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Abstract Quasi-phase matching (QPM) is a technique extensively utilized in nonlinear optics for enhancing the efficiency and stability of frequency conversion processes. However, the conventional QPM relies on periodically poled ferroelectric crystals, which are limited in availability. The 3R phase of molybdenum disulfide (3R-MoS2), a transition metal dichalcogenide (TMDc) with the broken inversion symmetry, stands out as a promising candidate for QPM, enabling efficient nonlinear process. Here, we experimentally demonstrate the QPM at nanoscale, utilizing van der Waals stacking of 3R-MoS2 layers with specific orientation to realize second harmonic generation (SHG) enhancement beyond the non QPM limit. We have also demonstrated enhanced spontaneous parametric down-conversion (SPDC) via QPM of 3R-MoS2 homo-structure, enabling more efficient generation of entangled photon pairs. The tunable capacity of 3R-MoS2 van der Waals stacking provides a platform for tuning phase-matching condition. This technique opens interesting possibilities for potential applications in nonlinear process and quantum technology.

Efficient quantum memories will be an essential building block of large-scale networked quantum systems and provide a link between flying photonic qubits and atomic or quasi-atomic local quantum processors. Memory efficiencies above 50% are required to be operating above the quantum no-cloning limit. High efficiency operation necessitates tailored photon source and memory pairs with matched bandwidths. In this paper, we explore the combination of an ultralow spectral bandwidth source of single photons from cavity-enhanced spontaneous parametric down-conversion with a hot gas-ensemble atomic memory. Our rubidium vapor gradient echo memory achieves 84% ± 3% recall efficiency of single photons: a record for single photon storage in a warm vapor platform that avoids bulky and complex systems, such as high vacuum and low temperature cryogenics.

Abstract Quantum mechanics offers the possibility of unconditionally secure communication between multiple remote parties. Security proofs for such protocols typically rely on bounding the capacity of the quantum channel in use. In a similar manner, Cramér-Rao bounds in quantum metrology place limits on how much information can be extracted from a given quantum state about some unknown parameters of interest. In this work we establish a connection between these two areas. We first demonstrate a three-party sensing protocol, where the attainable precision is dependent on how many parties work together. This protocol is then mapped to a secure access protocol, where only by working together can the parties gain access to some high security asset. Finally, we map the same task to a communication protocol where we demonstrate that a higher mutual information can be achieved when the parties work collaboratively compared to any party working in isolation.

The standard way to measure the performance of existing continuous variable quantum key distribution (CVQKD) protocols is by using the achievable secret key rate (SKR) with respect to one parameter while keeping all other parameters constant. However, this atomistic method requires many individual parameter analyses while overlooking the co-dependence of other parameters. In this work, a numerical tool is developed for comparing different CVQKD protocols while taking into account the simultaneous effects of multiple CVQKD parameters on the capability of protocols to produce positive SKRs. Using the transmittance, excess noise, and modulation amplitude parameter space, regions of positive SKR are identified to compare three discrete modulated (DM) CVQKD protocols. The results show that the M-QAM protocol outperforms the M-APSK and M-PSK protocols and that there is a non-linear increase in the capability to produce positive SKRs as the number of coherent states used for a protocol increases. The tool developed is beneficial for choosing the optimum protocol in unstable channels, such as free space, where the transmittance and excess noise fluctuate, providing a more holistic assessment of a protocol’s capability to produce positive SKRs.

