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The study of the angular momentum properties of fission fragments can shed light about the complex mechanisms that characterize the fission process. One quantity that is of significant interest, and has not yet been studied adequately, is the alignment of the fragments, which is the cause of anisotropy of the {\gamma} rays along the fission axis and has been observed in various past and recent experiments. In this work, we have performed calculations using the FIFRELIN code, in an attempt to quantify the alignment of the nuclear spins after neutron-emission. Under the statistical tensor formalism of angular distributions, the conversion-electron and the {\gamma}-ray angular distributions can be treated simultaneously in an event-by-event calculation. This enables a first prediction of the conversion-electron angular distribution with respect to the fission axis. An average value for the alignment of fission fragments is deduced for 252Cf, with the use of recent experimental data. The method used for the present work can serve as a starting point for future theoretical and experimental studies in terms of {\gamma} and conversion-electron spectroscopy in view of studying the spin alignment of individual fission fragments, which could further improve our understanding on the process of fission.

The emission of $\gamma$-rays after a neutron capture in a cryogenic detector can generate mono-energetic nuclear recoils in the sub-keV regime, of direct interest for the calibration of Dark Matter and Coherent Elastic Neutrino Nucleus Scattering experiments. Here we show that accurate predictions of the nuclear recoil spectra induced by neutron captures require taking into account the interplay between the development in time of the de-excitation $\gamma$-cascade of the target nucleus and that of the associated atomic collisions in matter. We present detailed simulations coupling the FIFRELIN code for the description of the $\gamma$-cascades and the IRADINA code for the modelling of the fast atomic movements in matter. Nuclear recoil spectra are predicted, and made available to the community, for concrete cases of Al$_2$O$_3$, Si, Ge and CaWO$_4$ crystals exposed to a low intensity beam of thermal neutrons. We find that timing effects cause new calibration peaks to emerge in the recoil spectra and also impact the shape of the continuous recoil distribution. We discuss how they could give access to a rich physics program, spanning the accurate study of the response of cryogenic detectors in the sub-keV range, tests of solid state physics simulations and tests of nuclear models.

Coherent elastic neutrino-nucleus scattering and low-mass Dark Matter detectors rely crucially on the understanding of their response to nuclear recoils. We report the first observation of a nuclear recoil peak at around 112 eV induced by neutron capture. The measurement was performed with a CaWO$_4$ cryogenic detector from the NUCLEUS experiment exposed to a $^{252}$Cf source placed in a compact moderator. The measured spectrum is found in agreement with simulations and the expected peak structure from the single-$\gamma$ de-excitation of $^{183}$W is identified with 3 $\sigma$ significance. This result demonstrates a new method for precise, in-situ, and non-intrusive calibration of low-threshold experiments.

Anomalies in past neutrino measurements have led to the discovery that these particles have non-zero mass and oscillate between their three flavors when they propagate. In the 2010's, similar anomalies observed in the antineutrino spectra emitted by nuclear reactors have triggered the hypothesis of the existence of a supplementary neutrino state that would be sterile i.e. not interacting via the weak interaction. The STEREO experiment was designed to study this scientific case that would potentially extend the Standard Model of Particle Physics. Here we present a complete study based on our full set of data with significantly improved sensitivity. Installed at the ILL (Institut Laue Langevin) research reactor, STEREO has accurately measured the antineutrino energy spectrum associated to the fission of 235U. This measurement confirms the anomalies whereas, thanks to the segmentation of the STEREO detector and its very short mean distance to the core (10~m), the same data reject the hypothesis of a light sterile neutrino. Such a direct measurement of the antineutrino energy spectrum suggests instead that biases in the nuclear experimental data used for the predictions are at the origin of the anomalies. Our result supports the neutrino content of the Standard Model and establishes a new reference for the 235U antineutrino energy spectrum. We anticipate that this result will allow to progress towards finer tests of the fundamental properties of neutrinos but also to benchmark models and nuclear data of interest for reactor physics and for observations of astrophysical or geo-neutrinos., Comment: 34 pages, 13 figures. Final version submitted to Nature

