Search

The AMoRE collaboration searches for neutrinoless double beta decay of $^{100}$Mo using molybdate scintillating crystals via low temperature thermal calorimetric detection. The early phases of the experiment, AMoRE-pilot and AMoRE-I, have demonstrated competitive discovery potential. Presently, the AMoRE-II experiment, featuring a large detector array with about 90 kg of $^{100}$Mo isotope, is under construction.This paper discusses the baseline design and characterization of the lithium molybdate cryogenic calorimeters to be used in the AMoRE-II detector modules. The results from prototype setups that incorporate new housing structures and two different crystal masses (316 g and 517 - 521 g), operated at 10 mK temperature, show energy resolutions (FWHM) of 7.55 - 8.82 keV at the 2.615 MeV $^{208}$Tl $\gamma$ line, and effective light detection of 0.79 - 0.96 keV/MeV. The simultaneous heat and light detection enables clear separation of alpha particles with a discrimination power of 12.37 - 19.50 at the energy region around $^6$Li(n, $\alpha$)$^3$H with Q-value = 4.785 MeV. Promising detector performances were demonstrated at temperatures as high as 30 mK, which relaxes the temperature constraints for operating the large AMoRE-II array.

AMoRE searches for the signature of neutrinoless double beta decay of $^{100}$Mo with a 100 kg sample of enriched $^{100}$Mo. Scintillating molybdate crystals coupled with a metallic magnetic calorimeter operate at milli-Kelvin temperatures to measure the energy of electrons emitted in the decay. As a demonstration of the full-scale AMoRE, we conducted AMoRE-I, a pre-experiment with 18 molybdate crystals, at the Yangyang Underground Laboratory for over two years. The exposure was 8.02 kg$\cdot$year (or 3.89 kg$_{\mathrm{^{100}Mo}}\cdot$year) and the total background rate near the Q-value was 0.025 $\pm$ 0.002 counts/keV/kg/year. We observed no indication of $0\nu\beta\beta$ decay and report a new lower limit of the half-life of $^{100}$Mo $0\nu\beta\beta$ decay as $ T^{0\nu}_{1/2}>3.0\times10^{24}~\mathrm{years}$ at 90\% confidence level. The effective Majorana mass limit range is $m_{\beta\beta}<$(210--610) meV using nuclear matrix elements estimated in the framework of different models, including the recent shell model calculations., Comment: 8 pages, 5 figures

AMoRE-II aims to search for neutrinoless double beta decay with an array of 423 Li$_2$$^{100}$MoO$_4$ crystals operating in the cryogenic system as the main phase of the Advanced Molybdenum-based Rare process Experiment (AMoRE). AMoRE has been planned to operate in three phases: AMoRE-pilot, AMoRE-I, and AMoRE-II. AMoRE-II is currently being installed at the Yemi Underground Laboratory, located approximately 1000 meters deep in Jeongseon, Korea. The goal of AMoRE-II is to reach up to $T^{0\nu\beta\beta}_{1/2}$ $\sim$ 6 $\times$ 10$^{26}$ years, corresponding to an effective Majorana mass of 15 - 29 meV, covering all the inverted mass hierarchy regions. To achieve this, the background level of the experimental configurations and possible background sources of gamma and beta events should be well understood. We have intensively performed Monte Carlo simulations using the GEANT4 toolkit in all the experimental configurations with potential sources. We report the estimated background level that meets the 10$^{-4}$counts/(keV$\cdot$kg$\cdot$yr) requirement for AMoRE-II in the region of interest (ROI) and show the projected half-life sensitivity based on the simulation study.

We report a study on the background of the Advanced Molybdenum-Based Rare process Experiment (AMoRE), a search for neutrinoless double beta decay (\znbb) of $^{100}$Mo. The pilot stage of the experiment was conducted using $\sim$1.9 kg of \CAMOO~ crystals at the Yangyang Underground Laboratory, South Korea, from 2015 to 2018. We compared the measured $\beta/\gamma$ energy spectra in three experimental configurations with the results of Monte Carlo simulations and identified the background sources in each configuration. We replaced several detector components and enhanced the neutron shielding to lower the background level between configurations. A limit on the half-life of $0\nu\beta\beta$ decay of $^{100}$Mo was found at $T_{1/2}^{0\nu} \ge 3.0\times 10^{23}$ years at 90\% confidence level, based on the measured background and its modeling. Further reduction of the background rate in the AMoRE-I and AMoRE-II are discussed.

