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The native gate set is fundamental to the performance of quantum devices, as it governs the accuracy of basic quantum operations and dictates the complexity of implementing quantum algorithms. Traditional approaches to extending gate sets often require accessing multiple transitions within an extended Hilbert space, leading to increased control complexity while offering only a limited set of gates. Here, we experimentally demonstrate a unified and highly versatile gate scheme capable of natively generating arbitrary two-qubit gates using only exchange interaction and qubit driving on a superconducting quantum processor, achieving maximum expressivity. Using a state-of-the-art transmon-coupler-transmon architecture, we achieve high fidelities averaging $99.37 \pm 0.07\%$ across a wide range of commonly used two-qubit unitaries. This outstanding performance, combined with reduced complexity, enables precise multipartite entangled state preparation, as demonstrated. To further enhance its applicability, we also show the high-fidelity realization of the unique B gate, which efficiently synthesizes the entire family of two-qubit gates. Our results highlight that fully exploiting the capabilities of a single interaction can yield a comprehensive and highly accurate gate set. With maximum expressivity, gate-time optimality, demonstrated high fidelity, and easy adaptability to other quantum platforms, our unified control scheme paves the way for optimal performance in quantum devices, offering exciting prospects for advancing quantum hardware and algorithm development.

The discovery of superconductivity with onset temperature of ~80 K in pressurized bilayer Ruddlesden-Popper La3Ni2O7-d has attracted much attention. Despite intense research, determination of the exact oxygen content and understanding of the relationship between superconductivity and oxygen content remain a big challenge. Here, we report a systematical study on the structure and physical properties of La3Ni2O7-d polycrystalline powders which were prepared using sol-gel method at ambient pressure and then annealed under various oxygen pressure. We found that high pO2 annealing with slow cooling results in a new phase, which can be modeled using the hybrid single-layer-trilayer La3Ni2O7 or the tetragonal bilayer La3Ni2O7. Scanning transmission electron microscopy (STEM) measurements revealed significant single layers and trilayers after high oxygen pressure annealing, evidencing damage of the bilayer structure. The superconducting transition under high pressure became weak for high pO2 annealed samples, which is consistent with the damage of the bilayer structure. Our results reveal that the bilayer structure is fragile and post-annealing under near atmosphere pressure of oxygen is suitable to maintain bilayer structure and increase oxygen content at the same time., Comment: 5 figures and 1 table

The search for quantum spin liquids (QSL) and chemical doping in such materials to explore superconductivity have continuously attracted intense interest. Here, we report the discovery of a potential QSL candidate, pyrochlore-lattice beta-NaYbO2. Colorless and transparent NaYbO2 single crystals, layered alpha-NaYbO2 (~250 um on edge) and octahedral beta-NaYbO2 (~50 um on edge), were grown for the first time. Synchrotron X-ray single crystal diffraction unambiguously determined that the newfound beta-NaYbO2 belongs to the three-dimensional pyrochlore structure characterized by the R-3m space group, corroborated by synchrotron X-ray and neutron powder diffraction and pair distribution function. Magnetic measurements revealed no long-range magnetic order or spin glass behavior down to 0.4 K with a low boundary spin frustration factor of 17.5, suggesting a potential QSL ground state. Under high magnetic fields, the potential QSL state was broken and spins order. Our findings reveal that NaYbO2 is a fertile playground for studying novel quantum states., Comment: This document is the unedited author's version of a Submitted Work that was subsequently accepted for publication in Journal of the American Chemical Society, copyright American Chemical Society after peer review. To access the final edited and published work, a link will be provided soon

Recently, the Ruddlesden-Popper bilayer nickelate La3Ni2O7 has been discovered as a high temperature superconductor with Tc near 80 K above 14 GPa.[1-3] The search for nickelate superconductors with higher Tc, the preparation of high-quality single crystals, and the removal of high-pressure conditions including single crystal growth under high gas pressure and achievement of high Tc superconductivity under high pressure, are the most challenging tasks. Here, we present ambient pressure flux growth of high-quality bilayer nickelate single crystals with superconductivity up to 91 K under high pressure. Single crystals of bilayer La3-xRxNi2O7-y with dimensions up to 220 um on the edge were successfully grown using flux method at atmosphere conditions. Single crystal X-ray diffraction, nuclear quadrupole resonance, energy dispersion spectroscopy and scanning transmission electron microscopy measurements evidenced high quality of bilayer La2SmNi2O7-y single crystals in average structure and local structure. Superconductivity has been observed in high pressure resistivity measurements of annealed La2SmNi2O7-y single crystals with Tc onset up to 91 K, which is the highest among the known superconducting nickelates. Our results not only demonstrate a new and easy-to-access method for synthesizing high-quality bilayer nickelate single crystals, but also providing a direction for discovering superconducting nickelates with higher Tc., Comment: 4 figures and 1 table

