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The nature of charge carriers in strange metals has become a topic of intense current investigation. Recent shot noise measurements in the quantum critical heavy fermion metal YbRh$_2$Si$_2$ revealed a suppression of the Fano factor that cannot be understood from electron-phonon scattering or strong electron correlations in a Fermi liquid, indicating loss of quasiparticles. The experiment motivates the consideration of shot noise in a variety of theoretical models in which quasiparticles may be lost. Here we study shot noise in systems with co-existing itinerant electrons and dispersive bosons, going beyond the regime where the bosons are on their own in thermal equilibrium. We construct the Boltzmann-Langevin equations for the coupled system, and show that adequate electron-boson couplings restore the Fano factor to its Fermi liquid value. Our findings point to the beyond-Landau form of quantum criticality as underlying the suppressed shot noise of strange metals in heavy fermion metals and beyond., Comment: 13 pages, 4 figures

The iron-based superconductor FeSe isovalently substituted with S displays an abundance of remarkable phenomena that have not been fully understood, at the center of which are apparent zero-energy excitations in the superconducting state in the tetragonal phase. The phenomenology has been generally consistent with the proposal of the so-called ultranodal states where Bogoliubov Fermi surfaces are present. Recently, nuclear magnetic resonance measurements have seen unusually large upturns in the relaxation rate as temperature decreases to nearly zero in these systems, calling for theoretical investigations. In this paper, we calculate the spin susceptibility of an ultranodal superconductor including correlation effects within the random phase approximation. Although the non-interacting mean-field calculation rarely gives an upturn in the low temperature relaxation rate within our model, we found that correlation strongly enhances scattering between coherent parts of the Bogoliubov Fermi surface, resulting in robust upturns when the interaction is strong. Our results suggest that in addition to the presence of Bogoliubov Fermi surfaces, correlation and multiband physics also play important roles in the system's low energy excitations.

Kagome metals offer a unique platform for investigating robust electron-correlation effects because of their lattice geometry, flat bands and multi-orbital nature. In the cases with active flat bands, recent theoretical studies have pointed to a rich phase diagram that contains not only electronic orders but also quantum criticality. Very recently, $\rm CsCr_3Sb_5$ has emerged as a strong candidate for exploring such new physics. Here, using effective tight-binding models obtained from ab initio calculations, we study the effects of electronic correlations and symmetries on the electronic structure of $\rm CsCr_3 Sb_5$. The effective tight-binding model and Fermi surface comprise multiple Cr-$d$ orbitals and Sb-$p$ orbitals. The introduction of Hubbard-Kanamori interactions leads to orbital-selective band renormalization dominated by the $d_{xz}$ band, concurrently producing emergent flat bands very close to the Fermi level. Our analysis sets the stage for further investigations into the electronic properties of $\rm CsCr_3Sb_5$, including electronic orders, quantum criticality and unconventional superconductivity, which promise to shed much new light into the electronic materials with frustrated lattices and bring about new connections with the correlation physics of a variety of strongly correlated systems., Comment: 6 + 6 pages, 4 + 5 figures

The interplay of topological electronic band structures and strong interparticle interactions provides a promising path towards the constructive design of robust, long-range entangled many-body systems. As a prototype for such systems, we here study an exactly integrable, local model for a fractionalized topological insulator. Using a controlled perturbation theory about this limit, we demonstrate the existence of topological bands of zeros in the exact fermionic Green's function and show that {in this model} they do affect the topological invariant of the system, but not the quantized transport response. Close to (but prior to) the Higgs transition signaling the breakdown of fractionalization, the topological bands of zeros acquire a finite ``lifetime''. We also discuss the appearance of edge states and edge zeros at real space domain walls separating different phases of the system. This model provides a fertile ground for controlled studies of the phenomenology of Green's function zeros and the underlying exactly solvable lattice gauge theory illustrates the synergetic cross-pollination between solid-state theory, high-energy physics and quantum information science., Comment: 5 papges, 9 pages supplement, 5 figures

The intersection of electronic topology and strong correlations offers a rich platform to discover exotic quantum phases of matter and unusual materials. An overarching challenge that impedes the discovery is how to diagnose strongly correlated electronic topology. Here, we develop a framework to address this outstanding question, and illustrate its power in the setting of electronic topology in Mott insulators. Based on single-particle Green's functions, the concept of a Green's function Berry curvature -- which is frequency dependent -- is introduced. We apply this notion in a system that contains symmetry-protected nodes in its noninteracting bandstructure; strong correlations drive the system into a Mott insulating state, creating contours in frequency-momentum space where the Green's function vanishes. The Green's function Berry flux of such zeros is found to be quantized, and is as such direct probe of the system's topology. Our framework allows for a systematic search of strongly correlated topological materials with Green's function topology., Comment: 38 pages, 13 figures including Supplemental Information

