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In iron-based superconductor Fe(Se,Te), a flat band-like feature near the Fermi level was observed around the Brillouin zone center in the superconducting state. It is under debate whether this is the evidence on the presence of the BCS-BEC crossover in the superconductor. High-resolution laser-based angle-resolved photoemission measurements are carried out on high quality single crystals of FeSe0.45Te0.55 superconductor to address the issue. By employing different polarization geometries, we have resolved and isolated the dyz band and the topological surface band, making it possible to study their superconducting behaviors separately. The dyz band alone does not form a flat band-like feature in the superconducting state and the measured dispersion can be well described by the BCS picture. We find that the flat band-like feature is formed from the combination of the dyz band and the topological surface state band in the superconducting state. These results reveal the origin of the flat band-like feature and rule out the presence of BCS-BEC crossover in Fe(Se,Te) superconductor.

In high temperature cuprate superconductors, it was found that in the overdoped region the superfluid density decreases with the increase of hole doping. One natural question is whether there exists normal fluid in the superconducting state in the overdoped region. In this paper, we have carried out high-resolution ultra-low temperature laser-based angle-resolved photoemission measurements on a heavily overdoped Bi2212 sample with a $T_{\mathrm{c}}$ of 48 K. We find that this heavily overdoped Bi2212 remains in the strong coupling regime with $2 \mathit{\Delta}_0 / k_{\mathrm{B}} T_{\mathrm{c}}=5.8$. The single-particle scattering rate is very small along the nodal direction ($\sim$5 meV) and increases as the momentum moves from the nodal to the antinodal regions. A hard superconducting gap opening is observed near the antinodal region with the spectral weight at the Fermi level fully suppressed to zero. The normal fluid is found to be negligibly small in the superconducting state of this heavily overdoped Bi2212. These results provide key information to understand the high $T_\mathrm{c}$ mechanism in the cuprate superconductors., Comment: 13 pages, 4 figures

The newly discovered Kagome superconductors AV$_3$Sb$_5$ (A=K, Rb and Cs) continue to bring surprises in generating unusual phenomena and physical properties, including anomalous Hall effect, unconventional charge density wave, electronic nematicity and time-reversal symmetry breaking. Here we report an unexpected emergence of multiple flat bands in the AV$_3$Sb$_5$ superconductors. By performing high-resolution angle-resolved photoemission (ARPES) measurements, we observed four branches of flat bands that span over the entire momentum space. The appearance of the flat bands is not anticipated from the band structure calculations and cannot be accounted for by the known mechanisms of flat band generation. It is intimately related to the evolution of van Hove singularities. It is for the first time to observe such emergence of multiple flat bands in solid materials. Our findings provide new insights in revealing the underlying mechanism that governs the unusual behaviors in the Kagome superconductors. They also provide a new pathway in producing flat bands and set a platform to study the flat bands related physics., Comment: 20 pages, 4 figures

The latest discovery of high temperature superconductivity near 80K in La3Ni2O7 under high pressure has attracted much attention. Many proposals are put forth to understand the origin of superconductivity.The determination of electronic structures is a prerequisite to establish theories to understand superconductivity in nickelates but is still lacking. Here we report our direct measurement of the electronic structures of La3Ni2O7 by high-resolution angle resolved photoemission spectroscopy. The Fermi surface and band structures of La3Ni2O7 are observed and compared with the band structure calculations. Strong electron correlations are revealed which are orbital- and momentum dependent. A flat band is formed from the Ni-3dz2 orbitals around the zone corner which is ~50meV below the Fermi level and exhibits the strongest electron correlation. In many theoretical proposals, this band is expected to play the dominant role in generating superconductivity in La3Ni2O7. Our observations provide key experimental information to understand the electronic structure and origin of high temperature superconductivity in La3Ni2O7., Comment: 20 pages, 5 figures

A kagome lattice of 3d transition metals hosts flat bands, Dirac fermions and saddle points. It provides a versatile platform for achieving topological superconductivity, anomalous Hall effect, unconventional density wave order and quantum spin liquid when the strong correlation, spin-orbit coupling or magnetic order are involved in such a lattice. Here, using laser-based angle-resolved photoemission spectroscopy in combination with density functional theory calculations, we investigate the electronic structure of the newly discovered kagome superconductor CsTi$_3$Bi$_5$, which is isostructural to the AV$_3$Sb$_5$ (A=K, Rb or Cs) kagome superconductors and possesses a perfect two-dimensional kagome network of Titanium. We directly observed a strikingly flat band derived from the local destructive interferences of Bloch wave functions within the kagome lattices. We also identify the type-II Dirac nodal loops around the Brillouin zone center, the type-III Dirac nodal loops around the zone corners and type-III Dirac nodal lines along the k$_z$ direction. In addition, around the Brillouin zone center, Z2 nontrivial topological surface states are also observed which is formed from the band inversion due to strong spin orbital coupling. The simultaneous existence of such multi-sets of nontrivial band structures in one kagome superconductor not only provides good opportunities to study related physics in the kagome lattice but also makes CsTi$_3$Bi$_5$ an ideal system to realize noval quantum phenomena by manipulating its chemical potential with chemical doping or pressure.