The precise modeling of the de-excitation of Gd isotopes is of great interest for experimental studies of neutrinos using Gd-loaded organic liquid scintillators. The FIFRELIN code was recently used within the purposes of the STEREO experiment for the modeling of the Gd de-excitation after neutron capture in order to achieve a good control of the detection efficiency. In this work, we report on the recent additions in the FIFRELIN de-excitation model with the purpose of enhancing further the de-excitation description. Experimental transition intensities from EGAF database are now included in the FIFRELIN cascades, in order to improve the description of the higher energy part of the spectrum. Furthermore, the angular correlations between {\gamma} rays are now implemented in FIFRELIN, to account for the relative anisotropies between them. In addition, conversion electrons are now treated more precisely in the whole spectrum range, while the subsequent emission of X rays is also accounted for. The impact of the aforementioned improvements in FIFRELIN is tested by simulating neutron captures in various positions inside the STEREO detector. A repository of up-to-date FIFRELIN simulations of the Gd isotopes is made available for the community, with the possibility of expanding for other isotopes which can be suitable for different applications., Comment: Corrected typos on author names on arXiv metadata

Different extensions of the standard model of particle physics, such as braneworld or mirror matter models, predict the existence of a neutron sterile state, possibly as a dark matter candidate. This Letter reports a new experimental constraint on the probability $p$ for neutron conversion into a hidden neutron, set by the STEREO experiment at the high flux reactor of the Institut Laue-Langevin. The limit is $p<3.1\times 10^{-11}$ at $95 \%$ C.L. improving the previous limit by a factor 13. This result demonstrates that short-baseline neutrino experiments can be used as competitive passing-through-walls neutron experiments to search for hidden neutrons., Comment: 5 pages, 3 figures

Angular distribution and correlation measurements are an essential part in nuclear structure experiments, especially when spectroscopic information of a specific nucleus is unknown. In most cases, the experimental determination of the spins, parities of the studied nuclear states, as well as the possible mixing between two electric/magnetic multipoles of a transition are determined using angular correlation measurements. In this work, the full effect of directional {\gamma}-correlations is simulated, by using the formal theory of angular distributions. The density matrix formalism along with its multipole expansions called statistical tensors is employed, enabling to perform a full simulation of the angular correlation effects in a cascade of an arbitrary number of {\gamma} transitions. A triple {\gamma} angular correlation simulation is demonstrated for the first time. The present approach was coupled with the Monte Carlo code FIFRELIN, which can simulate the de-excitation of fission fragments or of excited nuclei after neutron capture. It provides a complete description of the spatial distributions of all the {\gamma} rays in the cascade, that can be used for simulation purposes in various applications both in nuclear and particle physics. The potential for a novel approach in data analysis of angular correlation measurements is discussed thoroughly., Comment: 12 pages, 9 figures

The PROSPECT and STEREO collaborations present a combined measurement of the pure $^{235}$U antineutrino spectrum, without site specific corrections or detector-dependent effects. The spectral measurements of the two highest precision experiments at research reactors are found to be compatible with $\chi^2/\mathrm{ndf} = 24.1/21$, allowing a joint unfolding of the prompt energy measurements into antineutrino energy. This $\bar{\nu}_e$ energy spectrum is provided to the community, and an excess of events relative to the Huber model is found in the 5-6 MeV region. When a Gaussian bump is fitted to the excess, the data-model $\chi^2$ value is improved, corresponding to a $2.4\sigma$ significance.

