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We present 5 deg^2 (~250 pc^2) HCN, HNC, HCO+, and CO J=1-0 maps of the Orion B GMC, complemented with existing wide-field [CI] 492 GHz maps, as well as new pointed observations of rotationally excited HCN, HNC, H13CN, and HN13C lines. We detect anomalous HCN J=1-0 hyperfine structure line emission almost everywhere in the cloud. About 70% of the total HCN J=1-0 luminosity arises from gas at A_V < 8 mag. The HCN/CO J=1-0 line intensity ratio shows a bimodal behavior with an inflection point at A_V < 3 mag typical of translucent gas and UV-illuminated cloud edges. We find that most of the HCN J=1-0 emission arises from extended gas with n(H2) ~< 10^4 cm^-3, even lower density gas if the ionization fraction is > 10^-5 and electron excitation dominates. This result explains the low-A_V branch of the HCN/CO J=1-0 intensity ratio distribution. Indeed, the highest HCN/CO ratios (~0.1) at A_V < 3 mag correspond to regions of high [CI] 492 GHz/CO J=1-0 intensity ratios (>1) characteristic of low-density PDRs. Enhanced FUV radiation favors the formation and excitation of HCN on large scales, not only in dense star-forming clumps. The low surface brightness HCN and HCO+ J=1-0 emission scale with I_FIR (a proxy of the stellar FUV radiation field) in a similar way. Together with CO J=1-0, these lines respond to increasing I_FIR up to G0~20. On the other hand, the bright HCN J=1-0 emission from dense gas in star-forming clumps weakly responds to I_FIR once the FUV radiation field becomes too intense (G0>1500). The different power law scalings (produced by different chemistries, densities, and line excitation regimes) in a single but spatially resolved GMC resemble the variety of Kennicutt-Schmidt law indexes found in galaxy averages. As a corollary for extragalactic studies, we conclude that high HCN/CO J=1-0 line intensity ratios do not always imply the presence of dense gas., Comment: accepted for publication in A&A. 24 pages, 18 figures, plus Appendix. Abridged Abstract

We present the first detection of HCO$^+$ absorption in the Magellanic System. Using the Australia Telescope Compact Array (ATCA), we observed 9 extragalactic radio continuum sources behind the Magellanic System and detected HCO$^+$ absorption towards one source located behind the leading edge of the Magellanic Bridge. The detection is located at LSR velocity of $v=214.0 \pm 0.4\rm\,km\,s^{-1}$, with a full width at half maximum of $\Delta v=4.5\pm 1.0\rm\,km\,s^{-1}$ and optical depth of $\tau(\rm HCO^+)=0.10\pm 0.02$. Although there is abundant neutral hydrogen (HI) surrounding the sightline in position-velocity space, at the exact location of the absorber the HI column density is low, $<10^{20}\rm\,cm^{-2}$, and there is little evidence for dust or CO emission from Planck observations. While the origin and survival of molecules in such a diffuse environment remains unclear, dynamical events such as HI flows and cloud collisions in this interacting system likely play an important role., Comment: Accepted for publication in ApJ. 6 pages, 2 figures, 2 tables

To study the usefulness of \CFP\ as a tracer of the regions where C\p\ and \HH\ coexist in the interstellar medium. We used the Plateau de Bure Interferometer to synthesize \CFP\ J=1-0 absorption at 102.6 GHz toward the core of the distant HII region W49N at l = 43.2\degr, b=0.0\degr, and we modeled the fluorine chemistry in diffuse/translucent molecular gas. We detected \CFP\ absorption over a broad range of velocity showing that \CFP\ is widespread in the \HH-bearing Galactic disk gas. Originally detected in dense gas in the Orion Bar and Horsehead PDR, \CFP\ was subsequently detected in absorption from diffuse and translucent clouds seen toward \bll\ and 3C111. Here we showed that \CFP\ is distributed throughout the diffuse and translucent molecular disk gas with N(\CFP)/N(\HH) $= 1.5-2.0\times10^{-10}$, increasing to N(\CFP)/N(\HH) $= 3.5\times10^{-10}$ in one cloud at 39 \kms\ having higher N(\HH) $\approx 3\times10^{21}\pcc$. Models of the fluorine chemistry reproduce the observed column densities and relative abundance of HF, from which \CFP\ forms, but generally overpredict the the column density of \CFP\ by factors of 1.4-4. We show that a free space photodissociation rate $\Gamma \ga 10^{-9}\ps$, comparable to that of CH, might account for much of the discrepancy but a recent calculation finds a value about ten times smaller. In the heavily blended and kinematically complex spectra seen toward W49, \CFP\ absorption primarily traces the peaks of the \HH\ distribution., Comment: A&A in press