Nickelates have attracted enormous attention since the discovery of high-temperature superconductivity in La3Ni2O7 under high pressure. However, whether superconducting nickelate single crystals can be prepared at ambient pressure remains elusive. Here we report signature of superconductivity in pressurized La4Ni3O10-x single crystals grown from potassium carbonate flux at ambient pressure. Single crystal X-ray diffraction and scanning transmission electron microscopy investigations re-vealed high-quality single crystals with perfect stacking of trilayers. Resistivity measurements indicate that the metal-to-metal transition observed at ambient pressure was suppressed under high pressure, and a sharp drop occurred at ~30 K at 77.9 GPa, consistent with superconductivity in pressurized La4Ni3O10 single crystals grown by the floating zone method at an oxygen pressure of >18 bar. Our results not only provide an important path to prepare high-quality nickelate single crystals but also support superconductivity in nickelates under high pressure, promoting more systematic and in-depth research in this compelling field., Comment: 3 figures

Quasi-two-dimensional averievites with triangle-kagome-triangle trilayers are of interest due to their rich structural and magnetic transitions and strong spin frustration that are expected to host quantum spin liquid ground state with suitable substitution or doping. Herein, we report growth of bulk single crystals of averievite CsClCu5V2O10 with dimensions of several millimeters on edge in order to (1) address the open question whether the room temperature crystal structure is P-3m1, P-3, P21/c or else, (2) to elucidate the nature of phase transitions, and (3) to study direction-dependent physical properties. Single-crystal-to-single-crystal structural transitions at ~305 K and ~127 K were observed in the averievite CsClCu5V2O10 single crystals. The nature of the transition at ~305 K, which was reported as P-3m1-P21/c transition, was found to be a structural transition from high temperature P-3m1 to low temperature P-3 by combining variable temperature synchrotron X-ray single crystal and high-resolution powder diffraction. In-plane and out-of-plane magnetic susceptibility and heat capacity measurements confirm a first-order transition at 305 K, a structural transition at 127 K and an antiferromagnetic transition at 24 K. These averievites are thus ideal model systems for a deeper understanding of structural transitions and magnetism., Comment: 7 figures

Spins in strongly frustrated systems are of intense interest due to the emergence of intriguing quantum states including superconductivity and quantum spin liquid. Herein we report the discovery of cascade of phase transitions and large magnetic anisotropy in the averievite CsClCu5P2O10 single crystals. Under zero field, CsClCu5P2O10 undergoes a first-order structural transition at around 225 K from high temperature centrosymmetric P-3m1 to low temperature noncentrosymmetric P321, followed by an AFM transition at 13.6 K, another structural transition centering at ~3 K, and another AFM transition at ~2.18 K. Based upon magnetic susceptibility and magnetization data with magnetic fields perpendicular to the ab plane, a phase diagram, consisting of a paramagnetic state, two AFM states and four field-induced states including two magnetization plateaus, has been constructed. Our findings demonstrate that the quasi-2D CsClCu5P2O10 exhibits rich structural and metamagnetic transitions and the averievite family is a fertile platform for exploring novel quantum states., Comment: 15 pages, 5 figures

