Search

The transition matrix, frequently abbreviated as T-matrix, contains the complete information in a linear approximation of how a spatially localized object scatters an incident field. The T-matrix is used to study the scattering response of an isolated object and describes the optical response of complex photonic materials made from ensembles of individual objects. T-matrices of certain common structures, potentially, have been repeatedly calculated all over the world again and again. This is not necessary and constitutes a major challenge for various reasons. First, the resources spent on their computation represent an unsustainable financial and ecological burden. Second, with the onset of machine learning, data is the gold of our era, and it should be freely available to everybody to address novel scientific challenges. Finally, the possibility of reproducing simulations could tremendously improve if the considered T-matrices could be shared. To address these challenges, we found it important to agree on a common data format for T-matrices and to enable their collection from different sources and distribution. This document aims to develop the specifications for storing T-matrices and associated metadata. The specifications should allow maximum freedom to accommodate as many use cases as possible without introducing any ambiguity in the stored data. The common format will assist in setting up a public database of T-matrices., Comment: Submitted to the Journal of Quantitative Spectroscopy and Radiative Transfer

Wavefront shaping techniques allow waves to be focused on a diffraction-limited target deep inside disordered media. To identify the target position, a guidestar is required that typically emits a frequency-shifted signal. Here we present a noninvasive matrix approach operating at a single frequency only, based on the variation of the field scattered by a nonlinear target illuminated at two incident powers. The local perturbation induced by the nonlinearity serves as a guide for identifying optimal incident wavefronts. We demonstrate maximal focusing on electronic devices embedded in chaotic microwave cavities and extend our approach to temporal signals. Finally, we exploit the programmability offered by reconfigurable smart surfaces to enhance the intensity delivered to a nonlinear target. Our results pave the way for deep imaging protocols that use any type of nonlinearity as feedback, requiring only the measurement of a monochromatic scattering matrix.

A Coherent Perfect Absorber (CPA) exploits the interferometric nature of light to deposit all of a light field's incident energy into an otherwise weakly absorbing sample. The downside of this concept is that the necessary destructive interference in CPAs gets easily destroyed both by spectrally or spatially detuning the incoming light field. Each of these two limitations has recently been overcome by insights from exceptional-point physics and by using a degenerate cavity, respectively. Here, we show how these two concepts can be combined into a new type of cavity design, which allows broadband exceptional-point absorption of arbitrary wavefronts. We present two possible implementations of such a Massively Degenerate Exceptional-Point absorber and compare analytical results with numerical simulations., Comment: 6 pages, 4 figures, with Supplementary Materials (29 pages)

The physics of waves in time-varying media provides numerous opportunities for wave control that are unattainable with static media. In particular, Floquet systems with a periodic time modulation are currently of considerable interest. Here, we demonstrate how the scattering properties of a finite Floquet medium can be correctly described by a static Floquet scattering matrix, which satisfies a pseudo-unitary relation. This algebraic property is a consequence of the conservation of wave action for which we formulate here a continuity equation. Using this Floquet scattering matrix, we further demonstrate how it can be used to generalize also the seminal Wigner-Smith operator from static to Floquet systems. The eigenstates of the corresponding Floquet Wigner-Smith matrix are shown to be light pulses that are optimally shaped both in their spatial and temporal degrees of freedom for the optical micromanipulation of time-varying media.

The interaction of quantum light with matter is of great importance to a wide range of scientific disciplines, ranging from optomechanics to high precision measurements. A central issue we discuss here, is how to make optimal use of both the spatial and the quantum degrees of freedom of light for characterizing and manipulating arbitrary observable parameters in a linear scattering system into which suitably engineered light fields are injected. Here, we discuss a comprehensive framework based on a quantum operator that can be assembled solely from the scattering matrix of a system and its dependence on the corresponding local parameter, making this operator experimentally measurable from the far-field using only classical light. From this, the effect of quantum light in the near-field, i.e., in the vicinity of the target object, can be inferred. Based on this framework, it is straightforward to formulate optimal protocols on how to jointly design both the spatial shape and the quantum characteristics of light for micromanipulation as well as for parameter estimation in arbitrarily complex media. Also the forces of the quantum vacuum naturally emerge from this formalism. The aim of our tutorial is to bring different perspectives into alignment and thereby build a bridge between the different communities of wave control, quantum optics, micromanipulation, quantum metrology and vacuum physics., Comment: Tutorial article, 29 pages