Measurement estimation bounds for local quantum multiparameter estimation, which provide lower bounds on possible measurement uncertainties, have so far been formulated in two ways: by extending the classical Cramér-Rao bound (e.g., the quantum Cramér-Rao bound and the Nagaoka Cramér-Rao bound) and by incorporating the parameter estimation framework with the uncertainty principle, as in the Lu-Wang uncertainty relation. In this work, we present a general framework that allows a direct comparison between these different types of estimation limits. Specifically, we compare the attainability of the Nagaoka Cramér-Rao bound and the Lu-Wang uncertainty relation, using analytical and numerical techniques. We show that these two limits can provide different information about the physically attainable precision. We present an example where both limits provide the same attainable precision and an example where the Lu-Wang uncertainty relation is not attainable even for pure states. We further demonstrate that the unattainability in the latter case arises because the figure of merit underpinning the Lu-Wang uncertainty relation (the difference between the quantum and classical Fisher information matrices) does not necessarily agree with the conventionally used figure of merit (mean-squared error). The results offer insights into the general attainability and applicability of the Lu-Wang uncertainty relation. Furthermore, our proposed framework for comparing bounds of different types may prove useful in other settings.

Abstract It is a central fact in quantum mechanics that non-orthogonal states cannot be distinguished perfectly. In general, the optimal measurement for distinguishing such states is a collective measurement. However, to the best our knowledge, collective measurements have not been used to enhance quantum state discrimination to date. One of the main reasons for this is the fact that, in the usual state discrimination setting with equal prior probabilities, at least three copies of a quantum state are required to be measured collectively to outperform separable measurements. This is very challenging experimentally. In this work, by considering unequal prior probabilities, we propose and experimentally demonstrate a protocol for distinguishing two copies of single qubit states using collective measurements which achieves a lower probability of error than can be achieved by any non-entangling measurement. Additionally, we implemented collective measurements on three and four copies of the unknown state and found they performed poorly.

Abstract Quantum teleportation constitutes a fundamental tool for various applications in quantum communication and computation. However, state-of-the-art continuous-variable quantum teleportation is restricted to moderate fidelities and short-distance configurations. This is due to unavoidable experimental imperfections resulting in thermal decoherence during the teleportation process. Here we present a heralded quantum teleporter able to overcome these limitations through noiseless linear amplification. As a result, we report a high fidelity of 92% for teleporting coherent states using a modest level of quantum entanglement. Our teleporter in principle allows nearly complete removal of loss induced onto the input states being transmitted through imperfect quantum channels. We further demonstrate the purification of a displaced thermal state, impossible via conventional deterministic amplification or teleportation approaches. The combination of high-fidelity coherent state teleportation alongside the purification of thermalized input states permits the transmission of quantum states over significantly long distances. These results are of both practical and fundamental significance; overcoming long-standing hurdles en route to highly-efficient continuous-variable quantum teleportation, while also shining new light on applying teleportation to purify quantum systems from thermal noise.

Abstract The maximum amount of entanglement achievable under passive transformations by continuous-variable states is called the entanglement potential. Recent work has demonstrated that the entanglement potential is upper-bounded by a simple function of the squeezing of formation, and that certain classes of two-mode Gaussian states can indeed saturate this bound, though saturability in the general case remains an open problem. In this study, we introduce a larger class of states that we prove saturates the bound, and we conjecture that all two-mode Gaussian states can be passively transformed into this class, meaning that for all two-mode Gaussian states, entanglement potential is equivalent to squeezing of formation. We provide an explicit algorithm for the passive transformations and perform extensive numerical testing of our claim, which seeks to unite the resource theories of two characteristic quantum properties of continuous-variable systems.

The ability of quantum states to be in superposition is one of the key features that sets them apart from the classical world. This “coherence” is rigorously quantified by resource theories, which aim to understand how such properties may be exploited in quantum technologies. There has been much research on what the resource theory of coherence can reveal about quantum metrology, almost all of which has been from the viewpoint of Fisher information. We prove, however, that the relative entropy of coherence, and its recent generalization to positive operator-valued measures (POVMs), naturally quantify the performance of Bayesian metrology. In particular, we show how a coherence measure can be applied to an ensemble of states. We then prove that during parameter estimation, the ensemble relative entropy of coherence (C) is equal to the difference between the optimal Holevo information (X), and the mutual information attained by a measurement (I). We call this relation the CXI equality. The ensemble coherence lets us visualize how much information is locked away in superposition and hence is inaccessible with a given measurement scheme and quantifies the advantage that would be gained by using a joint measurement on multiple states. Our results hold regardless of how the parameter is encoded in the state, encompassing unitary, dissipative, and discrete settings. We consider both projective measurements and general POVMs. This work suggests new directions for research in coherence, provides a novel operation interpretation for the relative entropy of coherence and its POVM generalization, and introduces a new tool to study the role of quantum features in metrology.

