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The paper presents an experimental program on a structural system, consisting of three long-span portal frames. The primary structural members, including columns and rafters, were constructed using cold-rolled aluminium back-to-back built-up channel sections. The system configuration featured two bays of single-span cold-rolled aluminium portal frames connected in parallel by a series of purlins spanning between the rafters to create a free-standing structure. A total of three full-scale tests (Frame Tests 1,2 & 3) were conducted with two loading scenarios. Frame Tests 1&2, which were identical to ensure accuracy, were subjected to vertical loads only, while Frame Test 3 underwent testing with combined horizontal and vertical loads. In all the tests, the columns were unbraced. The main objectives of this paper are, first, to describe the test setups and observe the structural behaviours of the portal frame systems. Consequently, the ultimate capacities were determined, and the predominant failure modes of the portal systems were identified as flexural-torsional buckling of the unbraced columns. The paper also provides information on the mechanical properties of the aluminium alloy 5052-H36 materials used to fabricate the structural members and frame components, obtained from compressive and tensile coupon tests. Further, the elastic buckling loads of the columns in the frame systems are reported in this paper, as determined from the measured load-deformation curves. While this paper primarily delves into the behaviour of the cold-rolled aluminium portal frames with a focus on flexural torsional buckling failures of unbraced columns, the authors have also conducted a separate study on the same system. In that separate study, the portal frames with the columns predominantly restrained against flexural-torsional buckling were investigated to enhance the ultimate capacities of the portal frame systems. • Three full-scale portal frames fabricated from cold-rolled aluminium back-to-back built-up channel sections are tested. • Aluminium alloy 5052-H36 materials are used to fabricate the cold-rolled aluminium structural members and frame components. • Portal frames are tested under two loading cases, including vertical loads only and combined horizontal and vertical loads. • Observed failure mode of the portal frames is flexural-torsional buckling of the unbraced columns. • Elastic critical loads of the columns of the portal frame tests are determined using the measured load-deformation curves. [ABSTRACT FROM AUTHOR]