The control of thermal radiation by shaping its spatial and spectral emission characteristics plays a key role in many areas of science and engineering. Conventional approaches to tailor thermal emission using metamaterials are severely hampered both by the limited spatial resolution of the required sub-wavelength material structures and by the materials' strong absorption in the infrared. Here, we demonstrate a promising new approach based on the concept of topology. By changing a single parameter of a multilayer coating, we control the reflection topology of a surface, with the critical point of zero reflection being topologically protected. As a result, the boundaries between sub-critical and super-critical spatial domains host topological interface states with near-unity thermal emissivity. Our experimental demonstration of this effect shows that topological concepts enable unconventional manipulation of thermal light with promising applications for thermal management, energy harvesting and thermal camouflage., Comment: 10 pages, 4 figures

Speckle patterns are inherent features of coherent light propagation through complex media. As a result of interference, they are sensitive to multiple experimental parameters such as the configuration of disorder or the propagating wavelength. Recently, developments in wavefront shaping have enabled to control speckle pattern statistics and correlations, for example using the concept of the transmission matrix. In this article, we address the problem of correlating scattered fields across multiple degrees of freedom. We highlight the common points between the specific techniques already demonstrated and propose a general framework based on the singular value decomposition of a linear combination of multiple transmission matrices. Following analytical predictions, we experimentally illustrate the technique on spectral and temporal correlations and show that both the amplitude and the phase of the field correlations can be tuned. Our works open new perspectives in speckle correlation manipulation, with potential applications in coherent control and proposing a generalization of the concept speckle memory effect.

Light and sound waves have the fascinating property that they can move objects through the transfer of linear or angular momentum. This ability has led to the development of optical and acoustic tweezers, with applications ranging from biomedical engineering to quantum optics. Although impressive manipulation results have been achieved, the stringent requirement for a highly controlled, low-reverberant, and static environment still hinders the applicability of these techniques in many scenarios. Here, we overcome this challenge and demonstrate the manipulation of objects in disordered and dynamic media, by optimally tailoring the momentum of sound waves iteratively in the far field. The method does not require information about the object's physical properties or the spatial structure of the surrounding medium but relies only on a real-time scattering matrix measurement and a positional guidestar. Our experiment demonstrates the possibility of optimally moving and rotating objects, extending the reach of wave-based object manipulation to complex and dynamic scattering media. We envision new opportunities for biomedical applications, sensing, or manufacturing.

The strong coupling of quantum emitters to a cavity mode has been of paramount importance in the development of quantum optics. Recently, also the strong coupling to more than a single mode of an electromagnetic resonator has drawn considerable interest. We investigate how this multimode strong coupling regime can be harnessed to coherently control quantum systems. Specifically, we demonstrate that a Maxwell-Fish-Eye lens can be used to implement a pulsed excitation-exchange between two distant quantum emitters. This periodic exchange is mediated by single-photon pulses and can be extended to a photon-exchange between two atomic ensembles, for which the coupling strength is enhanced collectively., Comment: 8 pages, 7 figures. Accepted for publication in Physical Review Letters

Using waves to explore our environment is a widely used paradigm, ranging from seismology to radar technology, and from bio-medical imaging to precision measurements. In all of these fields, the central aim is to gather as much information as possible about an object of interest by sending a probing wave at it and processing the information delivered back to the detector. Here, we demonstrate that an electromagnetic wave scattered at an object carries locally defined and conserved information about all of the object's constitutive parameters. Specifically, we introduce here the density and flux of Fisher information for very general types of wave fields and identify corresponding sources and sinks of information through which all these new quantities satisfy a fundamental continuity equation. We experimentally verify our theoretical predictions by studying a movable object embedded inside a disordered environment and by measuring the corresponding Fisher information flux at microwave frequencies. Our results provide a new understanding of the generation and propagation of information and open up new possibilities for tracking and designing the flow of information even in complex environments., Comment: 17 pages, 4 figures, plus a methods section and supplementary material

We present a graph-based model for multiple scattering of light in integrated lithium niobate on insulator (LNOI) networks, which describes an open network of single-mode integrated waveguides with tunable scattering at the network nodes. We first validate the model at small scale with experimental LNOI resonator devices and show consistent agreement between simulated and measured spectral data. Then, the model is used to demonstrate a novel platform for on-chip multiple scattering in large-scale optical networks up to few hundred nodes, with tunable scattering behaviour and tailored disorder. Combining our simple graph-based model with material properties of LNOI, this platform creates new opportunities to control randomness in large optical networks.

