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Based on the three-dimensional field of molten pool and twin-roll strip casting experiments, this work verified the cracking mechanism of the strip by establishing mathematical model and rolling experiments. The results showed that due to the instability of the thermophysical field of the molten pool and the inconsistency of kiss curve height, the newly solidified strip will undergo incompatible deformation through the rolling. The stress concentration will appear around the large reduction area and then form slip bands. When plastic strain exceeds the limit of the metal, the oblique cracks will appear in the slip bands periodically or completely penetrate the strip. In addition, tensile cracks could also be produced by incompatible deformation. Therefore, keeping the uniformity and stability of the thermal physical field in molten pool is the key factor to restrain cracks.