Search

We report neutron scattering, pressure-dependent AC calorimetry, and AC magnetic susceptibility measurements of triangular lattice NaYbSe$_2$. We observe a continuum of scattering, which is reproduced by matrix product simulations, and no phase transition is detected in any bulk measurements. Comparison to heat capacity simulations suggest the material is within the Heisenberg spin liquid phase. AC Susceptibility shows a significant 23~mK downturn, indicating a gap in the magnetic spectrum. The combination of a gap with no detectable magnetic order, comparison to theoretical models, and comparison to other $A$YbSe$_2$ compounds all strongly indicate NaYbSe$_2$ is within the quantum spin liquid phase. The gap also allows us to rule out a gapless Dirac spin liquid, with a gapped $\mathbb{Z}_2$ liquid the most natural explanation., Comment: 5 pages, 4 figures; 7 pages and 13 figures supplemental materials

One of the prime material candidates to host the axion insulator state is EuIn$_{2}$As$_{2}$. First-principles calculations predicted the emergence of this exotic topological phase based on the assumption of a collinear antiferromagnetic structure. However, neutron scattering measurements revealed a more intricate magnetic ground state, characterized by two coexisting magnetic wavevectors, reached by successive thermal phase transitions. The proposed high and low temperature phases were a spin helix and a state with interpenetrating helical and antiferromagnetic order, termed a broken helix, respectively. Despite its complexity, the broken helix still protects the axion state because the product of time-reversal and a rotational symmetry is preserved. Here we identify the magnetic structure associated with these two phases using a multimodal approach that combines symmetry-sensitive optical probes, scattering, and group theoretical analysis. We find that the higher temperature phase hosts a nodal structure rather than a helix, characterized by a variation of the magnetic moment amplitude from layer to layer, with the moment vanishing entirely in every third Eu layer. The lower temperature structure is similar to the broken helix, with one important difference: the relative orientation of the magnetic structure and the lattice is not fixed, resulting in an `unpinned broken helix'. As a result of the breaking of rotational symmetry, the axion phase is not generically protected. Nevertheless, we show that it can be restored if the magnetic structure is tuned with externally-applied uniaxial strain. Finally, we present a spin Hamiltonian that identifies the spin interactions needed to account for the complex magnetic order in EuIn$_{2}$As$_{2}$. Our work highlights the importance of the multimodal approach in determining the symmetry of complex order-parameters., Comment: 32 pages, 21 figures

The Heisenberg triangular lattice quantum spin liquid and the phase transitions to nearby magnetic orders have received much theoretical attention, but clear experimental manifestations of these states are rare. This work investigates a new spin-half Yb$^{3+}$ delafossite material, KYbSe$_2$, whose inelastic neutron scattering spectra reveal a diffuse continuum with a sharp lower bound. Applying entanglement witnesses to the data reveals significant multipartite entanglement spread between its neighbors, and analysis of its magnetic exchange couplings shows close proximity to the triangular lattice Heisenberg quantum spin liquid. Key features of the data are reproduced by Schwinger-boson theory and tensor network calculations with a significant second-neighbor coupling $J_2$. The strength of the dynamical structure factor at the $K$ point shows a scaling collapse in $\hbar\omega/k_\mathrm{B}T$ down to 0.3 K, indicating a second-order quantum phase transition. Comparing this to previous theoretical work suggests that the proximate phase at larger $J_2$ is a gapped $\mathbb{Z}_2$ spin liquid, resolving a long-debated issue. We thus show that KYbSe$_2$ is close to a spin liquid phase, which in turn sheds light on the theoretical phase diagram itself., Comment: 6 pages main text, 6 pages methods, 7 pages supplemental information

The ferromagnetic phase of Co$_3$Sn$_2$S$_2$ is widely considered to be a topological Weyl semimetal, with evidence for momentum-space monopoles of Berry curvature from transport and spectroscopic probes. As the bandstructure is highly sensitive to the magnetic order, attention has focused on anomalies in magnetization, susceptibility and transport measurements that are seen well below the Curie temperature, leading to speculation that a "hidden" phase coexists with ferromagnetism. Here we report spatially-resolved measurements by Kerr effect microscopy that identify this phase. We find that the anomalies coincide with a deep minimum in domain wall (DW) mobility, indicating a crossover between two regimes of DW propagation. We demonstrate that this crossover is a manifestation of a 2D phase transition that occurs within the DW, in which the magnetization texture changes from continuous rotation to unidirectional variation. We propose that the existence of this 2D transition deep within the ferromagnetic state of the bulk is a consequence of a giant quality factor for magnetocrystalline anisotropy unique to this compound. This work broadens the horizon of the conventional binary classification of DWs into Bloch and N\'eel walls, and suggests new strategies for manipulation of domain walls and their role in electron and spin transport., Comment: 17+6 pages, revised version, to appear in Nature Communications