Light transport in a highly multimode fiber exhibits complex behavior in space, time, frequency and polarization, especially in the presence of mode coupling. The newly developed techniques of spatial wavefront shaping turn out to be highly suitable to harness such enormous complexity: a spatial light modulator enables precise characterization of field propagation through a multimode fiber, and by adjusting the incident wavefront it can accurately tailor the transmitted spatial pattern, temporal profile and polarization state. This unprecedented control leads to multimode fiber applications in imaging, endoscopy, optical trapping and microfabrication. Furthermore, the output speckle pattern from a multimode fiber encodes spatial, temporal, spectral and polarization properties of the input light, allowing such information to be retrieved from spatial measurements only. This article provides an overview of recent advances and breakthroughs in controlling light propagation in multimode fibers, and discusses newly emerging applications., Comment: 81 pages, 39 figures; invited review article for Advances in Optics and Photonics; feedback by the community is very welcome

Moving objects with optical or acoustical waves is a topic both of fundamental interest and of importance for a range of practical applications. One particularly intriguing example is the tractor beam, which pulls an object toward the wave's source, in opposition to the wave's momentum. In this study, we introduce a protocol that enables the identification of wave states that produce the optimal tractor force for arbitrary objects. Our method relies solely on the solution of a simple eigenvalue problem involving the system's measurable scattering matrix. Using numerical simulations, we demonstrate the efficacy of this wavefront shaping protocol for a representative set of different targets. Moreover, we show that the diffractive nature of waves enables the possibility of a tractor beam, that works even for targets where a geometric optics approach fails to explain the pulling forces.

Optical tweezers enable non-contact trapping of micro-scale objects using light. Despite their widespread use, it is currently not known how tightly it is possible to three-dimensionally trap micro-particles with a given photon budget. Reaching this elusive limit would enable maximally-stiff particle trapping for precision measurements on the nanoscale, and photon-efficient tweezing of light-sensitive objects. Here we solve this problem by customising a trapping light field to suit a specific particle, with the aim of simultaneously optimising trap stiffness in all three dimensions. Initially taking a theoretical approach, we develop an efficient multi-parameter optimisation routine to design bespoke optical traps for a wide range of micro-particles. We show that the confinement volume of micro-spheres held in these sculpted traps can be reduced by one-to-two orders-of-magnitude in comparison to a conventional optical tweezer of the same power. We go on to conduct proof-of-principle experiments, and use a wavefront shaping inspired strategy to suppress the Brownian fluctuations of optically trapped micro-spheres in every direction concurrently, thus demonstrating order-of-magnitude reductions in their confinement volumes. Our work paves the way towards the fundamental limits of optical control over the mesoscopic realm.

We study the superradiant emission of an inverted spin ensemble strongly coupled to a superconducting cavity. After fast inversion, we detune the spins from the cavity and store the inversion for tens of milliseconds, during which the remaining transverse spin components disappear. Switching back on resonance enables us to study the onset of superradiance. A weak trigger pulse of a few hundred photons shifts the superradiant burst to earlier times and imprints its phase onto the emitted radiation. For long hold times, the inversion decreases below the threshold for spontaneous superradiance. There, the energy stored in the ensemble can be used to amplify microwave pulses passing through the cavity.

The opportunity to manipulate small-scale objects pushes us to the limits of our understanding of physics. Particularly promising in this regard is the interdisciplinary field of levitation, in which light fields can be harnessed to isolate nano-particles from their environment by levitating them optically. When cooled down towards their motional quantum ground state, levitated systems offer the tantalizing prospect of displaying mesoscopic quantum properties. Currently restricted to single objects with simple shapes, the interest in levitation is currently moving towards the manipulation of more complex structures, such as those featuring multiple particles or different degrees of freedom. Unfortunately, current cooling techniques are mostly designed for single objects and thus cannot easily be multiplexed to address such coupled many-body systems. Here, we present an approach based on the spatial modulation of light in the far-field to cool down multiple nano-objects in parallel. Our procedure is based on the experimentally measurable scattering matrix and on its changes with time. We demonstrate how to compose from these ingredients a linear energy-shift operator, whose eigenstates are identified as the incoming wavefronts that implement the most efficient cooling of complex moving ensembles of levitated particles. Submitted in parallel with arxiv:2103.12592, this article provides a theoretical and numerical study of the expected cooling performance as well as of the robustness of the method against environmental parameters., Comment: Posted in parallel with arXiv:2103.12592, this preprint provides extended simulations and theoretical considerations on our far-field cooling scheme

