Search

The Dirac equation has resided among the greatest successes of modern physics since its emergence as the first quantum mechanical theory fully compatible with special relativity. This compatibility ensures that the expectation value of the velocity is less than the vacuum speed of light. Here, we show that the Dirac equation admits free-particle solutions where the peak amplitude of the wavefunction can travel at any velocity, including those exceeding the vacuum speed of light, despite having a subluminal velocity expectation value. The solutions are constructed by superposing basis functions with correlations in momentum space. These arbitrary velocity wavefunctions feature a near-constant profile and may impact quantum mechanical processes that are sensitive to the local value of the probability density as opposed to expectation values.

We show that the dynamics of high-intensity laser pulses undergoing self-focused propagation in a nonlinear medium can be understood in terms of the topological constraints imposed by the formation and evolution of spatiotemporal optical vortices (STOVs). STOVs are born from point phase defects on the sides of the pulse nucleated by spatiotemporal phase shear. These defects grow into closed loops of spatiotemporal vorticity that initially exclude the pulse propagation axis, but then reconnect to form a pair of toroidal vortex rings that wrap around it. STOVs constrain the intrapulse flow of electromagnetic energy, controlling the focusing-defocusing cycles and pulse splitting inherent to nonlinear pulse propagation. We illustrate this in two widely studied but very different regimes, relativistic self-focusing in plasma and non-relativistic self-focusing in gas, demonstrating that STOVs mediate nonlinear propagation irrespective of the detailed physics.

Spatiotemporal control encompasses a variety of techniques for producing laser pulses with dynamic intensity peaks that move independently of the group velocity. This controlled motion of the intensity peak offers a new approach to optimizing laser-based applications and enhancing signatures of fundamental phenomena. Here, we demonstrate spatiotemporal control with a plasma optic. A chirped laser pulse focused by a plasma lens exhibits a moving focal point, or "flying focus," that can travel at an arbitrary, predetermined velocity. Unlike currently used conventional or adaptive optics, a plasma lens can be located close to the interaction region and can operate at an orders of magnitude higher, near-relativistic intensity.

Inference of joule-class THz radiation sources from microchannel targets driven with hundreds of joule, picosecond lasers is reported. THz sources of this magnitude are useful for nonlinear pumping of matter and for charged-particle acceleration and manipulation. Microchannel targets demonstrate increased laser-THz conversion efficiency compared to planar foil targets, with laser energy to THz energy conversion up to approximately 0.9% in the best cases., Comment: 9 pages, 2 figures

Electron-positron pair creation occurs throughout the universe in the environments of extreme astrophysical objects, such as pulsar magnetospheres and black hole accretion disks. The difficulty of emulating these environments in the laboratory has motivated the use of ultrahigh-intensity laser pulses for pair creation. Here we show that the phase offset between a laser pulse and its second harmonic can be used to control the relative transverse motion of electrons and positrons created in the nonlinear Breit-Wheeler process. Analytic theory and particle-in-cell simulations of a head-on collision between a two-color laser pulse and electron beam predict that with an appropriate phase offset, the electrons will drift in one direction and the positrons in the other. The resulting current may provide a collective signature of nonlinear Breit-Wheeler, while the spatial separation resulting from the relative motion may facilitate isolation of positrons for subsequent applications or detection., Comment: 8 pages, 5 figures

Electrostatic waves play a critical role in nearly every branch of plasma physics from fusion to advanced accelerators, to astro, solar, and ionospheric physics. The properties of planar electrostatic waves are fully determined by the plasma conditions, such as density, temperature, ionization state, or details of the distribution functions. Here we demonstrate that electrostatic wavepackets structured with space-time correlations can have properties that are independent of the plasma conditions. For instance, an appropriately structured electrostatic wavepacket can travel at any group velocity, even backward with respect to its phase fronts, while maintaining a localized energy density. These linear, propagation-invariant wavepackets can be constructed with or without orbital angular momentum by superposing natural modes of the plasma and can be ponderomotively excited by space-time structured laser pulses like the flying focus.

"Flying focus" techniques produce laser pulses with dynamic focal points that travels distances much greater than a Rayleigh length. The implementation of these techniques in laser-based applications requires the design of optical configurations that can both extend the focal range and structure the radial group delay. This article describes a method for designing optical configurations that produce ultrashort flying focus pulses with arbitrary-trajectory focal points. The method is illustrated by several examples that employ an axiparabola for extending the focal range and either a reflective echelon or a deformable mirror-spatial light modulator pair for structuring the radial group delay. The latter configuration enables rapid exploration and optimization of flying foci, which could be ideal for experiments.