Electronic correlation effects are manifested in quantum materials when either the onsite Coulomb repulsion is large or the electron kinetic energy is small. The former is the dominant effect in the cuprate superconductors or heavy fermion systems while the latter in twisted bilayer graphene or geometrically frustrated metals. However, the simultaneous cooperation of both effects in the same quantum material--the design principle to produce a correlated topological flat bands pinned at the Fermi level--remains rare. Here, using angle-resolved photoemission spectroscopy, we report the observation of a flat band at the Fermi level in a 3$d$ pyrochlore metal CuV$_2$S$_4$. From a combination of first-principles calculations and slave-spin calculations, we understand the origin of this band to be a destructive quantum-interference effect associated with the V pyrochlore sublattice and further renormalization to the Fermi level by electron interactions in the partially filled V $t_{2g}$ orbitals. As a result, we find transport behavior that indicates a deviation from Fermi-liquid behavior as well as a large Sommerfeld coefficient. Our work demonstrates the pathway into correlated topology by constructing and pinning correlated flat bands near the Fermi level out of a pure $d$-electron system by the combined cooperation of local Coulomb interactions and geometric frustration in a pyrochlore lattice system., Comment: 23 pages, 4 figures, to appear in Nature Physics

There is extensive current interest about electronic topology in correlated settings. In strongly correlated systems, contours of Green's function zeros may develop in frequency-momentum space, and their role in correlated topology has increasingly been recognized. However, whether and how the zeros contribute to electronic properties is a matter of uncertainty. Here we address the issue in an exactly solvable model for Mott insulator. We show that the Green's function zeros contribute to several physically measurable correlation functions, in a way that does not run into inconsistencies. In particular, the physical properties remain robust to chemical potential variations up to the Mott gap as it should be based on general considerations. Our work sets the stage for further understandings on the rich interplay among topology, symmetry and strong correlations., Comment: 17 pages, 4 figures

The ability to reversibly toggle between two distinct states in a non-volatile method is important for information storage applications. Such devices have been realized for phase-change materials, which utilizes local heating methods to toggle between a crystalline and an amorphous state with distinct electrical properties. To expand such kind of switching between two topologically distinct phases requires non-volatile switching between two crystalline phases with distinct symmetries. Here we report the observation of reversible and non-volatile switching between two stable and closely-related crystal structures with remarkably distinct electronic structures in the near room temperature van der Waals ferromagnet Fe$_{5-\delta}$GeTe$_2$. From a combination of characterization techniques we show that the switching is enabled by the ordering and disordering of an Fe site vacancy that results in distinct crystalline symmetries of the two phases that can be controlled by a thermal annealing and quenching method. Furthermore, from symmetry analysis as well as first principle calculations, we provide understanding of the key distinction in the observed electronic structures of the two phases: topological nodal lines compatible with the preserved global inversion symmetry in the site-disordered phase, and flat bands resulting from quantum destructive interference on a bipartite crystaline lattice formed by the presence of the site order as well as the lifting of the topological degeneracy due to the broken inversion symmetry in the site-ordered phase. Our work not only reveals a rich variety of quantum phases emergent in the metallic van der Waals ferromagnets due to the presence of site ordering, but also demonstrates the potential of these highly tunable two-dimensional magnets for memory and spintronics applications.

Several unconventional superconductors show indications of zero-energy excitations in the superconducting state consistent with the existence of a so-called Bogoliubov Fermi surface (BFS). In particular, FeSe doped with S seems to acquire a nonzero density of states at zero energy at low temperatures when doped into the tetragonal phase, consistent with a previously proposed phenomenological theory assuming an anisotropic spin singlet pairing gap coexisting with a nonunitary interband triplet component. Here we search for a microscopic model that can support the coexistence of singlet pairing with other orders, including interband nonunitary triplet pairing, and discuss several candidates that indeed stabilize ground states with Bogoliubov Fermi surfaces. We show that with proper choice of the coupling strength of the various orders in our model, spontaneous breaking of $C_4$ rotational symmetry is realized at low temperatures, in accordance with recent angle-resolved photoemission experiments in Fe(Se,S) in the tetragonal phase., Comment: 13 pages, 5 figures

Phasons are collective low-energy modes that appear in disparate condensed matter systems such as quasicrystals, incommensurate structures, fluctuating charge density waves, and Moir\'e superlattices. They share several similarities with acoustic phonon modes, but they are not protected by any exact translational symmetry. As a consequence, they are subject to a wavevector independent damping, and they develop a finite pinning frequency, which destroy their acoustic linearly propagating dispersion. Under a few and simple well-motivated assumptions, we compute the phason density of states, and we derive the phason heat capacity as a function of the temperature. Finally, imagining a hypothetical s-wave pairing channel with electrons, we compute the critical temperature $T_c$ of the corresponding superconducting state as a function of phason damping using the Eliashberg formalism. We find that for large phason damping, the heat capacity is linear in temperature, showing a distinctive glass-like behavior. Additionally, we observe that the phason damping can strongly enhance the effective Eliashberg coupling, and we reveal a sharp non-monotonic dependence of the superconducting temperature $T_c$ on the phason damping, with a maximum located at the underdamped to overdamped crossover scale. Our simple computations confirm the potential role of overdamped modes in explaining the glassy properties of incommensurate structures, but also in possibly inducing strongly-coupled superconductivity therein, and enhancing the corresponding $T_c$., Comment: v2: appendices added, references added