Classical hydrodynamics is a remarkably versatile description of the coarse-grained behavior of many-particle systems once local equilibrium has been established. The form of the hydrodynamical equations is determined primarily by the conserved quantities present in a system. Some quantum spin chains are known to possess, even in the simplest cases, a greatly expanded set of conservation laws, and recent work suggests that these laws strongly modify collective spin dynamics even at high temperature. Here, by probing the dynamical exponent of the one-dimensional Heisenberg antiferromagnet KCuF$_3$ with neutron scattering, we find evidence that the spin dynamics are well described by the dynamical exponent $z=3/2$, which is consistent with the recent theoretical conjecture that the dynamics of this quantum system are described by the Kardar-Parisi-Zhang universality class. This observation shows that low-energy inelastic neutron scattering at moderate temperatures can reveal the details of emergent quantum fluid properties like those arising in non-Fermi liquids in higher dimensions., Comment: 12 pages and 4 figures. Includes 1 pages of methods and >> 1 pages Supplementary Information

Specialized computational chemistry packages have permanently reshaped the landscape of chemical and materials science by providing tools to support and guide experimental efforts and for the prediction of atomistic and electronic properties. In this regard, electronic structure packages have played a special role by using first-principledriven methodologies to model complex chemical and materials processes. Over the last few decades, the rapid development of computing technologies and the tremendous increase in computational power have offered a unique chance to study complex transformations using sophisticated and predictive many-body techniques that describe correlated behavior of electrons in molecular and condensed phase systems at different levels of theory. In enabling these simulations, novel parallel algorithms have been able to take advantage of computational resources to address the polynomial scaling of electronic structure methods. In this paper, we briefly review the NWChem computational chemistry suite, including its history, design principles, parallel tools, current capabilities, outreach and outlook., Comment: This article appeared in volume 152, issue 18, page 184102 of the Journal of Chemical Physics. It can be found at https://doi.org/10.1063/5.0004997

Weyl semimetals are crystals in which electron bands cross at isolated points in momentum space. Associated with each crossing point (or Weyl node) is an integer topological invariant known as the Berry monopole charge. The discovery of new classes of Weyl materials is driving the search for novel properties that derive directly from the Berry charge. The circular photogalvanic effect (CPGE), whereby circular polarized light generates a current whose direction depends on the helicity of the absorbed photons, is a striking example of a macroscopic property that emerges from Weyl topology. Recently, it was predicted that the rate of current generation associated with optical transitions near a Weyl node is proportional to its monopole charge and independent of material-specific parameters. In Weyl semimetals that retain mirror symmetry this universal photogalvanic current is strongly suppressed by opposing contributions from energy equivalent nodes of opposite charge. However, when all mirror symmetries are broken, as in chiral Weyl systems, nodes with opposite topological charge are no longer degenerate, opening a window of photon energies where the topological CPGE can emerge. In this work we test this theory through measurement of the photon-energy dependence of the CPGE in the chiral Weyl semimetal RhSi. The spectrum is fully consistent with a topological CPGE, as it reveals a response in a low-energy window that closes at 0.65 eV, in quantitative agreement with the theoretically-derived bandstucture., Comment: 33 pages, 4 + 6 figures

Pressure alters the physical, chemical and electronic properties of matter. The development of the diamond anvil cell (DAC) enables tabletop experiments to investigate a diverse landscape of high-pressure phenomena ranging from the properties of planetary interiors to transitions between quantum mechanical phases. In this work, we introduce and utilize a novel nanoscale sensing platform, which integrates nitrogen-vacancy (NV) color centers directly into the culet (tip) of diamond anvils. We demonstrate the versatility of this platform by performing diffraction-limited imaging (~600 nm) of both stress fields and magnetism, up to pressures ~30 GPa and for temperatures ranging from 25-340 K. For the former, we quantify all six (normal and shear) stress components with accuracy $<0.01$ GPa, offering unique new capabilities for characterizing the strength and effective viscosity of solids and fluids under pressure. For the latter, we demonstrate vector magnetic field imaging with dipole accuracy $<10^{-11}$ emu, enabling us to measure the pressure-driven $\alpha\leftrightarrow\epsilon$ phase transition in iron as well as the complex pressure-temperature phase diagram of gadolinium. In addition to DC vector magnetometry, we highlight a complementary NV-sensing modality using T1 noise spectroscopy; crucially, this demonstrates our ability to characterize phase transitions even in the absence of static magnetic signatures. By integrating an atomic-scale sensor directly into DACs, our platform enables the in situ imaging of elastic, electric and magnetic phenomena at high pressures., Comment: 18 + 50 pages, 4 + 19 figures

