104 results on '"Rohwer, Timm"'
Search Results
2. Delamination-assisted ultrafast wrinkle formation in a freestanding film
- Author
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Su, Yifan, Zong, Alfred, Kogar, Anshul, Lu, Di, Hong, Seung Sae, Freelon, Byron, Rohwer, Timm, Hwang, Harold Y., and Gedik, Nuh
- Subjects
Condensed Matter - Materials Science ,Condensed Matter - Mesoscale and Nanoscale Physics - Abstract
The ability to synthesize and control two-dimensional (2D) crystals creates numerous opportunities for studying emergent states of matter and their novel functionalities. Freestanding films provide a particularly versatile platform for materials engineering in 2D thanks to additional structural motifs not found in films adhered to a flat substrate. A ubiquitous example is wrinkles, yet little is known about how they can develop over as fast as a few picoseconds due to a lack of experimental probes to visualize their dynamics in real time at the nanoscopic scale. Here, we use ultrafast electron diffraction to directly observe light-activated wrinkling formation in a freestanding La$_{2/3}$Ca$_{1/3}$MnO$_3$ film. Via a ``lock-in'' analysis of a single mode of oscillation in the diffraction peak position, intensity, and width, we are able to quantitatively reconstruct how wrinkles develop at the picosecond timescale. Contrary to the common assumption of a fixed boundary condition for freestanding films, we found that wrinkle development is associated with ultrafast delamination at the contact point between the film boundary and the underlying substrate, avoiding a strain build-up in the film. Not only does our work provide a generic protocol to quantify wrinkling dynamics in freestanding films, it also highlights the importance of film-substrate interaction for determining the properties of freestanding structures., Comment: 14 pages, 15 figures, including supplemental material
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- 2022
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3. Author Correction: High gradient terahertz-driven ultrafast photogun
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Ying, Jianwei, He, Xie, Su, Dace, Zheng, Lingbin, Kroh, Tobias, Rohwer, Timm, Fakhari, Moein, Kassier, Günther H., Ma, Jingui, Yuan, Peng, Matlis, Nicholas H., Kärtner, Franz X., and Zhang, Dongfang
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- 2024
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4. Ultrafast electron diffractometer with Terahertz-driven pulse compression
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Zhang, Dongfang, Kroh, Tobias, Ritzkowsky, Felix, Rohwer, Timm, Fakhari, Moein, Cankaya, Huseyin, Calendron, Anne-Laure, Matlis, Nicholas H., and Kärtner, Franz X.
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Physics - Optics - Abstract
Terahertz (THz)-based electron manipulation has recently been shown to hold tremendous promise as a technology for manipulating and driving the next-generation of compact ultrafast electron sources. Here, we demonstrate an ultrafast electron diffractometer with THz-driven pulse compression. The electron bunches from a conventional DC gun are compressed by a factor of 10 and reach a duration of ~180 fs (FWHM) with 10,000 electrons/pulse at a 1 kHz repetition rate. The resulting ultrafast electron source is used in a proof-of-principle experiment to probe the photoinduced dynamics of single-crystal silicon. The THz-compressed electron beams produce high-quality diffraction patterns and enable observation of the ultrafast structural dynamics with improved time resolution. These results validate the maturity of THz-driven ultrafast electron sources for use in precision applications., Comment: 16 pages, 5 figures. arXiv admin note: text overlap with arXiv:1910.06639
- Published
- 2021
5. High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses
- Author
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Lee, Changmin, Rohwer, Timm, Sie, Edbert J., Zong, Alfred, Baldini, Edoardo, Straquadine, Joshua, Walmsley, Philip, Gardner, Dillon, Lee, Young S., Fisher, Ian R., and Gedik, Nuh
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Condensed Matter - Materials Science ,Condensed Matter - Other Condensed Matter - Abstract
Performing time and angle resolved photoemission spectroscopy (tr-ARPES) at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite recent advances, HHG-based setups still require large pulse energies (hundreds of $\mu$J to mJ) and their energy resolution is limited to tens of meV. Here, we present a novel 11 eV tr-ARPES setup that generates a flux of $5\times10^{10}$ photons/s and achieves an unprecedented energy resolution of 16 meV. It can be operated at high repetition rates (up to 250 kHz) while using input pulse energies down to 3 $\mu$J. We demonstrate these unique capabilities by simultaneously capturing the energy and momentum resolved dynamics in two well-separated momentum space regions of a charge density wave material ErTe$_3$. This novel setup offers opportunity to study the non-equilibrium band structure of solids with exceptional energy and time resolutions at high repetition rates.
- Published
- 2019
- Full Text
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6. Light-Induced Charge Density Wave in LaTe$_3$
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Kogar, Anshul, Zong, Alfred, Dolgirev, Pavel E., Shen, Xiaozhe, Straquadine, Joshua, Bie, Ya-Qing, Wang, Xirui, Rohwer, Timm, Tung, I-Cheng, Yang, Yafang, Li, Renkai, Yang, Jie, Weathersby, Stephen, Park, Suji, Kozina, Michael E., Sie, Edbert J., Wen, Haidan, Jarillo-Herrero, Pablo, Fisher, Ian R., Wang, Xijie, and Gedik, Nuh
- Subjects
Condensed Matter - Materials Science ,Condensed Matter - Strongly Correlated Electrons - Abstract
When electrons in a solid are excited with light, they can alter the free energy landscape and access phases of matter that are beyond reach in thermal equilibrium. This accessibility becomes of vast importance in the presence of phase competition, when one state of matter is preferred over another by only a small energy scale that, in principle, is surmountable by light. Here, we study a layered compound, LaTe$_3$, where a small in-plane (a-c plane) lattice anisotropy results in a unidirectional charge density wave (CDW) along the c-axis. Using ultrafast electron diffraction, we find that after photoexcitation, the CDW along the c-axis is weakened and subsequently, a different competing CDW along the a-axis emerges. The timescales characterizing the relaxation of this new CDW and the reestablishment of the original CDW are nearly identical, which points towards a strong competition between the two orders. The new density wave represents a transient non-equilibrium phase of matter with no equilibrium counterpart, and this study thus provides a framework for unleashing similar states of matter that are "trapped" under equilibrium conditions.
- Published
- 2019
- Full Text
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7. Dynamical slowing down in an ultrafast photo-induced phase transition
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Zong, Alfred, Dolgirev, Pavel E., Kogar, Anshul, Ergeçen, Emre, Yilmaz, Mehmet B., Bie, Ya-Qing, Rohwer, Timm, Tung, I-Cheng, Straquadine, Joshua, Wang, Xirui, Yang, Yafang, Shen, Xiaozhe, Li, Renkai, Yang, Jie, Park, Suji, Hoffmann, Matthias C., Ofori-Okai, Benjamin K., Kozina, Michael E., Wen, Haidan, Wang, Xijie, Fisher, Ian R., Jarillo-Herrero, Pablo, and Gedik, Nuh
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Condensed Matter - Strongly Correlated Electrons ,Condensed Matter - Materials Science - Abstract
Complex systems, which consist of a large number of interacting constituents, often exhibit universal behavior near a phase transition. A slowdown of certain dynamical observables is one such recurring feature found in a vast array of contexts. This phenomenon, known as critical slowing down, is well studied mostly in thermodynamic phase transitions. However, it is less understood in highly nonequilibrium settings, where the time it takes to traverse the phase boundary becomes comparable to the timescale of dynamical fluctuations. Using transient optical spectroscopy and femtosecond electron diffraction, we studied a photo-induced transition of a model charge-density-wave (CDW) compound, LaTe$_3$. We observed that it takes the longest time to suppress the order parameter at the threshold photoexcitation density, where the CDW transiently vanishes. This finding can be quantitatively captured by generalizing the time-dependent Landau theory to a system far from equilibrium. The experimental observation and theoretical understanding of dynamical slowing down may offer insight into other general principles behind nonequilibrium phase transitions in many-body systems.