A major goal of the Atacama Large Millimeter/submillimeter Array (ALMA) is to make accurate images with resolutions of tens of milliarcseconds, which at submillimeter (submm) wavelengths requires baselines up to ~15 km. To develop and test this capability, a Long Baseline Campaign (LBC) was carried out from September to late November 2014, culminating in end-to-end observations, calibrations, and imaging of selected Science Verification (SV) targets. This paper presents an overview of the campaign and its main results, including an investigation of the short-term coherence properties and systematic phase errors over the long baselines at the ALMA site, a summary of the SV targets and observations, and recommendations for science observing strategies at long baselines. Deep ALMA images of the quasar 3C138 at 97 and 241 GHz are also compared to VLA 43 GHz results, demonstrating an agreement at a level of a few percent. As a result of the extensive program of LBC testing, the highly successful SV imaging at long baselines achieved angular resolutions as fine as 19 mas at ~350 GHz. Observing with ALMA on baselines of up to 15 km is now possible, and opens up new parameter space for submm astronomy., Comment: 11 pages, 7 figures, 2 tables; accepted for publication in the Astrophysical Journal Letters; this version with small changes to affiliations

We modelled recent observations of UV absorption of HD and \HH\ in the Milky Way and toward damped/sub-damped Lyman alpha systems at z=0.18 and z $>$ 1.7. N(HD)/N(\HH) ratios reflect the separate self-shieldings of HD and \HH\ and the coupling introduced by deuteration chemistry. Locally, observations are explained by diffuse molecular gas with $ 16 \pccc \la$ n(H) $\la 128 \pccc $ if the cosmic-ray ionization rate per H-nucleus \zetaH $= 2\times 10^{-16}\ps$ as inferred from \H3\p\ and OH\p. The dominant influence on N(HD)/N(\HH) is the cosmic-ray ionization rate with a much weaker downward dependence on n(H) at Solar metallicity, but dust-extinction can drive N(HD) higher as with N(\HH). At z $>$ 1.7, N(HD) is comparable to the Galaxy but with 10x smaller N(\HH) and somewhat smaller N(\HH)/N(H I). Comparison of our Galaxy and the Magellanic Clouds shows that smaller \HH/H is expected at sub-Solar metallicity and we show by modelling that HD/\HH\ increases with density at low metallicity, opposite to the Milky Way. Observations of HD would be explained with higher n(H) at low metallicity but high-z systems have high HD/\HH\ at metallicity 0.04 $\la$ Z $\la$ 2 Solar. In parallel we trace dust-extinction and self-shielding effects. The abrupt \HH\ transition to \HH/H $\approx$ 1-10% occurs mostly from self-shielding although it is assisted by extinction for n(H) $\la 16 \pccc$. Interior \HH\ fractions are substantially increased by dust extinction below $\la 32\pccc$. At smaller n(H), \zetaH, small increases in \HH\ triggered by dust extinction can trigger abrupt increases in N(HD)., Comment: Accepted for Ap J

We explore the relationship between dust-emission derived reddening \EBV\ and atomic hydrogen column density N(H I) derived from 21 cm emission surveys. We consider measurements at galactic latitude $|b| \ga 20$\degr\ and \EBV\ $\la$ 0.1 mag where the interstellar gas is predominantly neutral and atomic and opacity corrections to 21cm H I profiles are small. Over the Galaxy at large at lower resolution in H I, and on smaller scales at higher resolution, we find that the reddening is always much smaller than would be expected from the usually-quoted relation N(H) $ = 5.8\times 10^{21}\pcc$ \EBV\ based on stellar reddening and {\it uv} absorption toward early-type stars. On wide scales, we find N(H I) = $8.3 \times 10^{21}\pcc$ \EBV. We cite various precedents for such a large N(H I)/\EBV\ ratio whenever wide-field 21cm emission surveys are considered, including when reddening based on galaxy counts or colors is substituted for the dust-emission derived reddening measure., Comment: Accepted for ApJ