Numerical modeling of electromagnetic waves is an important tool for understanding the interaction of light and matter, and lies at the core of computational electromagnetics. Traditional approaches to injecting and evolving electromagnetic waves, however, can be prohibitively expensive and complex for emerging problems of interest and can restrict the comparisons that can be made between simulation and theory. As an alternative, we demonstrate that electromagnetic waves can be incorporated analytically by decomposing the physics equations into analytic and computational parts. In particle-in-cell simulation of laser--plasma interaction, for example, treating the laser pulse analytically enables direct examination of the validity of approximate solutions to Maxwell's equations including Laguerre--Gaussian beams, allows lower-dimensional simulations to capture 3-D--like focusing, and facilitates the modeling of novel space--time structured laser pulses such as the flying focus. The flexibility and new routes to computational savings introduced by this analytic pulse technique are expected to enable new simulation directions and significantly reduce computational cost in existing areas., Comment: 26 pages, 9 figures

In cross-beam energy transfer (CBET), the interference of two laser beams ponderomotively drives an ion-acoustic wave that coherently scatters light from one beam into the other. This redirection of laser beam energy can severely inhibit the performance of direct-drive inertial confinement fusion (ICF) implosions. To assess the role of nonlinear and kinetic processes in direct-drive-relevant CBET, the energy transfer between two laser beams in the plasma conditions of an ICF implosion at the OMEGA laser facility was modeled using particle-in-cell simulations. For typical laser beam intensities, the simulations are in excellent agreement with linear kinetic theory, indicating that nonlinear processes do not play a role in direct-drive implosions. At higher intensities, CBET can be modified by pump depletion, backward stimulated Raman scattering, or ion trapping, depending on the plasma density.

Coherent light sources, such as free electron lasers, provide bright beams for biology, chemistry, physics, and advanced technological applications. Increasing the brightness of these sources requires progressively larger devices, with the largest being several km long (e.g., LCLS). Can we reverse this trend, and bring these sources to the many thousands of labs spanning universities, hospitals, and industry? Here we address this long-standing question by rethinking basic principles of radiation physics. At the core of our work is the introduction of quasi-particle-based light sources that rely on the collective and macroscopic motion of an ensemble of light-emitting charges to evolve and radiate in ways that would be unphysical when considering single charges. The underlying concept allows for temporal coherence and superradiance in fundamentally new configurations, providing radiation with clear experimental signatures and revolutionary properties. The underlying concept is illustrated with plasma accelerators but extends well beyond this case, such as to nonlinear optical configurations. The simplicity of the quasi-particle approach makes it suitable for experimental demonstrations at existing laser and accelerator facilities., Comment: 15 pages, 4 figures

The intensity peak of a "flying focus" travels at a programmable velocity over many Rayleigh ranges while maintaining a near-constant profile. Assessing the extent to which these features can enhance laser-based applications requires an accurate description of the electromagnetic fields. Here we present exact analytical solutions to Maxwell's equations for the electromagnetic fields of a constant-velocity flying focus, generalized for arbitrary polarization and orbital angular momentum. The approach combines the complex source-point method, which transforms multipole solutions into beam-like solutions, with the Lorentz invariance of Maxwell's equations. Propagating the fields backward in space reveals the space-time profile that an optical assembly must produce to realize these fields in the laboratory. Comparisons with simpler paraxial solutions provide conditions for their reliable use when modeling a flying focus.

White paper to the Proceedings of the U.S. Particle Physics Community Planning Exercise (Snowmass 2021): Linear colliders based on laser-plasma accelerators, Comment: Contribution to Snowmass 2021, Accelerator Frontier

We introduce the first approach to volumetrically generate relativistically thermal plasma at gas-jet--accessible density. Using fully kinetic simulations and theory, we demonstrate that two stages of direct laser acceleration driven by two laser pulses in an applied magnetic field can heat a significant plasma volume to multi-MeV average energy. The highest-momentum feature is 2D-isotropic, persists after the interaction, and includes the majority of electrons, enabling experimental access to bulk-relativistic, high-energy-density plasma in an optically diagnosable regime for the first time.