- Published
- 2019
- Full Text
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8. Ultrafast manipulation of mirror domain walls in a charge density wave
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Zong, Alfred, Shen, Xiaozhe, Kogar, Anshul, Ye, Linda, Marks, Carolyn, Chowdhury, Debanjan, Rohwer, Timm, Freelon, Byron, Weathersby, Stephen, Li, Renkai, Yang, Jie, Checkelsky, Joseph, Wang, Xijie, and Gedik, Nuh
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Condensed Matter - Materials Science - Abstract
Domain walls (DWs) are singularities in an ordered medium that often host exotic phenomena such as charge ordering, insulator-metal transition, or superconductivity. The ability to locally write and erase DWs is highly desirable, as it allows one to design material functionality by patterning DWs in specific configurations. We demonstrate such capability at room temperature in a charge density wave (CDW), a macroscopic condensate of electrons and phonons, in ultrathin 1T-TaS$_2$. A single femtosecond light pulse is shown to locally inject or remove mirror DWs in the CDW condensate, with probabilities tunable by pulse energy and temperature. Using time-resolved electron diffraction, we are able to simultaneously track anti-synchronized CDW amplitude oscillations from both the lattice and the condensate, where photo-injected DWs lead to a red-shifted frequency. Our demonstration of reversible DW manipulation may pave new ways for engineering correlated material systems with light.
- Published
- 2018
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9. Disentangling amplitude and phase dynamics of a charge density wave in a photo-induced phase transition
- Author
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Zong, Alfred, Kogar, Anshul, Bie, Ya-Qing, Rohwer, Timm, Lee, Changmin, Baldini, Edoardo, Ergeçen, Emre, Yilmaz, Mehmet B., Freelon, Byron, Sie, Edbert J., Zhou, Hengyun, Straquadine, Joshua, Walmsley, Philip, Dolgirev, Pavel E., Rozhkov, Alexander V., Fisher, Ian R., Jarillo-Herrero, Pablo, Fine, Boris V., and Gedik, Nuh
- Subjects
Condensed Matter - Materials Science ,Condensed Matter - Strongly Correlated Electrons - Abstract
Upon excitation with an intense ultrafast laser pulse, a symmetry-broken ground state can undergo a non-equilibrium phase transition through pathways dissimilar from those in thermal equilibrium. Determining the mechanism underlying these photo-induced phase transitions (PIPTs) has been a long-standing issue in the study of condensed matter systems. To this end, we investigate the light-induced melting of a unidirectional charge density wave (CDW) material, LaTe$_3$. Using a suite of time-resolved probes, we independently track the amplitude and phase dynamics of the CDW. We find that a quick ($\sim\,$1$\,$ps) recovery of the CDW amplitude is followed by a slower reestablishment of phase coherence. This longer timescale is dictated by the presence of topological defects: long-range order (LRO) is inhibited and is only restored when the defects annihilate. Our results provide a framework for understanding other PIPTs by identifying the generation of defects as a governing mechanism.
- Published
- 2018
- Full Text
- View/download PDF
10. Light-induced charge density wave in LaTe3
- Author
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Kogar, Anshul, Zong, Alfred, Dolgirev, Pavel E, Shen, Xiaozhe, Straquadine, Joshua, Bie, Ya-Qing, Wang, Xirui, Rohwer, Timm, Tung, I-Cheng, Yang, Yafang, Li, Renkai, Yang, Jie, Weathersby, Stephen, Park, Suji, Kozina, Michael E, Sie, Edbert J, Wen, Haidan, Jarillo-Herrero, Pablo, Fisher, Ian R, Wang, Xijie, and Gedik, Nuh
- Subjects
cond-mat.mtrl-sci ,cond-mat.str-el ,Mathematical Sciences ,Physical Sciences ,Fluids & Plasmas - Abstract
When electrons in a solid are excited with light, they can alter the freeenergy landscape and access phases of matter that are beyond reach in thermalequilibrium. This accessibility becomes of vast importance in the presence ofphase competition, when one state of matter is preferred over another by only asmall energy scale that, in principle, is surmountable by light. Here, we studya layered compound, LaTe$_3$, where a small in-plane (a-c plane) latticeanisotropy results in a unidirectional charge density wave (CDW) along thec-axis. Using ultrafast electron diffraction, we find that afterphotoexcitation, the CDW along the c-axis is weakened and subsequently, adifferent competing CDW along the a-axis emerges. The timescales characterizingthe relaxation of this new CDW and the reestablishment of the original CDW arenearly identical, which points towards a strong competition between the twoorders. The new density wave represents a transient non-equilibrium phase ofmatter with no equilibrium counterpart, and this study thus provides aframework for unleashing similar states of matter that are "trapped" underequilibrium conditions.
- Published
- 2020
11. Dynamical Slowing-Down in an Ultrafast Photoinduced Phase Transition
- Author
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Zong, Alfred, Dolgirev, Pavel E, Kogar, Anshul, Ergeçen, Emre, Yilmaz, Mehmet B, Bie, Ya-Qing, Rohwer, Timm, Tung, I-Cheng, Straquadine, Joshua, Wang, Xirui, Yang, Yafang, Shen, Xiaozhe, Li, Renkai, Yang, Jie, Park, Suji, Hoffmann, Matthias C, Ofori-Okai, Benjamin K, Kozina, Michael E, Wen, Haidan, Wang, Xijie, Fisher, Ian R, Jarillo-Herrero, Pablo, and Gedik, Nuh
- Subjects
cond-mat.str-el ,cond-mat.mtrl-sci ,Mathematical Sciences ,Physical Sciences ,Engineering ,General Physics - Abstract
Complex systems, which consist of a large number of interacting constituents, often exhibit universal behavior near a phase transition. A slowdown of certain dynamical observables is one such recurring feature found in a vast array of contexts. This phenomenon, known as critical slowing-down, is well studied mostly in thermodynamic phase transitions. However, it is less understood in highly nonequilibrium settings, where the time it takes to traverse the phase boundary becomes comparable to the timescale of dynamical fluctuations. Using transient optical spectroscopy and femtosecond electron diffraction, we studied a photoinduced transition of a model charge-density-wave (CDW) compound LaTe_{3}. We observed that it takes the longest time to suppress the order parameter at the threshold photoexcitation density, where the CDW transiently vanishes. This finding can be captured by generalizing the time-dependent Landau theory to a system far from equilibrium. The experimental observation and theoretical understanding of dynamical slowing-down may offer insight into other general principles behind nonequilibrium phase transitions in many-body systems.