The adiabatic theorem, a corollary of the Schr\"odinger equation, manifests itself in a profoundly different way in non-Hermitian arrangements, resulting in counterintuitive state transfer schemes that have no counterpart in closed quantum systems. In particular, the dynamical encirclement of exceptional points (EPs) in parameter space has been shown to lead to a chiral phase accumulation, non-adiabatic jumps, and topological mode conversion [1- 8]. Recent theoretical studies, however, have shown that contrary to previously established demonstrations, this behavior is not strictly a result of winding around a non-Hermitian degeneracy [9]. Instead, it appears to be mostly attributed to the non-trivial landscape of the Riemann surfaces, sometimes because of the presence of an exceptional point in the vicinity [9- 11]. In an effort to bring this counterintuitive aspect of non-Hermitian systems into light and confirm this hypothesis, we provide here the first set of experiments to directly observe the field evolution and chiral state conversion in an EP-excluding cycle in a slowly varying non- Hermitian system. To do so, a versatile yet unique fiber-based photonic emulator is realized that utilizes the polarization degrees of freedom in a quasi-common path single-ring arrangement. Our observations may open up new avenues for light manipulation and state conversion, while providing a foundation for understanding the intricacies of the adiabatic theorem in non-Hermitian systems.

One of the key insights in the emerging field of non-Hermitian photonics is that well-established concepts like the laser can be operated in reverse to realize a 'coherent perfect absorber' (CPA). While conceptually appealing, such CPAs are limited so far to a single, judiciously shaped wavefront or 'mode'. Here, we demonstrate how this limitation can be overcome by time-reversing a 'degenerate cavity laser', based on a unique cavity that self-images any incident light-field onto itself. Placing a weak, critically-coupled absorber into this cavity, we demonstrate that any incoming wavefront, even a complex and dynamically-varying speckle pattern, is absorbed with close to perfect efficiency in a massively parallel interference process. Moreover, the coherent nature of multi-mode absorption allows us to tune the degree of absorption over a wide range. These characteristics open-up interesting new possibilities for applications in light-harvesting, energy delivery, light control, and imaging., Comment: Updated version with color figures now being displayed correctly on different PDF readers

Getting to grips with the detrimental influence of disordered environments on wave propagation is an interdisciplinary endeavour spanning diverse research areas ranging from telecommunications \cite{basar_wireless_2019} and bio-medical imaging \cite{kubby_wavefront_2019} to seismology \cite{Campillo2003} and material engineering \cite{Chen2010,Molesky2018}. Wavefront shaping techniques are highly promising to overcome the effect of wave scattering as even opaque media feature open channels for which the incident light is fully transmitted \cite{Dorokhov1984,Gerardin2014,Sarma2016,Jeong18}. With this feature being restricted, however, to just a small subset of judiciously engineered states it remains out of reach to render an opaque sample translucent for any incident light field. Here we show that a structureless medium composed of randomly assembled scattering elements can be made fully transmitting to all incoming wavefronts by putting a customized complementary medium in front of it. This special situation is achieved when the reflection matrices of the two media surfaces facing each other satisfy a matrix generalization of the condition for critical coupling. We implement this protocol both numerically and experimentally for the design of electromagnetic waveguides with several dozen scattering elements placed inside of them. The translucent scattering media we introduce here also have the promising property of being able to store incident radiation in their interior for remarkably long times.

The complex temporal behavior of an ultrashort pulse of light propagating through a multiply scattering medium can be characterized experimentally through a time-gated transmission matrix. Using a spatial light modulator, we demonstrate here, that injecting singular vectors of this matrix allows us to optimally control energy deposition at any controllable delay time. Our approach provides insights into fundamental aspects of multi-spectral light scattering and could find applications in imaging or coherent control.

Coordinate transformations are a versatile tool to mould the flow of light, enabling a host of astonishing phenomena such as optical cloaking with metamaterials. Moving away from the usual restriction that links isotropic materials with conformal transformations, we show how non-conformal distortions of optical space are intimately connected to the complex refractive index distribution of an isotropic non-Hermitian medium. Remarkably, this insight can be used to circumvent the material requirement of working with refractive indices below unity, which limits the applications of transformation optics. We apply our approach to design a broadband unidirectional dielectric cloak, which relies on non-conformal coordinate transformations to tailor the nonHermitian refractive index profile around a cloaked object. Our insights bridge the fields of two-dimensional transformation optics and non-Hermitian photonics.