We wish to relate the degree scale structure of galactic diffuse clouds to sub-arcsecond atomic and molecular absorption spectra obtained against extragalactic continuum background sources. To do this, we used the ARO 12m telescope to map J=1-0 CO emission at 1' resolution over 30' fields around the positions of 11 background sources occulted by 20 molecular absorption line components, of which 11 had CO emission counterparts. We compare maps of CO emission to sub-arcsec atomic and molecular absorption spectra and to the large-scale distribution of interstellar reddening. The main results are: 1) Typical covering factors of individual features at the 1 K.km/s level were 20%. 2) CO-H2 conversion factors as much as 4-5 times below the mean value N(H2)/Wco = 2e20 H2 cm^-2 /(K.km/s) are required to explain the luminosity of CO emission at/above the level of 1 K.km/s. Small conversion factors and sharp variability of the conversion factor on arcminute scales are due primarily to CO chemistry and need not represent unresolved variations in reddening or total column density. Hence, like FERMI and PLANCK we see some gas that is dark in CO and other gas in which CO is overluminous per H2. A standard CO-H2 conversion factor applies overall owing to balance between the luminosities per H2 and surface covering factors of bright and dark CO., but with wide variations., Comment: 23 pages, 22 PostScript figures. Accepted for publication in Astronomy \& Astrophysics. Uses aa LaTeX macros

12C/13C isotopologue abundance anomalies have long been predicted for gas-phase chemistry in molecules other than CO and have recently been observed in the Taurus molecular cloud in several species hosting more than one carbon atom, i.e. CCH, CCS, CCCS and HC$_3$N. Here we work to ascertain whether these isotopologic anomalies actually result from the predicted depletion of the 13C+ ion in an oxygen-rich optically-shielded dense gas, or from some other more particular mechanism or mechanisms. We observed $\lambda$3mm emission from carbon, sulfur and nitrogen-bearing isotopologues of HNC, CS and \HH CS at three positions in Taurus(TMC1, L1527 and the ammonia peak) using the ARO 12m telescope. We saw no evidence of 12C/13C anomalies in our observations. Although the pool of C+ is likely to be depleted in 13C 13C is not depleted in the general pool of carbon outside CO, which probably exists mostly in the form of C^0. The observed isotopologic abundance anomalies are peculiar to those species in which they are found., Comment: Accepted for publication in The Astrophysical Journal (mail journal)

[This is truncated to suit the whims of the archivers ...] Parameter studies in LVG models are used to show how the low-lying rotational transitions of common polar molecules HCO+, HCN and CS vary with number density, column density and electron fraction; with molecular properties such as the charge state and permanent dipole moment; and with observational details such as the transition that is observed. Physically-based models are used to check the parameter studies and provide a basis for relating the few extant observations. The parameter studies of LVG radiative transfer models show that lines of polar molecules are uniformly brighter for ions, for lower J-values and for higher dipole moments. Excitation by electrons is more important for J=1-0 lines and contributes rather less to the brightness of CS J=2-1 lines. If abundances are like those seen in absorption, the HCO+ J=1-0 line will be the brightest line after CO, followed by HCN (1-0) and CS (2-1). Because of the very weak rotational excitation in diffuse clouds, emission brightnesses and molecular column densities retain a nearly-linear proportionality under fixed physical conditions, even when transitions are quite optically thick; this implies that changes in relative intensities among different species can be used to infer changes in their relative abundances., Comment: To appear in A&A

To interpret the galactic center H II region complexes as constituents of a barred galaxy's nuclear star-forming ring, we compare 18cm VLA radiocontinuumm, $8-22\mu$ MSX IR and 2.6mm BTL and ARO12m CO emission in the inner few hundred pc. Galactic center H II regions are comparable in their IR appearance, luminosity and SED to M17 or N!0, but the IR light distribution is strongly modified by extinction at 8-22$\mu$, locally and overall. In Sgr B2 at $l > 0.6$\degr strong radio H II regions are invisible in the IR. In two favorable cases, extinction from individual galactic center molecular clouds is shown to have $\tau \ga 1$ at 8-22$\mu$ independent of wavelength. The gas kinematics are mostly rotational but with systematic $\pm 30-50$ \kms non-circular motion. Sgr B and C both show the same shell and high-velocity cap structure. The H II regions lie in a slightly-inclined ring of radius $\approx$ 180 pc (1.2\degr) whose near side appears at higher latitude and lower velocity and contains Sgr B. Sgr C is on the far side and both Sgr B and C represent collisions with material inflowing along the galactic dust lanes. Sgr E is a coincidental aggregation of field objects seen tangent to the ring's outer edge. Most of the volume interior to the ring is probably devoid of dense gas and some emission seen at v=20-70 \kms toward Sgr A lies outside it, in the ring., Comment: 14 Figures 15 pages, submitted to A&A 9 May 2009, figures are slightly degraded in this version to accomodate on-screen viewing