Emergent phases often appear when the electronic kinetic energy is comparable to the Coulomb interactions. One approach to seek material systems as hosts of such emergent phases is to realize localization of electronic wavefunctions due to the geometric frustration inherent in the crystal structure, resulting in flat electronic bands. Recently, such efforts have found a wide range of exotic phases in the two-dimensional kagome lattice, including magnetic order, time-reversal symmetry breaking charge order, nematicity, and superconductivity. However, the interlayer coupling of the kagome layers disrupts the destructive interference needed to completely quench the kinetic energy. Here we demonstrate that an interwoven kagome network-a pyrochlore lattice-can host a three dimensional (3D) localization of electron wavefunctions. Meanwhile, the nonsymmorphic symmetry of the pyrochlore lattice guarantees all band crossings at the Brillouin zone X point to be 3D gapless Dirac points, which was predicted theoretically but never yet observed experimentally. Through a combination of angle-resolved photoemission spectroscopy, fundamental lattice model and density functional theory calculations, we investigate the novel electronic structure of a Laves phase superconductor with a pyrochlore sublattice, CeRu$_2$. We observe flat bands originating from both the Ce 4$f$ orbitals as well as from the 3D destructive interference of the Ru 4$d$ orbitals. We further observe the nonsymmorphic symmetry-protected 3D gapless Dirac cones at the X point. Our work establishes the pyrochlore structure as a promising lattice platform to realize and tune novel emergent phases intertwining topology and many-body interactions., Comment: 27 pages, 4 figures

The role of anharmonicity on superconductivity has often been disregarded in the past. Recently, it has been recognized that anharmonic decoherence could play a fundamental role in determining the superconducting properties (electron-phonon coupling, critical temperature, etc) of a large class of materials, including systems close to structural soft-mode instabilities, amorphous solids and metals under extreme high-pressure conditions. Here, we review recent theoretical progress on the role of anharmonic effects, and in particular certain universal properties of anharmonic damping, on superconductivity. Our focus regards the combination of microscopic-agnostic effective theories for bosonic mediators with the well-established BCS theory and Migdal-Eliashberg theory for superconductivity. We discuss in detail the theoretical frameworks, their possible implementation within first-principles methods, and the experimental probes for anharmonic decoherence. Finally, we present several concrete applications to emerging quantum materials, including hydrides, ferroelectrics and systems with charge density wave instabilities., Comment: matching the published version

Lattice symmetries are central to the characterization of electronic topology. Recently, it was shown that Green's function eigenvectors form a representation of the space group. This formulation has allowed the identification of gapless topological states even when quasiparticles are absent. Here we demonstrate the profundity of the framework in the extreme case, when interactions lead to a Mott insulator, through a solvable model with long-range interactions. We find that both Mott poles and zeros are subject to the symmetry constraints, and relate the symmetry-enforced spectral crossings to degeneracies of the original non-interacting eigenstates. Our results lead to new understandings of topological quantum materials and highlight the utility of interacting Green's functions toward their symmetry-based design., Comment: To appear in PRR Letter. 7 pages, 2 figures + Supplemental Material

Phonon softening is a ubiquitous phenomenon in condensed matter systems which is often associated with charge density wave (CDW) instabilities and anharmonicity. The interplay between phonon softening, CDW and superconductivity is a topic of intense debate. In this work, the effects of anomalous soft phonon instabilities on superconductivity are studied based on a recently developed theoretical framework that accounts for phonon damping and softening within the Migdal-Eliashberg theory. Model calculations show that the phonon softening in the form of a sharp dip in the phonon dispersion relation, either acoustic or optical (including the case of Kohn-type anomalies typically associated with CDW), can cause a manifold increase of the electron-phonon coupling constant $\lambda$. This, under certain conditions, which are consistent with the concept of optimal frequency introduced by Bergmann and Rainer, can produce a large increase of the superconducting transition temperature $T_c$. In summary, our results suggest the possibility of reaching high-temperature superconductivity by exploiting soft phonon anomalies restricted in momentum space., Comment: v3: matching the published version

Shot noise measures out-of-equilibrium current fluctuations and is a powerful tool to probe the nature of current-carrying excitations in quantum systems. Recent shot noise measurements in the heavy fermion strange metal YbRh$_2$Si$_2$ exhibit a strong suppression of the Fano factor ($F$) -- the ratio of the current noise to the average current in the DC limit. This system is representative of metals in which electron correlations are extremely strong. Here we carry out the first theoretical study on the shot noise of diffusive metals in the regime of strong correlations. A Boltzmann-Langevin equation formulation is constructed in a quasiparticle description in the presence of strong correlations. We find that $F = \sqrt{ 3}/{4}$ in such a correlation regime. Hence, the Fano factor suppression observed in experiments on YbRh$_2$Si$_2$ necessitates a loss of the quasiparticles. Our work opens the door to systematic theoretical studies of shot noise as a means of characterizing strongly correlated metallic phases and materials., Comment: 6+2 pages, 2+1 figures

Pair density waves (PDWs) are superconducting states formed by ``Cooper pairs" of electrons containing a non-zero center-of-mass momentum. They are characterized by a spatially modulated order parameter and may occur in a variety of emerging quantum materials such as cuprates, transition metal dichalcogenides (TMDs) and Kagome metals. Despite extensive theoretical and numerical studies seeking PDWs in a variety of lattices and interacting settings, there is currently no generic and robust mechanism that favors a modulated solution of the superconducting order parameter in the presence of time reversal symmetry. Here, we study the problem of two electrons subject to an anisotropic ($d$-wave) attractive potential. We solve the two-body Schrodinger wave equation exactly to determine the pair binding energy as a function of the center-of-mass momentum. We find that a modulated (finite momentum) pair is favored over a homogeneous (zero momentum) solution above a critical interaction. Using this insight from the exact two-body solution, we construct a BCS-like variational many-body wave function and calculate the free energy and superconducting gap as a function of the center-of-mass momentum. A zero temperature analysis of the energy shows that the conclusions of the two-body problem are robust in the many-body limit. Our results lay the theoretical and microscopic foundation for the existence of PDWs., Comment: 24 pages, 6 figures