The last decade has seen the development of a wide set of tools, such as wavefront shaping, computational or fundamental methods, that allow to understand and control light propagation in a complex medium, such as biological tissues or multimode fibers. A vibrant and diverse community is now working on this field, that has revolutionized the prospect of diffraction-limited imaging at depth in tissues. This roadmap highlights several key aspects of this fast developing field, and some of the challenges and opportunities ahead., Comment: submitted to J.Phys Photonics (IOP), 116 pages, 23 sections

Due to quantum noise fluctuations, the rate of error achievable in decision problems involving several possible configurations of a scattering system is subject to a fundamental limit known as the Helstrom bound. Here, we present a general framework to calculate and minimize this bound using coherent probe fields with tailored spatial distributions. As an example, we experimentally study a target located in between two disordered scattering media. We first show that the optimal field distribution can be directly identified using a general approach based on scattering matrix measurements. We then demonstrate that this optimal light field successfully probes the presence of the target with a number of photons that is reduced by more than two orders of magnitude as compared to unoptimized fields.

Quantum models based on few-mode Master equations have been a central tool in the study of resonator quantum electrodynamics, extending the seminal single-mode Jaynes-Cummings model to include loss and multiple modes. Despite their broad application range, previous approaches within this framework have either relied on a Markov approximation or a fitting procedure. By combining ideas from pseudomode and quasinormal mode theory, we develop a certification criterion for multi-mode effects in lossy resonators. It is based on a witness observable, and neither requires a fitting procedure nor a Markov approximation. Using the resulting criterion, we demonstrate that such multi-mode effects are important for understanding previous experiments in X-ray cavity QED with M\"ossbauer nuclei and that they allow one to tune the nuclear ensemble properties.

Spin ensembles with a comb-shaped spectrum have shown exciting properties as efficient quantum memories. Here, we present a rigorous theoretical study of such atomic frequency combs in the strong coupling limit of cavity QED, based on a full quantum treatment using tensor-network methods. Our results demonstrate that arbitrary multi-photon states in the cavity are almost perfectly absorbed by the spin ensemble and re-emitted as parity-flipped states at periodic time intervals. Fidelity values near unity are achieved in these revived states by compensating for energy shifts induced by the strong spin-cavity coupling through adjustments of individual coupling values of the teeth in the atomic frequency comb., Comment: 5 pages, 3 figures

Determining the ultimate precision limit for measurements on a sub-wavelength particle with coherent laser light is a goal with applications in areas as diverse as biophysics and nanotechnology. Here, we demonstrate that surrounding such a particle with a complex scattering environment does, on average, not have any influence on the mean quantum Fisher information associated with measurements on the particle. As a remarkable consequence, the average precision that can be achieved when estimating the particle's properties is the same in the ballistic and in the diffusive scattering regime, independently of the particle's position within its complex environment. This invariance law breaks down only in the regime of Anderson localization, due to increased speckle correlations. Finally, we show how these results connect to the mean quantum Fisher information achievable with spatially optimized input fields.

Light forces can be harnessed to levitate mesoscopic objects and cool them down towards their motional quantum ground state. Significant roadblocks on the way to scale up levitation from a single to multiple particles in close proximity are the requirements to constantly monitor the particles' positions as well as to engineer complex light fields that react fast and appropriately to their movements. Here, we present an approach that solves both problems at once. By exploiting the information stored in a time-dependent scattering matrix, we introduce a robust formalism enabling the identification of spatially modulated wavefronts, which simultaneously cool down multiple levitated objects of arbitrary shapes. An experimental implementation is suggested based on stroboscopic scattering-matrix measurements and time-adaptive injections of modulated light fields., Comment: This update includes a thermal noise analysis and an application of our far-field cooling approach to multiple trapped particles. Details of all derivations and extended numerical simulations are posted in the parallel submission arXiv:2206.01046

We study a multivariate, non-linear Hawkes process $Z^N$ on the complete graph with $N$ nodes. Each vertex is either excitatory (probability $p$) or inhibitory (probability $1-p$). We take the mean-field limit of $Z^N$, leading to a multivariate point process $\bar Z$. If $p\neq\tfrac12$, we rescale the interaction intensity by $N$ and find that the limit intensity process solves a deterministic convolution equation and all components of $\bar Z$ are independent. In the critical case, $p=\tfrac12$, we rescale by $N^{1/2}$ and obtain a limit intensity, which solves a stochastic convolution equation and all components of $\bar Z$ are conditionally independent.