In nonlinear Thomson scattering, a relativistic electron reflects and re-radiates the photons of a laser pulse, converting optical light to x rays or beyond. While this extreme frequency conversion offers a promising source for probing high-energy-density materials and driving uncharted regimes of nonlinear quantum electrodynamics, conventional nonlinear Thomson scattering has inherent tradeoffs in its scaling with laser intensity. Here we discover that the ponderomotive control afforded by spatiotemporal pulse shaping enables novel regimes of nonlinear Thomson scattering that substantially enhance the scaling of the radiated power, emission angle, and frequency with laser intensity. By appropriately setting the velocity of the intensity peak, a spatiotemporally shaped pulse can increase the power radiated by orders of magnitude. The enhanced scaling with laser intensity allows for operation at significantly lower electron energies and can eliminate the need for a high-energy electron accelerator., Comment: 23 pages, 4 figures

The performance of direct-drive inertial confinement fusion implosions relies critically on the coupling of laser energy to the target plasma. Cross-beam energy transfer (CBET), the resonant exchange of energy between intersecting laser beams mediated by ponderomotively driven ion-acoustic waves (IAW), inhibits this coupling by scattering light into unwanted directions. The variety of beam intersection angles and varying plasma conditions in an implosion results in IAWs with a range of phase velocities. Here we show that CBET saturates through a resonance detuning that depends on the IAW phase velocity and that results from trapping-induced modifications to the ion distribution functions. For smaller phase velocities, the modifications to the distribution functions can rapidly thermalize in the presence of mid-Z ions, leading to a blueshift in the resonant frequency. For larger phase velocities, the modifications can persist, leading to a redshift in the resonant frequency. Ultimately, these results may reveal pathways towards CBET mitigation and inform reduced models for radiation hydrodynamics codes to improve their predictive capability.

Laser wakefield accelerators rely on the extremely high electric fields of nonlinear plasma waves to trap and accelerate electrons to relativistic energies over short distances. When driven strongly enough, plasma waves break, trapping a large population of the background electrons that support their motion. This limits the maximum electric field. Here we introduce a novel regime of plasma wave excitation and wakefield acceleration that removes this limit, allowing for arbitrarily high electric fields. The regime, enabled by spatiotemporal shaping of laser pulses, exploits the property that nonlinear plasma waves with superluminal phase velocities cannot trap charged particles and are therefore immune to wave breaking. A laser wakefield accelerator operating in this regime provides energy tunability independent of the plasma density and can accommodate the large laser amplitudes delivered by modern and planned high-power, short pulse laser systems.

As an alternative inertial confinement fusion scheme with predicted high energy gain and more robust designs, shock ignition requires a strong converging shock driven by a shaped pulse with a high-intensity spike at the end to ignite a pre-compressed fusion capsule. Understanding nonlinear laser-plasma instabilities in shock ignition conditions is crucial to assess and improve the laser-shock energy coupling. Recent experiments conducted on the OMEGA-EP laser facility have for the first time demonstrated that such instabilities can $\sim$100\% deplete the first 0.5 ns of the high-intensity laser pump. Analysis of the observed laser-generated blast wave suggests that this pump-depletion starts at 0.01--0.02 critical density and progresses to 0.1--0.2 critical density. This pump-depletion is also confirmed by the time-resolved stimulated Raman backscattering spectra. The dynamics of the pump-depletion can be explained by the breaking of ion-acoustic waves in stimulated Brillouin scattering. Such strong pump-depletion would inhibit the collisional laser energy absorption but may benefit the generation of hot electrons with moderate temperatures for electron shock ignition [Shang et al. Phys. Rev. Lett. 119 195001 (2017)].

The success of direct laser-driven inertial confinement fusion (ICF) relies critically on the efficient coupling of laser light to plasma. At ignition scale, the absolute stimulated Raman scattering (SRS) instability can severely inhibit this coupling by redirecting and strongly depleting laser light. This Letter describes a new dynamic saturation regime of the absolute SRS instability. The saturation occurs when spatiotemporal fluctuations in the ion-acoustic density detune the instability resonance. The dynamic saturation mitigates the strong depletion of laser light and enhances its transmission through the instability region, explaining the coupling of laser light to ICF targets at higher plasma densities.

An overview from the past and an outlook for the future of fundamental laser-plasma interactions research enabled by emerging laser systems.