The field just West of the galactic supernova remnant W28 (l=6.4\degr, b=-0.2\degr) harbors 3 of 5 newly-discovered 1720 OH maser spots and two recently-discovered candidate supernova candidates (one of which is a $\gamma$-ray source), as well as several compact and classical HII regions. Here, we analyze a datacube of CO J=1-0 emission having 1\arcmin and 1 \kms resolution, made with on-the-fly mapping over the region $5\degr \le l \le 6\degr, -1\degr \le b \le 0.5\degr$}. {Extended and often very bright CO emission was detected at the velocities of the 1720 MHz OH masers and around the supernova remnant G5.55+0.32 which lacks a maser. A new bipolar outflow which is marginally resolved at 1\arcmin resolution and strong in CO (12K) was detected at the periphery of G5.55+0.32, coincident with an MSX source; there is also a bright rim of CO just beyond the periphery of the radio remnant. The OH maser near G5.71-0.08 lies on a shell of strongly-emitting molecular gas (up to 20K) . At the -21 \kms velocity of G5.4-1.2, CO covers much of the field but is weak (3 K) and undisturbed near the remnant. The extended molecular gas around the compact H II region and outflow in G5.89-0.39 (W28A2) is shown for the first time.}, Comment: 6 Pages, 3 figures submitted to A&A 4 May 2009

Methods: The microscopic equations of H2-formation and protonation are integrated numerically over time in such a manner that the overall structures evolve self-consistently under benign conditions. Results: The equilibrium H2 formation timescale in an H I cloud with N(H) ~ 4x10^{20}/cm^2 is 1-3 x 10^7 yr, nearly independent of the assumed density or H2 formation rate constant on grains, etc. Attempts to speed up the evolution of the H2-fraction would require densities well beyond the range usually considered typical of diffuse gas. The calculations suggest that, under benign, quiescent conditions, formation of H2 is favored in larger regions having moderate density, consistent with the rather high mean kinetic temperatures measured in H2, 70-80 K. Formation of H3+ is essentially complete when H2-formation equilibrates but the final abundance of H3+ appears more nearly at the very last instant. Chemistry in a weakly-molecular gas has particular properties so that the abundance patterns change appreciably as gas becomes more fully molecular, either in model sequences or with time in a single model. One manifestation of this is that the predicted abundance of H3+ is much more weakly dependent on the cosmic-ray ionization rate when n(H2)/n(H) < 0.05. In general, high abundances of H3+ do not enhance the abundances of other species (e.g. HCO+) but late-time OH formation proceeds most vigourously in more diffuse regions having modest density, extinction and H2 fraction and somewhat higher fractional ionization, suggesting that atypically high OH/H2 abundance ratios might be found optically in diffuse clouds having modest extinction.

Aims: We show the existence of a small family of inner-galaxy dust lanes and dust lane standing shocks beyond the two major ones that were previously known to exist Methods: We analyze images of CO emission in the inner regions of the Galaxy Results: The peculiar kinematics of the major dust lane features are repeated in several other distinct instances at l > 0deg, in one case at a contrary location 100 pc above the galactic equator at l > 3degr at the upper extremity of Clump 2. Like the previously-known dust lanes, these new examples are alsoassociated with localized, exceptionally broad line profiles believed to be characteristic of the shredding of neutral gas at the standing dust lane shocks. Conclusions: There may be secondary dust lane and standing shocks in the Milky Way bulge. The vertical structure provides a temporal sequence for understanding the secular evolution of gas flow in the bar.

Context: Over the past thirty years a wealth of observations of CO and other molecules in optical/uv absorption in diffuse clouds has accumulated for which no comparable CO emission line data exist. Aims: To acquire mm-wave J=1-0 CO emission line profiles toward a substantial sample of commonly-studied optical/uv absorption line targets and to compare with the properties of the absorbing gas, especially the predicted emission line strengths. Methods: Using the ARO 12m telescope we observed mm-wavelength J=1-0 CO emission with spectral resolution R ~ 3x10^6 and spatial resolution 1' toward a sample of 110 lines of sight previously studied in optical/uv absorption lines of CO, \HH, CH, etc. Results: Interstellar CO emission was detected along 65 of the 110 lines of sight surveyed and there is a general superabundance of CO emission given the distribution of galactic latitudes in the survey sample. Much of the emission is optically thick or very intense and must emanate from dark clouds or warm dense gas near HII regions. Conclusions: Judging from the statistical superabundance of CO emission, seen also in the total line of sight reddening, the OB star optical/uv absorption line targets must be physically associated with the large quantities of neutral gas whose CO emission was detected, in which case they are probably influencing the absorbing gas by heating and/or photoionizing it. This explains why CO/H2 and 12CO/13CO ratios differ somewhat between $uv$ and mm-wave absorption line studies. Because the lines of sight have been preselected to have AV < 1 mag, relatively little of the associated material actually occults the targets, making it difficult for CO emission line observations to isolate the foreground gas contribution.