- Published
- 2019
12. Evidence for topological defects in a photoinduced phase transition
- Author
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Zong, Alfred, Kogar, Anshul, Bie, Ya-Qing, Rohwer, Timm, Lee, Changmin, Baldini, Edoardo, Ergeçen, Emre, Yilmaz, Mehmet B, Freelon, Byron, Sie, Edbert J, Zhou, Hengyun, Straquadine, Joshua, Walmsley, Philip, Dolgirev, Pavel E, Rozhkov, Alexander V, Fisher, Ian R, Jarillo-Herrero, Pablo, Fine, Boris V, and Gedik, Nuh
- Subjects
cond-mat.mtrl-sci ,cond-mat.str-el ,Mathematical Sciences ,Physical Sciences ,Fluids & Plasmas - Abstract
Upon excitation with an intense ultrafast laser pulse, a symmetry-brokenground state can undergo a non-equilibrium phase transition through pathwaysdissimilar from those in thermal equilibrium. Determining the mechanismunderlying these photo-induced phase transitions (PIPTs) has been along-standing issue in the study of condensed matter systems. To this end, weinvestigate the light-induced melting of a unidirectional charge density wave(CDW) material, LaTe$_3$. Using a suite of time-resolved probes, weindependently track the amplitude and phase dynamics of the CDW. We find that aquick ($\sim\,$1$\,$ps) recovery of the CDW amplitude is followed by a slowerreestablishment of phase coherence. This longer timescale is dictated by thepresence of topological defects: long-range order (LRO) is inhibited and isonly restored when the defects annihilate. Our results provide a framework forunderstanding other PIPTs by identifying the generation of defects as agoverning mechanism.
- Published
- 2019
13. All-optical three-dimensional electron pulse compression
- Author
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Wong, Liang Jie, Freelon, Byron, Rohwer, Timm, Gedik, Nuh, and Johnson, Steven G.
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Physics - Optics ,Physics - Chemical Physics ,Physics - Instrumentation and Detectors ,78A15, 78A35, 78A60, 83A05 - Abstract
We propose an all-optical, three-dimensional electron pulse compression scheme in which Hermite-Gaussian optical modes are used to fashion a three-dimensional optical trap in the electron pulse's rest frame. We show that the correct choices of optical incidence angles are necessary for optimal compression. We obtain analytical expressions for the net impulse imparted by Hermite-Gaussian free-space modes of arbitrary order. Although we focus on electrons, our theory applies to any charged particle and any particle with non-zero polarizability in the Rayleigh regime. We verify our theory numerically using exact solutions to Maxwell's equations for first-order Hermite-Gaussian beams, demonstrating single-electron pulse compression factors of $>10^{2}$ in both longitudinal and transverse dimensions with experimentally realizable optical pulses. The proposed scheme is useful in ultrafast electron imaging for both single- and multi-electron pulse compression, and as a means of circumventing temporal distortions in magnetic lenses when focusing ultrashort electron pulses., Comment: 21 pages, 7 figures
- Published
- 2014
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14. Delamination-Assisted Ultrafast Wrinkle Formation in a Freestanding Film
- Author
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Su, Yifan, primary, Zong, Alfred, additional, Kogar, Anshul, additional, Lu, Di, additional, Hong, Seung Sae, additional, Freelon, Byron, additional, Rohwer, Timm, additional, Wang, Bai Yang, additional, Hwang, Harold Y., additional, and Gedik, Nuh, additional
- Published
- 2023
- Full Text
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15. Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution
- Author
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Sie, Edbert J., Rohwer, Timm, Lee, Changmin, and Gedik, Nuh
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- 2019
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16. Design and construction of a compact, high-repetition-rate ultrafast electron diffraction instrument
- Author
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Freelon, Byron, Rohwer, Timm, Zong, Alfred, Kogar, Anshul, Zhou, Hengyun, Wong, Liang Jie, Ergeçen, Emre, Gedik, Nuh, and School of Electrical and Electronic Engineering
- Subjects
Ultrafast Electron Diffraction ,Electrical and electronic engineering [Engineering] ,Condensed matter - Abstract
We present the design and performance of a compact ultrafast electron diffraction instrument. The diffractometer provides a means of examining time-resolved ultrafast dynamical properties of solids. The system's utilization is discussed in terms of instrument parameters and diffraction data from selected condensed matter samples. The difractometer's performance is highlighted in terms of detection sensitivity, instrumental temporal resolution, and the electron beam transverse coherence length. Following specific details of the construction, we present a practical discussion of parameters such as repetition rate and provide advice on general construction approaches for laboratory-based, keV ultrafast electron diffractometers. In addition, design guidance for constructing a compact electron gun source that is well-suited for studying diffraction from hard condensed matter is given. A unique data acquisition scheme, utilizing high laser repetition rates, is presented. Nanyang Technological University Published version This work was supported by the U.S. Department of Energy, BES DMSE (building of the experimental setup, data taking, and analysis), and the Gordon and Betty Moore Foundation’s EPiQS Initiative Grant No. GBMF9459 (instrumentation). L.J.W. was supported by the Nanyang Assistant Professorship start-up grant. T.R. received funding from the Humboldt Postdoctoral Fellowship. B.F. would like to thank the MIT Physics Department for generous support. B.F. acknowledges support from the Welch Foundation (Grant No. L-E001-19921203) and the Texas Center for Superconductivity at the University of Houston (TcSUH).
- Published
- 2023
17. Combining time-resolved optical (TOS), electronic (trARPES) and structural (UED) probes on the class of rare earth tritellurides RTe3
- Author
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Rohwer Timm, Zong Alfred, Kogar Anshul, Bie Ya-Qing, Lee Changmin, Baldini Edoardo, Ergecen Emre, Yilmaz Mehmet B., Freelon Byron, Sie Edbert J., Zhou Hengyun, Straquadine Joshua, Walmsley Philip, Dolgirev Pavel E., Rozhkov Alexander V., Fisher Ian R., Jarillo-Herrero Pablo, Fine Boris V., and Gedik Nuh
- Subjects
Physics ,QC1-999 - Abstract
The combination of EUV based time-resolved Angle-Resolved-Photo-Electron-Spectroscopy (trARPES), Ultrafast-Electron-Diffraction (UED) and Transient-Optical-Spectroscopy (TOS) facilitates a comprehensive study and all-embracing analysis of correlated dynamics, exemplified on the system of Charge-Density-Waves (CDW’s) in rare earth tritellurides (RTe3).
