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It is particularly appealing for efficient active terahertz (THz) modulators using photonic structures to enhance light–matter interaction. Here, an optical controlled THz modulator is proposed that combines lead sulfide (PbS) quantum dots with subwavelength metallic split-ring resonators (SRRs) for providing field enhancement. The modulation depth reaches 60.3%, which is approximately 3 times larger than the PbS quantum dots film without SRRs (as reference) in the frequency range of 0.1–1.1 THz. Such significant enhanced THz modulation is mainly due to the local THz field enhancement caused by the SRRs, which is consistent with the simulation result.

The transport properties of charge carriers in MXene, a promising material, have been studied using terahertz time-domain spectroscopy (THz-TDS) to examine its potential applications in optical and electronic devices. However, previous studies have been limited by narrow frequency ranges, which have hindered the understanding of the intrinsic mechanisms of carrier transport in MXenes. To address this issue, ultrabroadband THz-TDS with frequencies of up to 15 THz to investigate the complex photoconductances of MXene (Ti 3 C 2 T x ) films with different thicknesses are employed. The findings indicate that the electronic localization is substrate-dependent, and this effect decreases with an increase in the number of layers. This is attributed to the screening effect of the high carrier density in Ti 3 C 2 T x . Additionally, the layer-independent photocarrier relaxations revealed by optical pump THz probe spectroscopy (OPTP) provide evidence of the carrier heating-induced screening effect. These results are significant for practical applications in both scientific research and various industries., (© 2023 Wiley‐VCH GmbH.)