The energy loss of heavy ions in thin Mylar and nickel foils was measured accurately using fission fragments from $^{239}Pu(n_{th},f)$, mass and energy separated by the Lohengrin separator at ILL. The detection setup, placed at the focal plane of the Lohengrin separator enabled to measure precisely the kinetic energy difference of selected fragments after passing through the sample. From these data, the stopping powers in Mylar and nickel layers were extracted and compared to calculations. Whereas large deviations are observed with SRIM-2013 for Mylar, fairly good agreements are obtained with the semi-empirical approach of Knyazheva et al. and the calculations contained within the DPASS database. In nickel, SRIM-2013 and Knyazheva model are in agreement with our data within about 10 %, while large deviations are observed with DPASS. We used our data to provide updated parameters for the Knyazheva et al. model and rescale DPASS database for nickel and Mylar., Comment: 19 pages, 18 figures

The development of low-threshold detectors for the study of coherent elastic neutrino-nucleus scattering and for the search for light dark matter necessitates methods of low-energy calibration. We suggest this can be provided by the nuclear recoils resulting from the $\gamma$ emission following thermal neutron capture. In particular, several MeV-scale single-$\gamma$ transitions induce well-defined nuclear recoil peaks in the 100 eV range. Using the FIFRELIN code, complete schemes of $\gamma$-cascades for various isotopes can be predicted with high accuracy to determine the continuous background of nuclear recoils below the calibration peaks. We present a comprehensive experimental concept for the calibration of CaWO$_4$ and Ge cryogenic detectors at a research reactor. For CaWO$_4$ the simulations show that two nuclear recoil peaks at 112.5 eV and 160.3 eV should be visible above background simply in the spectrum of the cryogenic detector. Then we discuss how the additional tagging for the associated $\gamma$ increases the sensitivity of the method and extends its application to a wider energy range and to Ge cryogenic detectors., Comment: 21 pages, 8 figures

This article reports the measurement of the $^{235}$U-induced antineutrino spectrum shape by the STEREO experiment. 43'000 antineutrinos have been detected at about 10 m from the highly enriched core of the ILL reactor during 118 full days equivalent at nominal power. The measured inverse beta decay spectrum is unfolded to provide a pure $^{235}$U spectrum in antineutrino energy. A careful study of the unfolding procedure, including a cross-validation by an independent framework, has shown that no major biases are introduced by the method. A significant local distortion is found with respect to predictions around $E_\nu \simeq 5.3$ MeV. A gaussian fit of this local excess leads to an amplitude of $A = 12.1 \pm 3.4\%$ (3.5$\sigma$)., Comment: This is the Accepted Manuscript version of an article accepted for publication in J. Phys. G: Nucl. Part. Phys.. IOP Publishing Ltd is not responsible for any errors or omissions in this version of the manuscript or any version derived from it. The Version of Record is available online at https://doi.org/10.1088/1361-6471/abd37a. 34 pages, 14 figures

We comment on the claimed observation [arXiv:arXiv:2005.05301] of sterile neutrino oscillations by the Neutrino-4 collaboration. Such a claim, which requires the existence of a new fundamental particle, demands a level of rigor commensurate with its impact. The burden lies with the Neutrino-4 collaboration to provide the information necessary to prove the validity of their claim to the community. In this note, we describe aspects of both the data and analysis method that might lead to an oscillation signature arising from a null experiment and describe additional information needed from the Neutrino-4 collaboration to support the oscillation claim. Additionally, as opposed to the assertion made by the Neutrino-4 collaboration, we also show that the method of 'coherent summation' using the $L/E$ parameter produces similar results to the methods used by the PROSPECT and the STEREO collaborations., Comment: 5 pages, 3 figures

We report a measurement of the antineutrino rate from the fission of U-235 with the STEREO detector using 119 days of reactor turned on. In our analysis, we perform several detailed corrections and achieve the most precise single measurement at reactors with highly enriched U-235 fuel. We measure an IBD cross section per fission of $\sigma_f$ = (6.34 $\pm$ 0.06 [stat] $\pm$ 0.15 [sys] $\pm$ 0.15 [model]) $\times$ 10${}^{-43}$ cm${}^{2}$/fission and observe a rate deficit of (5.2 $\pm$ 0.8 [stat] $\pm$ 2.3 [sys] $\pm$ 2.3 [model])% compared to the model, consistent with the deficit of the world average. Testing U-235 as the sole source of the deficit, we find a tension between the results of lowly and highly enriched U-235 fuel of 2.1 standard deviations., Comment: 7 pages, 1 figure