- Published
- 2019
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18. Parameter sensitivities in tilted-pulse-front based terahertz setups and their implications for high-energy terahertz source design and optimization
- Author
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Kroh, Tobias, primary, Rohwer, Timm, additional, Zhang, Dongfang, additional, Demirbas, Umit, additional, Cankaya, Huseyin, additional, Hemmer, Michaël, additional, Hua, Yi, additional, Zapata, Luis, additional, Pergament, Mikhail, additional, Kaertner, Franz, additional, and Matlis, Nicholas, additional
- Published
- 2022
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19. Field Enhanced, Compact S-Band Gun Employing a Pin Cathode
- Author
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Bazrafshan, Reza, Fakhari, Moein, Flöttmann, Klaus, Kaernter, Franz, Matlis, Nicholas, and Rohwer, Timm
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History ,Physics::Accelerator Physics ,MC2: Photon Sources and Electron Accelerators ,Computer Science Applications ,Education ,Accelerator Physics - Abstract
S-band RF-guns are highly developed for production of low emittance relativistic electron bunches, but need powerful klystrons for driving. Here, we present the design and first experimental tests of a compact S-band gun, which can accelerate electrons up to 180 keV powered by only 10 kW from a compact rack-mountable solid-state amplifier. A pin-cathode is used to enhance the RF electric field on the cathode up to 100 MV/m as in large-scale S-band guns. An electron bunch is generated through photoemission off a flat copper surface on the pin excited by a UV laser pulse followed by a focusing solenoid producing a low emittance bunch with 0.1 mm mrad transverse emittance for up to 100 fC bunch charge. We are currently in the conditioning phase of the gun and first experiments show good agreement with simulations. The compact gun will serve three purposes: (i) it can be used directly for ultrafast electron diffraction; (ii) as an injector into a THz booster producing 0.3MeV to 2 MeV electron bunches for ultrafast electron diffraction; (iii) The system in (ii) serves as an injector into a THz linear accelerator producing a 20 MeV beam for the AXSIS X-ray source project., Proceedings of the 13th International Particle Accelerator Conference, IPAC2022, Bangkok, Thailand
- Published
- 2022
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20. Design of a Compact 180-Degree Single-Shot Energy Spectrometer Based on a Halbach Dipole Magnet
- Author
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Bazrafshan, Reza, Fakhari, Moein, Kaernter, Franz, Matlis, Nicholas, and Rohwer, Timm
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Physics::Accelerator Physics ,MC2: Photon Sources and Electron Accelerators ,Accelerator Physics - Abstract
In the AXSIS project at DESY, we develop compact THz accelerating structures for a table-top x-ray source. Acceleration is achieved by passing the electron beam through a dielectric-loaded waveguide powered by multi-cycle THz radiation. The final electron energy strongly depends on THz-power injected into the LINAC and timing. Thus in first experiments we expect large energy fluctuations and a large range of energies to cover. We designed an electron energy spectrometer for a wide range of final energies covering 5 to 20 MeV in a single-shot. Here, we present the design of an energy spectrometer which uses a compact dipole magnet based on the Halbach array concept to deflect the electron beam through a 180° path intercepted by a Fiber Optic Scintillator (FOS) mounted inside the vacuum perpendicular to the beam. The 180-degree bending geometry provides the possibility of having the focus point of all energies at the same distance from the magnet edge which makes the design simpler and more compact. It also removes the necessity of installing a safety dipole at the end of the accelerator. A slit system at the spectrometer entrance increases resolution to better than 0.2%., Proceedings of the 13th International Particle Accelerator Conference, IPAC2022, Bangkok, Thailand
- Published
- 2022
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21. Parameter sensitivities in tilted-pulse-front based terahertz setups and their implications for high-energy terahertz source design and optimization
- Author
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Kroh, Tobias, Rohwer, Timm, Zhang, Dongfang, Demirbas, Uemit, Cankaya, Huseyin, Hemmer, Michael, Hua, Yi, Zapata, Luis, Pergament, Mikhail, Kärtner, Franz, and Matlis, Nicholas
- Subjects
Physics::Optics ,ddc:530 - Abstract
Optics express 30(14), 24186 - 24206 (2022). doi:10.1364/OE.457773, Despite the popularity and ubiquity of the tilted-pulse-front technique for single-cycle terahertz (THz) pulse generation, there is a deficit of experimental studies comprehensively mapping out the dependence of the performance on key setup parameters. The most critical parameters include the pulse-front tilt, the effective length of the pump pulse propagation within the crystal as well as effective length over which the THz beam interacts with the pump before it spatially walks off. Therefore, we investigate the impact of these parameters on the conversion efficiency and the shape of the THz beam via systematically scanning the 5D parameter space spanned by pump fluence, pulse-front-tilt, crystal-position (2D), and the pump size experimentally. We verify predictions so far only made by theory regarding the optimum interaction lengths and map out the impact of cascading on the THz radiation generation process. Furthermore, distortions imposed on the spatial THz beam profile for larger than optimum interaction lengths are observed. Finally, we identify the most sensitive parameters and, based on our findings, propose a robust optimization strategy for tilted-pulse-front THz setups. These findings are relevant for all THz strong-field applications in high demand of robust high-energy table-top single-cycle THz sources such as THz plasmonics, high-harmonic generation in solids as well as novel particle accelerators and beam manipulators., Published by Optica Publishing Group, Washington, DC
- Published
- 2022
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22. Single-Sided Pumped Compact Terahertz Driven Booster Accelerator
- Author
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Kroh, Tobias, Bazrafshan, Reza, Fakhari, Moein, Kärtner, Franz, Kawase, Keigo, Matlis, Nicholas, Pergament, Mikhail, Rohwer, Timm, Vahdani, Mostafa, and Zhang, Dongfang
- Subjects
MC3: Novel Particle Sources and Acceleration Techniques ,Physics::Accelerator Physics ,Physics::Optics ,Novel Particle Sources and Acceleration Techniques [MC3] ,Accelerator Physics - Abstract
Proceedings of the 13th International Particle Accelerator Conference, IPAC2022, Bangkok, Thailand 13th International Particle Accelerator Conference, IPAC, Bangkok, Thailand, 12 Jun 2022 - 17 Jun 2022; [Geneva] : JACoW Publishing, Geneva, Switzerland 625-627 (2022). doi:10.18429/JACoW-IPAC2022-MOPOMS003, Scaling the RF-accelerator concept to terahertz (THz) frequencies brings several compelling advantages, including compactness, intrinsic timing between the photoemission and driving field sources, and high field gradients associated with the short THz wavelength and high breakdown threshold. Recent demonstrations of such THz powered accelerators relied on two counter-propagating single-cycle THz pulses. However, to achieve high energy gains in the acceleration process high energy THz pulses are needed which in turn require complex optical setups. Here, we present on the development of a matchbox sized multi-layered accelerator designed to boost the 50 keV output of a DC electron gun to energies of ~400 keV that only requires a single THz pulse to be powered. An integrated tunable mirror inside the structure interferes the front of the driving THz pulse with its rear part such that the field in the interaction region is optimized for efficient acceleration. This reduces the complexity of the required optical setup. Such a compact booster accelerator is very promising as electron source in ultrafast electron diffraction experiments and as booster stage prior to THz based LINACs., Published by JACoW Publishing, Geneva, Switzerland, [Geneva]
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- 2022
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23. Compact Multi-Layered THz-driven Photogun
- Author
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Kroh, Tobias, Seyedfakhari, Moein, Rohwer, Timm, Zhang, Dongfang, Pergament, Mikhail, Matlis, Nicholas, and Kärtner, Franz
- Abstract
All-optical terahertz (THz) based compact accelerators promise to enable new science due to unique features such as reduced space charge broadening of the generated electron bunches and reduced timing-jitter. While prototypes of THz based devices have been demonstrated and showed exceptional capabilities to accelerate and manipulate electron beams on sub-ps timescales, development of practical THz-powered photoguns, however, has lagged due to challenges associated with the physical miniaturization and the larger THz energies required for the driving pulses. Here, we present on the progress of developing a modular all-optically driven setup that allows to power multi-layered electron photo-guns with the potential to reach several hundreds of keV. The modular concept enables convenient exchange of accelerating structures allowing rapid prototyping. As a first prototype, a 3-layered structure designed to reach 200 keV electron energy is presented. Such miniaturized electron sources are promising for seeding compact THz driven accelerators or to deliver ultrafast bunches in electron diffraction experiments.
