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Electromagnetic waves are described by not only polarization ellipses but also cyclically rotating vectors tracing out them. The corresponding fields are respectively directionless steady line fields and directional instantaneous vector fields. Here we study the seminal topic of electromagnetic scattering from the perspective of instantaneous vector fields and uncover how the global topology of the momentum sphere regulates local distributions of tangent scattered fields. Structurally-stable generic singularities of vector fields move cyclically along lines of linear polarizations and at any instant their index sum has to be the Euler characteristic $\chi=2$. This contrasts sharply with steady line fields, of which generic singularities constrained by the Euler characteristic locate on points of circular polarizations. From such unique perspective of instantaneous singularities, we discovered that for circularly-polarized waves scattered by electromagnetic duality-symmetric particles, since linearly-polarized scatterings are prohibited by helicity conservation, there must exist at least one dark direction along which the scattering is strictly zero. Two such dark directions can be tuned to overlap, along which the scattering would remain zero for arbitrary incident polarizations. We have essentially revealed that \textit{polarizations underdescribe vectorial electromagnetic waves and the instantaneous perspective is indispensable}. The complementarity we discover provides broader and deeper insights into not only electromagnetism, but also other branches of wave physics where singularities are generic and ubiquitous., Comment: Wei Liu acknowledges many illuminating correspondences with Sir Michael Berry, whose monumental paper with J. F. Nye on phase singularities was published 50 years ago

Compared with well-developed free space polarization converters, polarization conversion between TE and TM modes in waveguide is generally considered to be caused by shape birefringence, like curvature, morphology of waveguide cross section and scattering. Here, we reveal a hidden polarization conversion mechanism in X-cut lithium niobate microrings, that is the conversion can be implemented by birefringence of waveguides, which will also introduce an unavoidable avoided-mode crossing. In the experiment, we find that this mode crossing results in severe suppression of one sideband in local nondegenerate four-wave mixing and disrupts the cascaded four-wave mixing on this side. Simultaneously, we proposed, for the first time to our best knowledge, one two-dimensional method to simulate the eigenmodes (TE and TM) in X-cut microrings, which avoids the obstacle from large computational effort in three-dimensional anisotropic microrings simulation, and the mode crossing point. This work will provide an entirely novel approach to the design of polarization converters and simulation for monolithic photonics integrated circuits, and may be helpful to the studies of missed temporal dissipative soliton formation in X-cut lithium niobate rings.

It was proved that the joint operation of electromagnetic reciprocity and $n$-fold ($n\geq3$) rotational symmetry would secure arbitrary polarization-independent backscattering efficiency [Phys. Rev. B \textbf{103}, 045422 (2021)]. Here we remove the restriction of reciprocity and study the backscatterings of plane waves by rotationally symmetric magneto-optical structures, with collinear incident wavevector, rotational axis and externally applied magnetic field. It is revealed that though nonreciprocity removes the degeneracy of backscattering efficiencies for circularly-polarized incident waves of opposite handedness, the remaining rotational symmetry is sufficient to guarantee that the efficiency is related to the polarization ellipticity only, having nothing to do with the orientations of the polarization ellipses. Moreover, the backscattering efficiency reaches its extremes (maximum or minimum values) always for circularly-polarized incident waves, and for other polarizations the efficiency is their ellipticity-weighted arithmetic average. The principles we have revealed are dictated by rotational symmetries only, which are irrelevant to specific geometric or optical parameters and are intrinsically robust against any rotational-symmetry preserving perturbations. The correlations we have discovered could be further exploited for fundamental explorations in nonreciprocal photonics and practical applications including polarimetry and ellipsometry., Comment: 6 pages and 4 figures; Comments to welcome

Frequency-dependent nonlinear process in microresonators is widely acknowledged, but there is no theory available to calculate the conversion efficiency for each resonance of the ring, except for the phase-matching one. Similarly for azimuth-dependent nonlinear process in birefringent rings, there is a lack of theory to analysis the conversion efficiency for each azimuth of the ring. Consequently, it leads to old-fashioned or ill-considered coupling position and inefficient energy conversion in birefringent microrings. Here, we introduce spatio-temporal coupled-mode equation to describe mode spatial properties in the cavity, compensating for the deficiency of temporal coupled-mode equation in describing sophisticated responses. By this equation, we find that over a wide frequency range, the extremely strong second-harmonic generation can be achieved at different azimuth under different pumps in an X-cut lithium niobate microring, which is important for realizing an efficient entangled quantum light source, for example. This work will provide new ideas and guidelines for design and applications of monolithic birefringent photonic integrated circuits with high efficiency.