Context: An unexpectedly complex polyatomic chemistry exists in diffuse clouds, allowing detection of species such as C2H, C3H2, H2CO and NH3 which have relative abundances that are strikingly similar to those inferred toward the dark cloud TMC-1 Aims: We probe the limits of complexity of diffuse cloud polyatomic chemistry. Methods: We used the IRAM Plateau de Bure Interferometer to search for galactic absorption from low-lying J=2-1 rotational transitions of A- and E-CH3OH near 96.740 GHz and used the VLA to search for the J=8-7 transition of HC5N at 21.3 GHz. Results: Neither CH3OH nor HC5N were detected at column densities well below those of all polyatomics known in diffuse clouds and somewhat below the levels expected from comparison with TMC-1. The HCN/HC5N ratio is at least 3-10 times higher in diffuse gas than toward TMC-1. Conclusions: It is possible to go to the well once (or more) too often

Methods: 12CO emission is imaged in position and position-velocity space analyzed statistically, and then compared with maps of total reddening and with models of the C+ - CO transition in H2-bearing diffuse clouds. Results: Around Zeta Oph, 12CO emission appears in two distinct intervals of reddening centered near EBV = 0.4 and 0.65 mag, of which < 0.2 mag is background material. Within either interval, the integrated 12CO intensity varies up to 6-12 K-km/s compared to 1.5 K-km/s toward Zeta Oph. Nearly 80% of the individual profiles have velocity dispersions < 0.6 km/s, which are subsonic at the kinetic temperature derived from H2 toward Zeta Oph, 55 K. Partly as a result, 12CO emission exposes the internal, turbulent, supersonic (1-3 km/s) gas flows with especial clarity in the cores of strong lines. The flows are manifested as resolved velocity gradients in narrow, subsonically-broadened line cores. Conclusions: The scatter between N(CO) and EBV in global, CO absorption line surveys toward bright stars is present in the gas seen around Zeta Oph, reflecting the extreme sensitivity of N(12CO) to ambient conditions. The two-component nature of the optical absorption toward Zeta Oph is coincidental and the star is occulted by a single body of gas with a complex internal structure, not by two distinct clouds. The very bright 12CO lines in diffuse gas arise at N(H2) ~ 10^21/cm^2 in regions of modest density n(H) ~ 200-500/cc and somewhat more complete C+-CO conversion. Given the variety of structure in the foreground gas, it is apparent that only large surveys of absorption sightlines can hope to capture the intrinsic behavior of diffuse gas., Comment: 2009 A&A, in press

Aims: Our aims are threefold: a) To compare the $uv$ and mm-wave results; b) to interpret 13CO and 12CO abundances in terms of the physical processes which separately and jointly determine them; c) to interpret observed J=1-0 rotational excitation and line brightness in terms of ambient gas properties. Methods: A simple phenomenological model of CO formation as the immediate descendant of quiescently-recombining HCO+ is used to study the accumulation, fractionation and rotational excitation of CO in more explicit and detailed models of H2-bearing diffuse/H I clouds Results: The variation of N(CO) with N(H2) is explained by quiescent recombination of a steady fraction n(HCO+)/n(H2) = 2 x 10^{-9}. Observed N(12CO))/N(13CO) ratios generally do not require a special chemistry but result from competing processes and do not provide much insight into the local gas properties, especially the temperature. J=1-0 CO line brightnesses directly represent N(CO), not N(H2), so the CO-H2 conversion factor varies widely; it attains typical values at N(12CO) \la 10^{16}cm^{-2}. Models of CO rotational excitation account for the line brightnesses and CO-H2 conversion factors but readily reproduce the observed excitation temperatures and optical depths of the rotational transitions only if excitation by H-atoms is weak -- as seems to be the case for the very most recent calculations of these excitation rates., Comment: 11 pages, 6 figures, A&A 2007 or 2008 (in press)

Using data from IRAM's Plateau de Bure Interferometer and 30 m Telescope, we discuss the mm-wave absorption lines of CS, SO, H2S and HCS+ which arise in diffuse clouds occulting several extragalactic continuum sources. Typical relative abundances are X(CS)/X(HCO+) ~ 2, X(CS)/X(SO) ~ 2, X(CS)/X(H2S) ~ 6 and X(CS)/X(HCS+) ~ 13., Comment: Accepted by A&A 2002-Jan-10