Strange-metal behavior has been observed in materials ranging from high-temperature superconductors to heavy fermion metals. In conventional metals, current is carried by quasiparticles; although it has been suggested that quasiparticles are absent in strange metals, direct experimental evidence is lacking. We measured shot noise to probe the granularity of the current-carrying excitations in nanowires of the heavy fermion strange metal YbRh2Si2. When compared with conventional metals, shot noise in these nanowires is strongly suppressed. This suppression cannot be attributed to either electron-phonon or electron-electron interactions in a Fermi liquid, which suggests that the current is not carried by well-defined quasiparticles in the strange-metal regime that we probed. Our work sets the stage for similar studies of other strange metals., Comment: 22 pages, 4 figures; 21 pages supplementary text, 11 supplementary figures

Topological phononic insulators are the counterpart of three-dimensional quantum spin Hall insulators in phononic systems and, as such, their topological surfaces are characterized by Dirac cone-shaped gapless edge states arising as a consequence of a bulk-boundary correspondence. We propose a theoretical framework for the possible superconducting phase in these materials, where the attractive interaction between electrons is mediated by topological phonons in nontrivial boundary modes. Within the BCS limit, we develop a self-consistent two-band gap equation, whose solutions show that the superconducting critical temperature has a non-monotonic behaviour with respect to the phononic frequency in the Kramers-like point. This remarkable behaviour is produced by a resonance, that occurs when electrons and phonons on the topological surfaces have the same energy: this effectively increases the electron-phonon interaction and hence the Cooper pair binding energy, thus establishing an optimal condition for the superconducting phase. With this mechanism, the $T_{c}$ can be increased by well over a factor two, and the maximum enhancement occurs in the degenerate phononic flat-band limit.

Charge order in kagome metals is of extensive current interest. Recently, a charge density wave was discovered in the magnetic binary kagome metal FeGe. In analogy to its predecessor, the non-magnetic $A$V$_3$Sb$_5$ ($A$=K, Cs, Rb), the in-plane ordering occurs at the $M$ point. In contrast, however, the system manifestly shows effects of substantial correlations. Here we identify the topological bands crossing the Fermi energy (E$_F$) in FeGe and characterize the correlation-induced renormalization of these bands. We then derive a charge order from an effective model comprising topological kagome `flat' bands in the presence of a magnetic order. We demonstrate edge states as well as excess out-of-plane magnetic moment associated with the charge order; both are fingerprints of non-trivial band topology and consistent with recent experimental observations. Our results point to FeGe as an ideal platform to realize and elucidate correlated topological physics., Comment: 10 pages, 9 figures including Supplemental Material

Kagome materials often host exotic quantum phases, including spin liquids, Chern gap, charge order, and superconductivity. Existing scanning microscopy studies of the kagome charge order have been limited to non-kagome surface layers. Here we tunnel into the kagome lattice of FeGe to uncover features of the charge order. Our spectroscopic imaging identifes a 2x2 charge order in the magnetic kagome lattice, resembling that discovered in kagome superconductors. Spin-mapping across steps of unit-cell-height demonstrates that this charge order emerges from spin-polarized electrons with an antiferromagnetic stacking order. We further uncover the correlation between antiferromagnetism and charge order anisotropy, highlighting the unusual magnetic coupling of the charge order. Finally, we detect a pronounced edge state within the charge order energy gap, which is robust against the irregular shape of the kagome lattice edges. We discuss our results with the theoretically considered topological features of the kagome charge order including orbital magnetism and bulk-boundary correspondence.

In weakly coupled BCS superconductors, only electrons within a tiny energy window around the Fermi energy, $E_F$, form Cooper pairs. This may not be the case in strong coupling superconductors such as cuprates, FeSe, SrTiO$_3$ or cold atom condensates where the pairing scale, $E_B$, becomes comparable or even larger than $E_F$. In cuprates, for example, a plausible candidate for the pseudogap state at low doping is a fluctuating pair density wave, but no microscopic model has yet been found which supports such a state. In this work, we write an analytically solvable model to examine pairing phases in the strongly coupled regime and in the presence of anisotropic interactions. Already for moderate coupling we find an unusual finite temperature phase, below an instability temperature $T_i$, where local pair correlations have non-zero center-of-mass momentum but lack long-range order. At low temperature, this fluctuating pair density wave can condense either to a uniform $d$-wave superconductor or the widely postulated pair-density wave phase depending on the interaction strength. Our minimal model offers a unified microscopic framework to understand the emergence of both fluctuating and long range pair density waves in realistic systems., Comment: 13 pages, 6 figures including Supplemental Material