While all media can exhibit first-order conductivity describing current linearly proportional to electric field, $E$, the second-order conductivity, $\sigma^{(2)}$ , relating current to $E^2$, is nonzero only when inversion symmetry is broken. Second order nonlinear optical responses are powerful tools in basic research, as probes of symmetry breaking, and in optical technology as the basis for generating currents from far-infrared to X-ray wavelengths. The recent surge of interest in Weyl semimetals with acentric crystal structures has led to the discovery of a host of $\sigma^{(2)}$ -related phenomena in this class of materials, such as polarization-selective conversion of light to dc current (photogalvanic effects) and the observation of giant second-harmonic generation (SHG) efficiency in TaAs at photon energy 1.5 eV. Here, we present measurements of the SHG spectrum of TaAs revealing that the response at 1.5 eV corresponds to the high-energy tail of a resonance at 0.7 eV, at which point the second harmonic conductivity is approximately 200 times larger than seen in the standard candle nonlinear crystal, GaAs. This remarkably large SHG response provokes the question of ultimate limits on $\sigma^{(2)}$ , which we address by a new theorem relating frequency-integrated nonlinear response functions to the third cumulant (or "skewness") of the polarization distribution function in the ground state. This theorem provides considerable insight into the factors that lead to the largest possible second-order nonlinear response, specifically showing that the spectral weight is unbounded and potentially divergent when the possibility of next-neighbor hopping is included., Comment: 7 pages, 4 figures

We study the intrinsic transport anisotropy and fermiology of the quasi one-dimensional superconductor Ta$_4$Pd$_3$Te$_{16}$. Below $T^*=20$ K we detect a thermodynamic phase transition that predominantly affects the conductivity perpendicular to the quasi one-dimensional chains, consistent with a thermodynamic transition related to the presence of charge order that precedes superconductivity. Remarkably the Fermi surface pockets detected by de Haas-van Alphen (dHvA) oscillations are unaffected by this transition, suggesting that the ordered state does not break any translational symmetries but rather alters the scattering of the quasiparticles themselves., Comment: 8 pages, 5 figures

Although Weyl fermions have proven elusive in high-energy physics, their existence as emergent quasiparticles has been predicted in certain crystalline solids in which either inversion or time-reversal symmetry is broken\cite{WanPRB2011,BurkovPRL2011, WengPRX2015,HuangNatComm2015}. Recently they have been observed in transition metal monopnictides (TMMPs) such as TaAs, a class of noncentrosymmetric materials that heretofore received only limited attention \cite{XuScience2015, LvPRX2015, YangNatPhys2015}. The question that arises now is whether these materials will exhibit novel, enhanced, or technologically applicable electronic properties. The TMMPs are polar metals, a rare subset of inversion-breaking crystals that would allow spontaneous polarization, were it not screened by conduction electrons \cite{anderson1965symmetry,shi2013ferroelectric,kim2016polar}. Despite the absence of spontaneous polarization, polar metals can exhibit other signatures of inversion-symmetry breaking, most notably second-order nonlinear optical polarizability, $\chi^{(2)}$, leading to phenomena such as optical rectification and second-harmonic generation (SHG). Here we report measurements of SHG that reveal a giant, anisotropic $\chi^{(2)}$ in the TMMPs TaAs, TaP, and NbAs. With the fundamental and second harmonic fields oriented parallel to the polar axis, the value of $\chi^{(2)}$ is larger by almost one order of magnitude than its value in the archetypal electro-optic materials GaAs \cite{bergfeld2003second} and ZnTe \cite{wagner1998dispersion}, and in fact larger than reported in any crystal to date., Comment: Published in Nature Physics

We study the interplay of interactions and disorder in a one-dimensional fermion lattice coupled adiabatically to infinite reservoirs. We employ both the functional renormalization group (FRG) as well as matrix product state techniques, which serve as an accurate benchmark for small systems. Using the FRG, we compute the length- and temperature-dependence of the conductance averaged over $10^4$ samples for lattices as large as $10^{5}$ sites. We identify regimes in which non-ohmic power law behavior can be observed and demonstrate that the corresponding exponents can be understood by adapting earlier predictions obtained perturbatively for disordered Luttinger liquids. In presence of both disorder and isolated impurities, the conductance has a universal single-parameter scaling form. This lays the groundwork for an application of the functional renormalization group to the realm of many-body localization.