Studies into scatterings of photonic structures have been so far overwhelmingly focused on their dependencies on the spatial and spectral morphologies of the incident waves. In contrast, the evolution of scattering properties through another parameter space of incident directions (momentum space) has attracted comparably little attention, though of profound importance for various scattering-related applications. Here we investigate, from the perspective of quasi-normal modes (QNMs), the momentum-space scattering extremizations with respect to varying incident directions of plane waves. It is revealed that for effective single-QNM excitations, scatterings are maximized exactly along those directions where the QNM radiation reaches its maximum, with matched incident and radiation polarizations. For an arbitrary direction, when the incident polarization is tuned to be orthogonal to that of the mode radiation, the QNM cannot be excited and thus the scatterer becomes invisible with null scatterings. The principles we have revealed are protected by fundamental laws of reciprocity and energy conservation (optical theorem), which can be further expanded and applied for other branches of wave physics., Comment: 5 pages, 3 figures, and comments to welcome

Growing uniform oxides with various thickness on TMDs is one of the biggest challenges to integrate TMDs into complementary metal oxide semiconductor (CMOS) logic circuits. Here, we report a layer-by-layer oxidation of atomically thin MoTe2 flakes via ozone (O3) exposure. The thickness of MoOx oxide film could be tuning with atomic-level accuracy simply by varying O3 exposure time. Additionally, MoOx-covered MoTe2 shows a hole-dominated transport behavior. Our findings point to a simple and effective strategy for growing homogenous surface oxide film on MoTe2, which is promising for several purposes in metal-oxide-semiconductor transistor, ranging from surface passivation to dielectric layers.

Van der Waals junctions of two-dimensional materials with an atomically sharp interface open up unprecedented opportunities to design and study functional heterostructures. Semiconducting transition metal dichalcogenides have shown tremendous potential for future applications due to their unique electronic properties and strong light-matter interaction. However, many important optoelectronic applications, such as broadband photodetection, are severely hindered by their limited spectral range and reduced light absorption. Here, we present a p-g-n heterostructure formed by sandwiching graphene with a gapless bandstructure and wide absorption spectrum in an atomically thin p-n junction to overcome these major limitations. We have successfully demonstrated a MoS2-graphene-WSe2 heterostructure for broadband photodetection in the visible to short-wavelength infrared range at room temperature that exhibits competitive device performance, including a specific detectivity of up to 1011 Jones in the near-infrared region. Our results pave the way toward the implementation of atomically thin heterostructures for broadband and sensitive optoelectronic applications., Comment: Submitted to Nano Letters; 25 pages, 4 figures, 7 supplementary figures

Two-dimensional transition metal dichalcogenides are emerging with tremendous potential in many optoelectronic applications due to their strong light-matter interactions. To fully explore their potential in photoconductive detectors, high responsivity and weak signal detection are required. Here, we present high responsivity phototransistors based on few-layer rhenium disulfide (ReS2). Depending on the back gate voltage, source drain bias and incident optical light intensity, the maximum attainable photoresponsivity can reach as high as 88,600 A W-1, which is a record value compared to other two-dimensional materials with similar device structures and two orders of magnitude higher than that of monolayer MoS2. Such high photoresponsivity is attributed to the increased light absorption as well as the gain enhancement due to the existence of trap states in the few-layer ReS2 flakes. It further enables the detection of weak signals, as successfully demonstrated with weak light sources including a lighter and limited fluorescent lighting. Our studies underscore ReS2 as a promising material for future sensitive optoelectronic applications., Comment: Accepted by Advanced Functional Materials; 25 pages, 4 figures, 2 supplementary figures

Plasmonics can be used to improve absorption in optoelectronic devices and has been intensively studied for solar cells and photodetectors. Graphene has recently emerged as a powerful plasmonic material. It shows significantly less losses compared to traditional plasmonic materials such as gold and silver and its plasmons can be tuned by changing the Fermi energy with chemical or electrical doping. Here we propose the usage of graphene plasmonics for light trapping in optoelectronic devices and show that the excitation of localized plasmons in doped, nanostructured graphene can enhance optical absorption in its surrounding media including both bulky and two-dimensional materials by tens of times, which may lead to a new generation of highly efficient, spectrally selective photodetectors in mid-infrared and THz ranges. The proposed concept could even revolutionize the field of plasmonic solar cells if graphene plasmons in the visible and near-infrared are realized., Comment: 20 pages, 6 figures

In this letter, we show that asymmetric transmission of circularly polarized waves through a nanostructured planar chiral graphene film can be observed in terahertz range. The asymmetric transmission effect of monatomic layer graphene closely resembles that of metallic planar chiral nanostructures which has previously been demonstrated. And the relative enantiomeric difference in the total transmission varies with the change of graphene's Fermi level. The plasmonic excitation in the graphene nanostructure is the enantiometically sensitive which is asymmetric for opposite propagating directions. This phenomenon will deepen our understanding of light-matter interactions in planar chiral structures and may find applications in polarization-sensitive devices, sensors, detectors and other areas., Comment: 4 pages, 4 figures