We present a minimal theory of superconductivity enhancement in ferroelectric-type materials. Simple expressions for the optical mode responsible for the soft mode transition are assumed. A key role is played by the anharmonic phonon damping which is modulated by an external control parameter (electron doping or mechanical strain) causing the appearance of the soft mode. It is shown that the enhancement in the superconducting critical temperature $T_{c}$ upon approaching the ferroelectric transition from either side is due to the Stokes electron-phonon scattering processes promoted by strong phonon damping effects., Comment: Synopsis in APS Physics at: https://physics.aps.org/articles/v15/s11

The interplay between interactions and topology in quantum materials is of extensive current interest. Strong correlations are known to be important for insulating topological states, as exemplified by the fractional quantum Hall effect. For the metallic case, whether and how they can drive topological states that have no free-electron counterparts is an open and pressing question. We introduce a general framework for lattice symmetries to constrain single-particle excitations even when they are not quasiparticles, and substantiate it in a periodic Anderson model with two channels of conduction electrons. We demonstrate that symmetry constrains correlation-induced emergent excitations to produce non-Fermi liquid topological phases. The loss of quasiparticles in these phases is manifested in a non-Fermi liquid form of spectral and transport properties, whereas its topological nature is characterized by surface states and valley and spin Hall conductivities. We also identify candidate materials to realize the proposed phases. Our work opens a door to a variety of non-Fermi liquid topological phases in a broad range of strongly correlated materials., Comment: 46 pages, 3 figures main text + 11 figures supplementary information

Electron correlations amplify quantum fluctuations and, as such, they have been recognized as the origin of a rich landscape of quantum phases. Whether and how they lead to gapless topological states is an outstanding question, and a framework that allows for determining novel phases and identifying new materials is in pressing need. Here we advance a general approach, in which strong correlations cooperate with crystalline symmetry to drive gapless topological states. We test this materials design principle by exploring Kondo lattice models and materials whose space group symmetries may promote different kinds of electronic degeneracies, with a particular focus on square-net systems. Weyl-Kondo nodal-line semimetals -- with nodes pinned to the Fermi energy -- are identified. We describe how this approach can be applied to discover strongly correlated topological semimetals, identify three heavy fermion compounds as new candidates, provide first direct experimental evidence for our prediction in Ce$_2$Au$_3$In$_5$, and discuss how our approach may lead to many more. Our findings illustrate the potential of the proposed materials design principle to guide the search for new topological metals in a broad range of strongly correlated systems., Comment: To appear in Nature Physics; submitted version of the manuscript (the accepted version will appear in the journal); 35 pages, 4 figures main text + 8 figures supplementary information

There have been extensive recent developments on kagome metals, such as T$_m$X$_n$ (T= Fe, Co and X= Sn, Ge) and $A$V$_3$Sb$_5$ ($A=$ Cs, K, Rb). An emerging issue is the nature of correlated phases when topologically \textit{non-trivial} bands cross the Fermi level. Here, we consider an extended Hubbard model on the kagome lattice in the presence of spin-orbit couplings, involving a Kramer's pair of bands that have opposite Chern numbers and are isolated in the band structure. We construct an effective model in a time-reversal (T) symmetric lattice description. We determine the correlated phases of this model and identify a density-wave order in the phase diagram. We show that this order is T-breaking, which originates from the Wannier orbitals lacking a common Wannier center -- a fingerprint of the underlying $Z_2$ topology. Implications of our results for the correlation physics of the kagome metals are discussed., Comment: 14 pages, 8 figures, 3 tables including Supplemental Material

Despite concerted efforts, the problem of dilute local moments embedded in a correlated conduction electron host such as Nd$_{1-x}$Ce$_x$CuO$_2$ persists due to lack of analytically controllable models. Here, we address the question: how do local moments couple to correlated but integrable hosts? We describe the conduction electrons by the model of Hatsugai-Kohmoto (HK) which has undergone a recent resurgence arising from its exact solvability, existence of Luttinger surfaces, and connections to Sachdev-Ye-Kitaev (SYK) thermodynamics. We derive an exact low energy "Kondo-HK" Hamiltonian and show the existence of additional spin-exchange coupling that is relevant in the renormalization group (RG) sense. This term is ferromagnetic and does not vanish at low energies yielding an algebraic enhancement of the Kondo temperature. "Poor man's" scaling of couplings exhibits an exotic step-like RG flow between UV-IR fixed points attributed to severely restricted scattering phase space. This phenomenon is analogous to the flow of central charge in Zamolodchikov's diagonal resonance scattering in integrable quantum field theories., Comment: 8 pages, 2 figures

The pairing of two electrons on a Fermi surface due to an infinitesimal attraction between them always results in a superconducting instability at zero temperature ($T=0$). The equivalent question of pairing instability on a Luttinger surface (LS) -- a contour of zeros of the propagator -- instead leads to a quantum critical point (QCP) that separates a non-Fermi liquid (NFL) and superconductor. A surprising and little understood aspect of pair fluctuations at this QCP is that their thermodynamics maps to that of the Sachdev-Ye-Kitaev (SYK) model in the strong coupling limit. Here, we offer a simple justification for this mapping by demonstrating that (i) LS models share the reparametrization symmetry of the $q\rightarrow \infty$ SYK model with $q$-body interactions \textcolor{black}{close to the LS}, and (ii) the enforcement of gauge invariance results in a $\frac{1}{\sqrt{\tau}}$ ($\tau\sim T^{-1}$) behavior of the fluctuation propagator near the QCP, as is a feature of the fundamental SYK fermion., Comment: 7+ pages, 3 figures