It is typically assumed that disorder is essential to realize Anderson localization. Recently, a number of proposals have suggested that an interacting, translation invariant system can also exhibit localization. We examine these claims in the context of a one-dimensional spin ladder. At intermediate time scales, we find slow growth of entanglement entropy consistent with the phenomenology of many-body localization. However, at longer times, all finite wavelength spin polarizations decay in a finite time, independent of system size. We identify a single length scale which parametrically controls both the eventual spin transport times and the divergence of the susceptibility to spin glass ordering. We dub this long pre-thermal dynamical behavior, intermediate between full localization and diffusion, quasi-many body localization., Comment: 7 pages, 7 figures

We study finite-temperature transport properties of the one-dimensional Hubbard model using the density matrix renormalization group. Our aim is two-fold: First, we compute both the charge and the spin current correlation function of the integrable model at half filling. The former decays rapidly, implying that the corresponding Drude weight is either zero or very small. Second, we calculate the optical charge conductivity sigma(omega) in presence of small integrability-breaking next-nearest neighbor interactions (the extended Hubbard model). The DC conductivity is finite and diverges as the temperature is decreased below the gap. Our results thus suggest that the half-filled, gapped Hubbard model is a normal charge conductor at finite temperatures. As a testbed for our numerics, we compute sigma(omega) for the integrable XXZ spin chain in its gapped phase.

We show that the magnetization of a single `qubit' spin weakly coupled to an otherwise isolated disordered spin chain exhibits periodic revivals in the localized regime, and retains an imprint of its initial magnetization at infinite time. We demonstrate that the revival rate is strongly suppressed upon adding interactions after a time scale corresponding to the onset of the dephasing that distinguishes many-body localized phases from Anderson insulators. In contrast, the ergodic phase acts as a bath for the qubit, with no revivals visible on the time scales studied. The suppression of quantum revivals of local observables provides a quantitative, experimentally observable alternative to entanglement growth as a measure of the `non-ergodic but dephasing' nature of many-body localized systems., Comment: 5 pages + appendices. v4: published version

The quantum evolution after a metallic lead is suddenly connected to an electron system contains information about the excitation spectrum of the combined system. We exploit this type of "quantum quench" to probe the presence of Majorana fermions at the ends of a topological superconducting wire. We obtain an algebraically decaying overlap (Loschmidt echo) ${\cal L}(t)=| < \psi(0) | \psi(t) > |^2\sim t^{-\alpha}$ for large times after the quench, with a universal critical exponent $\alpha$=1/4 that is found to be remarkably robust against details of the setup, such as interactions in the normal lead, the existence of additional lead channels or the presence of bound levels between the lead and the superconductor. As in recent quantum dot experiments, this exponent could be measured by optical absorption, offering a new signature of Majorana zero modes that is distinct from interferometry and tunneling spectroscopy., Comment: 9 pages + appendices, 4 figures. v3: published version

We study the spin- and energy dynamics in one-dimensional spin-1/2 systems induced by local quantum quenches at finite temperatures using a time-dependent density matrix renormalization group method. System sizes are chosen large enough to ensure that the time-dependent data for the accesible time scales represents the behavior in the thermodynamic limit. As a main result, we observe a ballistic spreading of perturbations of the energy density in the integrable spin-1/2 XXZ chain for all temperatures and exchange anisotropies, related to the divergent thermal conductivity in this model and the exact conservation of the energy current. In contrast, the spin dynamics is ballistic in the massless phase, but shows a diffusive behavior at high temperatures in the easy-axis phase in the case of a vanishing background spin density. We extract a quantitative estimate for the spin diffusion constant from the time dependence of the spatial variance of the spin density, which agrees well with values obtained from current-current correlation functions using an Einstein relation. As an example for non-integrable models, we consider two-leg ladders, for which we observe indications of diffusive energy and spin dynamics. The relevance of our results for recent experiments with quantum magnets and bosons in optical lattices is discussed.

Finite-temperature transport properties of one-dimensional systems can be studied using the time dependent density matrix renormalization group via the introduction of auxiliary degrees of freedom which purify the thermal statistical operator. We demonstrate how the numerical effort of such calculations is reduced when the physical time evolution is augmented by an additional time evolution within the auxiliary Hilbert space. Specifically, we explore a variety of integrable and non-integrable, gapless and gapped models at temperatures ranging from T=infty down to T/bandwidth=0.05 and study both (i) linear response where (heat and charge) transport coefficients are determined by the current-current correlation function and (ii) non-equilibrium driven by arbitrary large temperature gradients. The modified DMRG algorithm removes an 'artificial' build-up of entanglement between the auxiliary and physical degrees of freedom. Thus, longer time scales can be reached.

Many low-dimensional materials are well described by integrable one-dimensional models such as the Hubbard model of electrons or the Heisenberg model of spins. However, the small perturbations to these models required to describe real materials are expected to have singular effects on transport quantities: integrable models often support dissipationless transport, while weak non-integrable terms lead to finite conductivities. We use matrix-product-state methods to obtain quantitative values of spin/electrical and thermal conductivities in an almost integrable gapless chain (an XXZ spin chain with staggered fields, or equivalently a spinless fermion chain with staggered on-site potentials). The results at low temperatures validate a scaling theory based on bosonization.