Discrete-variable (DV) quantum key distribution (QKD) based on single-photon detectors and sources have been successfully deployed for long-range secure key distribution. On the other hand, continuous-variable (CV) quantum key distribution (QKD) based on coherent detectors and sources is currently lagging behind in terms of loss and noise tolerance. An important discerning factor between DV-QKD and CV-QKD is the effect of phase noise, which is known to be more relevant in CV-QKD. In this article, we investigate the effect of phase noise on DV-QKD and CV-QKD protocols, including the six-state protocol and squeezed-state protocol, in a thermal-loss channel but with the assumed availability of perfect sources and detectors. We find that in the low phase noise regime but high thermal noise regime, CV-QKD can tolerate more loss compared to DV-QKD. We also compare the secret key rate as an additional metric for the performance of QKD. Requirements for this quantity to be high vastly extend the regions at which CV-QKD performs better than DV-QKD. Our analysis addresses the questions of how phase noise affects DV-QKD and CV-QKD and why the former has historically performed better in a thermal-loss channel.

Abstract Decoherence is detrimental to quantum key distribution (QKD) over large distances. One of the proposed solutions is to use quantum repeaters, which divide the total distance between the users into smaller segments to minimise the effects of the losses in the channel. Here we introduce a measurement-device-independent protocol which uses high-dimensional states prepared by two distant trusted parties and a coherent total photon number detection for the entanglement swapping measurement at the repeater station. We present an experimentally feasible protocol that can be implemented with current technology as the required states reduce down to the single-photon level over large distances. This protocol outperforms the existing measurement-device-independent and twin-field QKD protocols by achieving better key rates in general and higher transmission distance in total when experimental imperfections are considered. It also surpasses the fundamental limit of the repeaterless bound at a much shorter transmission distance in comparison to the existing TF-QKD protocols.

Abstract Quantum correlation often refers to correlations exhibited by two or more local subsystems under a suitable measurement. These correlations are beyond the framework of classical statistics and the associated classical probability distribution. Quantum entanglement is the most well-known of such correlations and plays an important role in quantum information theory. However, there exist non-entangled states that still possess quantum correlations which cannot be described by classical statistics. One such measure that captures these non-classical correlations is discord. Here we introduce a new measure of quantum correlations which we call entropic accord that fits between entanglement and discord. It is defined as the optimised minimax mutual information of the outcome of the projective measurements between two parties. We show a strict hierarchy exists between entanglement, entropic accord and discord for two-qubit states. We study two-qubit states which shows the relationship between the three entropic quantities. In addition to revealing a class of correlations that are distinct from discord and entanglement, the entropic accord measure can be inherently more intuitive in certain contexts.

Abstract Satellite geodesy uses the measurement of the motion of one or more satellites to infer precise information about the Earth’s gravitational field. In this work, we consider the achievable precision limits on such measurements by examining approximate models for the three main noise sources in the measurement process of the current Gravitational Recovery and Climate Experiment (GRACE) Follow-On mission: laser phase noise, accelerometer noise and quantum noise. We show that, through time-delay interferometry, it is possible to remove the laser phase noise from the measurement, allowing for almost three orders of magnitude improvement in the signal-to-noise ratio. Several differential mass satellite formations are presented which can further enhance the signal-to-noise ratio through the removal of accelerometer noise. Finally, techniques from quantum optics have been studied, and found to have great promise for reducing quantum noise in other alternative mission configurations. We model the spectral noise performance using an intuitive 1D model and verify that our proposals have the potential to greatly enhance the performance of near-future satellite geodesy missions.