We employ Momentum-Resolved Electron Energy Loss Spectroscopy (M-EELS) on Bi2.1Sr1.9CaCu2O8+x to resolve the issue of the kink feature in the electron dispersion widely observed in the cuprates. To this end, we utilize the GW approximation to relate the density response function measured in in M-EELS to the self-energy, isolating contributions from phonons, electrons, and the momentum dependence of the effective interaction to the decay rates. The phononic contributions, present in the M-EELS spectra due to electron-phonon coupling, lead to kink features in the corresponding single-particle spectra at energies between 40 meV and 80 meV, independent of the doping level. We find that a repulsive interaction constant in momentum space is able to yield the kink attributed to phonons in ARPES. Hence, our analysis of the M-EELS spectra points to local repulsive interactions as a factor that enhances the spectroscopic signatures of electron-phonon coupling in cuprates. We conclude that the strength of the kink feature in cuprates is determined by the combined action of electron-phonon coupling and electron-electron interactions.

Electron-phonon superconductors at high pressures have displayed the highest values of critical superconducting temperature $T_c$ on record, now rapidly approaching room temperature. Despite the importance of high-$P$ superconductivity in the quest for room-temperature superconductors, a mechanistic understanding of the effect of pressure and its complex interplay with phonon anharmonicity and superconductivity is missing, as numerical simulations can only bring system-specific details clouding out key players controlling the physics. Here we develop a minimal model of electron-phonon superconductivity under an applied pressure which takes into account the anharmonic decoherence of the optical phonons. We find that $T_c$ behaves non-monotonically as a function of the ratio $\Gamma/\omega_0$, where $\Gamma$ is the optical phonon damping and $\omega_0$ the optical phonon energy at zero pressure and momentum. Optimal pairing occurs for a critical ratio $\Gamma/\omega_0$ when the phonons are on the verge of decoherence ("diffuson-like" limit). Our framework gives insights into recent experimental observations of $T_c$ as a function of pressure in the complex BCS material TlInTe$_2$.

Bogoliubov Fermi surfaces (BFSs) are topologically protected regions of zero energy excitations in a superconductor whose dimension equals that of the underlying normal state Fermi surface. Examples of Hamiltonians exhibiting this "ultranodal" phase are known to preserve charge-conjugation ($C$) and parity ($P$) but break time-reversal ($T$). In this work, we provide examples of model Hamiltonians that do not necessarily preserve this symmetry pattern but have well-defined sign-changing Pfaffians yielding BFSs. While their topological character has not been recognized previously, some of the models we present have been extensively studied in prior literature. We further examine thermodynamic and electronic properties arising from the ultranodal state. In particular, we study the effect of a weak Zeeman field close to the topological transition and propose distinguishing features of BFSs using residual specific heat and tunneling conductance. Our calculation of the superfluid density in a toy multi-band model indicates a window of interband pairing strength where BFSs are stable with a positive superfluid density. We also present additional signatures of BFSs in spin-polarized spectral weight and total magnetization measurements., Comment: 13 pages, 8 figures

A theory of superconductivity is presented where the effect of anharmonicity, as entailed in the acoustic, or optical, phonon damping, is explicitly considered in the pairing mechanism. The gap equation is solved including diffusive Akhiezer damping for longitudinal acoustic phonons or Klemens damping for optical phonons, with a damping coefficient which, in either case, can be directly related to the Gruneisen parameter and hence to the anharmonic coefficients in the interatomic potential. The results show that the increase of anharmonicity has a strikingly non-monotonic effect on the critical temperature $T_{c}$. The optimal damping coefficient yielding maximum $T_c$ is set by the velocity of the bosonic mediator. This theory may open up unprecedented opportunities for material design where $T_{c}$ may be tuned via the anharmonicity of the interatomic potential, and presents implications for the superconductivity in the recently discovered hydrides, where anharmonicity is very strong and for which the anharmonic damping is especially relevant., Comment: v2: matching the published version

A theory of phonon-mediated superconductivity in strong-coupling amorphous materials is developed based on an effective description of structural disorder and its effect on the vibrational spectrum. The theory accounts for the diffusive-like transport of vibrational excitations due to disorder-induced scattering within the Eliashberg theory of strong-coupling superconductivity. The theory provides a good analytical description of the Eliashberg function $\alpha^{2}F(\omega)$ in comparison with experiments, and allows one to disentangle the effects of transverse and longitudinal excitations on the Eliashberg function. In particular, it shows that the transverse excitations play a crucial role in driving an increase or excess in the Eliashberg function at low energy, which is related to the boson peak phenomenon in vibrational spectra of glasses. This low-energy excess, on one hand drives an enhancement of the electron-phonon coupling but at the same time reduces the characteristic energy scale $\omega_{log}$ in the Allen-Dynes formula. As a consequence, the non-monotonicity of $T_{c}$ as a function of alloying (disorder) in $\text{Pb}$-based systems can be rationalized. The case of $\text{Al}$-based systems, where disorder increases $T_{c}$ from the start, is also analyzed. General material-design principles for enhancing $T_{c}$ in amorphous superconductors are presented., Comment: matching the final version published in PRB