The construction of a butt-end multicell matrix proportional counter (MMPC) is presented in the work. Each cell is a butt-end proportional counter with a 5 mm cathode diameter and 0.8 mm circular anode diameter. In the example of the $3\times3$ matrix, it is shown that the gas multiplication of the central cell depends on the potentials at the anodes of the peripheral cells, the drift electrode, the forming rings, and the surrounding metal parts of the structure. The amplitude characteristics were measured when the MMPC was filled with mixtures of 96.3\% Ar + 3.7\% Xe and 90\% Ar + 10\% CH$_4$ at pressures of 620 Torr and 62 Torr. The calibration was carried out with $\alpha$-particles and $\gamma$-quanta from a $^{238}$Pu source. For photons with energies of 7.5 keV, a resolution of 26\% was obtained. It is shown that, based on MMPC, it is possible to fabricate recording surfaces of arbitrary configuration., Comment: 7 pages, 4 figures

The activity of $^{222}$Rn and its daughter isotopes was measured in the air of several underground laboratories of the Baksan Neutrino Observatory at various distances from the entrance. The measurements were carried out with the help of the cylindrical ionionization air chamber. We found that the radon content in the ventilated airflow within the measurement accuracy does not depend on the distance travelled along the adit. In addition, we observed that the radon content increases abruptly in those locations where underground gases and water are released. As a result, we review various mechanisms of air enrichment with radon. We also outline our research methodology and present the results of our measurements of radon release from the rocky walls of the underground laboratory. Finally, we present the results of the measurements of the radon content of various ground and underground water sources., Comment: 11 pages, 9 figures, 1 table

A new method for correcting the charge signal from the large proportional counter is proposed. The correction method makes it possible to take into account the loss of primary ionization electrons in the presence of weakly increasing micro impurities of electronegative gases during long-term measurements. It allows increasing the efficiency of the selection of useful events and thereby increasing the sensitivity to $2\nu2K$-decay in $^{124}$Xe at the level of $2\times10^{22}$ from over six years of measurements using a large proportional counter. Analysis of the calibration data, taking into account the new method for correcting the energy release in the detector, made it possible to register events from double $K$ photoionization by a single photon., Comment: 4 pages, 3 figures, to appear in the proceedings of the 17th International Conference on Topics in Astroparticle and Underground Physics (TAUP-2021) 26 August to 3 September 2021

Results of a comparative analysis of the $^{214}$Po ($T_{1/2}= 163.47\pm0.03$ $\mu$s), $^{213}$Po ($T_{1/2}=3.705 \pm 0.001$ $\mu$s) and $^{212}$Po ($T_{1/2}=294.09\pm0.07$ ns) half-life annular variation parameters are presented. It is shown that two independent sequential sets of the $^{214}$Po $\tau$-values $(\tau\equiv T_{1/2})$ obtained in the spaced laboratories can be described by sinusoidal functions. The sinusoid curve with amplitude $A=(5.0 \pm1.5) \cdot 10^{-4}$, period $\omega=(365\pm 8)$ days, and phase $\phi=(170 \pm 7)$ days approximates the set of $^{214}$Po $\tau$ values obtained at BNO INR RAS during the $\sim$973 days starting on January 4, 2012. The function approximates a set of $\tau$-values with a time duration of $\sim1460$ days obtained at the KhNU has an amplitude $A=(4.9\pm1.8)\cdot10^{-4}$, a period $\omega= (377\pm13)$ days and a phase $\phi=(77\pm10)$ days. The $^{213}$Po $\tau$-value set with a time duration of $\sim1700$ days can be described by a sinusoidal function with an amplitude $A=(3.9\pm1.2)\cdot10^{-4}$, a period $\omega= (370\pm13)$ days and a phase $\phi=(130\pm9)$ days. The $^{212}$Po $\tau$-value set with a time duration of $\sim670$ days can be described by a sinusoidal function with an amplitude $A=(7.5\pm1.6)\cdot10^{-4}$, a period $\omega= (375\pm13)$ days and a phase $\phi=(40\pm10)$ days., Comment: 6 pages, 5 figures, Prepared for the proceedings of The 5th International Conference on Particle Physics and Astrophysics (ICPPA-2020)

