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In a PN junction, the separation between positive and negative charges leads to diode transport. In the past few years, the intrinsic diode transport in noncentrosymmetric polar conductors has attracted great interest, because it suggests novel nonlinear applications and provides a symmetry-sensitive probe of Fermi surface. Recently, such studies have been extended to noncentrosymmetric superconductors, realizing the superconducting diode effect. Here, we show that, even in a centrosymmetric crystal without directional charge separation, the spins of an antiferromagnet (AFM) can generate a spatial directionality, leading to an AFM diode effect. We observe large second-harmonic transport in a nonlinear electronic device enabled by the compensated AFM state of even-layered MnBi2Te4. We also report a novel electrical sum-frequency generation (SFG), which has been rarely explored in contrast to the well-known optical SFG in wide-gap insulators. We demonstrate that the AFM enables an in-plane field-effect transistor and harvesting of wireless electromagnetic energy. The electrical SFG establishes a powerful method to study nonlinear electronics built by quantum materials. The AFM diode effect paves the way for potential device concepts including AFM logic circuits, self-powered AFM spintronics, and other applications that potentially bridge nonlinear electronics with AFM spintronics., Comment: 33+8 pages, 14+2 figures. arXiv admin note: text overlap with arXiv:2306.09575

We study the charmed meson and baryon production and elliptic flow in ultra-relativistic nucleus-nucleus collisions at the LHC energies. The space-time evolution of quark-gluon plasma (QGP) produced in these energetic collisions is obtained via the (3+1)-dimensional CLVisc hydrodynamics model, the heavy quark dynamics inside the QGP is simulated using an improved Langevin model that incorporates both elastic and inelastic parton energy loss processes, and the heavy quark hadronization is simulated utilizing a comprehensive coalescence-fragmentation model. Using our combined approach, we first calculate charmed hadron ratios, $\Lambda_c/D^0$ and $D_s/D^0$, as well as their elliptic flow ($v_2$) as a function of transverse momentum ($p_T$) for different centralities in Pb+Pb collisions at $\sqrt{s_{NN}}=5.02$~TeV. Due to strangeness enhancement and parton coalescence effects, $D_s/D^0$ and $\Lambda_c/D^0$ ratios increase from peripheral to central collisions, and such centrality dependence for $\Lambda_c/D^0$ is stronger than $D_s/D^0$. We further predict the $p_T$ and centrality dependences of charmed hadron chemistry and $v_2$ in smaller Xe+Xe, Ar+Ar and O+O collisions at the LHC energies. Strong centrality and system size dependences for $\Lambda_c/D^0$ and $D_s/D^0$ ratios are observed across four collision systems. As for charmed hadron flow, both system size and collision geometry are important to understand the centrality dependence of $v_2$ in different collision systems. Our study provides a significant reference for studying heavy quark evolution and hadronizaiton in large and small systems in relativistic nuclear collisions., Comment: 12 pages, 10 figures

Diode effects are of great interest for both fundamental physics and modern technologies. Electrical diode effects (nonreciprocal transport) have been observed in Weyl systems. Optical diode effects arising from the Weyl fermions have been theoretically considered but not probed experimentally. Here, we report the observation of a nonlinear optical diode effect (NODE) in the magnetic Weyl semimetal CeAlSi, where the magnetization introduces a pronounced directionality in the nonlinear optical second-harmonic generation (SHG). We show demonstrate a six-fold change of the measured SHG intensity between opposite propagation directions over a bandwidth exceeding 250 meV. Supported by density-functional theory, we establish the linearly dispersive bands emerging from Weyl nodes as the origin of this broadband effect. We further demonstrate current-induced magnetization switching and thus electrical control of the NODE. Our results advance ongoing research to identify novel nonlinear optical/transport phenomena in magnetic topological materials and further opens new pathways for the unidirectional manipulation of light., Comment: 20 pages, 4 figures, SI included

Quantum geometry - the geometry of electron Bloch wavefunctions - is central to modern condensed matter physics. Due to the quantum nature, quantum geometry has two parts, the real part quantum metric and the imaginary part Berry curvature. The studies of Berry curvature have led to countless breakthroughs, ranging from the quantum Hall effect in 2DEGs to the anomalous Hall effect (AHE) in ferromagnets. However, in contrast to Berry curvature, the quantum metric has rarely been explored. Here, we report a new nonlinear Hall effect induced by quantum metric by interfacing even-layered MnBi2Te4 (a PT-symmetric antiferromagnet (AFM)) with black phosphorus. This novel nonlinear Hall effect switches direction upon reversing the AFM spins and exhibits distinct scaling that suggests a non-dissipative nature. Like the AHE brought Berry curvature under the spotlight, our results open the door to discovering quantum metric responses. Moreover, we demonstrate that the AFM can harvest wireless electromagnetic energy via the new nonlinear Hall effect, therefore enabling intriguing applications that bridges nonlinear electronics with AFM spintronics., Comment: 19 pages, 4 figures and a Supplementary Materials with 66 pages, 4 figures and 3 tables. Originally submitted to Science on Oct. 5, 2022