The STEREO experiment is a very short baseline reactor antineutrino experiment. It is designed to test the hypothesis of light sterile neutrinos being the cause of a deficit of the observed antineutrino interaction rate at short baselines with respect to the predicted rate, known as the reactor antineutrino anomaly. The STEREO experiment measures the antineutrino energy spectrum in six identical detector cells covering baselines between 9 and 11 m from the compact core of the ILL research reactor. In this article, results from 179 days of reactor turned on and 235 days of reactor turned off are reported at a high degree of detail. The current results include improvements in the modelling of detector optical properties and the gamma-cascade after neutron captures by gadolinium, the treatment of backgrounds, and the statistical method of the oscillation analysis. Using a direct comparison between antineutrino spectra of all cells, largely independent of any flux prediction, we find the data compatible with the null oscillation hypothesis. The best-fit point of the reactor antineutrino anomaly is rejected at more than 99.9% C.L., Comment: 31 pages, 35 figures, for supplemental data see http://doi.org/10.17182/hepdata.92323

The STEREO experiment measures the electron antineutrino spectrum emitted in a research reactor using the inverse beta decay reaction on H nuclei in a gadolinium loaded liquid scintillator. The detection is based on a signal coincidence of a prompt positron and a delayed neutron capture event. The simulated response of the neutron capture on gadolinium is crucial for the comparison with data, in particular in the case of the detection efficiency. Among all stable isotopes, $^{155}$Gd and $^{157}$Gd have the highest cross sections for thermal neutron capture. The excited nuclei after the neutron capture emit gamma rays with a total energy of about 8 MeV. The complex level schemes of $^{156}$Gd and $^{158}$Gd are a challenge for the modeling and prediction of the deexcitation spectrum, especially for compact detectors where gamma rays can escape the active volume. With a new description of the Gd(n,${\gamma}$) cascades obtained using the FIFRELIN code, the agreement between simulation and measurements with a neutron calibration source was significantly improved in the STEREO experiment. A database of ten millions of deexcitation cascades for each isotope has been generated and is now available for the user., Comment: 5 pages, 3 figures

The reactor antineutrino anomaly might be explained by the oscillation of reactor antineutrinos toward a sterile neutrino of eV mass. In order to explore this hypothesis, the STEREO experiment measures the antineutrino energy spectrum in six different detector cells covering baselines between 9 and 11 m from the compact core of the ILL research reactor. In this Letter, results from 66 days of reactor turned on and 138 days of reactor turned off are reported. A novel method to extract the antineutrino rates has been developed based on the distribution of the pulse shape discrimination parameter. The test of a new oscillation toward a sterile neutrino is performed by comparing ratios of cells, independent of absolute normalization and of the prediction of the reactor spectrum. The results are found to be compatible with the null oscillation hypothesis and the best fit of the reactor antineutrino anomaly is excluded at 97.5\% C.L.

The STEREO experiment is a very short baseline reactor antineutrino experiment aiming at testing the hypothesis of light sterile neutrinos as an explanation of the deficit of the observed neutrino interaction rate with respect to the predicted rate, known as the Reactor Antineutrino Anomaly. The detector center is located 10 m away from the compact, highly $^{235}$U enriched core of the research nuclear reactor of the Institut Laue Langevin in Grenoble, France. This paper describes the STEREO site, the detector components and associated shielding designed to suppress the external sources of background which were characterized on site. It reports the performances in terms of detector response and energy reconstruction., Comment: 32 pages, 17 figures