The study of low-yield effects requires not only good quality of the original data but also puts high requirements for their processing procedures to increase the efficiency of the selection of useful events. The exploiting of the large cylindrical proportional counter's electrostatic topology allows improving the extrapolation of information about the primary ionization of a multipoint event. Long-term calibration measurements with an external $^{109}$Cd-source allowed the development of a new method for analyzing the pulse shape from a sizeable proportional counter. Optimized analysis of the current's pulse shape from the electron cloud of primary ionization in the counter improved the resolution and energy calibration. As a result, the efficiency of selecting useful events was increased by 25\%., Comment: 6 pages, 6 figures, Prepared for the proceedings of The 5th International Conference on Particle Physics and Astrophysics (ICPPA-2020)

The Advanced Molybdenum-based Rare process Experiment (AMoRE) aims to search for neutrinoless double beta decay (0$\nu\beta\beta$) of $^{100}$Mo with $\sim$100 kg of $^{100}$Mo-enriched molybdenum embedded in cryogenic detectors with a dual heat and light readout. At the current, pilot stage of the AMoRE project we employ six calcium molybdate crystals with a total mass of 1.9 kg, produced from $^{48}$Ca-depleted calcium and $^{100}$Mo-enriched molybdenum ($^{48\textrm{depl}}$Ca$^{100}$MoO$_4$). The simultaneous detection of heat(phonon) and scintillation (photon) signals is realized with high resolution metallic magnetic calorimeter sensors that operate at milli-Kelvin temperatures. This stage of the project is carried out in the Yangyang underground laboratory at a depth of 700 m. We report first results from the AMoRE-Pilot $0\nu\beta\beta$ search with a 111 kg$\cdot$d live exposure of $^{48\textrm{depl}}$Ca$^{100}$MoO$_4$ crystals. No evidence for $0\nu\beta\beta$ decay of $^{100}$Mo is found, and a upper limit is set for the half-life of 0$\nu\beta\beta$ of $^{100}$Mo of $T^{0\nu}_{1/2} > 9.5\times10^{22}$ y at 90% C.L.. This limit corresponds to an effective Majorana neutrino mass limit in the range $\langle m_{\beta\beta}\rangle\le(1.2-2.1)$ eV.

Description of the TAU-4 installation intended for long-term monitoring of the half-life value $T_{1/2}$ of the $^{212}$Po is presented. Natural thorium used as a source of the mother's chain. The methods of measurement and data processing are described. The comparative results of short test measurements carried out in the ground (680 h) and underground (564 h) laboratories are given. Averaged value $T_{1/2}$ =$294.09\pm 0.07$ ns of the $^{212}$Po half-life has been found for the ground level data set similar one for the underground data set. The solar-daily variations with amplitudes $A_{So}=(11.7\pm 5.2)\times10^{-4}$ for the ground data and $A_{So}=(7.5\pm 4.1)\times10^{-4}$ for the underground one were found in a series of $\tau$ values., Comment: 6 pages, 5 figures, the talk at ICPPA2018, October 22-26, Moscow

We describe the Monte Carlo (MC) simulation package of the `2K-CAPTURE' setup and discuss the agreement of its output with data. The `2K-CAPTURE' MC simulates the energy loss of particles in detector and components of the passive shield and generates the resulting response in working volume large proportional counter (LPC). The simulation accounts for absorption, reemission, and scattering of both photons and neutrons and tracks them until they either are absorbed. The algorithm proceeds with a detailed simulation of the electronics chain. The MC is tuned using data collected with radioactive calibration source deployed in the internal channel of the installation. The simulation reproduces the energy response of the detector corresponding to distribution of the generated pointwise clusters of a charge of primary ionization in LPC., Comment: 6 pages, 5 figures, 1 table, presented at IV international conference on particle physics and astrophysics

