dynamically-disordered quantum networks., Comment: 15 pages, 4 figures

Entangled two-photon absorption spectroscopy (TPA) has been widely recognized as a powerful tool for revealing relevant information about the structure of complex molecular systems. However, to date, the experimental implementation of this technique has remained elusive, mainly because of two major difficulties. First, the need to perform multiple experiments with two-photon states bearing different temporal correlations, which translates in the necessity to have at the experimenter's disposal tens, if not hundreds, of sources of entangled photons. Second, the need to have \emph{a priori} knowledge of the absorbing medium's lowest-lying intermediate energy level. In this work, we put forward a simple experimental scheme that successfully overcomes these two limitations. By making use of a temperature-controlled entangled-photon source, which allows the tuning of the central frequencies of the absorbed photons, we show that the TPA signal, measured as a function of the temperature of the nonlinear crystal that generates the paired photons, and a controllable delay between them, carries all information about the electronic level structure of the absorbing medium, which can be revealed by a simple Fourier transformation., Comment: 8 pages, 3 figures

The quantum theory of electromagnetic radiation predicts characteristic statistical fluctuations for light sources as diverse as sunlight, laser radiation and molecule fluorescence. Indeed, these underlying statistical fluctuations of light are associated with the fundamental physical processes behind their generation. In this contribution, we demonstrate that the manipulation of the quantum electromagnetic fluctuations of a pair of vacuum states leads to a novel family of quantum-correlated multiphoton states with tunable mean photon numbers and degree of correlation. Our technique relies on the use of conditional measurements to engineer the excitation mode of the field through the simultaneous subtraction of photons from two-mode squeezed vacuum states. The experimental generation of multiphoton states with quantum correlations by means of photon subtraction unveils novel mechanisms to control fundamental properties of light. As a remarkable example, we demonstrate the engineering of a quantum correlated state of light, with nearly Poissonian photon statistics, that constitutes the first step towards the generation of entangled lasers. Our technique enables a robust protocol to prepare quantum states with multiple photons in high-dimensional spaces and, as such, it constitutes a novel platform for exploring quantum phenomena in mesoscopic systems.

Quantum coherence, the physical property underlying fundamental phenomena such as multi-particle interference and entanglement, has emerged as a valuable resource upon which modern technologies are founded. In general, the most prominent adversary of quantum coherence is noise arising from the interaction of the associated dynamical system with its environment. Under certain conditions, however, the existence of noise may drive quantum and classical systems to endure intriguing nontrivial effects. In this vein, here we demonstrate, both theoretically and experimentally, that when two indistinguishable non-interacting particles co-propagate through quantum networks affected by non-dissipative noise, the system always evolves into a steady state in which coherences accounting for particle indistinguishabilty perpetually prevail. Furthermore, we show that the same steady state with surviving quantum coherences is reached even when the initial state exhibits classical correlations., Comment: arXiv admin note: substantial text overlap with arXiv:1709.04336

We demonstrate that when a waveguide beam splitter (BS) is excited by N indistinguishable photons, the arising multiphoton states evolve in a way as if they were coupled to each other with coupling strengths that are identical to the ones exhibited by a discrete fractional Fourier system. Based on the properties of the discrete fractional Fourier transform, we then derive a multiphoton suppression law for 50/50 BSs, thereby generalizing the Hong-Ou-Mandel effect. Furthermore, we examine the possibility of performing simultaneous multiphoton quantum random walks by using a single waveguide BS in combination with photon number resolving detectors. We anticipate that the multiphoton lattice-like structures unveiled in this work will be useful to identify new effects and applications of high-dimensional multiphoton states., Comment: Accepted for publication in JOSA B on June 26, 2018

We report the first experimental observation of multiple transitions showing the emergence and disappearance of slowly decaying eigenmodes in a dissipative, Floquet electronic system with synthetic components. Conventional wisdom has it that such transitions occur at exceptional points, and avoided-level-crossing driven phenomena in purely dissipative systems are formerly unexplored. Remarkably, in our system, the slowly decaying eigenmodes emerge without exceptional points. Our experimental setup makes use of an LC oscillator inductively coupled to an RLC oscillator, where the time-periodic (Floquet) inductive coupling and resistive-heating losses can be independently controlled by means of external voltage signals. With a Floquet dissipation, we observe that slowly-decaying eigenmodes emerge at vanishingly small dissipation strength in the weak coupling limit. With a moderate, Floquet coupling, multiple instances of their emergence and disappearance are observed. With an asymmetric dimer model, we show that these transitions, driven by avoided-level-crossing in purely dissipative systems, are generically present in both static and Floquet domains.

