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Conductive materials are required for sensing and actuation purposes in microfluidic devices. Electrical and mechanical properties of aligned CNTs/PDMS nanocomposites fabricated in AC and quasi-AC electric fields were measured. Field emission scanning electron microscope and elemental mapping were used to evaluate the microstructural properties of fabricated specimens. Results showed that nanocomposite properties were dependent on CNT concentration. A homogenized and nonagglomerated composite was obtained using a quasi-AC electric field with the voltage of 1075 V zero to peak at a frequency of 100 Hz and current of 35 milliamps when applied to suspension for 2 hours at 80 °C. The aligned nanocomposite with 1 wt% of CNT exhibited an electrical conductivity, Young's modulus, and tensile strength of 10-6 S/cm, 7.23 MPa, and 1.02 MPa, respectively. [ABSTRACT FROM AUTHOR]