The results of the experimental search for two-neutrino $2K$-capture in $^{124}$Xe with a large copper proportional counter obtained by processing the data for an exposure of 37.7 kg$\times$day are presented. The experimental setup is located at the Underground Low-Background Laboratory of the Baksan Neutrino Observatory at a depth of 4900 m w.e. The combination of methods of selection of useful signals with a unique set of characteristics and the event topology taken into account allowed us to suppress the background in the energy region of interest. A new half-life limit for $2K(2\nu)$-capture in $^{124}$Xe was determined: T$_{1/2}\geq7.7\cdot10^{21}$ yrs (90\% C.L.)., Comment: 5 pages, 4 figures; to be published in PEPAN

A device with the parent $^{229}$Th source was constructed to search for variations of the daughter $^{213}$Po half-life ($T_{1/2} = 4.2$ $\mu$s). A solar-daily variation with amplitude $A_{So}=(5.3 \pm 1.1) \times 10^{-4}$, a lunar-daily variation with amplitude $A_L = (4.8 \pm 2.1) \times 10^{-4}$, and a sidereal-daily variation with amplitude $A_S = (4.2 \pm 1.7) \times 10^{-4}$ were found upon proceeding the data series over a 622-day interval (from July 2015 to March 2017). The $^{213}$Po half-life mean value is found to be $T_{1/2} = 3.705 \pm 0.001$ $\mu$s. The obtained half-life is in good agreement with some of the literature values obtained with great accuracy., Comment: 6 pages, 9 figures; to be published in PEPAN

A search for resonant absorption of the solar axion by $^{83}\rm{Kr}$ nuclei was performed using the proportional counter installed inside the low-background setup at the Baksan Neutrino Observatory. The obtained model independent upper limit on the combination of isoscalar and isovector axion-nucleon couplings $|g_3-g_0|\leq 8.4\times 10^{-7}$ allowed us to set the new upper limit on the hadronic axion mass of $m_{A}\leq 65$ eV (95\% C.L.) with the generally accepted values $S$=0.5 and $z$=0.56., Comment: 4 pages, 2 figures, Proceedings of the 13th Patras Workshop on Axions, WIMPs and WISP, May 15th to 19th 2017, Thessaloniki, Greece

We carried out the comparative study of the signal from the decay of double $K$-shell vacancy production that follows after single $K$-shell electron capture of $^{81}$Kr and double $K$-shell electron capture of $^{78}$Kr. The radiative decay of a the double $1s$ vacancy state was identified by detecting the triple coincidence of two $K$ X-rays and several Auger electrons in the $ECEC$-decay, or by detecting two $K$ X-rays and (Auger electrons + ejected $K$-shell electron) in the $EC$ decay. The number of $K$-shell vacancies per the $K$-electron capture, produced as a result of the shake-off process, has been measured for the decay of $^{81}$Kr. The probability for this decay was found to be $P_{KK}=(5.7\pm0.8)\times10^{-5}$ with a systematic error of $(\Delta P_{KK})_{syst}=\pm0.4 \times10^{-5}$. For the $^{78}{\rm{Kr}}(2\nu2K)$ decay, the comparative study of single- and double-capture decays allowed us to obtain the signal-to-background ratio to be 15/1. The half-life $T_{1/2}^{2\nu2K}(g.s. \rightarrow g.s.) = [1.9^{+1.3}_{-0.7}(stat)\pm0.3(syst)]\times 10^{22}$ y is determined from the analysis of data that have been accumulated over 782 days of live measurements in the experiment that used samples consisted of 170.6 g of $^{78}$Kr., Comment: 17 pages, 9 figures, 1 table