Diffusive random walks feature the surprising property that the average length of all possible random trajectories that enter and exit a finite domain is determined solely by the domain boundary. Changes in the diffusion constant or the mean-free path, that characterize the diffusion process, leave the mean path length unchanged. Here we demonstrate experimentally that this result can be transferred to the scattering of waves, even when wave interference leads to marked deviations from a diffusion process. Using a versatile microwave setup, we establish the mean path length invariance for the crossover to Anderson localization and for the case of a band gap in a photonic crystal. We obtain these results on the mean path length solely based on a transmission matrix measurement through a novel procedure that turns out to be more robust to absorption and incomplete measurement in the localized regime as compared to an assessment based on the full scattering matrix.

The memory effect in disordered systems is a key physical phenomenon that has been employed for optical imaging, metrology, and communication through opaque media. Under the conventional memory effect, when the incident beam is tilted slightly, the transmitted pattern tilts in the same direction. However, the "memory" is limited in its angular range and tilt direction. Here, we present a general approach to customize the memory effect by introducing an angular memory operator. Its eigenstates possess perfect correlation for tilt angles and directions that can be arbitrarily chosen separately for the incident and transmitted waves, and can be readily realized with wavefront shaping. This work reveals the power of wavefront shaping in creating any desired memory for applications of classical and quantum waves in complex systems.

Speckle patterns are ubiquitous in optics and have multiple applications for which the control of their spatial correlations is essential. Here, we report on a method to engineer speckle correlations behind a scattering medium through the singular value decomposition of the transmission matrix. We not only demonstrate control over the speckle grain size and shape but also realize patterns with non-local correlations. Moreover, we show that the reach of our method extends also along the axial dimension, allowing volumetric speckle engineering behind scattering layers.

Random scattering of light in disordered media is an intriguing phenomenon of fundamental relevance to various applications. While techniques such as wavefront shaping and transmission matrix measurements have enabled remarkable progress for advanced imaging concepts, the most successful strategy to obtain clear images through a disordered medium remains the filtering of ballistic light. Ballistic photons with a scattering-free propagation are, however, exponentially rare and no method so far can increase their proportion. To address these limitations, we introduce and experimentally implement here a new set of optical states that we term Scattering Invariant Modes (SIMs), whose transmitted field pattern is the same, irrespective of whether they scatter through a disordered sample or propagate ballistically through a homogeneous medium. We observe SIMs that are only weakly attenuated in dense scattering media, and show in simulations that their correlations with the ballistic light can be used to improve imaging inside scattering materials.

The efficient transfer of excitations between different levels of a quantum system is a task with many applications. Among the various protocols to carry out such a state transfer in driven systems, rapid adiabatic passage (RAP) is one of the most widely used. Here we show both theoretically and experimentally that adding a suitable amount of loss to the driven Hamiltonian turns a RAP protocol into a scheme for encircling an exceptional point including the chiral state transfer associated with it. Our work thus discloses an intimate connection between a whole body of literature on RAP and recent studies on the dynamics in the vicinity of an exceptional point, which we expect to serve as a bridge between the disjoint communities working on these two scenarios., Comment: 5 pages, 4 figures in main text; 14 pages supplementary material

The effect of PT-symmetry breaking in coupled systems with balanced gain and loss has recently attracted considerable attention and has been demonstrated in various photonic, electrical and mechanical systems in the classical regime. Here we generalize the definition of PT symmetry to finite-dimensional open quantum systems, which are described by a Markovian master equation. Specifically, we show that the invariance of this master equation under a certain symmetry transformation implies the existence of stationary states with preserved and broken parity symmetry. As the dimension of the Hilbert space grows, the transition between these two limiting phases becomes increasingly sharp and the classically expected PT-symmetry breaking transition is recovered. This quantum-to-classical correspondence allows us to establish a common theoretical framework to identify and accurately describe PT-symmetry breaking effects in a large variety of physical systems, operated both in the classical and quantum regimes., Comment: 15 pages, 3 figures

The use of coherent light for precision measurements has been a key driving force for numerous research directions, ranging from biomedical optics to semiconductor manufacturing. Recent work demonstrates that the precision of such measurements can be significantly improved by tailoring the spatial profile of light fields used for estimating an observable system parameter. These advances naturally raise the intriguing question of which states of light can provide the ultimate measurement precision. Here, we introduce a general approach to determine the optimal coherent states of light for estimating any given parameter, regardless of the complexity of the system. Our analysis reveals that the light fields delivering the ultimate measurement precision are eigenstates of a Hermitian operator which quantifies the Fisher information based on the system's scattering matrix. To illustrate this concept, we experimentally show that these maximum information states can probe the phase or the position of an object that is hidden by a disordered medium with a precision improved by an order of magnitude as compared to unoptimized states. Our results enable optimally precise measurements in arbitrarily complex systems, thus establishing a new benchmark for metrology and imaging applications.