The ability to fast reset a qubit state is crucial for quantum information processing. However, to actively reset a qubit requires engineering a pathway to interact with a dissipative bath, which often comes with the cost of reduced qubit protection from the environment. Here, we present a novel multi-purpose architecture that enables fast reset and protection of superconducting qubits during control and readout. In our design, two on-chip diplexers are connected by two transmission lines. The high-pass branch provides a flat passband for convenient allocation of readout resonators above the qubit frequencies, which is preferred for reducing measurement-induced state transitions. In the low-pass branch, we leverage a standing-wave mode below the maximum qubit frequency for a rapid reset. The qubits are located in the common stopband to inhibit dissipation during coherent operations. We demonstrate resetting a transmon qubit from its first excited state to the ground state in 100 ns, achieving a residual population of 2.7%. The reset time may be further shortened to 27 ns by exploiting the coherent population inversion effect. We further extend the technique to resetting the qubit from its second excited state. Our approach promises scalable implementation of fast reset and qubit protection during control and readout, adding to the toolbox of dissipation engineering., Comment: 8 pages, 4 figures

Shear Alfven wave parametric decay instability (PDI) provides a potential path toward significant wave dissipation and plasma heating. However, fundamental questions regarding how PDI is excited in a realistic three-dimensional (3D) open system and how critically the finite perpendicular wave scale--as found in both laboratory and space plasmas--affects the excitation remain poorly understood. Here, we present the first 3D, open-boundary, hybrid kinetic-fluid simulations of kinetic Alfven wave PDI in low-beta plasmas. Key findings are that the PDI excitation is strongly limited by the wave damping present, including electron-ion collisional damping (represented by a constant resistivity) and geometrical attenuation associated with the finite-scale Alfven wave, and ion Landau damping of the child acoustic wave. The perpendicular wave scale alone, however, plays no discernible role: waves of different perpendicular scales exhibit similar instability growth as long as the magnitude of the parallel ponderomotive force remains unchanged. These findings are corroborated by theoretical analysis and estimates. The new understanding of 3D kinetic Alfv\'en wave PDI physics is essential for laboratory study of the basic plasma process and may also help evaluate the relevance/role of PDI in low-beta space plasmas., Comment: 8 pages, 3 figures

$\alpha$-TeO2 is widely used in acousto-optic devices due to its excellent physical properties. Conventionally, $\alpha$-TeO2 single crystals were grown using melt methods. Here, we report for the first time the growth of $\alpha$-TeO2 single crystals using the aqueous solution method below 100 {\deg}C. Solubility curve of $\alpha$-TeO2 was measured, and then single crystals with dimensions of 3.5x3.5x2.5 mm3 were successfully grown using seed crystals that were synthesized from spontaneous nucleation. The as-grown single crystals belong to the P41212 space group, evidenced by single crystal X-ray diffraction and Rietveld refinement on powder diffraction. Rocking curve measurements show that the as-grown crystals exhibit high crystallinity with a full-width at half maxima (FWHM) of 57.2''. Ultraviolet-Visible absorption spectroscopy indicates the absorption edge is 350 nm and the band gap is estimated to be 3.58 eV. The density and Vickers hardness of as-grown single crystals are measured to be 6.042 g/cm3 and 404 kg/mm2, repectively. Our findings provide an easy-to-access and energy-saving method for growing single crystals of inorganic compounds., Comment: 14 pages, 8 figures

Advancement of technologies relies on discovery of new materials with emerging physical properties that are determined by their crystal structures. Ruddlesden-Popper (R-P) phases with formula of $A_{n+1}$$B_n$$X_{3n+1}$ (n=1,2,3...) are among one of the most widely studied class of materials due to their electrical, optical, magnetic, thermal properties and their combined multifunctional properties(Ref.1-6). In R-P phases, intergrowth is well-known in the short range(Ref.7-9); however, no existing compounds have been reported to have different n mixed in bulk single crystals. Here we design a hybrid R-P nickelate $La_2NiO_4$$La_3Ni_2O_7$ by alternatively stacking bilayers, which is the active structural motif in the newly discovery high-$T_c$ superconductor $La_3Ni_2O_7$ and single layers of the antiferromagnetic insulator $La_2NiO_4$. We report the successful synthesis of $La_2NiO_4$$La_3Ni_2O_7$ single crystals, and X-ray diffraction and real-space imaging vis STEM show that the crystal structure consists of single layers and bilayers of $NiO_6$ octahedral stacking alternatively perpendicular to the ab plane, characterized by the orthorhombic Immm (No.71) space group. Resistivity measurements indicate a peculiar insulator-to-metal transition around 140 K on cooling. Correlated density functional theory calculations corroborate this finding, and reveal that the single layer becomes paramagnetic metallic due to charge transfer via LaO layers. The discovery of $La_2NiO_4$$La_3Ni_2O_7$ opens a door to access a completely new family of 3D hybrid R-P phases with the formula of $A_{n+1}$$B_n$$X_{3n+1}$$A'_{m+1}$$B'_m$$X'_{3m+1}$ which potentially host a plethora of emerging physical properties for various applications., Comment: 27 pages, 4 figures