Using circularly-polarized light to control quantum matter is a highly intriguing topic in physics, chemistry and biology. Previous studies have demonstrated helicity-dependent optical control of spatial chirality and magnetization $M$. The former is central for asymmetric synthesis in chemistry and homochirality in bio-molecules, while the latter is of great interest for ferromagnetic spintronics. In this paper, we report the surprising observation of helicity-dependent optical control of fully-compensated antiferromagnetic (AFM) order in 2D even-layered MnBi$_2$Te$_4$, a topological Axion insulator with neither chirality nor $M$. We further demonstrate helicity-dependent optical creation of AFM domain walls by double induction beams and the direct reversal of AFM domains by ultrafast pulses. The control and reversal of AFM domains and domain walls by light helicity have never been achieved in any fully-compensated AFM. To understand this optical control, we study a novel type of circular dichroism (CD) proportional to the AFM order, which only appears in reflection but is absent in transmission. We show that the optical control and CD both arise from the optical Axion electrodynamics, which can be visualized as a Berry curvature real space dipole. Our Axion induction provides the possibility to optically control a family of $\mathcal{PT}$-symmetric AFMs such as Cr$_2$O$_3$, CrI$_3$ and possibly novel states in cuprates. In MnBi$_2$Te$_4$, this further opens the door for optical writing of dissipationless circuit formed by topological edge states.

While ferromagnets have been known and exploited for millennia, antiferromagnets (AFMs) were only discovered in the 1930s. The elusive nature indicates AFMs' unique properties: At large scale, due to the absence of global magnetization, AFMs may appear to behave like any non-magnetic material; However, such a seemingly mundane macroscopic magnetic property is highly nontrivial at microscopic level, where opposite spin alignment within the AFM unit cell forms a rich internal structure. In topological AFMs, such an internal structure leads to a new possibility, where topology and Berry phase can acquire distinct spatial textures. Here, we study this exciting possibility in an AFM Axion insulator, even-layered MnBi$_2$Te$_4$ flakes, where spatial degrees of freedom correspond to different layers. Remarkably, we report the observation of a new type of Hall effect, the layer Hall effect, where electrons from the top and bottom layers spontaneously deflect in opposite directions. Specifically, under no net electric field, even-layered MnBi$_2$Te$_4$ shows no anomalous Hall effect (AHE); However, applying an electric field isolates the response from one layer and leads to the surprising emergence of a large layer-polarized AHE (~50%$\frac{e^2}{h}$). Such a layer Hall effect uncovers a highly rare layer-locked Berry curvature, which serves as a unique character of the space-time $\mathcal{PT}$-symmetric AFM topological insulator state. Moreover, we found that the layer-locked Berry curvature can be manipulated by the Axion field, E$\cdot$B, which drives the system between the opposite AFM states. Our results achieve previously unavailable pathways to detect and manipulate the rich internal spatial structure of fully-compensated topological AFMs. The layer-locked Berry curvature represents a first step towards spatial engineering of Berry phase, such as through layer-specific moir\'e potential., Comment: A revised version of this article is published in Nature

Recent experiments have observed large anisotropic collective flows in high multiplicity proton-lead collisions at the Large Hadron Collider (LHC), which indicates the possible formation of mini quark-gluon plasma (QGP) in small collision systems. However, no jet quenching has been confirmed in such small systems so far. To understand this intriguing result, the system size scan experiments have been proposed to bridge the gap between large and small systems. In this work, we perform a systematic study on both heavy and light flavor jet quenching in different collision systems at the LHC energies. Using our state-of-the-art jet quenching model, which combines the next-to-leading-order perturbative QCD framework, a linear Boltzmann transport model and the (3+1)-dimensional viscous hydrodynamics simulation, we provide a good description of nuclear modification factor $R_{\rm AA}$ for charged hadrons and $D$ mesons in central and mid-central Pb+Pb and Xe+Xe collisions measured by CMS collaboration. We further predict the transverse momentum and centrality dependences of $R_{AA}$ for charged hadrons, $D$ and $B$ mesons in Pb+Pb, Xe+Xe, Ar+Ar and O+O collisions at the LHC energies. Our numerical results show a clear system size dependence for both light and heavy flavor hadron $R_{AA}$ across different collision systems. Sizable jet quenching effect is obtained for both heavy and light flavor hadrons in central O+O collisions at the LHC energies. Our study provides a significant bridge for jet quenching from large to small systems, and should be helpful for finding the smallest QGP droplet and the disappearance of QGP in relativistic nuclear collisions., Comment: 12 pages, 8 figures

Topological electrons in semimetals are usually vulnerable to chemical doping and environment change, which restricts their potential application in future electronic devices. In this paper we report that the type-II Dirac semimetal $\mathbf{VAl_3}$ hosts exceptional, robust topological electrons which can tolerate extreme change of chemical composition. The Dirac electrons remain intact even after a substantial part of V atoms have been replaced in the $\mathbf{V_{1-x}Ti_xAl_3}$ solid solutions. This Dirac semimetal state ends at $x=0.35$ where a Lifshitz transition to $p$-type trivial metal occurs. The V-Al bond is completely broken in this transition as long as the bonding orbitals are fully depopulated by the holes donated from Ti substitution. In other words, the Dirac electrons in $\mathbf{VAl_3}$ are protected by the V-Al bond whose molecular orbital is their bonding gravity center. Our understanding on the interrelations among electron count, chemical bond and electronic properties in topological semimetals suggests a rational approach to search robust, chemical-bond-protected topological materials.