A high-intensity laser pulse propagating through a medium triggers an ionization front that can accelerate and frequency-upshift the photons of a second pulse. The maximum upshift is ultimately limited by the accelerated photons outpacing the ionization front or the ionizing pulse refracting from the plasma. Here we apply the flying focus--a moving focal point resulting from a chirped laser pulse focused by a chromatic lens--to overcome these limitations. Theory and simulations demonstrate that the ionization front produced by a flying focus can frequency-upshift an ultrashort optical pulse to the extreme ultraviolet over a centimeter of propagation. An analytic model of the upshift predicts that this scheme could be scaled to a novel table-top source of spatially coherent x-rays., Comment: 7 pages, 4 figures, 1 table

Broad bandwidth, infrared light sources have the potential to revolutionize inertial confinement fusion (ICF) by suppressing laser-plasma instabilities. There is, however, a tradeoff: The broad bandwidth precludes high efficiency conversion to the ultraviolet, where laser-plasma interactions are weaker. Operation in the infrared could intensify the role of resonance absorption, an effect long suspected to be the shortcoming of early ICF experiments. Here we present simulations exploring the effect of bandwidth on resonance absorption. In the linear regime, bandwidth has little effect on resonance absorption; in the nonlinear regime, bandwidth suppresses enhanced absorption resulting from the electromagnetic decay instability. These findings evince that regardless of bandwidth, an ICF implosion will confront at least linear levels of resonance absorption.

A chirped laser pulse focused by a chromatic lens exhibits a dynamic, or "flying," focus in which the trajectory of the peak intensity decouples from the group velocity. In a medium, the flying focus can trigger an ionization front that follows this trajectory. By adjusting the chirp, the ionization front can be made to travel at an arbitrary velocity along the optical axis. We present analytical calculations and simulations describing the propagation of the flying focus pulse, the self-similar form of its intensity profile, and ionization wave formation. The ability to control the speed of the ionization wave and, in conjunction, mitigate plasma refraction has the potential to advance several laser-based applications, including Raman amplification, photon acceleration, high harmonic generation, and THz generation.

An intense, short laser pulse incident on a transparent dielectric can excite electrons from valence to the conduction band. As these electrons undergo scattering, both from phonons and ions, they emit bremsstrahlung radiation. Here we present a theory of bremsstrahlung emission appropriate for laser pulse-dielectric interactions. Simulations of the interaction, incorporating this theory, illustrate characteristics of the radiation (power, energy and spectra) for arbitrary ratios of electron collision frequency to radiation frequency. The conversion efficiency of laser pulse energy into bremsstrahlung radiation depends strongly on both the intensity and duration of the pulse, saturating at values of about 10e-5. Depending on whether the intensity is above or below the damage threshold of the material, the emission can originate either from the surface or the bulk of the dielectric respectively. The bremsstrahlung emission may provide a broadband light source for diagnostics.

The wealth of work in backward Raman amplification in plasma has focused on the extreme intensity limit, however backward Raman amplification may also provide an effective and practical mechanism for generating intense, broad bandwidth, long-wavelength infrared radiation (LWIR). An electromagnetic simulation coupled with a relativistic cold fluid plasma model is used to demonstrate the generation of picosecond pulses at a wavelength of 10 microns with terawatt powers through backward Raman amplification. The effects of collisional damping, Landau damping, pump depletion, and wave breaking are examined, as well as the resulting design considerations for a LWIR Raman amplifier.

Raman backscattered radiation of intense laser pulses in plasma is investigated for a wide range of intensities relevant to laser wakefield acceleration. The weakly nonlinear dispersion relation for Raman backscattering predicts an intensity and density dependent frequency shift that is opposite to that suggested by a simple relativistic consideration. This observation has been benchmarked against experimental results, providing a novel diagnostic for laser-plasma interactions.

A laser pulse guided in a curved plasma channel can excite wakefields that steer electrons along an arched trajectory. As the electrons are accelerated along the curved channel, they emit synchrotron radiation. We present simple analytical models and simulations examining laser pulse guiding, wakefield generation, electron steering, and synchrotron emission in curved plasma channels. For experimentally realizable parameters, a ~2 GeV electron emits 0.1 photons per cm with an average photon energy of multiple keV.