The AMoRE (Advanced Mo-based Rare process Experiment) project is a series of experiments that use advanced cryogenic techniques to search for the neutrinoless double-beta decay of \mohundred. The work is being carried out by an international collaboration of researchers from eight countries. These searches involve high precision measurements of radiation-induced temperature changes and scintillation light produced in ultra-pure \Mo[100]-enriched and \Ca[48]-depleted calcium molybdate ($\mathrm{^{48depl}Ca^{100}MoO_4}$) crystals that are located in a deep underground laboratory in Korea. The \mohundred nuclide was chosen for this \zeronubb decay search because of its high $Q$-value and favorable nuclear matrix element. Tests have demonstrated that \camo crystals produce the brightest scintillation light among all of the molybdate crystals, both at room and at cryogenic temperatures. $\mathrm{^{48depl}Ca^{100}MoO_4}$ crystals are being operated at milli-Kelvin temperatures and read out via specially developed metallic-magnetic-calorimeter (MMC) temperature sensors that have excellent energy resolution and relatively fast response times. The excellent energy resolution provides good discrimination of signal from backgrounds, and the fast response time is important for minimizing the irreducible background caused by random coincidence of two-neutrino double-beta decay events of \mohundred nuclei. Comparisons of the scintillating-light and phonon yields and pulse shape discrimination of the phonon signals will be used to provide redundant rejection of alpha-ray-induced backgrounds. An effective Majorana neutrino mass sensitivity that reaches the expected range of the inverted neutrino mass hierarchy, i.e., 20-50 meV, could be achieved with a 200~kg array of $\mathrm{^{48depl}Ca^{100}MoO_4}$ crystals operating for three years., Comment: 93 pages

A construction of a thermal neutron testing detector with a thin [ZnS(Ag)+$^6$LiF] scintillator is described. Results of an investigation of sources of the detector pulse origin and the pulse features in a ground and underground conditions are presented. Measurements of the scintillator own background, registration efficiency and a neutron flux at different objects of the BNO INR RAS were performed. The results are compared with the ones measured by the $^3$He proportional counter., Comment: 6 pages, 6 figures, 1 tables

A method of measurements of the environmental neutron background at the Baksan Neutrino Observatory of the INR RAS are described. Measurements were done by using of a proportional counter filled with mixture of Ar(2 at)+$^3$He(4 at). The results obtained at the surface and the underground laboratory of the BNO INR RAS are presented. It is shown that a neutron background in the underground laboratory at the 4900 m w.e. depth is decreased by $\sim 260$ times without any special shield in a comparison with the Earth surface. A neutron flux density in the 5-1323.5~cm air height region is constant within the determination error and equal to $(7.1\pm0.1_{\rm{stat}}\pm0.3_{\rm{syst}})\times10^{-3}$ s$^{-1}\cdot$cm$^{-2}$., Comment: 5 pages, 4 figures, 2 tables

The construction and characteristics of the cylindrical ion pulse ionization chamber (CIPIC) with a working volume of 3.2 L are described. The chamber is intended to register alpha-particles from the $^{222}$Rn and its daughter's decays in the filled air sample. The detector is less sensitive to electromagnetic pick-ups and mechanical noises. The digital pulse processing method is proposed to improve the energy resolution of the ion pulse ionization chamber. An energy resolution of 1.6% has been achieved for the 5.49 MeV alpha-line. The dependence of the energy resolution on high voltage and working media pressure has been investigated and the results are presented., Comment: 7 pages, 7 figures, submitted to NIM A

We report on the study of thermal neutron flux using monitors based on mixture of ZnS(Ag) and LiF enriched with a lithium-6 isotope at the deep underground laboratory DULB-4900 at the Baksan Neutrino Observatory. An annual modulation of thermal neutron flux in DULB-4900 is observed. Experimental evidences were obtained of correlation between the long-term thermal neutron flux variations and the absolute humidity of the air in laboratory. The amplitude of the modulation exceed 5\% of total neutron flux., Comment: 9 pages, 9 figures, Talk at The International Workshop on Prospects of Particle Physics: "Neutrino Physics and Astrophysics" February 01 - Ferbuary 08, 2015, Valday, Russia

The results of a search for two neutrino mode of double K-capture of Xe-124 using a large copper low-background proportional counter are presented. Data collected during 3220 hours of measurements with 58.6 g of $^{124}$Xe provides us to a new limit on the half-life of Xe-124 regarding 2K-capture at the level: T_{1/2} >= 2.0*10^{21} years at a 90\% confidence level., Comment: 9 pages, 4 figures, Talk at The International Workshop on Prospects of Particle Physics: "Neutrino Physics and Astrophysics" February 01 - Ferbuary 08, 2015, Valday, Russia