The space and time configurations of the dissociation of $^8$He into $^6$He+$n$+$n$, on C and Pb targets, have been explored simultaneously for the first time. The final-state interactions in the $n$-$n$ and $^6$He-$n$ channels are successfully described within a model that considers independent emission of neutrons from a Gaussian volume with a given lifetime. The dissociation on C target exhibits a dominant sequential decay through the ground state of $^7$He, consistent with neutrons being emitted from a Gaussian volume of $r_{nn}^{\rm{rms}}=7.3\pm0.6$~fm with a $n$-$n$ delay in the sequential channel of $1400\pm400$~fm/$c$, in agreement with the lifetime of $^7$He. The lower-statistics data on Pb target correspond mainly to direct breakup, and are well described using the $n$-$n$ volume measured, without any $n$-$n$ delay. The validity of the phenomenological model used is discussed., Comment: Accepted for publication in J. Phys. G, 11 pages, 5 figures

The Daya Bay, Double Chooz and RENO experiments recently observed a significant distortion in their detected reactor antineutrino spectra, being at odds with the current predictions. Although such a result suggests to revisit the current reactor antineutrino spectra modeling, an alternative scenario, which could potentially explain this anomaly, is explored in this letter. Using an appropriate statistical method, a study of the Daya Bay experiment energy scale is performed. While still being in agreement with the {\gamma} calibration data and Boron 12 measured spectrum, it is shown that a O(1%) deviation of the energy scale reproduces the distortion observed in the Daya Bay spectrum, remaining within the quoted calibration uncertainties. Potential origins of such a deviation, which challenge the energy calibration of these detectors, are finally discussed.

The characteristic properties of the hot nuclear matter existing at the time of fragment formation in the multifragmentation events produced in the reaction $^{64}$Zn + $^{112}$Sn at 40 MeV/nucleon are studied. A kinematical focusing method is employed to determine the multiplicities of evaporated light particles, associated with isotopically identified detected fragments. From these data the primary isotopic yield distributions are reconstructed using a Monte Carlo method. The reconstructed yield distributions are in good agreement with the primary isotope distributions obtained from AMD transport model simulations. Utilizing the reconstructed yields, power distribution, Landau free energy, characteristic properties of the emitting source are examined. The primary mass distributions exhibit a power law distribution with the critical exponent, $A^{-2.3}$, for $A \geq 15$ isotopes, but significantly deviates from that for the lighter isotopes. Landau free energy plots show no strong signature of the first order phase transition. Based on the Modified Fisher Model, the ratios of the Coulomb and symmetry energy coefficients relative to the temperature, $a_{c}/T$ and $a_{sym}/T$, are extracted as a function of A. The extracted $a_{sym}/T$ values are compared with results of the AMD simulations using Gogny interactions with different density dependencies of the symmetry energy term. The calculated $a_{sym}/T$ values show a close relation to the symmetry energy at the density at the time of the fragment formation. From this relation the density of the fragmenting source is determined to be $\rho /\rho_{0} = (0.63 \pm 0.03 )$. Using this density, the symmetry energy coefficient and the temperature of fragmenting source are determined in a self-consistent manner as $a_{sym} = (24.7 \pm 3.4) MeV$ and $T=(4.9 \pm 0.2)$ MeV.

For the first time primary hot isotope distributions are experimentally reconstructed in intermediate heavy ion collisions and used with antisymmetrized molecular dynamics (AMD) calculations to determine density, temperature and symmetry energy coefficient in a self-consistent manner. A kinematical focusing method is employed to reconstruct the primary hot fragment yield distributions for multifragmentation events observed in the reaction system $^{64}$Zn + $^{112}$Sn at 40 MeV/nucleon. The reconstructed yield distributions are in good agreement with the primary isotope distributions of AMD simulations. The experimentally extracted values of the symmetry energy coefficient relative to the temperature, $a_{sym}/T$, are compared with those of the AMD simulations with different density dependence of the symmetry energy term. The calculated $a_{sym}/T$ values changes according to the different interactions. By comparison of the experimental values of $a_{sym}/T$ with those of calculations, the density of the source at fragment formation was determined to be $\rho /\rho_{0} = (0.63 \pm 0.03 )$. Using this density, the symmetry energy coefficient and the temperature are determined in a self-consistent manner as $a_{sym} = (24.7 \pm 1.9) MeV$ and $T=(4.9 \pm 0.2)$ MeV

