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High Q-factors are of utmost importance to minimize losses of superconducting radio-frequency cavities deployed in continuous wave particle accelerators. This study elucidates the surface treatment that can maximize the Q-factors in high-beta 650 MHz elliptical niobium cavities. State-of-the-art surface treatments are applied in many single-cell cavities, and surface resistance studies are performed to understand the microwave dissipation at this unexplored frequency. The nitrogen doping treatment is confirmed to be necessary to maximize the Q-factors at medium RF fields. We applied this treatment in five-cell high-beta 650 MHz cavities and demonstrated that extremely high Q-factors were obtained at medium RF fields with this treatment. We also demonstrated that adding a cold electropolishing step after N-doping is crucial to push the quench field of multicell cavities to higher gradients.

Nb3Sn is a promising next-generation material for superconducting radiofrequency cavities, with significant potential for both large scale and compact accelerator applications. However, so far, Nb3Sn cavities have been limited to cw accelerating fields <18 MV/m. In this paper, new results are presented with significantly higher fields, as high as 24 MV/m in single cell cavities. Results are also presented from the first ever Nb3Sn-coated 1.3 GHz 9-cell cavity, a full-scale demonstration on the cavity type used in production for the European XFEL and LCLS-II. Results are presented together with heat dissipation curves to emphasize the potential for industrial accelerator applications using cryocooler-based cooling systems. The cavities studied have an atypical shiny visual appearance, and microscopy studies of witness samples reveal significantly reduced surface roughness and smaller film thickness compared to typical Nb3Sn films for superconducting cavities. Possible mechanisms for increased maximum field are discussed as well as implications for physics of RF superconductivity in the low coherence length regime. Outlook for continued development is presented.

We report on an effort to improve the performance of superconducting radiofrequency cavities by the use of heat treatment in a temperature range sufficient to dissociate the natural surface oxide. We find that the residual resistance is significantly decreased, and we find an unexpected reduction in the BCS resistance. Together these result in extremely high quality factor values at relatively large accelerating fields Eacc ~20 MV/m: Q0 of 3-4x10^11 at <1.5 K and Q0 ~5x10^10 at 2.0 K. In one cavity, measurements of surface resistance versus temperature showed an extremely small residual resistance of just 0.63+/-0.06 nOhms at 16 MV/m. SIMS measurements confirm that the oxide was significantly dissociated, but they also show the presence of nitrogen after heat treatment. We also present studies of surface oxidation via exposure to air and to water, as well as the effects of very light surface removal via HF rinse. The possibilities for applications and the planned future development are discussed., Comment: 9 pages, 9 figures

When a superconducting radiofrequency cavity is cooled through its critical temperature, ambient magnetic flux can become "frozen in" to the superconductor, resulting in degradation of the quality factor. This is especially problematic in applications where quality factor is a cost driver, such as in the CW linac for LCLS-II. Previously, it had been unknown how to prevent flux from being trapped during cooldown in bulk niobium cavities, but recent R&D studies showed near-full flux expulsion can be achieved through high temperature heat treatment and cooling cavities through the superconducting transition with a spatial thermal gradient over the surface. In this paper, we describe the first accelerator implementation of these procedures, in cryomodules that are currently being produced for LCLS-II. We compare the performance of cavities under different conditions of heat treatment and thermal gradient during cooldown, showing a substantial improvement in performance when both are applied, enabling cryomodules to reach and, in many cases, exceed a Q0 of ~3x10^10., Comment: 11 pages

In this paper we present the discovery of a new surface treatment applied to superconducting radio frequency (SRF) niobium cavities, leading to unprecedented accelerating fields of 49 MV/m in TESLA-shaped cavities, in continuous wave (CW); the corresponding peak magnetic fields are the highest ever measured in CW, about 210 mT. For TESLA-shape cavities the maximum quench field ever achieved was ~45 MV/m - reached very rarely- with most typical values being below 40 MV/m. These values are reached for niobium surfaces treated with electropolishing followed by the so called mild bake, a 120C vacuum bake (for 48 hours for fine grain and 24 hours for large grain surfaces). We discover that the addition during the mild bake of a step at 75C for few hours, before the 120C, increases systematically the quench fields up to unprecedented values of 49 MV/m. The significance of the result lays not only in the relative improvement, but in the proof that niobium surfaces can sustain and exceed CW radio frequency magnetic fields much larger than Hc1, pointing to an extrinsic nature of the current field limitations, and therefore to the potential to reach accelerating fields well beyond the current state of the art.