The results of investigation of Xe-127 radioactive isotope production in the xenon sample enriched in Xe-124, Xe-126, Xe-128 are presented. The isotope is supposed to be the source of the background events in the low-background experiment on search for 2K-capture of Xe-124. In this work we consider two channels of Xe-127 production: the neutron knock-out from Xe-128 nucleus by cosmogenic muons and the neutron capture by Xe-126 nucleus. For the first channel the upper limit of the cross section of Xe-127 production was found to be sigma >= 0.007 barn at 95\% C.L. For the second channel the value obtained for the cross section was found to be equal to sigma =(2.74+-0.4) barn, which coincides well, within the statistical error, with reference value., Comment: Talk at The International Workshop on Prospects of Particle Physics: "Neutrino Physics and Astrophysics" Ferbuary 1 - 8, 2015, Valday,Russia, 4 pages, 5 figures, 1 tabel (to be published in PEPAN)

The brief description of installation TAU-2 intended for long-term monitoring of the half-life value $\tau$ ($\tau_{1/2}$) of the $^{214}$Po is presented. The methods of measurement and processing of collected data are reported. The results of analysis of time series values $\tau$ with different time step are presented. Total of measurement time was equal to 590 days. Averaged value of the $^{214}$Po half-life was obtained $\tau=163.46\pm0.04$ $\mu$s. The annual variation with an amplitude $A=(8.9\pm2.3)\cdot10^{-4}$, solar-daily variation with an amplitude $A_{So}=(7.5\pm1.2)\cdot10^{-4}$, lunar-daily variation with an amplitude $A_L=(6.9\pm2.0)\cdot10^{-4}$ and sidereal-daily variation with an amplitude $A_S=(7.2\pm1.2)\cdot10^{-4}$ were found in a series of $\tau$ values. The maximal values of amplitude are observed at the moments when the projections of the installation Earth location velocity vectors toward the source of possible variation achieve its maximal magnitudes., Comment: Talk at The International Workshop on Prospects of Particle Physics: "Neutrino Physics and Astrophysics" February 1 - Ferbuary 8, 2015, Valday,Russia, 7 pages, 12 figure (to be published in PEPAN)

A search for resonant absorption of the solar axion by $^{83}\rm{Kr}$ nuclei was performed using the proportional counter installed inside the low-background setup at the Baksan Neutrino Observatory. The obtained model independent upper limit on the combination of isoscalar and isovector axion-nucleon couplings $|g_3-g_0|\leq 1.69\times 10^{-6}$ allowed us to set the new upper limit on the hadronic axion mass of $m_{A}\leq 130$ eV (95\% C.L.) with the generally accepted values $S$=0.5 and $z$=0.56., Comment: 5 pages, 2 figures, Proceedings of the 10th Patras Workshop on Axions, WIMPs and WISP 29 June - 4 July 2014, CERN, Geneva, Switzerland

The experimental search for solar hadronic axions is started at the Baksan Neutrino Observatory of the Institute for Nuclear Researches Russian Academy of Science. It is assumed that axions are created in the Sun during M1-transition between the first thermally excited level at 9.4 keV and the ground state in Kr-83. The experiment is based on axion detection via resonant absorption process by the same nucleus in the detector. The big copper proportional counter filled with krypton is used to detect signals from axions. The experimental setup is situated in the deep underground low background laboratory. No evidence of axion detection were found after the 26.5 days data collection. Resulting new upper limit on axion mass is m_{A} < 130 eV at 95% C.L., Comment: Talk at the International Workshop on Prospects of Particle Physics: "Neutrino Physics and Astrophysics" Jan 26 - Ferb 2, 2014, Valday, Russia, 10 pages, 5 figures