The amount of information that a noisy channel can transmit has been one of the primary subjects of interest in information theory. In this work we consider a practically-motivated family of optical quantum channels that can be implemented without an external energy source. We optimize the Holevo information over procedures that encode information in attenuations and phase-shifts applied by these channels on a resource state of finite energy. It is shown that for any given input state and environment temperature, the maximum Holevo information can be achieved by an encoding procedure that uniformly distributes the channel's phase-shift parameter. Moreover for large families of input states, any maximizing encoding scheme has a finite number of channel attenuation values, simplifying the codewords to a finite number of rings around the origin in the output phase space. The above results and numerical evidence suggests that this property holds for all resource states. Our results are directly applicable to the quantum reading of an optical memory in the presence of environmental thermal noise.

Quantum mechanics has withstood every experimental test thus far. However, it relies on ad-hoc postulates which require experimental verification. Over the past decade there has been a great deal of research testing these postulates, with numerous tests of Born’s rule for determining probabilities and the complex nature of the Hilbert space being carried out. Although these tests are yet to reveal any significant deviation from textbook quantum theory, it remains important to conduct such tests in different configurations and using different quantum states. Here we perform the first such test using coherent states of light in a three-arm interferometer combined with homodyne detection. Our proposed configuration requires additional assumptions, but importantly allows us to use quantum states which exist in a larger Hilbert space compared to previous tests. For testing Born’s rule, we find that the third order interference is bounded to be $\kappa = 0.002\pm0.004$ and for testing whether quantum mechanics is complex or not we find a Peres parameter of $F = 1.0000 \pm 0.0003$ ( F = 1 corresponds to the expected complex quantum mechanics). We also design and implement a test of Glauber’s theory of optical coherence.

Abstract Finding the optimal attainable precisions in quantum multiparameter metrology is a non-trivial problem. One approach to tackling this problem involves the computation of bounds which impose limits on how accurately we can estimate certain physical quantities. One such bound is the Holevo Cramér–Rao bound on the trace of the mean squared error matrix. The Holevo bound is an asymptotically achievable bound when one allows for any measurement strategy, including collective measurements on many copies of the probe. In this work, we introduce a tighter bound for estimating multiple parameters simultaneously when performing separable measurements on a finite number of copies of the probe. This makes it more relevant in terms of experimental accessibility. We show that this bound can be efficiently computed by casting it as a semidefinite programme. We illustrate our bound with several examples of collective measurements on finite copies of the probe. These results have implications for the necessary requirements to saturate the Holevo bound.

This work compares the performance of single- and two-qubit probes for estimating several phase rotations simultaneously under the action of different noisy channels. We compute the quantum limits for this simultaneous estimation using collective and individual measurements by evaluating the Holevo and Nagaoka–Hayashi Cramér-Rao bounds, respectively. Several quantum noise channels are considered, namely the decohering channel, the amplitude damping channel, and the phase damping channel. For each channel, we find the optimal single- and two-qubit probes. Where possible we demonstrate an explicit measurement strategy that saturates the appropriate bound and we investigate how closely the Holevo bound can be approached through collective measurements on multiple copies of the same probe. We find that under the action of the considered channels, two-qubit probes show enhanced parameter estimation capabilities over single-qubit probes for almost all non-identity channels, i.e., the achievable precision with a single-qubit probe degrades faster with increasing exposure to the noisy environment than that of the two-qubit probe. However, in sufficiently noisy channels, we show that it is possible for single-qubit probes to outperform maximally entangled two-qubit probes. This work shows that, in order to reach the ultimate precision limits allowed by quantum mechanics, entanglement is required in both the state preparation and state measurement stages. It is hoped the tutorial-esque nature of this paper will make it easily accessible.

