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An open question in mechanics is whether mechanical resonators can be made nonlinear with vibrations approaching the quantum ground state. This requires engineering a mechanical nonlinearity far beyond what has been realized thus far. Here we discovered a mechanism to boost the Duffing nonlinearity by coupling the vibrations of a nanotube resonator to single-electron tunneling and by operating the system in the ultrastrong coupling regime. Remarkably, thermal vibrations become highly nonlinear when lowering the temperature. The average vibration amplitude at the lowest temperature is 13 times the zero-point motion, with approximately 42% of the thermal energy stored in the anharmonic part of the potential. Our work paves the way for realizing mechanical Schrodinger cat states [1], mechanical qubits [2, 3], and quantum simulators emulating the electron-phonon coupling [4].

Driven nanomechanical resonators based on low-dimensional materials are routinely and efficiently detected with electrical mixing measurements. However, the measured signal is a non-trivial combination of the mechanical eigenmode displacement and an electrical contribution, which makes the extraction of the driven mechanical response challenging. Here, we report a simple yet reliable method to extract solely the driven mechanical vibrations by eliminating the contribution of pure electrical origin. This enables us to measure the spectral mechanical response as well as the driven quadratures of motion. We further show how to calibrate the measured signal into units of displacement. Additionally, we utilize the pure electrical contribution to directly determine the effective mass of the measured mechanical mode. Our method marks a key step forward in the study of nanoelectromechanical resonators based on low-dimensional materials in both the linear and the nonlinear regime.

We report the first study on the thermal behaviour of the stiffness of individual carbon nanotubes, which is achieved by measuring the resonance frequency of their fundamental mechanical bending modes. We observe a reduction of the Young's modulus over a large temperature range with a slope $-(173\pm 65)$ ppm/K in its relative shift. These findings are reproduced by two different theoretical models based on the thermal dynamics of the lattice. These results reveal how the measured fundamental bending modes depend on the phonons in the nanotube via the Young's modulus. An alternative description based on the coupling between the measured mechanical modes and the phonon thermal bath in the Akhiezer limit is discussed.