We study the real-time dynamics of spin chains driven out of thermal equilibrium by an initial temperature gradient T_L \neq T_R using density matrix renormalization group methods. We demonstrate that the nonequilibrium energy current saturates fast to a finite value if the linear-response thermal conductivity is infinite, i.e. if the Drude weight D is nonzero. Our data suggests that a nonintegrable dimerized chain might support such dissipationless transport (D>0). We show that the steady-state value J_E of the current for arbitrary T_L \neq T_R is of the functional form J_E=f(T_L)-f(T_R), i.e. it is completely determined by the linear conductance. We argue for this functional form, which is essentially a Stefan-Boltzmann law in this integrable model; for the XXX ferromagnet, f can be computed via thermodynamic Bethe ansatz in good agreement with the numerics. Inhomogeneous systems exhibiting different bulk parameters as well as Luttinger liquid boundary physics induced by single impurities are discussed briefly.

We study one-dimensional spinless fermions at zero and finite temperature T using the density matrix renormalization group. We consider nearest as well as next-nearest neighbor interactions; the latter render the system inaccessible by a Bethe ansatz treatment. Using an infinite-system alogrithm we demonstrate the emergence of Luttinger liquid physics at low energies for a variety of static correlation functions as well as for thermodynamic properties. The characteristic power law suppression of the momentum distribution n(k) function at T=0 can be directly observed over several orders of magnitude. At finite temperature, we show that n(k) obeys a scaling relation. The Luttinger liquid parameter and the renormalized Fermi velocity can be extracted from the density response function, the specific heat, and/or the susceptibility without the need to carry out any finite-size analysis. We illustrate that the energy scale below which Luttinger liquid power laws manifest vanishes as the half-filled system is driven into a gapped phase by large interactions.

We propose an easily implemented approach to study time-dependent correlation functions of one dimensional systems at finite temperature T using the density matrix renormalization group. The entanglement growth inherent to any time-dependent calculation is significantly reduced if the auxiliary degrees of freedom which purify the statistical operator are time evolved with the physical Hamiltonian but reversed time. We exploit this to investigate the long time behavior of current correlation functions of the XXZ spin-1/2 Heisenberg chain. This allows a direct extraction of the Drude weight D at intermediate to large T. We find that D is nonzero -- and thus transport is dissipationless -- everywhere in the gapless phase. At low temperatures we establish an upper bound to D by comparing with bosonization.

A direct signature of electron transport at the metallic surface of a topological insulator is the Aharonov-Bohm oscillation observed in a recent study of Bi_2Se_3 nanowires [Peng et al., Nature Mater. 9, 225 (2010)] where conductance was found to oscillate as a function of magnetic flux $\phi$ through the wire, with a period of one flux quantum $\phi_0=h/e$ and maximum conductance at zero flux. This seemingly agrees neither with diffusive theory, which would predict a period of half a flux quantum, nor with ballistic theory, which in the simplest form predicts a period of $\phi_0$ but a minimum at zero flux due to a nontrivial Berry phase in topological insulators. We show how h/e and h/2e flux oscillations of the conductance depend on doping and disorder strength, provide a possible explanation for the experiments, and discuss further experiments that could verify the theory., Comment: 4 pages, 3 figures; v2. added data for weak antilocalization

We study a realization of a 1d chain of Majorana bound states at the interfaces between alternating ferromagnetic and superconducting regions at a quantum spin Hall insulator edge. In the limit of well separated Majoranas, the system can be mapped to the transverse field Ising model. The disordered critical point can be reached by tuning the relative magnitude or phases of the ferromagnetic and superconducting order parameters. We compute the voltage dependence of the tunneling current from a metallic tip into the Majorana chain as a direct probe of the random critical state., Comment: 5 pages, 3 figures

The photocurrent in an optically active metal is known to contain a component that switches sign with the helicity of the incident radiation. At low frequencies, this current depends on the orbital Berry phase of the Bloch electrons via the "anomalous velocity" of Karplus and Luttinger. We consider quantum wells in which the parent material, such as GaAs, is not optically active and the relevant Berry phase only arises as a result of quantum confinement. Using an envelope approximation that is supported by numerical tight-binding results, it is shown that the Berry phase contribution is determined for realistic wells by a cubic Berry phase intrinsic to the bulk material, the well width, and the well direction. These results for the magnitude of the Berry-phase effect suggest that it may already have been observed in quantum well experiments., Comment: 4 pages, 2 figures

An odd number of gapless Dirac fermions is guaranteed to exist at a surface of a strong topological insulator. We show that in a thin-film geometry and under external bias, electron-hole pairs that reside in these surface states can condense to form a coherent exciton condensate, similar in general terms to the exciton condensate recently argued to exist in a biased graphene bilayer, but with different topological properties. Such a `topological' exciton condensate (TEC) exhibits a host of unusual properties; the most interesting among them is the fractional charge +-e/2 carried by a singly quantized vortex in the TEC order parameter., Comment: 4 pages, 1 figure, version to appear in PRL (minor stylistic changes). For related work and info visit http://www.physics.ubc.ca/~franz/