The design changes of the Baksan low-background TAU-1 and TAU-2 set-ups allowed to improve a sensitivity of Po-214 half-life (\tau) measurements up to the 2.5 x 10^{-4} are described. Different possible sources of systematic errors influencing on the $\tau$-value are studed. An annual variation of Po-214 half-life time measurements with an amplitude of A=(6.9 \pm 3) x 10^{-4} and a phase of (\phi=93 \pm 10) days was found in a sequence of the week-collected \tau-values obtained from the TAU-2 data sample with total duration of 480 days. 24 hours' variation of the \tau-value measurements with an amplitude of A=(10.0 \pm 2.6) x 10^{-4} and phase of (\phi=1 \pm 0.5) hours was found in a solar day 1 hour step \tau-value sequence formed from the same data sample. It was found that the Po-214 half-life averaged at 480 days is equal to (163.45 \pm 0.04) mks., Comment: 17 pages, 6 figures, accepted for publication in Journal of Physics of Elementary Particles and Atomic Nuclei

First result of experiment for searching of 2K-capture of Xe-124 with the large-volume copper proportional counter is given. The 12 litre sample with 63.3% (44 g) of Xe-124 was used in measurements. The limit on the half-life of Xe-124 with regard to 2K(2\nu)-capture for the ground state of Te-124 has been found: T_{1/2} > 4.67x10^{20} y (90% C.L.). A sample with volume 52 L comprising of Xe-124 (10.6 L - 58.6 g) and Xe-126 (14.1 L - 79.3 g) will used at the next step of the experiment to increase a sensitivity of 2K-caption of Xe-124 registration. In this case sensitivity to the investigated process will be at the level of S=1.46 x 10^{21} y (90% C.L.) for 1 year measurement., Comment: Talk at the International Workshop on Prospects of Particle Physics: "Neutrino Physics and Astrophysics" Jan 26 - Ferb 2, 2014, Valday, Russia, 9 pages, 4 figure and 2 tables

The results of measurements of natural radioactive isotopes content in different source materials of natural and enriched composition used for CaMoO4 scintillation crystal growing are presented. The crystals are to be used in the experiment to search for double neutrinoless betas-decay of Mo-100., Comment: Contribution to Proc. of Int. Workshop on Radiopure Scintillators RPSCINT 2013, 17-20.09.2013, Kyiv, Ukraine; to be published in EPJ Web of Conferences; 4 pages, 2 figure and 1 tables

A concise technical characteristic of a new low-background laboratory DULB-4900 of the BNO INR RAS is presented. The technique and the results of background measurements in the Hall, ordinary box and low-background box are presented. Rn-222 contamination in the laboratory air has been measured by direct detection of gamma-radiation of its daughter Bi-214 distributed over the volume of the low-background box. The results of the data analysis are presented., Comment: 5 pages, 6 figures

A method and results of an experimental test of the time stability of the half-life of alpha-decay Po-214 nuclei are presented. Two underground installations aimed at monitoring the time stability have been constructed. Time of measurement exceeds 1038 days for one set up and 562 days for the other. It was found that amplitude of possible annual variation of Po-214 half-life does not exceed 0.2% of the mean value. The limit on the deviation of the decay curve from exponent at 0.034\times T_{1/2}

Results of a search for Kr-78 double K-capture at the second stage of the experiment with high-pressure copper proportional counters are presented. The method is based on comparison of spectra measured with natural and enriched krypton. The total exposure of the low background measurements is for Kr-78 152 g*yr and for Kr-nat 106 g*yr. An excess of events was observed in the analysis of Kr-78 selected data collected during 2008-2010 years. This excess could correspond to a double K-capture of Kr-78 with the half-life of T_{1/2}(2K,2\nu + 0\nu)=[1.4^{+2.2}_{-0.7}]\cdot 10^{22}$ yr (90% C.L.), Comment: Proceedings for the XV-th International School "Particles and Cosmology", May 26 - June 2, 2011 Troitsk, Moscow Region, Russian Federation. 4 pages, 5 figures

Search for \beta \beta -decay of Xe-136 with two high pressure proportional counters is carried out in Baksan Neutrino Observatory. The experiment is based on comparision of spectra measured with natural and enriched xenon. The measured halfe life is equal to T_{1/2}=5.5^{+4.6}_{-1.7} \cdot 10^{21} yr (67% C.L.) for \beta \beta 2\nu -decay mode. No evidence has been found for neutrinoless \beta \beta -decay. The decay half life limit based on data measured during 17280 h is T_{1/2}(\beta\beta 0\nu)\geq 4.9 \cdot 10^{23} yr (90% C.L.)., Comment: 4 pages, 8 figure, proceedings for XV-th International School "Particles and Cosmology" May 26 - June 2, 2011 Troitsk, Moscow Region, Russian Federation