Isotope yields have been analyzed within the framework of a Modified Fisher Model to study the power law yield distribution of isotopes in the multifragmentation regime. Using the ratio of the mass dependent symmetry energy coefficient relative to the temperature, $a_{sym}/T$, extracted in previous work and that of the pairing term, $a_{p}/T$, extracted from this work, and assuming that both reflect secondary decay processes, the experimentally observed isotope yields have been corrected for these effects. For a given I = N - Z value, the corrected yields of isotopes relative to the yield of $^{12}C$ show a power law distribution, $Y(N,Z)/Y(^{12}C) \sim A^{-\tau}$, in the mass range of $1 \le A \le 30$ and the distributions are almost identical for the different reactions studied. The observed power law distributions change systematically when I of the isotopes changes and the extracted $\tau$ value decreases from 3.9 to 1.0 as I increases from -1 to 3. These observations are well reproduced by a simple de-excitation model, which the power law distribution of the primary isotopes is determined to $\tau^{prim} = 2.4 \pm 0.2$, suggesting that the disassembling system at the time of the fragment formation is indeed at or very near the critical point., Comment: 5 pages, 5 figures

We discuss experimental evidence for a nuclear phase transition driven by the different concentration of neutrons to protons. Different ratios of the neutron to proton concentrations lead to different critical points for the phase transition. This is analogous to the phase transitions occurring in 4He-3He liquid mixtures. We present experimental results which reveal the N/A (or Z/A) dependence of the phase transition and discuss possible implications of these observations in terms of the Landau Free Energy description of critical phenomena., Comment: 14 pages, 18 figures

Isoscaling is derived within a recently proposed modified Fisher model where the free energy near the critical point is described by the Landau O(m^6) theory. In this model m = (N-Z)/A is the order parameter, a consequence of (one of) the symmetries of the nuclear Hamiltonian. Within this framework we show that isoscaling depends mainly on this order parameter through the 'external (conjugate) field' H. The external field is just given by the difference in chemical potentials of the neutrons and protons of the two sources. To distinguish from previously employed isoscaling relationships, this approach is dubbed: m - scaling. We discuss the relationship between this framework and the standard isoscaling formalism and point out some substantial differences in interpretation of experimental results which might result. These should be investigated further both theoretically and experimentally., Comment: 14 pages, 5 figures

The ratio of the symmetry energy coefficient to temperature, $a_sym/T$, in Fermi energy heavy ion collisions, has been experimentally extracted as a function of the fragment atomic number using isoscaling parameters and the variance of the isotope distributions. The extracted values have been compared to the results of calculations made with an Antisymmetrized Molecular Dynamics (AMD) model employing a statistical decay code to account for deexcitation of excited primary fragments. The experimental values are in good agreement with the values calculated but are significantly different from those characterizing the yields of the primary AMD fragments., Comment: 12 pages, 6 figures

The relative isobaric yields of fragments produced in a series of heavy ion induced multifragmentation reactions have been analyzed in the framework of a Modified Fisher Model, primarily to determine the ratio of the symmetry energy coefficient to the temperature, $a_a/T$, as a function of fragment mass A. The extracted values increase from 5 to ~16 as A increases from 9 to 37. These values have been compared to the results of calculations using the Antisymmetrized Molecular Dynamics (AMD) model together with the statistical decay code Gemini. The calculated ratios are in good agreement with those extracted from the experiment. In contrast, the ratios determined from fitting the primary fragment distributions from the AMD model calculation are ~ 4 and show little variation with A. This observation indicates that the value of the symmetry energy coefficient derived from final fragment observables may be significantly different than the actual value at the time of fragment formation. The experimentally observed pairing effect is also studied within the same simulations. The Coulomb coefficient is also discussed., Comment: 10 pages, 12 figures

A beta-decay study of Cu-77 has been performed at the ISOLDE mass separator with the aim to deduce its beta-decay properties and to obtain spectroscopic information on Zn-77. Neutron-rich copper isotopes were produced by means of proton- or neutron-induced fission reactions on U-238. After the production, Cu-77 was selectively laser ionized, mass separated and sent to different detection systems where beta-gamma and beta-n coincidence data were collected. We report on the deduced half-live, decay scheme, and possible spin assignment of 77Cu.