We study the S=1 square lattice Heisenberg antiferromagnet with spatially anisotropic nearest neighbor couplings $J_{1x}$, $J_{1y}$ frustrated by a next-nearest neighbor coupling $J_{2}$ numerically using the density-matrix renormalization group (DMRG) method and analytically employing the Schwinger-Boson mean-field theory (SBMFT). Up to relatively strong values of the anisotropy, within both methods we find quantum fluctuations to stabilize the N\'{e}el ordered state above the classically stable region. Whereas SBMFT suggests a fluctuation-induced first order transition between the N\'{e}el state and a stripe antiferromagnet for $1/3\leq J_{1x}/J_{1y}\leq 1$ and an intermediate paramagnetic region opening only for very strong anisotropy, the DMRG results clearly demonstrate that the two magnetically ordered phases are separated by a quantum disordered region for all values of the anisotropy with the remarkable implication that the quantum paramagnetic phase of the spatially isotropic $J_{1}$-$J_{2}$ model is continuously connected to the limit of decoupled Haldane spin chains. Our findings indicate that for S=1 quantum fluctuations in strongly frustrated antiferromagnets are crucial and not correctly treated on the semiclassical level., Comment: 10 pages, 10 figures

We present an approach to tune the effective mass in an oxide semiconductor by a double doping mechanism. We demonstrate this in a model oxide system Sr$_{1-x}$La$_x$TiO$_{3-\delta}$, where we can tune the effective mass ranging from 6--20$\mathrm{m_e}$ as a function of filling or carrier concentration and the scattering mechanism, which are dependent on the chosen lanthanum and oxygen vacancy concentrations. The effective mass values were calculated from the Boltzmann transport equation using the measured transport properties of thin films of Sr$_{1-x}$La$_x$TiO$_{3-\delta}$. Our method, which shows that the effective mass decreases with carrier concentration, provides a means for understanding the nature of transport processes in oxides, which typically have large effective mass and low electron mobility, contrary to the tradional high mobility semiconductors., Comment: 5 pages with 4 figures

The topological insulator is an electronic phase stabilized by spin-orbit coupling that supports propagating edge states and is not adiabatically connected to the ordinary insulator. In several ways it is a spin-orbit-induced analogue in time-reversal-invariant systems of the integer quantum Hall effect (IQHE). This paper studies the topological insulator phase in disordered two-dimensional systems, using a model graphene Hamiltonian introduced by Kane and Mele as an example. The nonperturbative definition of a topological insulator given here is distinct from previous efforts in that it involves boundary phase twists that couple only to charge, does not refer to edge states, and can be measured by pumping cycles of ordinary charge. In this definition, the phase of a Slater determinant of electronic states is determined by a Chern parity analogous to Chern number in the IQHE case. Numerically we find, in agreement with recent network model studies, that the direct transition between ordinary and topological insulators that occurs in band structures is a consequence of the perfect crystalline lattice. Generically these two phases are separated by a metallic phase, which is allowed in two dimensions when spin-orbit coupling is present. The same approach can be used to study three-dimensional topological insulators., Comment: 12 pages, 10 figures

The thermal conductance by phonons of a quasi-one-dimensional solid with isotope or defect scattering is studied using the Landauer formalism for thermal transport. The conductance shows a crossover from localized to Ohmic behavior, just as for electrons, but the nature of this crossover is modified by delocalization of phonons at low frequency. A scalable numerical transfer-matrix technique is developed and applied to model quasi-one-dimensional systems in order to confirm simple analytic predictions. We argue that existing thermal conductivity data on semiconductor nanowires, showing an unexpected linear dependence, can be understood through a model that combines incoherent surface scattering for short-wavelength phonons with nearly ballistic long-wavelength phonons. It is also found that even when strong phonon localization effects would be observed if defects are distributed throughout the wire, localization effects are much weaker when defects are localized at the boundary, as in current experiments., Comment: 13 pages

The search for semiconductors with high thermoelectric figure of merit has been greatly aided by theoretical modeling of electron and phonon transport, both in bulk materials and in nanocomposites. Recent experiments have studied thermoelectric transport in ``strongly correlated'' materials derived by doping Mott insulators, whose insulating behavior without doping results from electron-electron repulsion, rather than from band structure as in semiconductors. Here a unified theory of electrical and thermal transport in the atomic and ``Heikes'' limit is applied to understand recent transport experiments on sodium cobaltate and other doped Mott insulators at room temperature and above. For optimal electron filling, a broad class of narrow-bandwidth correlated materials are shown to have power factors (the electronic portion of the thermoelectric figure of merit) as high at and above room temperature as in the best semiconductors., Comment: 4 pages, 4 figures