The origin of the high temperature superconductivity in the iron-based superconductors remains elusive after being extensively studied for more than a decade. Determination of the pairing symmetry is essential in understanding the superconductivity mechanism. In the iron-based superconductors that have hole pockets around the Brillouin zone center and electron pockets around the zone corners, the pairing symmetry is generally considered to be s$_\pm$, endowing a sign change in the superconducting gap between the hole and electron pockets. For the iron-based superconductors with only hole pockets, however, a couple of pairing scenarios have been proposed but the exact symmetry is still highly controversial. Here we report our determination of the pairing symmetry in KFe$_2$As$_2$ which is a prototypical iron-based superconductor with hole pockets both around the zone center and around the zone corners. By taking laser-based angle resolved photoemission measurements with super-high resolution and at ultra-low temperature, we have precisely determined the superconducting gap distribution and identified the locations of the gap nodes on all the Fermi surface around the zone center and the zone corners. The complete superconducting gap structure, in combination with the observation of the spin resonance in neutron scattering, provides strong evidence on the s$_\pm$ pairing symmetry in KFe$_2$As$_2$ with a gap sign reversal between the hole pockets around the zone center and the hole pockets around the zone corners. These results unify the pairing symmetry in the hole-doped iron-based superconductors and point to the spin fluctuation as the pairing glue in generating superconductivity.

The electronic structure and the physical properties of quantum materials can be significantly altered by charge carrier doping and magnetic state transition. Here we report a discovery of a giant and reversible electronic structure evolution with doping in a magnetic topological material. By performing high-resolution angle-resolved photoemission measurements on EuCd2As2,we found that a huge amount of hole doping can be introduced into the sample surface due to surface absorption. The electronic structure exhibits a dramatic change with the hole doping which can not be described by a rigid band shift. Prominent band splitting is observed at high doping which corresponds to a doping-induced magnetic transition at low temperature (below -15 K) from an antiferromagnetic state to a ferromagnetic state. These results have established a detailed electronic phase diagram of EuCd2As2 where the electronic structure and the magnetic structure change systematically and dramatically with the doping level. They further suggest that the transport, magnetic and topological properties of EuCd2As2 can be greatly modified by doping. These work will stimulate further investigations to explore for new phenomena and properties in doping this magnetic topological material., Comment: 22 pages,5 figures

The Kagome superconductors AV3Sb5 (A=K, Rb, Cs) have received enormous attention due to their nontrivial topological electronic structure, anomalous physical properties and superconductivity. Unconventional charge density wave (CDW) has been detected in AV3Sb5. High-precision electronic structure determination is essential to understand its origin. Here we unveil electronic nature of the CDW phase in our high-resolution angle-resolved photoemission measurements on KV3Sb5. We have observed CDW-induced Fermi surface reconstruction and the associated band folding. The CDW-induced band splitting and the associated gap opening have been revealed at the boundary of the pristine and reconstructed Brillouin zones. The Fermi surface- and momentum-dependent CDW gap is measured and the strongly anisotropic CDW gap is observed for all the V-derived Fermi surface. In particular, we have observed signatures of the electron-phonon coupling in KV3Sb5. These results provide key insights in understanding the nature of the CDW state and its interplay with superconductivity in AV3Sb5 superconductors., Comment: 21 pages, 5 figures

Impurity pinning has long been discussed to have a profound effect on the dynamics of an incommensurate charge density wave (CDW), which would otherwise slide through the lattice without resistance. Here we visualize the impurity pinning evolution of the CDW in ZrTe3 using the variable temperature scanning tunneling microscopy (STM). At low temperatures, we observe a quasi-1D incommensurate CDW modulation moderately correlated to the impurity positions, indicating a weak impurity pinning. As we raise the sample temperature, the CDW modulation gets progressively weakened and distorted, while the correlation with the impurities becomes stronger. Above the CDW transition temperature, short-range modulations persist with the phase almost all pinned by impurities. The evolution from weak to strong impurity pinning through the CDW transition can be understood as a result of losing phase rigidity.