In their ground states, atomic nuclei are quantum Fermi liquids. At finite temperatures and low densities, these nuclei may undergo a phase change similar to, but substantially different from, a classical liquid gas phase transition. As in the classical case, temperature is the control parameter while density and pressure are the conjugate variables. At variance with the classical case, in the nucleus the difference between the proton and neutron concentrations acts as an additional order parameter, for which the symmetry potential is the conjugate variable. Different ratios of the neutron to proton concentrations lead to different critical points for the phase transition. This is analogous to the phase transitions occurring in $^{4}$He-$^{3}$He liquid mixtures. We present experimental results which reveal the N/Z dependence of the phase transition and discuss possible implications of these observations in terms of the Landau Free Energy description of critical phenomena., Comment: 5 pages, 4 figures

The sizes, temperatures and free neutron to proton ratios of the initial interaction zones produced in the collisions of 40 MeV/nucleon $^{40}$Ar + $^{112}$Sn and 55 MeV/nucleon$^{27}$Al + $^{124}$Sn are derived using total detected neutron plus charged particle multiplicity as a measure of the impact parameter range and number of participant nucleons. The size of the initial interaction zone, determined from a coalescence model analysis, increases significantly with decreasing impact parameter. The temperatures and free neutron to proton ratios in the interaction zones are relatively similar for different impact parameter ranges and evolve in a similar fashion., Comment: 7 pages, 8 figures

Experimental analyses of moderate temperature nuclear gases produced in the violent collisions of 35 MeV/nucleon$^{64}$Zn projectiles with $^{92}$Mo and $^{197}$Au target nuclei reveal a large degree of alpha particle clustering at low densities. For these gases, temperature and density dependent symmetry energy coefficients have been derived from isoscaling analyses of the yields of nuclei with A $\leq 4$. At densities of 0.01 to 0.05 times the ground state density of symmetric nuclear matter, the temperature and density dependent symmetry energies are 10.7 to 13.5 MeV. These values are much larger than those obtained in mean field calculations. They are in quite good agreement with results of a recently proposed Virial Equation of State calculation., Comment: 9 pages, 7 figures. This is the version taking into account referee comments

We analyzed the experimental data of the pre-scission neutron multiplicity in connection with fission fragments in the reaction $^{58}$Ni+$^{208}$Pb at the incident energy corresponding to the excitation energy of compound nucleus $E^{*}$=185.9 MeV, which was performed by D\'{e}MoN group. The relation between the pre-scission neutron multiplicity and each reaction process having different reaction time is investigated. In order to study the fusion-fission process accompanied by neutron emission, the fluctuation-dissipation model combined with a statistical model is employed. It is found that the fusion-fission process and the quasi-fission process are clearly distinguished in correlation with the pre-scission neutron multiplicity., Comment: 11 figures

The kinetic energy variation of emitted light clusters has been employed as a clock to explore the time evolution of the temperature for thermalizing composite systems produced in the reactions of 26A, 35A and 47A MeV $^{64}$Zn with $^{58}$Ni, $^{92}$Mo and $^{197}$Au. For each system investigated, the double isotope ratio temperature curve exhibits a high maximum apparent temperature, in the range of 10-25 MeV, at high ejectile velocity. These maximum values increase with increasing projectile energy and decrease with increasing target mass. The time at which the maximum in the temperature curve is reached ranges from 80 to 130 fm/c after contact. For each different target, the subsequent cooling curves for all three projectile energies are quite similar. Temperatures comparable to those of limiting temperature systematics are reached 30 to 40 fm/c after the times corresponding to the maxima, at a time when AMD-V transport model calculations predict entry into the final evaporative or fragmentation stage of de-excitation of the hot composite systems. Evidence for the establishment of thermal and chemical equilibrium is discussed., Comment: 9 pages, 5 figures