Radiation pressure can be used to enable optomechanical control and manipulation of the quantum state of a mechanical oscillator. Optomechanical interaction can also be mediated by photothermal effects which, although frequently overlooked, may compete with radiation pressure interaction. Understanding of how these phenomena affect the coherent exchange of information between optical and mechanical degrees of freedom is often underdeveloped, particularly in mesoscale high-power systems where photothermal effects can fully dominate the interaction. Here we report an effective theoretical model to predict and successfully reconstruct the dynamics of a unique optomechanical system: a cavity-enhanced setup for macroscopic optical levitation, where a free-standing mirror acts as the optomechanical oscillator. We decompose the photothermal interaction into two opposing light-induced effects, photothermal expansion, and thermo-optic effects. We then reconstruct a heuristic model that links the intracavity field to four types of cavity length changes caused by acoustic ( $x_\textrm{ac}$ ), centre of mass ( $x_\textrm{lev}$ ), photothermal ( $x_\textrm{ex}$ ) and thermo-optic ( $x_\textrm{re}$ ) displacements. This offers refined predictions with a higher degree of agreement with experimental results. Our work provides a means to precisely model the photothermal effect of high power optomechanical systems, as well as for developing more precise photothermal modeling of photonics systems for precision sensing and quantum measurements.

The potential of 2D materials for space applications has been surfaced recently, however a comprehensive assessment of their suitability is currently missing. Here, the authors investigate the radiation effects in Earth’s atmosphere on various devices based on 2D transition metal dichalcogenides and hexagonal boron nitride.

Strong nonlinear interactions between single photons have important applications in optical quantum information processing. Demonstrations of these interactions in cold atomic ensembles have largely been limited to exploiting slow light generated using electromagnetically induced transparency (EIT). However, these EIT implementations have limited achievable phase shifts due to spontaneous emission. Here, we demonstrate and characterize a scheme free from these limitations using gradient echo memory with inferred single photon phase shifts of 0.07 ± 0.02 μ rad. Excellent agreement with theoretical modelling was observed. Degradation of memory efficiency was observed for large phase shifts but strategies to overcome that are presented.

Quantum theory is the foundation of modern physics. Some of its basic principles, such as Born's rule, however, are based on postulates which require experimental testing. Any deviation from Born's rule would result in higher-order interference and can thus be tested in an experiment. Here, we report on such a test with a quantum light source based on a color center in hexagonal boron nitride (hBN) coupled to a microcavity. Our room-temperature photon source features a narrow-linewidth, high-efficiency, high-purity, and on-demand single-photon generation. With the single-photon source we can increase the interferometric sensitivity of our three-path interferometer compared to conventional laser-based light sources by fully suppressing the detector nonlinearity. We thereby obtain a tight bound on the third-order interference term of 3.96(523)×10^{−4}. We also measure an interference visibility of 98.58% for our single photons emitted from hBN at room temperature, which provides a promising route for using the hBN platform as light source for phase-encoding schemes in quantum key distribution.

Cloning an unknown quantum state is challenging and the limit on the quality of clones is set by the no-cloning theorem. Here, the authors demonstrated the surpassing of such a limit using an effective quantum cloner based on a hybrid probabilistic-deterministic linear amplifier.

We analyze the precision limits for a simultaneous estimation of a pair of conjugate parameters in a displacement channel using Gaussian probes. Having a set of squeezed states as an initial resource, we compute the Holevo Cramér-Rao bound to investigate the best achievable estimation precisions if only passive linear operations are allowed to be performed on the resource prior to probing the channel. The analysis reveals the optimal measurement scheme and allows us to quantify the best precision for one parameter when the precision of the second conjugate parameter is fixed. To estimate the conjugate parameter pair with equal precision, our analysis shows that the optimal probe is obtained by combining two squeezed states with orthogonal squeezing quadratures on a 50:50 beam splitter. If different importance is attached to each parameter, then the optimal mixing ratio is no longer 50:50. Instead, it follows a simple function of the available squeezing and the relative importance between the two parameters.

A scheme is presented to perform longitudinal and transverse spatial phase coding of continuous-wave optical beams. This phase coding scheme has an information storage capacity which scales with the power of the read-out optical beam, and can be extended to implement a multiplex array detector.