Superconductivity results from an instability of the Fermi surface -- contour of \textit{poles} of the single particle propagator -- to an infinitesimally small attraction between electrons. Here, we instead discuss the analogous problem on a model \textit{Luttinger} surface, or contour of \textit{zeros} of the Green function. At zero temperature ($\beta \rightarrow \infty$) and a critical interaction strength ($u_{c\infty}$) characterized by the residue of self-energy pole, we find that the pair susceptibility diverges leading to a superconducting instability. We evaluate the pair fluctuation partition function and find that the spectral density in the normal state has an interaction-driven, power-law $\frac{1}{\sqrt{\omega}}$ type, van-Hove singularity (vHS) indicating non-Fermi liquid (NFL) physics. Crucially, in the strong coupling limit ($\beta u \gg 1$), the leading order fluctuation free energy terms in the normal state of this NFL-SC transition resemble the equivalent $\left(O(1)\right)$ terms of the Sachdev-Ye-Kitaev (SYK) model. This free energy contribution takes a simple form $-\beta F = \beta u_{c\infty} - \gamma~\text{ln}\left(\beta u_{c \infty}\right)$ where $\gamma$ is a constant equal to $\frac{1}{2}$. Weak impurity scattering ($\tau \gg \beta^{-1}$) leaves the low-energy spectral density unaffected, but leads to an interaction-driven enhancement of superconductivity. Our results shed light on the role played by order-parameter fluctuations in providing the key missing link between Mott physics and strongly coupled toy-models exhibiting gravity duals., Comment: 16 pages, 6 figures including Appendices

Bogoliubov Fermi surfaces are contours of zero-energy excitations that are protected in the superconducting state. Here we show that multiband superconductors with dominant spin singlet, intraband pairing of spin-1/2 electrons can undergo a transition to a state with Bogoliubov Fermi surfaces if spin-orbit coupling, interband pairing and time reversal symmetry breaking are also present. These latter effects may be small, but drive the transition to the topological state for appropriate nodal structure of the intra-band pair. Such a state should display nonzero zero-bias density of states and corresponding residual Sommerfeld coefficient as for a disordered nodal superconductor, but occurring even in the pure case. We present a model appropriate for iron-based superconductors where the topological transition associated with creation of a Bogoliubov Fermi surface can be studied. The model gives results that strongly resemble experiments on FeSe$_{1-x}$S$_x$ across the nematic transition, where this ultranodal behavior may already have been observed., Comment: 7 pages, 2 figures

With substantial evidence of glassy behavior in the phase diagram of high $T_c$ superconductors and its co-existence with superconductivity, we attempt to answer the question: what are the properties of a superconducting state where the force driving cooper pairing becomes dissipative? We find that when the bosonic mediator is local, dissipation acts to reduce the superconducting critical temperature ($T_c$). On the other hand, contrary to na\"{i}ve expectations, $T_c$ behaves non-monotonically with dissipation for a non-local mediator -- weakly dissipative bosons at different energy scales act coherently to give rise to an increase in $T_c$ and eventually destroy superconductivity when the dissipation exceeds a critical value. The critical value occurs when dissipative effects become comparable to the energy scale associated with the spatial stiffness of the mediator, at which point, $T_c$ acquires a maximum. We outline consequences of our results to recent proton irradiation experiments (M. Leroux et al.,~\cite{Welp2018}) on the cuprate superconductor La$_{2-x}$Ba$_x$CuO$_4$ (LBCO) which observe a disorder induced increase in $T_c$ even when the transition temperature of the proximate charge density wave (CDW) is unaffected by the presence of irradiation. Our mechanism is a novel way to raise $T_c$ that does not require a `tug-of-war' -type scenario between two competing phases., Comment: 3 figures, 6 pages

We study an anisotropic holographic bottom-up model displaying a quantum phase transition (QPT) between a topologically trivial insulator and a non-trivial Weyl semimetal phase. We analyze the properties of quantum chaos in the quantum critical region. We do not find any universal property of the Butterfly velocity across the QPT. In particular it turns out to be either maximized or minimized at the quantum critical point depending on the direction of propagation. We observe that instead of the butterfly velocity, it is the dimensionless information screening length that is always maximized at a quantum critical point. We argue that the null-energy condition (NEC) is the underlying reason for the upper bound, which now is just a simple combination of the number of spatial dimensions and the anisotropic scaling parameter., Comment: v1: 24 pages, 9 figures; v2: minor additions in main text and references; v3: minor changes in presentation (jhep version)

We propose a theoretical framework for the detection of order parameter fluctuations in three dimensions using ultrafast coherent phonon spectroscopy. We focus our attention on long wavelength charge density fluctuations (plasmons), and charged nematic fluctuations where the direction of the propagation vector is fixed perpendicular to the plane of anisotropy. By treating phonons and light classically and decoupling interactions to integrate out the fermionic degrees of freedom, we arrive at an effective theory of order parameter fluctuations about the spatially uniform saddle-point solution. We find that, due to the $(k_x^2-k_y^2) (B_{1g})$ symmetry of the form factor appearing in the vertex, nematic fluctuations couple to light only at fourth order, unlike isotropic density fluctuations which couple at second order. Hence, to lowest order, the interaction between electrons and the electromagnetic field contributes a driving force for plasmon oscillations while it provides a frequency shift for nematic fluctuations. From the resulting coupled harmonic oscillator equations of motion, we argue that ultrafast coherent phonon spectroscopy could be a useful tool to extract and analyze various electronic properties of interest such as the frequency of the collective mode and the coupling between electrons and phonons. Specific experiments are proposed on the normal state of FeSe to observe the frequency shift predicted here resulting directly from orbital ordering (nematic) fluctuations. Our paper presents a new mechanism for generating coherent phonons from long-range interactions (coherent long-range interaction induced phonons) that does not require the existence of multiple bands to act as intermediary states for quasiparticles., Comment: 13 pages, 4 figures