Ultrashort long-wave infrared (LWIR) laser pulses can resonantly excite vibrations in N2 and O2 through a two-photon transition. The absorptive, vibrational component of the ultrafast optical nonlinearity grows in time, starting smaller than, but quickly surpassing, the electronic, rotational, and vibrational refractive components. The growth of the vibrational component results in a novel mechanism of 3rd harmonic generation, providing an additional two-photon excitation channel, fundamental + 3rd harmonic. The original and emergent two-photon excitations drive the resonance exactly out of phase, causing spatial decay of the absorptive, vibrational nonlinearity. This nearly eliminates two-photon vibrational absorption. Here we present simulations and analytical calculations demonstrating how these processes modify the ultrafast optical nonlinearity in air. The results reveal nonlinear optical phenomena unique to the LWIR regime of ultrashort pulse propagation in atmosphere.

Adaptive optics (AO) systems rely on the principle of reciprocity, or symmetry with respect to the interchange of point sources and receivers. These systems use the light received from a low power emitter on or near a target to compensate profile aberrations acquired by a laser beam during linear propagation through random media. If, however, the laser beam propagates nonlinearly, reciprocity is broken, potentially undermining AO correction. Here we examine the consequences of this breakdown. While discussed for general random and nonlinear media, we consider specific examples of Kerr-nonlinear, turbulent atmosphere.

We present results of energetic laser-ion acceleration from a tailored, near solid density gas target. Colliding hydrodynamic shocks compress a pure hydrogen gas jet into a 70 {\mu}m thick target prior to the arrival of the ultra-intense laser pulse. A density scan reveals the transition from a regime characterized by a wide angle, low energy beam to one of a more focused beam with a high energy halo. In the latter case, three dimensional simulations show the formation of a Z-pinch driven by the axial current resulting from laser wakefield accelerated electrons. Ions at the rear of the target are then accelerated by a combination of space charge fields from accelerated electrons and Coulombic repulsion as the pinch dissipates., Comment: 4 pages, 6 figues plus supplemental. arXiv admin note: substantial text overlap with arXiv:1507.04594

The electronic, rotational, and vibrational components of the ultrafast optical nonlinearity in H$_2$ and D$_2$ are measured directly and absolutely at intensities up to the ionization threshold of $\sim$10$^{14}$ W/cm$^2$. As the most basic nonlinear interactions of the simplest molecules exposed to high fields, these results constitute a benchmark for high field laser-matter theory and simulation., Comment: 20 pages, 5 figures. References fixed

An ideal plasma lens can provide the focusing power of a small f-number, solid-state focusing optic at a fraction of the diameter. An ideal plasma lens, however, relies on a steady-state, linear laser pulse-plasma interaction. Ultrashort multi-petawatt (MPW) pulses possess broad bandwidths and extreme intensities, and, as a result, their interaction with the plasma lens is neither steady state nor linear. Here we examine nonlinear and time-dependent modifications to plasma lens focusing, and show that these result in chromatic and phase aberrations and amplitude distortion. We find that a plasma lens can provide enhanced focusing for 30 fs pulses with peak power up to ~1 PW. The performance degrades through the MPW regime, until finally a focusing penalty is incurred at ~10 PW.

In the cavitation regime of plasma-based accelerators, a population of high-energy electrons tailing the driver can undergo betatron motion. The motion results in X-ray emission, but the brilliance and photon energy are limited by the electrons' initial transverse coordinate. To overcome this, we exploit parametrically unstable betatron motion in a cavitated, axially modulated plasma. Theory and simulations are presented showing that the unstable oscillations increase both the total X-ray energy and average photon energy.

The physical processes associated with propagation of a high-power (power > critical power for self-focusing) laser beam in water include nonlinear focusing, stimulated Raman scattering (SRS), optical breakdown and plasma formation. The interplay between nonlinear focusing and SRS is analyzed for cases where a significant portion of the pump power is channeled into the Stokes wave. Propagation simulations and an analytical model demonstrate that the Stokes wave can re-focus the pump wave after the power in the latter falls below the critical power. It is shown that this novel focusing mechanism is distinct from cross-phase focusing. While discussed here in the context of propagation in water, the gain-focusing phenomenon is general to any medium supporting nonlinear focusing and stimulated forward Raman scattering.

