Christoph Kern, Hugo Delgado-Granados, Viviana Burbano, Nicole Bobrowski, Armando Saballos, Mike Burton, Hendra Gunawan, Gustavo Garzón, Zoraida Chacón, Mattias Johansson, Nia Haerani, Philippe Kowalski, Fabio Vita, Mathieu M. Yalire, Francisco Montalvo, Giuseppe Salerno, Fredy Apaza, Thor H. Hansteen, Joakim Möller, Vladimir Conde, Maarten de Moor, Claudia Rivera, Charlotte Barrington, Geoffroy Avard, F. Vasconez, Salvatore Inguaggiato, Pablo Masias, Deborah Fernandez, Fidel Costa, Christian Joseph Clarito, Ulrich Platt, Gustavo Chigna, Manne Kihlman, Benoit Taisne, Andrea Di Muro, Bo Galle, Gabriela Velasquez, Santiago Arellano, Claudia Bucarey, Silvana Hidalgo, and Earth Observatory of Singapore
Volcanic plumes are common and far-reaching manifestations of volcanic activity during and between eruptions. Observations of the rate of emission and composition of volcanic plumes are essential to recognize and, in some cases, predict the state of volcanic activity. Measurements of the size and location of the plumes are important to assess the impact of the emission from sporadic or localized events to persistent or widespread processes of climatic and environmental importance. These observations provide information on volatile budgets on Earth, chemical evolution of magmas, and atmospheric circulation and dynamics. Space-based observations during the last decades have given us a global view of Earth's volcanic emission, particularly of sulfur dioxide (SO2). Although none of the satellite missions were intended to be used for measurement of volcanic gas emission, specially adapted algorithms have produced time-averaged global emission budgets. These have confirmed that tropospheric plumes, produced from persistent degassing of weak sources, dominate the total emission of volcanic SO2. Although space-based observations have provided this global insight into some aspects of Earth's volcanism, it still has important limitations. The magnitude and short-term variability of lower-atmosphere emissions, historically less accessible from space, remain largely uncertain. Operational monitoring of volcanic plumes, at scales relevant for adequate surveillance, has been facilitated through the use of ground-based scanning differential optical absorption spectrometer (ScanDOAS) instruments since the beginning of this century, largely due to the coordinated effort of the Network for Observation of Volcanic and Atmospheric Change (NOVAC). In this study, we present a compilation of results of homogenized post-analysis of measurements of SO2 flux and plume parameters obtained during the period March 2005 to January 2017 of 32 volcanoes in NOVAC. This inventory opens a window into the short-term emission patterns of a diverse set of volcanoes in terms of magma composition, geographical location, magnitude of emission, and style of eruptive activity. We find that passive volcanic degassing is by no means a stationary process in time and that large sub-daily variability is observed in the flux of volcanic gases, which has implications for emission budgets produced using short-term, sporadic observations. The use of a standard evaluation method allows for intercomparison between different volcanoes and between ground- and space-based measurements of the same volcanoes. The emission of several weakly degassing volcanoes, undetected by satellites, is presented for the first time. We also compare our results with those reported in the literature, providing ranges of variability in emission not accessible in the past. The open-access data repository introduced in this article will enable further exploitation of this unique dataset, with a focus on volcanological research, risk assessment, satellite-sensor validation, and improved quantification of the prevalent tropospheric component of global volcanic emission. Published version Initial implementation of the network was funded by the EU FP6 NOVAC project (https://cordis.europa.eu/ project/rcn/75513/factsheet/en, last access: 1 October 2020). Recent funding for this work was provided by the Alfred P. Sloan Foundation’s Deep Carbon Observatory programme (https://deepcarbon. net/, last access: 1 October 2020), Chalmers University of Technology, the Swedish National Space Agency (career grant no. 149/18), and the ECMWF CAMS_81 Global and Regional Emissions project. The authors are thankful for the valuable support from the USGS–USAID Volcano Disaster Assistance Program (https: //volcanoes.usgs.gov/vdap/, last access: 1 October 2020) provided to NOVAC since 2015.