The topological invariants of a time-reversal-invariant band structure in two dimensions are multiple copies of the $\mathbb{Z}_2$ invariant found by Kane and Mele. Such invariants protect the topological insulator and give rise to a spin Hall effect carried by edge states. Each pair of bands related by time reversal is described by a single $\mathbb{Z}_2$ invariant, up to one less than half the dimension of the Bloch Hamiltonians. In three dimensions, there are four such invariants per band. The $\mathbb{Z}_2$ invariants of a crystal determine the transitions between ordinary and topological insulators as its bands are occupied by electrons. We derive these invariants using maps from the Brillouin zone to the space of Bloch Hamiltonians and clarify the connections between $\mathbb{Z}_2$ invariants, the integer invariants that underlie the integer quantum Hall effect, and previous invariants of ${\cal T}$-invariant Fermi systems., Comment: 4 pages

Systems near to quantum critical points show universal scaling in their response functions. We consider whether this scaling is reflected in their fluctuations; namely in current-noise. Naive scaling predicts low-temperature Johnson noise crossing over to noise power $\propto E^{z/(z+1)}$ at strong electric fields. We study this crossover in the metallic state at the 2d z=1 superconductor/insulator quantum critical point. Using a Boltzmann-Langevin approach within a 1/N-expansion, we show that the current noise obeys a scaling form $S_j=T \Phi[T/T_{eff}(E)]$ with $T_{eff} \propto \sqrt{E}$. We recover Johnson noise in thermal equilibrium and $S_j \propto \sqrt{E}$ at strong electric fields. The suppression from free carrier shot noise is due to strong correlations at the critical point. We discuss its interpretation in terms of a diverging carrier charge $\propto 1/\sqrt{E}$ or as out-of-equilibrium Johnson noise with effective temperature $\propto \sqrt{E}$., Comment: 5 pages

The $s=1$ spinor Bose condensate at zero temperature supports ferromagnetic and polar phases that combine magnetic and superfluid ordering. We analyze the topological defects of the polar condensate, correcting previous studies, and show that the polar condensate in two dimensions is unstable at any finite temperature; instead there is a nematic or paired superfluid phase with algebraic order in $\exp(2 i \theta)$, where $\theta$ is the superfluid phase, and no magnetic order. The Kosterlitz-Thouless transition out of this phase is driven by unbinding of half-vortices (the spin-disordered version of the combined spin and phase defects found by Zhou), and the anomalous universal $8 T_c / \pi$ stiffness jump at the transition is confirmed in numerical simulations. The anomalous stiffness jump is a clear experimental signature of this phase and the corresponding phase transition., Comment: 4 pages, 2 figures; published version

An electron propagating through a solid carries spin angular momentum in addition to its mass and charge. Of late there has been considerable interest in developing electronic devices based on the transport of spin, which offer potential advantages in dissipation, size, and speed over charge-based devices. However, these advantages bring with them additional complexity. Because each electron carries a single, fixed value (-e) of charge, the electrical current carried by a gas of electrons is simply proportional to its total momentum. A fundamental consequence is that the charge current is not affected by interactions that conserve total momentum, notably collisions among the electrons themselves. In contrast, the electron's spin along a given spatial direction can take on two values, "up" and "down", so that the spin current and momentum need not be proportional. Although the transport of spin polarization is not protected by momentum conservation, it has been widely assumed that, like the charge current, spin current is unaffected by electron-electron (e-e) interactions. Here we demonstrate experimentally not only that this assumption is invalid, but that over a broad range of temperature and electron density, the flow of spin polarization in a two-dimensional gas of electrons is controlled by the rate of e-e collisions.

The stability to interactions and disorder of the quantum spin Hall effect (QSHE) proposed for time-reversal-invariant 2D systems is discussed. The QSHE requires an energy gap in the bulk and gapless edge modes that conduct spin-up and spin-down excitations in opposite directions. When the number of Kramers pairs of edge modes is odd, certain one-particle scattering processes are forbidden due to a topological $\mathbb{Z}_2$ index. We show that in a many-body description, there are other scattering processes that can localize the edge modes and destroy the QSHE: the region of stability for both classes of models (even or odd number of Kramers pairs) is obtained explicitly in the chiral boson theory. For a single Kramers pair the QSHE is stable to weak interactions and disorder, while for two Kramers pairs it is not; however, the two-pair case can be stabilized by {\it either} finite attractive or repulsive interactions. For the simplest case of a single pair of edge modes, it is shown that changing the screening length in an edge with screened Coulomb interactions can be used to drive a phase transition between the QSHE state and the ordinary insulator., Comment: 6 pages, 2 figures