Optical beams propagating through air acquire phase distortions from turbulent fluctuations in the refractive index. While these distortions are usually deleterious to propagation, beams reflected in a turbulent medium can undergo a local recovery of spatial coherence and intensity enhancement referred to as enhanced backscatter (EBS). Using a combination of lab-scale experiments and simulations, we investigate the EBS of optical beams reflected from corner cubes and rough surfaces, and identify the regimes in which EBS is most distinctly observed., Comment: 10 pages, 8 figures

The axial dependence of femtosecond filamentation in air is measured under conditions of varying laser pulsewidth, energy, and focusing f-number. Filaments are characterized by the ultrafast z-dependent absorption of energy from the laser pulse and diagnosed by measuring the local single cycle acoustic wave generated. Results are compared to 2D+1 simulations of pulse propagation, whose results are highly sensitive to the instantaneous (electronic) part of the nonlinear response of $N_2$ and $O_2$. We find that recent measurements of the nonlinear refractive index ($n_2$) in [J.K. Wahlstrand et al., Phys. Rev. A. 85, 043820 (2012)] provide the best match and an excellent fit between experiments and simulations., Comment: 15 pages, 4 figures

A scheme of wake field generation for positron acceleration using hollow or donut shaped electron driver beams is studied. An annular shaped, electron free region forms around a hollow driver beam creating a favorable region (longitudinal field is accelerating and transverse field is focusing and radially linear) for positron acceleration. Accelerating gradients of the order of 10 GV/m are produced by a hollow electron beam driver with FACET like parameters. The peak accelerating field increases linearly with the total charge in the beam driver while the axial size of the favorable region ($\sim$ one plasma wavelength) remains approximately fixed. The radial size drops with the total charge but remains large enough for the placement of a witness positron beam. We simulate an efficient acceleration of a 23 GeV positron beam to 35.4 GeV with a maximum energy spread of 0.4\% and very small emittance over a plasma length of 140 cm., Comment: 5 figures, Submitted to Physical Review Letters

Compton scattered x-rays can be generated using a configuration consisting of a single, ultra-intense laser pulse, and a shaped gas target. The gas target incorporates a hydrodynamically formed density spike, which nonlinearly scatters the incident pump radiation, to produce a counter-propagating electromagnetic wiggler. This self-generated wiggler field Compton scatters from electrons accelerated in the laser wakefield of the pump radiation. The nonlinear scattering mechanism in the density spike is examined theoretically and numerically in order to optimize the Compton scattered radiation. It is found that narrow-band x-rays are produced by moderate intensity pump radiation incident on the quarter-critical surface of the density spike, while high fluence, broadband x-rays are produced by high intensity pump radiation reflected near the critical surface.

We investigate, through simulation, the modifications to Bessel and Airy beams during propagation through atmospheric turbulence. We find that atmospheric turbulence disrupts the quasi-non-diffracting nature of Bessel and Airy beams when the transverse coherence length (Fried parameter) nears the initial aperture diameter or diagonal respectively. The turbulence induced transverse phase distortion limits the effectiveness of Bessel and Airy beams for applications requiring propagation over long distances in the turbulent atmosphere.

A nonlocal quantum model is presented for calculating the atomic dielectric response to a strong laser electric field. By replacing the Coulomb potential with a nonlocal potential in the Schrodinger equation, a 3+1D calculation of the time-dependent electric dipole moment can be replaced with a 0+1D integral equation, offering significant computational savings. The model is benchmarked against an established ionization model and \textit{ab initio} simulation of the time-dependent Schrodinger equation. The reduced computational overhead makes the model a promising candidate to incorporate full quantum mechanical time dynamics in laser pulse propagation simulations., Comment: 10 pages, 8 figures

The energy gain in laser wakefield acceleration (LWFA) is ultimately limited by dephasing, occurring when accelerated electrons outrun the accelerating phase of the wakefield. We apply quasi-phasematching, enabled by axially modulated plasma channels, to overcome this limitation. By matching the modulation period to the dephasing length, a relativistic electron can undergo energy gain over several dephasing lengths. Theory and simulations are presented showing that at a weakly relativistic laser intensity, ~10^17 W/cm2, and millijoule level pulse energies, quasi-phasematched LWFA results in energy gains of 50 MeV larger than standard LWFA.

We investigate, through simulation, the evolution of polarization states during atmospheric propagation of high power, ultrashort laser pulses. A delayed rotational response model handling arbitrary, transverse polarization couples both the amplitude and phase of the polarization states. We find that, while circularly and linearly polarized pulses maintain their polarization, elliptically polarized pulses become depolarized due to energy equilibration between left and right circularly polarized states. The depolarization can be detrimental to remote radiation generation schemes and obscures time-integrated polarization measurements.