Image inverse halftoning is a classic image restoration task, aiming to recover continuous-tone images from halftone images with only bilevel pixels. Because the halftone images lose much of the original image content, inverse halftoning is a classic ill-problem. Although existing inverse halftoning algorithms achieve good performance, their results lose image details and features. Therefore, it is still a challenge to recover high-quality continuous-tone images. In this paper, we propose an end-to-end multiscale progressively residual learning network (MSPRL), which has a UNet architecture and takes multiscale input images. To make full use of different input image information, we design a shallow feature extraction module to capture similar features between images of different scales. We systematically study the performance of different methods and compare them with our proposed method. In addition, we employ different training strategies to optimize the model, which is important for optimizing the training process and improving performance. Extensive experiments demonstrate that our MSPRL model obtains considerable performance gains in detail restoration.

Large-amplitude Alfv\'en waves are subject to parametric decays which can have important consequences in space, astrophysical, and fusion plasmas. Though the Alfv\'en wave parametric decay instability was predicted decades ago, observational evidence is limited, stimulating considerable interest in laboratory demonstration of the instability and associated numerical modeling. Here, we report novel hybrid simulation of the Alfv\'en wave parametric decay instability in a laboratory relevant plasma (based on the Large Plasma Device), using realistic wave injection and wave-plasma parameters. Considering only collisionless damping, we identify the threshold Alfv\'en wave amplitudes and frequencies required for triggering the instability in the bounded plasma. These threshold behaviors are corroborated by simple theoretical considerations. Other effects not included in the present model such as finite transverse scale and ion-neutral collision are briefly discussed. These hybrid simulations demonstrate a promising tool for investigating laboratory Alfv\'en wave dynamics that can provide guidance for future laboratory demonstration of the parametric decay instability., Comment: 8 pages, 3 figures

The parametric decay of finite-size Alfv\'en waves in nonperiodic low-beta plasmas is investigated using one-dimensional hybrid simulations. Compared with the usual small periodic system, a wave packet in a large system under the absorption boundary condition shows different decay dynamics, including reduced energy transfer and localized density cavitation and ion heating. The resulting Alfv\'en wave dynamics are influenced by several factors of the instability including the growth rate, central wave frequency, and unstable bandwidth. A final steady state of the wave packet may be achieved when the instability does not have enough time to develop within the residual packet, and the packet size shows well-defined scaling dependencies on the growth rate, wave amplitude, and plasma beta. Under the proper conditions enhanced secondary decay can also be excited in the form of a narrow, amplified wavepacket. These results may help interpret laboratory and spacecraft observations of Alfv\'en waves, and refine our understanding of associated energy transport and ion heating., Comment: 11 pages, 5 figures

Relativistic temperature electrons higher than 0.5 MeV are generated typically with laser intensities of about 10$^{18}$ W/cm$^{2}$. Their generation with high repetition rate lasers that operate at non-relativistic intensities ($\simeq$10$^{16}$ W/cm$^{2}$) is cardinal for the realization of compact, ultra-short, bench-top electron sources. New strategies, capable of exploiting different aspects of laser-plasma interaction, are necessary for reducing the required intensity. We report here, a novel technique of dynamic target structuring of microdroplets, capable of generating 200 keV and 1 MeV electron temperatures at 1/100th of the intensity required by ponderomotive scaling($10^{18}$ W/cm$^2$) to generate relativistic electron temperature. Combining the concepts of pre-plasma tailoring, optimized scale length and micro-optics, this method achieves two-plasmon decay boosted electron acceleration with "non-ideal" ultrashort (25 fs) pulses at $4\times10^{16}$ W/cm$^2$, only. With shot repeatability at kHz, this precise in-situ targetry produces directed, imaging quality beam-like electron emission up to 6 MeV with milli-joule class lasers, that can be transformational for time-resolved, microscopic studies in all fields of science., Comment: Main text- 9 pages, 4 figures. Comments are welcome