A new test stand dedicated to Superconducting Radiofrequency (SRF) cryomodule testing, CMTS1, has been commissioned and is now in operation at Fermilab. The first device to be cooled down and powered in this facility is the prototype 1.3 GHz cryomodule assembled at Fermilab for LCLS-II. We describe the demonstrated capabilities of CMTS1, report on steps taken during commissioning, provide an overview of first test results, and survey future plans., Comment: 4 pp. Proceedings of LINAC2016, East Lansing, MI, USA

Expulsion of ambient flux has been shown to be crucial to obtain high quality factors in bulk niobium SRF cavities. However, there remain many questions as to what properties of the niobium material determine its flux expulsion behavior. In this paper, we present first results from a new study of two cavities that were specially fabricated to study flux expulsion. Both cavities were made from large grain ingot niobium slices, one of which had its slices rolled prior to fabrication, and none these slices were annealed prior to measurement. Expulsion measurements indicate that a dense network of grain boundaries is not necessary for a cavity to have near-complete flux trapping behavior up to large thermal gradients. The results also contribute to a body of evidence that cold work is a strong determinant of flux expulsion behavior in SRF-grade niobium., Comment: 7 pages, 10 figures

SRF cavity quality factors can be accurately measured using RF-power based techniques only when the cavity is very close to critically coupled. This limitation is from systematic errors driven by non-ideal RF components. When the cavity is not close to critically coupled, these systematic effects limit the accuracy of the measurements. The combination of the complex base-band envelopes of the cavity RF signals in combination with a trombone in the circuit allow the relative calibration of the RF signals to be extracted from the data and systematic effects to be characterized and suppressed. The improved calibration allows accurate measurements to be made over a much wider range of couplings. Demonstration of these techniques during testing of a single-spoke resonator with a coupling factor of near 7 will be presented, along with recommendations for application of these techniques.

The radio-frequency surface resistance of niobium resonators is incredibly reduced when nitrogen impurities are dissolved as interstitial in the material, conferring ultra-high Q-factors at medium values of accelerating field. This effect has been observed in both high and low temperature nitrogen treatments. As a matter of fact, the peculiar anti Q-slope observed in nitrogen doped cavities, i.e. the decreasing of the Q-factor with the increasing of the radio-frequency field, come from the decreasing of the BCS surface resistance component as a function of the field. Such peculiar behavior has been considered consequence of the interstitial nitrogen present in the niobium lattice after the doping treatment. The study here presented show the field dependence of the BCS surface resistance of cavities with different resonant frequencies, such as: 650 MHz, 1.3 GHz, 2.6 GHz and 3.9 GHz, and processed with different state-of-the-art surface treatments. These findings show for the first time that the anti Q-slope might be seen at high frequency even for clean Niobium cavities, revealing useful suggestion on the physics underneath the anti Q-slope effect., Comment: To be published in Proceedings of SRF 2017

We report the finding of new surface treatments that permit to manipulate the niobium resonator nitrogen content in the first few nanometers in a controlled way, and the resonator fundamental Mattis-Bardeen surface resistance and residual resistance accordingly. In particular, we find surface infusion conditions that systematically a) increase the quality factor of these 1.3 GHz superconducting radio frequency (SRF) bulk niobium resonators, up to very high gradients; b) increase the achievable accelerating gradient of the cavity compared to its own baseline with state-of-the-art surface processing. Cavities subject to the new surface process have larger than two times the state of the art Q at 2K for accelerating fields > 35 MV/m. Moreover, very high accelerating gradients ~ 45 MV/m are repeatedly reached, which correspond to peak magnetic surface fields of 190 mT, among the highest measured for bulk niobium cavities. These findings open the opportunity to tailor the surface impurity content distribution to maximize performance in Q and gradients, and have therefore very important implications on future performance and cost of SRF based accelerators. They also help deepen the understanding of the physics of the RF niobium cavity surface.

Previous work has demonstrated that the radio frequency surface resistance of niobium resonators is dramatically reduced when nitrogen impurities are dissolved as interstitial in the material. The origin of this effect is attributed to the lowering of the Mattis and Bardeen surface resistance contribution with increasing accelerating field. Meanwhile, an enhancement of the sensitivity to trapped magnetic field is typically observed for such cavities. In this paper we conduct the first systematic study on these different components contributing to the total surface resistance as a function of different levels of dissolved nitrogen, in comparison with standard surface treatments for niobium resonators. Adding these results together we are able to show for the first time which is the optimum surface treatment that maximizes the Q-factor of superconducting niobium resonators as a function of expected trapped magnetic field in the cavity walls. These results also provide new insights on the physics behind the change in the field dependence of the Mattis and Bardeen surface resistance, and of the trapped magnetic vortex induced losses in superconducting niobium resonators.