Results of a search for Kr-78 double K-capture with the large low-background proportional counter (2005-2008 years) at the Baksan Neutrino Observatory are presented. An experimental method and characteristics of detectors are described. Basic features of the digitized pulses processing using wavelet transform are considered. With due account taken of the analysis of individual noise characteristic it has been shown that the appropriate choice of both wavelet characteristics and sequence of processing algorithms allows one to decrease the background in the energy region of useful events with a unique set of characteristics by ~2000 times. New limit on the half-life of Kr-78 with regard to 2K-capture has been found: T_{1/2} >= 2.4E21 yrs (90% C.L.)., Comment: 12 pages, 9 figures

A pulse shape analysis algorithm and a method for suppressing the noise component of signals from a large copper proportional counter in the experiment aimed at searching for 2K capture of Kr-78 are described. These signals correspond to a compound event with different numbers of charge clusters due to from primary ionization is formed by these signals. A technique for separating single- and multipoint events and determining the charge in individual clusters is presented. Using the Daubechies wavelets in multiresolutional signal analysis, it is possible to increase the sensitivity and the resolution in extraction of multipoint events in the detector by a factor of 3-4., Comment: 10 pages, 8 figures. submitted to Instruments and Experimental Techniques; ISSN 0020/4412

The results of the experiment searching for 2K-capture with large low-background proportional counter are presented. The comparison of spectra of the background of the proportional counter filled with Kr enriched in $^{78}$Kr (8400 hr) and with natural Kr (3039 hr) is given. A new limit on the half-life of $^{78}$Kr with regard to 2K-capture, T$_{1/2}\geq2.0\cdot10^{21}$ yrs (95% C.L.) has been obtained., Comment: 4 pages, 7 postscript figures, talk at the XIV-th Int. School "Particles and Cosmology"

The construction of an ion pulse ionization chamber aimed at measuring ultra-low levels of surface alpha-activity of different samples is described. The results of measurement carried out with alpha-source and copper samples and light-reflecting film VM2000 are presented., Comment: 6 pages, 7 postscript figures, talk at the XIV-th Int. School "Particles and Cosmology"

The experiment for the 2$\beta$-decay of $^{136}$Xe search with two high-pressure copper proportional counters has been held in Baksan neutrino observatory. The search for the process is based on comparison of spectra measured with natural and enriched xenon. No evidence has been found for 2$\beta$(2$\nu$)- and 2$\beta$(0$\nu$)-decay. The decay half lifetime limit based on data measured during 8000 h is T$_{1/2}$$\geq8.5\cdot10^{21}$yr for 2$\nu$-mode and T$_{1/2}$$\geq3.1\cdot10^{23}$yr for 0$\nu$-mode (90%C.L.)., Comment: 9 pages, 8 figures; talk at the NANP'05 Conference; submitted to Phys. At. Nucl

A technique to search for 2K-capture of $^{78}$Kr with large low-background proportional counter filled with an enriched in $^{78}$Kr up to 99.8% sample of Krypton at a pressure of 4.51 is described in this paper. The results of first measurements are presented. Analysis of data collected during 159 hours yielded new limit to the half-life of $^{78}$Kr with regard to 2K-capture (T$_{1/2}\geq6\cdot10^{21}$ yr (90% C.L.)). Sensitivity of the facility to the process for one year of measurement was evaluated to be $\texttt{S}=1.0\cdot10^{22}$ yr (90% C.L.)., Comment: 4 pages, 5 figures; talk at the NANP'05 Conference; submitted to Phys. At. Nucl

In this article the measurement results of proportional counter working characteristics filled with CF$_4$ and Xe ($0\div5$% Xe) additions at different pressures ($0.8\div14.8$ $at$) are presented. We have found that a bit of Xe addition reduces working voltage necessary to get the same gas amplification by two times against pure CF$_4$, it improves as well the resolution of the counter and increases limit gas amplification by more than ten times., Comment: 7 pages, 8 figures