Spiking activity in cortical networks is nonlinear in nature. The linear-nonlinear cascade model, some versions of which are also known as point-process generalized linear model, can efficiently capture the nonlinear dynamics exhibited by such networks. Of particular interest in such models are theoretical predictions of spike train statistics. However, due to the moment-closure problem, approximations are inevitable. We suggest here a series expansion that explains how higher-order moments couple to lower-order ones. Our approach makes predictions in terms of certain integrals, the so-called loop integrals. In previous studies these integrals have been evaluated numerically, but numerical instabilities are sometimes encountered rendering the results unreliable. Analytic solutions are presented here to overcome this problem, and to arrive at more robust evaluations. We were able to deduce these analytic solutions by switching to Fourier space and making use of complex analysis, specifically Cauchy's residue theorem. We formalized the loop integrals and explicitly solved them for specific response functions. To quantify the importance of these corrections for spike train cumulants, we numerically simulated spiking networks and compared their sample statistics to our theoretical predictions. Our results demonstrate that the magnitude of the nonlinear corrections depends on the working point of the nonlinear network dynamics, and that it is related to the eigenvalues of the mean-field stability matrix. For our example, the corrections for the firing rates are in the range between 4 % and 21 % on average. Precise and robust predictions of spike train statistics accounting for nonlinear effects are, for example, highly relevant for theories involving spike-timing dependent plasticity (STDP)., Comment: 45 pages, 8 figures

Spectral fingerprints of molecules are mostly accessible in the terahertz and mid-infrared ranges, such that efficient molecular-detection technologies rely on broadband coherent light sources at such frequencies. THz Quantum Cascade Lasers can achieve octave-spanning bandwidths. However, their tunability and wavelength selectivity is often constrained by the geometry of their cavity. The recently introduced Quantum Cascade Random Lasers represent alternative sources of THz light, in which random scattering provides the required field confinement. The random resonator geometry greatly relaxes wavelength selectivity, thus producing radiation that is both spectrally broadband and collimated in the far-field. Yet, the intrinsic randomness of these devices' spectral emission strongly restricts the scope of their potential applications. In this work, we demonstrate the all-optical adaptive control and tuning of Quantum Cascade Random Lasers. The specificity of our random-laser sources is exploited to locally modify the system's permittivity with a near-infrared (NIR) laser beam and thereby substantially reconfigure the distribution of disorder. Using a spatial light modulator combined with an optimization procedure, the NIR illumination is spatially modulated to reshape the spectral emission and transform the initially multimode laser into a single mode source, which could be harnessed to perform self-referenced spectroscopic measurements. Moreover, we show that local NIR perturbations can be used to sense linear and nonlinear interactions amongst modes in the near field. Our work points the way towards the design of broadly tunable THz sources with greatly relaxed fabrication constraints., Comment: 11 pages, 3 figures

The manipulation of small objects with light has become an indispensable tool in many areas of research ranging from physics to biology and medicine. Here we demonstrate how to implement micro-manipulation at the optimal level of efficiency for targets of arbitrary shape and inside complex environments such as disordered media. Our approach is to design wave-fronts in the far-field that have optimal properties in the near-field of the target such as to apply to it the strongest possible force, pressure or torque as well as to achieve the most efficient focus at the target position. Free of any iterative optimization, our approach only relies on a simple eigenvalue problem established from the scattering matrix of the system and its dependence on the target parameters. To illustrate this theoretical concept, we perform a proof-of-principle experiment in the microwave regime, which fully confirms our predictions.

The optical memory effect has emerged as a powerful tool for imaging through multiple-scattering media; however, the finite angular range of the memory effect limits the field of view. Here, we demonstrate experimentally that selective coupling of incident light into a high-transmission channel increases the angular memory-effect range. This enhancement is attributed to the robustness of the high-transmission channels against perturbations such as sample tilt or wavefront tilt. Our work shows that the high-transmission channels provide an enhanced field of view for memory effect-based imaging through diffusive media.