Quench of superconducting radio-frequency cavities frequently leads to the lowered quality factor Q0, which had been attributed to the additional trapped magnetic flux. Here we demonstrate that the origin of this magnetic flux is purely extrinsic to the cavity by showing no extra dissipation (unchanged Q0) after quenching in zero magnetic field, which allows us to rule out intrinsic mechanisms of flux trapping such as generation of thermal currents or trapping of the rf field. We also show the clear relation of dissipation introduced by quenching to the orientation of the applied magnetic field and the possibility to fully recover the quality factor by requenching in the compensated field. We discover that for larger values of the ambient field, the Q-factor degradation may become irreversible by this technique, likely due to the outward flux migration beyond the normal zone opening during quench. Our findings are of special practical importance for accelerators based on low- and medium-beta accelerating structures residing close to focusing magnets, as well as for all high-Q cavity-based accelerators.

Q0 determinations based on RF power measurements are subject to at least three potentially large systematic effects that have not been previously appreciated. Instrumental factors that can systematically bias RF based measurements of Q0 are quantified and steps that can be taken to improve the determination of Q0 are discussed.

Even when cooled through its transition temperature in the presence of an external magnetic field, a superconductor can expel nearly all external magnetic flux. This Letter presents an experimental study to identify the parameters that most strongly influence flux trapping in high purity niobium during cooldown. This is critical to the operation of superconducting radiofrequency cavities, in which trapped flux degrades the quality factor and therefore cryogenic efficiency. Flux expulsion was measured on a large survey of 1.3 GHz cavities prepared in various ways. It is shown that both spatial thermal gradient and high temperature treatment are critical to expelling external magnetic fields, while surface treatment has minimal effect. For the first time, it is shown that a cavity can be converted from poor expulsion behavior to strong expulsion behavior after furnace treatment, resulting in a substantial improvement in quality factor. Future plans are described to build on this result in order to optimize treatment for future cavities., Comment: 5 pages

Cool-down dynamics of superconducting accelerating cavities became particularly important for obtaining very high quality factors in SRF cavities. Previous studies proved that when cavity is cooled fast, the quality factor is higher than when cavity is cooled slowly. This has been discovered to derive from the fact that a fast cool-down allows better magnetic field expulsion during the superconducting transition. In this paper we describe the first experiment where the temperature all around the cavity was mapped during the cavity cool-down through transition temperature, proving the existence of two different transition dynamics: a sharp superconducting-normal conducting transition during fast cool-down which favors flux expulsion and nucleation phase transition during slow cool-down, which leads to full flux trapping.

Previous studies on magnetic flux expulsion as a function of cooling details have been performed for superconducting niobium cavities with the cavity beam axis placed parallel respect to the helium cooling flow, and findings showed that for sufficient cooling thermogradients all magnetic flux could be expelled and very low residual resistance could be achieved. In this paper we investigate the flux trapping and its impact on radio frequency surface resistance when the resonators are positioned perpendicularly to the helium cooling flow, which is representative of how superconducting radio-frequency (SRF) cavities are cooled in an accelerator. We also extend the studies to different directions of applied magnetic field surrounding the resonator. Results show that in the cavity horizontal configuration there is a different impact of the various field components on the final surface resistance, and that several parameters have to be considered to understand flux dynamics. A newly discovered phenomenon of concentration of flux lines at the cavity top leading to cavity equator temperature rise is presented.

Ambient magnetic field, if trapped in the penetration depth, leads to the residual resistance and therefore sets the limit for the achievable quality factors in superconducting niobium resonators for particle accelerators. Here we show that a complete expulsion of the magnetic flux can be performed and leads to: 1) record quality factors $Q > 2\times10^{11}$ up to accelerating gradient of 22 MV/m; 2) $Q\sim3\times10^{10}$ at 2 K and 16 MV/m in up to 190 mG magnetic fields. This is achieved by large thermal gradients at the normal/superconducting phase front during the cooldown. Our findings open up a way to ultra-high quality factors at low temperatures and show an alternative to the sophisticated magnetic shielding implemented in modern superconducting accelerators.

We report a strong effect of the cooling dynamics through $T_\mathrm{c}$ on the amount of trapped external magnetic flux in superconducting niobium cavities. The effect is similar for fine grain and single crystal niobium and all surface treatments including electropolishing with and without 120$^\circ$C baking and nitrogen doping. Direct magnetic field measurements on the cavity walls show that the effect stems from changes in the flux trapping efficiency: slow cooling leads to almost complete flux trapping and higher residual resistance while fast cooling leads to the much more efficient flux expulsion and lower residual resistance.