- Published
- 2022
24. Compact-Two-Octave-Spanning Perpendicular Kicker of MeV Electrons Based on a Cubic Magnet Dipole Array
- Author
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Rohwer, Timm, Bazrafshan, Reza, Kärtner, Franz, Matlis, Nicholas, and Vagin, Pavel
- Subjects
Physics::Accelerator Physics ,Accelerator Physics ,MC6: Beam Instrumentation, Controls, Feedback and Operational Aspects - Abstract
New compact particle acceleration structures, including but not limited to plasma, THz and direct laser driven accelerators, have in common that they cover a wide energy range of potential final energies and often show a large energy spread. Moreover, they may initially have a rather large emittance. To analyze the energy range of a single shot and/or to deflect the beam to safely dump the electrons away from an end-station requires an electron kicker covering a large energy range. Here, we present a magnetic dipole structure based on a 2D Halbach array. For the current experimental test accelerator in AXSIS, an electron beam in the energy range from 4 to 20 MeV is deflected by 90 degree and energetically dispersed. In direct contrast to a simple magnetic dipole, an array of cubic magnet blocks with tailored magnetization directions allows a focusing of the beam for both longitudinal and transverse directions at 90 degree bend. A generic algorithm optimizes the magnetic field array to the predefined deflection angle and divergence. The modular array structure, in combination with the algorithm enables a simple exchange of magnets to adapt for different beam parameters., Proceedings of the 13th International Particle Accelerator Conference, IPAC2022, Bangkok, Thailand
- Published
- 2022
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25. Progress on Development of AXSIS: A Femtosecond THz-Driven MeV Accelerator and keV X-Ray Source
- Author
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Matlis, Nicholas, Bazrafshan, Reza, Fakhari, Moein, Kärtner, Franz, Kroh, Tobias, Pergament, Mikhail, Rohwer, Timm, Vahdani, Mostafa, and Zhang, Dongfang
- Subjects
MC3: Novel Particle Sources and Acceleration Techniques ,Novel Particle Sources and Acceleration Techniques [MC3] ,Accelerator Physics - Abstract
[Ebook] 13th International Particle Accelerator Conference : June 12-17, 2022, Impact Forum, Muangthong Thani, Bangkok, Thailand : conference proceedings / Chanwattana, Thakonwat , [Geneva] : JACoW Publishing, July 2022, IPAC'22 13th International Particle Accelerator Conference, IPAC'22, Bangkok, Thailand, 12 Jun 2022 - 17 Jun 2022; [Geneva] : JACoW Publishing, Geneva, Switzerland 621-624 (2022). doi:doi:10.18429/JACoW-IPAC2022-MOPOMS001, We report on the design and progress in implementing a THz-driven relativistic electron accelerator and associated X-ray source, the AXSIS Facility at DESY. We have developed a full layout of the machine based on a THz gun followed by a multi-cycle dielectric loaded metal waveguide THz linear accelerator to generate 20 MeV level, 10 fs electron bunches. The required THz pulse energies are on the mJ-level for the gun and multi-10-mJ-level for the THz linac. Customized laser technologies have been developed allowing for the generation of these pulses up to 1 kHz repetition rate. The generated electron bunches are then focused into a counter propagating optical pulse ’optical undulator’ to generate X-rays in the 6-7 keV range. We will discuss the overall layout of the machine, status of its implementation and technical challenges in the different components as well as diagnostics of this new type of accelerator and X-ray source., Published by JACoW Publishing, Geneva, Switzerland, [Geneva]
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- 2022
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26. Interaction Lengths in Tilted-pulse-front Terahertz Setups
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Kroh, Tobias, primary, Rohwer, Timm, additional, Demirbas, Umit, additional, Çankaya, Huseyin, additional, Hemmer, Michael, additional, Hua, Yi, additional, Pergament, Mikhail, additional, Matlis, Nicholas H., additional, and Kärtner, Franz X., additional
- Published
- 2022
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27. Collapse of long-range charge order tracked by time-resolved photoemission at high momenta
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Rohwer, Timm, Hellmann, Stefan, Wiesenmayer, Martin, Sohrt, Christian, Stange, Ankatrin, Slomski, Bartosz, Carr, Adra, Liu, Yanwei, Avila, Luis Miaja, Kallane, Matthias, Mathias, Stefan, Kipp, Lutz, Rossnagel, Kai, and Bauer, Michael
- Subjects
Analysis ,Usage ,Electric properties ,Condensed matter -- Electric properties -- Analysis -- Usage ,Emission spectroscopy -- Usage -- Analysis -- Electric properties - Abstract
The electronic properties of many condensed matter systems are determined by large-momentum electron states, often located near the edge of the first Brillouin zone (BZ), the unit cell of crystalline [...], Intense femtosecond ([10.sup.-15] s) light pulses can be used to transform electronic, magnetic and structural order in condensed-matter systems on timescales of electronic and atomic motion (1,2,3). This technique is particularly useful in the study (4,5) and in the control (6) of materials whose physical properties are governed by the interactions between multiple degrees of freedom. Time- and angle-resolved photoemission spectroscopy is in this context a direct and comprehensive, energy- and momentum-selective probe of the ultrafast processes that couple to the electronic degrees of freedom (7-10). Previously, the capability of such studies to access electron momentum space away from zero momentum was, however, restricted owing to limitations of the available probing photon energy (10,11). Here, using femtosecond extreme-ultraviolet pulses delivered by a high-harmonic-generation source, we use time- and angle-resolved photoemission spectroscopy to measure the photoinduced vaporization of a charge-ordered state in the potential excitonic insulator 1T-Ti[Se.sub.2] (refs 12, 13). By way of stroboscopic imaging of electronic band dispersions at large momentum, in the vicinity of the edge of the first Brillouin zone, we reveal that the collapse of atomic-scale periodic long-range order happens on a timescale as short as 20 femtoseconds. The surprisingly fast response of the system is assigned to screening by the transient generation of free charge carriers. Similar screening scenarios are likely to be relevant in other photoinduced solid-state transitions and may generally determine the response times. Moreover, as electron states with large momenta govern fundamental electronic properties in condensed matter systems (14), we anticipate that the experimental advance represented by the present study will be useful to study the ultrafast dynamics and microscopic mechanisms of electronic phenomena in a wide range of materials.