Electronic matter waves traveling through the weak and smoothly varying disorder potential of a semi-conductor show branching behavior instead of a smooth spreading of flow. By transferring this phenomenon to optics, we show how the branched flow of light can be controlled to propagate along a single branch rather than through many of them at the same time. Our method is based on shaping the incoming wavefront and only requires partial knowledge of the system's transmission matrix. We show that the light flowing along a single branch has a broadband frequency stability such that we can even steer pulses along selected branches - a prospect with many interesting possibilities for wave control in disordered environments., Comment: 6 pages, 5 figures, including appendix

We present a theoretical study on the nonlinear dynamics and stationary states of an inhomogeneously broadened spin ensemble coupled to a single-mode cavity driven by an external drive with constant amplitude. Assuming a sizeable number of constituents within the ensemble allows us to use a semiclassical approach and to formally reduce the theoretical description to the Maxwell-Bloch equations for the cavity and spin amplitudes. We explore the critical slowing-down effect, quench dynamics, and asymptotic behavior of the system near a steady-state dissipative phase transition accompanied by a bistability effect. Some of our theoretical findings have recently been successfully verified in a specific experimental realization based on a spin ensemble of negatively charged nitrogen-vacancy centers in diamond strongly coupled to a single-mode microwave cavity (see Science Adv. 3, e1701626 (2017))., Comment: 11 pages, 6 figures

We numerically study the dynamics and stationary states of a spin ensemble strongly coupled to a single-mode resonator subjected to loss and external driving. Employing a generalized cumulant expansion approach we analyze finite-size corrections to a semiclassical description of amplitude bistability, which is a paradigm example of a driven-dissipative phase transition. Our theoretical model allows us to include inhomogeneous broadening of the spin ensemble and to capture in which way the quantum corrections approach the semiclassical limit for increasing ensemble size $N$. We set up a criterion for the validity of the Maxwell-Bloch equations and show that close to the critical point of amplitude bistability even very large spin ensembles consisting of up to $10^4$ spins feature significant deviations from the semiclassical theory., Comment: 12 pages, 6 figures

We demonstrate a new design principle for unidirectionally invisible non-Hermitian structures that are not only invisible for one specific wavelength but rather for a broad frequency range. Our idea is based on the concept of constant-intensity waves, which can propagate even through highly disordered media without back-scattering or intensity variations. Contrary to already existing invisibility studies, our new design principle requires neither a specific symmetry (like $\mathcal{PT}$-symmetry) nor periodicity, and can thus be applied in a much wider context. This generality combined with broadband frequency stability allows a pulse to propagate through a disordered medium as if the medium was entirely uniform., Comment: 7 pages, 7 figures, including appendix

We report on a novel dynamical phenomenon in electron spin resonance experiments of phosphorus donors. When strongly coupling the paramagnetic ensemble to a superconducting lumped element resonator, the coherent exchange between these two subsystems leads to a train of periodic, self-stimulated echos after a conventional Hahn echo pulse sequence. The presence of these multi-echo signatures is explained using a simple model based on spins rotating on the Bloch sphere, backed up by numerical calculations using the inhomogeneous Tavis-Cummings Hamiltonian.

We analyze the collective dynamics of hierarchically structured networks of densely connected spiking neurons. These networks of sub-networks may represent interactions between cell assemblies or different nuclei in the brain. The dynamical activity pattern that results from these interactions depends on the strength of synaptic coupling between them. Importantly, the overall dynamics of a brain region in the absence of external input, so called ongoing brain activity, has been attributed to the dynamics of such interactions. In our study, two different network scenarios are considered: a system with one inhibitory and two excitatory sub-networks, and a network representation with three inhibitory sub-networks. To study the effect of synaptic strength on the global dynamics of the network, two parameters for relative couplings between these sub-networks are considered. For each case, a co-dimension two bifurcation analysis is performed and the results have been compared to large-scale network simulations. Our analysis shows that Generalized Lotka-Volterra (GLV) equations, well-known in predator-prey studies, yield a meaningful population-level description for the collective behavior of spiking neuronal interaction, which have a hierarchical structure. In particular, we observed a striking equivalence between the bifurcation diagrams of spiking neuronal networks and their corresponding GLV equations. This study gives new insight on the behavior of neuronal assemblies, and can potentially suggest new mechanisms for altering the dynamical patterns of spiking networks based on changing the synaptic strength between some groups of neurons.