We report a surface treatment that systematically improves the quality factor of niobium radio frequency cavities beyond the expected limit for niobium. A combination of annealing in a partial pressure of nitrogen or argon gas and subsequent electropolishing of the niobium cavity surface leads to unprecedented low values of the microwave surface resistance, and an improvement in the efficiency of the accelerating structures up to a factor of 3, reducing the cryogenic load of superconducting cavities for both pulsed and continuous duty cycles. The field dependence of the surface resistance is reversed compared to standardly treated niobium.

We investigate the effect of high temperature treatments followed by only high-pressure water rinse (HPR) of superconducting radio frequency (SRF) niobium cavities. The objective is to provide a cost effective alternative to the typical cavity processing sequence, by eliminating the material removal step post furnace treatment while preserving or improving the RF performance. The studies have been conducted in the temperature range 800-1000C for different conditions of the starting substrate: large grain and fine grain, electro-polished (EP) and centrifugal barrel polished (CBP) to mirror finish. An interesting effect of the grain size on the performances is found. Cavity results and samples characterization show that furnace contaminants cause poor cavity performance, and a practical solution is found to prevent surface contamination. Extraordinary values of residual resistances ~ 1 nOhm and below are then consistently achieved for the contamination-free cavities. These results lead to a more cost-effective processing and improved RF performance, and, in conjunction with CBP, open a potential pathway to acid-free processing.

In Fermilab we are build and tested several superconducting Single Spoke Resonators (SSR1, \beta=0.22) which can be used for acceleration of low beta ions. Fist two cavities performed very well during cold test in Vertical Test Station at FNAL. One dressed cavity was also tested successfully in Horizontal Test Station. Currently we are building 8 cavity cryomodule for PIXIE project. Additional 10 cavities were manufactured in the industry and on-going cold test results will be presented in this poster., Comment: 3 pp. 3rd International Particle Accelerator Conference (IPAC 2012) 20-25 May 2012, New Orleans, Louisiana

Magnetic field enhancement has been studied in the past through replica and cavity cutting. Considerable progress of niobium cavity manufacturing and processing has been made since then. Wide variety of single cell cavities has been analyzed through replica technique. Their RF performances were compared in corresponding to geometric RF surface quality. It is concluded that the surface roughness affects cavity performance mostly in secondary role. The other factors must have played primary role in cavity performance limitations., Comment: 4 pp. Applied Superconductivity Conference (ASC 2010) 1-6 Aug 2010. Washington, D.C

In the recently commissioned superconducting RF cavity test facility at Fermilab (SCTF), a 325 MHz, {\beta}=0.22 superconducting single-spoke resonator (SSR1) has been tested for the first time with its input power coupler. Previously, this cavity had been tested CW with a low power, high Qext test coupler; first as a bare cavity in the Fermilab Vertical Test Stand and then fully dressed in the SCTF. For the tests described here, the design input coupler with Qext ~ 106 was used. Pulsed power was provided by a Toshiba E3740A 2.5 MW klystron., Comment: 3 pp. Particle Accelerator, 24th Conference (PAC'11) 28 Mar - 1 Apr 2011: New York, USA

We have made heat capacity measurements of superfluid He-4 at temperatures very close to the lambda point, T(sub lambda) , in a constant heat flux, Q, when the helium sample is heated from above. In this configuration the helium enters a self-organized (SOC) heat transport state at a temperature T(sub SOC)(Q), which for Q greater than or = 100 nW/sq cm lies below T(sub lambda). At low Q we observe little or no deviation from the bulk Q = 0 heat capacity up to T(sub SOC)(Q); beyond this temperature the heat capacity appears to be sharply depressed, deviating dramatically from its bulk behaviour. This marks the formation and propagation of a SOC/superfluid two phase state, which we confirm with a simple model. The excellent agreement between data and model serves as an independent confirmation of the existence of the SOC state. As Q is increased (up to 6 micron W/sq cm) we observe a Q dependant depression in the heat capacity that occurs just below T(sub SOC)(Q), when the entire sample is still superfluid. This is due to the emergence of a large thermal resistance in the sample, which we have measured and used to model the observed heat capacity depression. Our measurements of the superfluid thermal resistivity are a factor of ten larger than previous measurements by Baddar et al.

We describe an experimental setup and a series of experiments with a column of helium- 4 heated from above close to its transition to the superfluid state.