1. Aerosol Effects on Water Cloud Properties in Different Atmospheric Regimes.
- Author
-
Khatri, P., Yoshida, K., and Hayasaka, T.
- Subjects
AIR pollution control ,CLOUD condensation nuclei ,AIR pollution ,AEROSOLS ,ATMOSPHERIC aerosols ,WEATHER control ,ATMOSPHERE - Abstract
Aerosol‐cloud interaction remains one of the least understood processes in climate science arena, despite its profound impacts in radiation and water budget perturbations. The aerosol effects on clouds largely depend on aerosol characteristics. Here, we implemented 17‐year (2003–2020) data set of aerosol, cloud, and meteorological factors collected over East Asia—a highly polluted region with recent decreasing trend of air pollution due to control measures—to elucidate atmospheric regime‐dependent aerosol effects on water cloud properties by simultaneously accessing the response of air pollution control measures in cloud field. The study found a very close relationship between aerosol loading and cloud properties modifications in the continental region of East Asia with a significant response of air pollution control measures in the cloud field. The study further revealed that aerosols of the polluted continental atmosphere affected cloud micro‐ and macro‐physics differently than aerosols of the clean maritime atmosphere: in the former, increased aerosol loading increased the stability under cloud base and then enhanced cloud droplet collision‐coalescence process, resulting to increase cloud droplet size by decreasing cloud top height; whereas in the latter, increased aerosol loading decreased cloud droplet size without notable influence in the atmosphere thermodynamics and cloud top height. This study further showed a complex aerosol‐cloud interaction process in the polluted maritime atmosphere due to the mixed effect of polluted continental and clean maritime atmospheres. In all atmospheric regimes, cloud fraction was found to increase with the increase of aerosol loading. Plain Language Summary: Aerosols can act as cloud condensation nuclei to modify water cloud properties and then climate system and water cycle. At the same time, these aerosols scatter and absorb solar radiation, which can perturb atmospheric heating. Such change in the atmospheric heating can also play an important role in cloud properties modification. Because of such different routes, aerosol‐cloud interaction (ACI) remains one of the least understood topics in climate science. As ACI is strongly driven by aerosol property, it is important to investigate ACI process for different atmospheric backgrounds. This study analyzed a long‐term data of aerosol, cloud, and meteorological factors collected over East Asia, which is one of the major air pollution regions in the world, although air pollution is decreasing gradually in recent years. By analyzing data corresponding to different atmospheric regimes, we showed that aerosols of continental atmosphere can modify cloud micro‐ and macro‐physics by modifying atmospheric thermodynamics; whereas aerosols of maritime atmosphere are less capable to modify atmospheric thermodynamics, but they can decrease cloud droplet size. On the other hand, we found a complex ACI in polluted maritime atmosphere due to mixed effect of polluted continental and maritime atmospheric regimes. Key Points: Continental aerosols of East Asia were noted to strongly modulate cloud properties in time series analysesIncreased aerosols of polluted continental atmosphere increased cloud droplet size by modulating atmospheric thermodynamicsIncreased aerosols of clean maritime atmosphere decreased cloud droplet size without notable influence in atmospheric thermodynamics [ABSTRACT FROM AUTHOR]
- Published
- 2023
- Full Text
- View/download PDF