In this contribution we analyze virtual-state spectroscopy --- a unique tool for extracting information about the virtual states that contribute to the two-photon excitation of an absorbing medium --- as implemented by means of intense entangled beams with tunable spectral correlations. We provide a thorough description of all contributing terms (classical and quantum) in the two-photon absorption signal, as well as the limits imposed by the power of the pump that produces the entangled beams on the observability of the spectral lines of the virtual transitions. We find that virtual-state spectroscopy may be implemented with entangled twin beams carrying up to $10^4$ photon pairs. This implies that, in principle, one might be able to detect two-photon absorption signals up to four orders of magnitude larger than previously reported, thus paving the way towards the first experimental realization of the virtual-state spectroscopy technique., Comment: 8 pages, 5 figures, in print J. Opt. Soc. Am. B

Quantum coherence, the physical property underlying fundamental phenomena such as multi-particle interference and entanglement, has emerged as a valuable resource upon which exotic modern technologies are founded. In general, the most prominent adversary of quantum coherence is noise arising from the interaction of the associated dynamical system with its environment. Under certain conditions, however, the existence of noise may drive quantum and classical systems to endure intriguing nontrivial effects. Along these lines, here we demonstrate, both theoretically and experimentally, that when two indistinguishable particles co-propagate through quantum networks affected by noise, the system always evolves into a steady state in which coherences between certain separable states perpetually prevail. Furthermore, we show that the same steady state with surviving quantum coherences is reached irrespectively of the configuration in which the particles are prepared.

We use the concept of two-particle probability amplitude to derive the stochastic evolution equation for two-particle four-point correlations in tight-binding networks affected by diagonal dynamic disorder. It is predicted that in the presence of dynamic disorder, the average spatial wave function of indistinguishable particle pairs delocalizes and populates all network sites including those which are weakly coupled in the absence of disorder. Interestingly, our findings reveal that correlation elements accounting for particle indistinguishability are immune to the impact of dynamic disorder.

In this work we demonstrate single microparticle transport enabled by noise in a one dimensional optical lattice with periodic symmetric potentials and a small constant external force. The one dimensional lattice is implemented by six focused beams with holographic optical tweezers, where a microparticle is trapped in three dimensions. Transport initiates when dynamical disorder is added to the diffracted laser power at each trap ($\pm 30\%$) at a fixed frequency (0 to 35 Hz), while the direction of motion is set by the constant external force. We find that transport is only achieved within a narrow noise frequency range, which is consistent with simulations, and the predicted behavior and observations of noise-induced energy transport in quantum and classical systems. To our knowledge this is the first direct observation of noise-assisted transport in a colloidal system.

We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to successfully extract information about the intermediate material states that contribute to the two-photon excitation of an absorbing medium. Robustness of the presented method is examined with respect to the applied intervals of the frequency chirp., Comment: new version, accepted in Chemical Physics, 14 pages, 4 figures

Noise is generally thought as detrimental for energy transport in coupled oscillator networks. However, it has been shown that for certain coherently evolving systems, the presence of noise can enhance, somehow unexpectedly, their transport efficiency; a phenomenon called environment-assisted quantum transport (ENAQT) or dephasing-assisted transport. Here, we report on the experimental observation of such effect in a network of coupled electrical oscillators. We demonstrate that by introducing stochastic fluctuations in one of the couplings of the network, a relative enhancement in the energy transport efficiency of $22.5 \pm 3.6\,\%$ can be observed.