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- 2011
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28. Compact Terahertz-Powered Electron Photo-Gun
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Kroh, Tobias, Aßmann, Ralph, Çankaya, Huseyin, Demirbas, Uemit, Dinter, Hannes, Fakhari, Moein, Hemmer, Michael, Kärtner, Franz, Kellermeier, Max Joseph, Matlis, Nicholas, Pergament, Mikhail, and Rohwer, Timm
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MC3: Novel Particle Sources and Acceleration Techniques ,Physics::Optics ,Physics::Accelerator Physics ,Novel Particle Sources and Acceleration Techniques [MC3] ,Accelerator Physics - Abstract
Proceedings of the 12th International Particle Accelerator Conference, IPAC2021, Campinas, SP, Brazil 12th International Particle Accelerator Conference, IPAC 2021, Campinas, Brazil, 24 Nov 2021 - 28 Nov 2021; JACoW Publishing, Geneva, Switzerland 2983-2985 (2021). doi:doi:10.18429/JACoW-IPAC2021-WEPAB158, Novel accelerator concepts such as all-optical THz based compact accelerators promise to enable new science due to unique features such as reduced timing-jitter and improved space-charge broadening of the generated electron bunches. However, multi-keV electron photo-guns based on short single-cycle THz pulses for acceleration have not been demonstrated experimentally so far. Here, we present a modular THz-driven electron gun with both tunable interaction length and output orifice allowing optimization of the sub-mm interaction volume. First extraction of multi-keV electrons is demonstrated and the parameter space as well as resulting performance of the THz-driven gun by varying the timing of the two single-cycle THz pulses and the UV photo-excitation pulse are explored. Such compact gun prototypes are not only promising as injectors for compact THz-based LINACs but also as source for ultrafast electron diffraction experiments., Published by JACoW Publishing, Geneva, Switzerland
- Published
- 2021
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29. Ultrafast electron diffraction powered with a Terahertz-driven pulse compressor
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Zhang, Dongfang, primary, Kroh, Tobias, additional, Ritzkowsky, Felix, additional, Rohwer, Timm, additional, Fakhari, Moein, additional, Cankaya, Huseyin, additional, Calendron, Anne-Laure, additional, Matlis, Nicholas H., additional, and Kartner, Franz X., additional
- Published
- 2021
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- View/download PDF
30. Ultrafast electron diffractometer with Terahertz-driven pulse compression
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Zhang, Dongfang, primary, Kroh, Tobias, additional, Ritzkowsky, Felix, additional, Rohwer, Timm, additional, Fakhari, Moein, additional, Cankaya, Huseyin, additional, Calendron, Anne-Laure, additional, Matlis, Nicholas H., additional, and Kärtner, Franz X., additional
- Published
- 2021
- Full Text
- View/download PDF
31. THz-Enhanced DC Ultrafast Electron Diffractometer
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Zhang, Dongfang, primary, Kroh, Tobias, additional, Ritzkowsky, Felix, additional, Rohwer, Timm, additional, Fakhari, Moein, additional, Cankaya, Huseyin, additional, Calendron, Anne-Laure, additional, Matlis, Nicholas H., additional, and Kärtner, Franz X., additional
- Published
- 2021
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32. Compact THz Photogun Transversely Pumped By Twin Single-Cycle Pulses
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Kroh, Tobias, primary, Rohwer, Timm, additional, Dinter, Hannes, additional, Kellermeier, Max, additional, Fakhari, Moein, additional, Hemmer, Michael, additional, Demirbas, Umit, additional, Çankaya, Huseyin, additional, Pergament, Mikhail, additional, Aßmann, Ralph, additional, Matlis, Nicholas H., additional, and Kärtner, Franz X., additional
- Published
- 2021
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33. High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses
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Lee, Changmin, primary, Rohwer, Timm, additional, Sie, Edbert J., additional, Zong, Alfred, additional, Baldini, Edoardo, additional, Straquadine, Joshua, additional, Walmsley, Philip, additional, Gardner, Dillon, additional, Lee, Young S., additional, Fisher, Ian R., additional, and Gedik, Nuh, additional
- Published
- 2020
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34. High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses
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Massachusetts Institute of Technology. Department of Physics, Massachusetts Institute of Technology. Materials Research Laboratory, Lee, Changmin, Rohwer, Timm, Sie, Edbert Jarvis, Zhong, Alfred, Baldini, Edoardo, Gardner, Dillion R., Lee, Young S, Gedik, Nuh, Massachusetts Institute of Technology. Department of Physics, Massachusetts Institute of Technology. Materials Research Laboratory, Lee, Changmin, Rohwer, Timm, Sie, Edbert Jarvis, Zhong, Alfred, Baldini, Edoardo, Gardner, Dillion R., Lee, Young S, and Gedik, Nuh
- Abstract
Swiss National Science Foundation (Fellowships P2ELP2_172290 and P400P2_183842), United States. Department of Energy. Office of Basic Energy Sciences. Division of Materials Sciences and Engineering (Grant DE-FG02-08ER46521), United States. Army Research Office (Grant W911NF-15-1-0128), Gordon and Betty Moore Foundation (EPiQS Initiative (Grant GBMF4540)), United States. Department of Energy. Office of Basic Energy Science (Contract DE-AC02-76SF00515)
- Published
- 2020
35. Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution
- Author
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Massachusetts Institute of Technology. Department of Physics, Sie, Edbert J., Rohwer, Timm, Lee, Changmin, Gedik, Nuh, Massachusetts Institute of Technology. Department of Physics, Sie, Edbert J., Rohwer, Timm, Lee, Changmin, and Gedik, Nuh
- Abstract
Gordon and Betty Moore Foundation. Emergent Phenomena in Quantum Systems (EpiQS) initiative (Grant GBMF4540)
- Published
- 2020
36. Combining time-resolved optical (TOS), electronic (trARPES) and structural (UED) probes on the class of rare earth tritellurides RTe₃
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Massachusetts Institute of Technology. Department of Physics, MIT Materials Research Laboratory, Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science, Rohwer, Timm, Zong, Alfred, Kogar, Anshul, Bie, Yaqing, Lee, Changmin, Baldini, Edoardo, Ergecen, Emre, Yilmaz, Mehmet B, Freelon, Byron, Sie, Edbert Jarvis, Zhou, Hengyun, Jarillo-Herrero, Pablo, Gedik, Nuh, Massachusetts Institute of Technology. Department of Physics, MIT Materials Research Laboratory, Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science, Rohwer, Timm, Zong, Alfred, Kogar, Anshul, Bie, Yaqing, Lee, Changmin, Baldini, Edoardo, Ergecen, Emre, Yilmaz, Mehmet B, Freelon, Byron, Sie, Edbert Jarvis, Zhou, Hengyun, Jarillo-Herrero, Pablo, and Gedik, Nuh
- Abstract
The combination of EUV based time-resolved Angle-Resolved-Photo-Electron-Spectroscopy (trARPES), Ultrafast-Electron-Diffraction (UED) and Transient-Optical-Spectroscopy (TOS) facilitates a comprehensive study and all-embracing analysis of correlated dynamics, exemplified on the system of Charge-Density-Waves (CDW’s) in rare earth tritellurides (RTe3).