Randomly diluted quantum boson and spin models in two dimensions combine the physics of classical percolation with the well-known dimensionality dependence of ordering in quantum lattice models. This combination is rather subtle for models that order in two dimensions but have no true order in one dimension, as the percolation cluster near threshold is a fractal of dimension between 1 and 2: two experimentally relevant examples are the O(2) quantum rotor and the Heisenberg antiferromagnet. We study two analytic descriptions of the O(2) quantum rotor near the percolation threshold. First a spin-wave expansion is shown to predict long-ranged order, but there are statistically rare points on the cluster that violate the standard assumptions of spin-wave theory. A real-space renormalization group (RSRG) approach is then used to understand how these rare points modify ordering of the O(2) rotor. A new class of fixed points of the RSRG equations for disordered 1D bosons is identified and shown to support the existence of long-range order on the percolation backbone in two dimensions. These results are relevant to experiments on bosons in optical lattices and superconducting arrays, and also (qualitatively) for the diluted Heisenberg antiferromagnet.

The Karplus-Luttinger anomalous velocity is shown to lead to electric-field-induced charge accumulation in nearly ferromagnetic noncollinear magnets with itinerant electrons, like $MnSi$. For helical magnetic ordering, the balance between this accumulation and the Coulomb interaction leads to a nonequilibrium charge density wave state with the period of the helix, even when such accumulation is forbidden by an approximate gauge-like symmetry in the absence of electric field. We compute the strength of such charge accumulation as an example of how unexpected many-electron physics is induced by the inclusion of the one-electron Karplus-Luttinger term whenever the local exchange field felt by conduction electrons does not satisfy the current-free Maxwell equations., Comment: 5 pages and 1 figure

The phase diagram of the uniaxially anisotropic $s=1$ antiferromagnet on the kagom\'e lattice includes a critical line exactly described by the classical three-color model. This line is distinct from the standard geometric classical criticality that appears in the classical limit ($s \to \infty$) of the 2D XY model; the $s=1$ geometric T=0 critical line separates two unconventional plaquette-ordered phases that survive to nonzero temperature. The experimentally important correlations at finite temperature and the nature of the transitions into these ordered phases are obtained using the mapping to the three-color model and a combination of perturbation theory and a variational ansatz for the ordered phases. The ordered phases show sixfold symmetry breaking and are similar to phases proposed for the honeycomb lattice dimer model and $s=1/2$ $XXZ$ model. The same mapping and phase transition can be realized also for integer spins $s \geq 2$ but then require strong on-site anisotropy in the Hamiltonian., Comment: 5 pages, 2 figures

For quantum critical spin chains without disorder, it is known that the entanglement of a segment of N>>1 spins with the remainder is logarithmic in N with a prefactor fixed by the central charge of the associated conformal field theory. We show that for a class of strongly random quantum spin chains, the same logarithmic scaling holds for mean entanglement at criticality and defines a critical entropy equivalent to central charge in the pure case. This effective central charge is obtained for Heisenberg, XX, and quantum Ising chains using an analytic real-space renormalization group approach believed to be asymptotically exact. For these random chains, the effective universal central charge is characteristic of a universality class and is consistent with a c-theorem., Comment: 4 pages, 3 figures

Some frustrated magnets and superconducting arrays possess unusual symmetries that cause the free energy or other physics of a $D$-dimensional quantum or classical problem to be that of a different problem in a reduced dimension $d

The reduction of 2D superconducting or antiferromagnetic order by random dilution is studied as a model for the 2D diluted Heisenberg antiferromagnet (DHAF) La$_2$Cu$_{1-p}$(Zn,Mg)$_p$O$_4$ and randomly inhomogeneous 2D suerconductors. We show in simplified models that long-range order can persist at the percolation threshold despite the presence of disordered one-dimensional segments, contrary to the classical case. When long-range order persists to the percolation threshold, charging effects (in the superconductor) or frustrating interactions (in the antiferromagnet) can dramatically modify the stiffness of the order. This quantum destruction of stiffness is used to model neutron scattering data on La$_2$Cu$_{1-p}$(Zn,Mg)$_p$O$_4$. In a certain simplified model, there is a sharp stiffness transition between ``stiff'' and ``floppy'' ordered phases., Comment: 4 pages, 3 figures

Experiments studying vibrational effects on electronic transport through single molecules have observed several seemingly inconsistent behaviors, ranging from up to 30 harmonics of a vibrational frequency in one experiment, to an absence of higher-harmonic peaks in another. We study the different manifestations of electronic-vibrational coupling in inelastic and elastic electron transport through single molecules. For the case of inelastic transport, higher harmonics are shown to be damped by additional small factors beyond powers of the electron-vibration coupling constant $\lambda$. Two mechanisms greatly increase the size of secondary peaks in inelastic transport: coupling between electron transport and spatial motion of the molecule, and the ``pumping'' of higher vibrational modes of the molecule when vibrational excitations do not completely relax between electron transits.