- Published
- 2020
37. Light-induced charge density wave in LaT₃
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Massachusetts Institute of Technology. Department of Physics, MIT Materials Research Laboratory, Kogar, Anshul, Zong, Alfred, Bie, Yaqing, Wang, Xirui, Rohwer, Timm, Yang, Yafang, Jarillo-Herrero, Pablo, Gedik, Nuh, Massachusetts Institute of Technology. Department of Physics, MIT Materials Research Laboratory, Kogar, Anshul, Zong, Alfred, Bie, Yaqing, Wang, Xirui, Rohwer, Timm, Yang, Yafang, Jarillo-Herrero, Pablo, and Gedik, Nuh
- Abstract
When electrons in a solid are excited by light, they can alter the free energy landscape and access phases of matter that are out of reach in thermal equilibrium. This accessibility becomes important in the presence of phase competition, when one state of matter is preferred over another by only a small energy scale that, in principle, is surmountable by the excitation. Here, we study a layered compound, LaTe3, where a small lattice anisotropy in the a–c plane results in a unidirectional charge density wave (CDW) along the c axis1,2. Using ultrafast electron diffraction, we find that, after photoexcitation, the CDW along the c axis is weakened and a different competing CDW along the a axis subsequently emerges. The timescales characterizing the relaxation of this new CDW and the reestablishment of the original CDW are nearly identical, which points towards a strong competition between the two orders. The new density wave represents a transient non-equilibrium phase of matter with no equilibrium counterpart, and this study thus provides a framework for discovering similar states of matter that are ‘trapped’ under equilibrium conditions., United States. Department of Energy. Office of Basic Energy Science. Division Accelerator & Detector R&D program (Contracts DE-AC02-05-CH11231 and DE-AC02-76SF00515 (MeV UED at SLAC), United States. Department of Energy. Office of Basic Energy Science (Contract DE-AC02-76SF00515), United States. Department of Energy. Office of Basic Energy Science (Award DE-SC0001088), Gordon and Betty Moore Foundation EPiQS Initiative (Grant GBMF4541 (sample preparation and characterization))
- Published
- 2020
38. Commissioning-Stages and Radio-Protection Concept for the THz-Linac Based Accelerator 'AXSIS' at DESY
- Author
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Burkart, Florian, Aßmann, Ralph, Dorda, Ulrich, Kärtner, Franz, Marchetti, Barbara, Matlis, Nicholas, and Rohwer, Timm
- Subjects
MC3: Novel Particle Sources and Acceleration Techniques ,Accelerator Physics - Abstract
The dedicated accelerator R facility SINBAD at DESY hosts the AXSIS accelerator. This project is funded by the European Research Council to develop a compact source for attosecond serial X-ray crystallography and spectroscopy. For that purpose, in one of the arcs of the SINBAD facility and the neighboring laser labs, an accelerator research site is being constructed where a fully THz-driven accelerator (electron gun and linac, 30MeV) will be installed. The current status of the hardware installation of the electron beam accelerator is presented. Furthermore, the required radio-protection measures and maximum beam parameters are presented. In this contribution the commissioning plans and the staging of the beam operation for the accelerator complex will be shown and discussed in detail., Proceedings of the 10th Int. Particle Accelerator Conf., IPAC2019, Melbourne, Australia
- Published
- 2019
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39. Robust optimization of single-cycle THz setups based on phase-matching via tilted pulse fronts using an incident-fluence metric
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Kroh, Tobias, primary, Rohwer, Timm, additional, Wang, Lu, additional, Demirbas, Umit, additional, Cankaya, Huseyin, additional, Pergament, Mikhail, additional, Kärtner, Franz, additional, and Matlis, Nicholas, additional
- Published
- 2020
- Full Text
- View/download PDF
40. Light-induced charge density wave in LaTe3
- Author
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Kogar, Anshul, primary, Zong, Alfred, additional, Dolgirev, Pavel E., additional, Shen, Xiaozhe, additional, Straquadine, Joshua, additional, Bie, Ya-Qing, additional, Wang, Xirui, additional, Rohwer, Timm, additional, Tung, I-Cheng, additional, Yang, Yafang, additional, Li, Renkai, additional, Yang, Jie, additional, Weathersby, Stephen, additional, Park, Suji, additional, Kozina, Michael E., additional, Sie, Edbert J., additional, Wen, Haidan, additional, Jarillo-Herrero, Pablo, additional, Fisher, Ian R., additional, Wang, Xijie, additional, and Gedik, Nuh, additional
- Published
- 2019
- Full Text
- View/download PDF
41. Ultrafast manipulation of mirror domain walls in a charge density wave
- Author
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Massachusetts Institute of Technology. Department of Physics, Zong, Guo, Kogar, Anshul, Ye, Linda, Chowdhury, Debanjan, Rohwer, Timm, Freelon, Byron, Checkelsky, Joseph, Gedik, Nuh, Shen, Xiaozhe, Marks, Carolyn, Weathersby, Stephen, Li, Renkai, Yang, Jie, Wang, Xijie, Massachusetts Institute of Technology. Department of Physics, Zong, Guo, Kogar, Anshul, Ye, Linda, Chowdhury, Debanjan, Rohwer, Timm, Freelon, Byron, Checkelsky, Joseph, Gedik, Nuh, Shen, Xiaozhe, Marks, Carolyn, Weathersby, Stephen, Li, Renkai, Yang, Jie, and Wang, Xijie
- Abstract
Domain walls (DWs) are singularities in an ordered medium that often host exotic phenomena such as charge ordering, insulator-metal transition, or superconductivity. The ability to locally write and erase DWs is highly desirable, as it allows one to design material functionality by patterning DWs in specific configurations. We demonstrate such capability at room temperature in a charge density wave (CDW), a macroscopic condensate of electrons and phonons, in ultrathin 1T-TaS₂. A single femtosecond light pulse is shown to locally inject or remove mirror DWs in the CDW condensate, with probabilities tunable by pulse energy and temperature. Using time-resolved electron diffraction, we are able to simultaneously track anti-synchronized CDW amplitude oscillations from both the lattice and the condensate, where photoinjected DWs lead to a red-shifted frequency. Our demonstration of reversible DW manipulation may pave new ways for engineering correlated material systems with light.
- Published
- 2019
42. Evidence for topological defects in a photoinduced phase transition
- Author
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Zong, Alfred, primary, Kogar, Anshul, additional, Bie, Ya-Qing, additional, Rohwer, Timm, additional, Lee, Changmin, additional, Baldini, Edoardo, additional, Ergeçen, Emre, additional, Yilmaz, Mehmet B., additional, Freelon, Byron, additional, Sie, Edbert J., additional, Zhou, Hengyun, additional, Straquadine, Joshua, additional, Walmsley, Philip, additional, Dolgirev, Pavel E., additional, Rozhkov, Alexander V., additional, Fisher, Ian R., additional, Jarillo-Herrero, Pablo, additional, Fine, Boris V., additional, and Gedik, Nuh, additional
- Published
- 2018
- Full Text
- View/download PDF
43. Ultrafast manipulation of mirror domain walls in a charge density wave
- Author
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Zong, Alfred, primary, Shen, Xiaozhe, additional, Kogar, Anshul, additional, Ye, Linda, additional, Marks, Carolyn, additional, Chowdhury, Debanjan, additional, Rohwer, Timm, additional, Freelon, Byron, additional, Weathersby, Stephen, additional, Li, Renkai, additional, Yang, Jie, additional, Checkelsky, Joseph, additional, Wang, Xijie, additional, and Gedik, Nuh, additional
- Published
- 2018
- Full Text
- View/download PDF
44. Self-amplified photo-induced gap quenching in a correlated electron material
- Author
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Massachusetts Institute of Technology. Department of Physics, Francis Bitter Magnet Laboratory (Massachusetts Institute of Technology), Rohwer, Timm, Mathias, S., Eich, S., Urbancic, J., Michael, S., Carr, A. V., Emmerich, S., Stange, A., Popmintchev, T., Wiesenmayer, M., Ruffing, A., Jakobs, S., Hellmann, S., Matyba, P., Chen, C., Kipp, L., Bauer, M., Kapteyn, H. C., Schneider, H. C., Rossnagel, K., Murnane, M. M., Aeschlimann, M., Massachusetts Institute of Technology. Department of Physics, Francis Bitter Magnet Laboratory (Massachusetts Institute of Technology), Rohwer, Timm, Mathias, S., Eich, S., Urbancic, J., Michael, S., Carr, A. V., Emmerich, S., Stange, A., Popmintchev, T., Wiesenmayer, M., Ruffing, A., Jakobs, S., Hellmann, S., Matyba, P., Chen, C., Kipp, L., Bauer, M., Kapteyn, H. C., Schneider, H. C., Rossnagel, K., Murnane, M. M., and Aeschlimann, M.
- Abstract
Capturing the dynamic electronic band structure of a correlated material presents a powerful capability for uncovering the complex couplings between the electronic and structural degrees of freedom. When combined with ultrafast laser excitation, new phases of matter can result, since far-from-equilibrium excited states are instantaneously populated. Here, we elucidate a general relation between ultrafast non-equilibrium electron dynamics and the size of the characteristic energy gap in a correlated electron material. We show that carrier multiplication via impact ionization can be one of the most important processes in a gapped material, and that the speed of carrier multiplication critically depends on the size of the energy gap. In the case of the charge-density wave material 1T-TiSe[subscript 2], our data indicate that carrier multiplication and gap dynamics mutually amplify each other, which explains—on a microscopic level—the extremely fast response of this material to ultrafast optical excitation.
- Published
- 2017
45. Combining time-resolved optical (TOS), electronic (trARPES) and structural (UED) probes on the class of rare earth tritellurides RTe3.
- Author
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Rohwer, Timm, Zong, Alfred, Kogar, Anshul, Bie, Ya-Qing, Lee, Changmin, Baldini, Edoardo, Ergecen, Emre, Yilmaz, Mehmet B., Freelon, Byron, Sie, Edbert J., Zhou, Hengyun, Straquadine, Joshua, Walmsley, Philip, Dolgirev, Pavel E., Rozhkov, Alexander V., Fisher, Ian R., Jarillo-Herrero, Pablo, Fine, Boris V., Gedik, Nuh, and Cerullo, G.
- Subjects
TELLURIDES ,PHOTOELECTRON spectroscopy ,CHARGE density waves ,ELECTRON diffraction ,MATHEMATICAL combinations - Abstract
The combination of EUV based time-resolved Angle-Resolved-Photo-Electron-Spectroscopy (trARPES), Ultrafast-Electron-Diffraction (UED) and Transient-Optical-Spectroscopy (TOS) facilitates a comprehensive study and all-embracing analysis of correlated dynamics, exemplified on the system of Charge-Density-Waves (CDW's) in rare earth tritellurides (RTe3). [ABSTRACT FROM AUTHOR]
- Published
- 2019
- Full Text
- View/download PDF
46. All-optical three-dimensional electron pulse compression
- Author
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Massachusetts Institute of Technology. Department of Mathematics, Massachusetts Institute of Technology. Department of Physics, Wong, Liang Jie, Freelon, Byron, Rohwer, Timm, Gedik, Nuh, Johnson, Steven G., Massachusetts Institute of Technology. Department of Mathematics, Massachusetts Institute of Technology. Department of Physics, Wong, Liang Jie, Freelon, Byron, Rohwer, Timm, Gedik, Nuh, and Johnson, Steven G.
- Abstract
We propose an all-optical, three-dimensional electron pulse compression scheme in which Hermite–Gaussian optical modes are used to fashion a three-dimensional optical trap in the electron pulse's rest frame. We show that the correct choices of optical incidence angles are necessary for optimal compression. We obtain analytical expressions for the net impulse imparted by Hermite–Gaussian free-space modes of arbitrary order. Although we focus on electrons, our theory applies to any charged particle and any particle with non-zero polarizability in the Rayleigh regime. We verify our theory numerically using exact solutions to Maxwell's equations for first-order Hermite–Gaussian beams, demonstrating single-electron pulse compression factors of >10[superscript 2] in both longitudinal and transverse dimensions with experimentally realizable optical pulses. The proposed scheme is useful in ultrafast electron imaging for both single- and multi-electron pulse compression, and as a means of circumventing temporal distortions in magnetic lenses when focusing ultrashort electron pulses. Other applications include the creation of flat electron beams and ultrashort electron bunches for coherent terahertz emission., United States. Army Research Office (Contract No. W911NF-13-D-0001), United States. Defense Advanced Research Projects Agency (DARPA Young Faculty Award, Grant No. D13AP00050), Alexander von Humboldt-Stiftung, Singapore. Agency for Science, Technology and Research
- Published
- 2015
47. All-optical three-dimensional electron pulse compression
- Author
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Wong, Liang Jie, primary, Freelon, Byron, additional, Rohwer, Timm, additional, Gedik, Nuh, additional, and Johnson, Steven G, additional
- Published
- 2015
- Full Text
- View/download PDF
48. Temporal Lenses for Three-Dimensional Electron Pulse Compression
- Author
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Wong, Liang Jie, primary, Freelon, Byron, additional, Rohwer, Timm, additional, Gedik, Nuh, additional, and Johnson, Steven G., additional
- Published
- 2015
- Full Text
- View/download PDF
49. Probing the switching state of a surface-mounted azobenzene derivative using femtosecond XUV photoemission
- Author
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Grunau, Jan, primary, Heinemann, Nils, additional, Rohwer, Timm, additional, Zargarani, Dordaneh, additional, Kuhn, Sonja, additional, Jung, Ullrich, additional, Kipp, Lutz, additional, Magnussen, Olaf, additional, Herges, Rainer, additional, and Bauer, Michael, additional
- Published
- 2012
- Full Text
- View/download PDF
50. CDW-superlattice suppression probed in time-resolved XUV-photoemission at the border of the Brillouin zone
- Author
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Rohwer, Timm, primary, Hellmann, Stefan, additional, Wiesenmayer, Martin, additional, Sohrt, Christian, additional, Stange, Ankatrin, additional, Slomski, Bartosz, additional, Kipp, Lutz, additional, Rossnagel, Kai, additional, and Bauer, Michael, additional
- Published
- 2010
- Full Text
- View/download PDF
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