Recent photoemission spectroscopy measurements (T. J. Reber et al., arXiv:1509.01611) of cuprate superconductors have inferred that the self-energy exhibits critical scaling over an extended doping regime, thereby calling into question the conventional wisdom that critical scaling exists only at isolated points. In particular, this new state of matter, dubbed a power-law liquid, has a self-energy whose imaginary part scales as $\Sigma^{\prime\prime}\sim(\omega^{2}+\pi^{2}T^{2})^{\alpha}$, with $\alpha=1$ in the overdoped Fermi-liquid state and $\alpha\leq0.5$ in the optimal to underdoped regime. Previously, we showed that this self-energy can arise from interactions between electrons and unparticles, a scale-invariant sector that naturally emerges from strong correlations. Here, taking the self-energy as a given, we first reconstruct the real part of the self-energy. We find that the resultant quasiparticle weight vanishes for any doping level less than optimal, implying an absence of particle-like excitations in the underdoped regime. Consequently, the Fermi velocity vanishes and the effective mass diverges for $\alpha\leq\frac{1}{2}$, in agreement with earlier experimental observations. We then use the self-energy to reconstruct the spectral function and compute the superconducting $T_c$ within the BCS formalism. We find that the $T_c$ has a dome-like structure, implying that broad scale invariance manifested in the form of a power-law liquid is the likely cause of the superconducting dome in the cuprates., Comment: 9 pages, 6 figures. to be published in Phys. Rev. B

We devise a model to explain why twisted bi-layer graphene (TBLG) exhibits insulating behavior when $\nu=2,3$ charges occupy a unit moir\'e cell, a feature attributed to Mottness, but not for $\nu=1$, clearly inconsistent with Mott insulation. We compute $r_s=E_U/E_K$, where $E_U$ and $E_K$ are the potential and kinetic energies, respectively, and show that (i) the Mott criterion lies at a density $10^4$ higher than in the experiments and (ii) a transition to a series of Wigner crystalline states exists as a function of $\nu$. We find, for $\nu=1$, $r_s$ fails to cross the threshold ($r_s = 37$) for the triangular lattice and metallic transport ensues. However, for $\nu=2$ and $\nu=3$, the thresholds, $r_s=22$, and $r_s=17$, respectively are satisfied for a transition to Wigner crystals (WCs) with a honeycomb ($\nu=2$) and kagome ($\nu=3$) structure. We believe, such crystalline states form the correct starting point for analyzing superconductivity., Comment: Version accepted in Nano Letters

We address the question of the mismatch between the zero momentum limits of the transverse and longitudinal dielectric functions for a fixed direction of the driving field observed in the cuprates. This question translates to whether or not the order in which the longitudinal and transverse momentum transfers are taken to zero commute. While the two limits commute for both isotropic and anisotropic Drude metals, we argue that a scaleless vertex interaction that depends solely on the angle between scattered electron momenta is sufficient to achieve non-commutativity of the two limits even for a system that is inherently isotropic. We demonstrate this claim for a simple case of the Drude conductivity modified by electron-boson interactions through appropriate vertex corrections, and outline possible consequences of our result to optical and electron energy loss spectroscopy (EELS) measurements close to zero momentum transfer, Comment: 7 pages, 1 figure including Supplemental Material

We study a single-channel Kondo effect using a recently developed holographic large-$N$ technique. In order to obtain resistivity of this model, we introduce a probe field. The gravity dual of a localized fermionic impurity in 1+1-dimensional host matter is constructed by embedding a localized 2-dimensional Anti-de Sitter (\ads{2})-brane in the bulk of \ads{3}. This helps us construct an impurity charge density which acts as a source to the bulk equation of motion of the probe gauge field. The functional form of the charge density is obtained independently by solving the equations of motion for the fields confined to the \ads{2}-brane. The asymptotic solution of the probe field is dictated by the impurity charge density, which in turn, affects the current-current correlation functions, and hence the resistivity. Our choice of parameters tunes the near-boundary impurity current to be marginal, resulting in a $\log T$ behavior in the UV resistivity, as is expected for the Kondo problem. The resistivity at the IR fixed point turns out to be zero, signaling a complete screening of the impurity., Comment: v2: 15 pages, typos corrected, few more clarifications added

Motivated by recent bounds for charge diffusion in critical matter, we investigate the question: What sets the scale for charge diffusion in a scale-invariant system? To make our statements precise, we analyze the diffusion pole in an exactly solvable model for a Mott transition in the presence of a long-range interaction term. To achieve scale invariance, we limit our discussion to the flat-band regime. We find in this limit that the diffusion pole which would normally obtain at finite energy is pushed to zero energy resulting in a vanishing of the diffusion constant. This occurs even in the presence of interactions in certain limits, indicating the robustness of this result to the inclusion of a scale in the problem. Consequently, scale-invariance precludes any reasonable definition of the diffusion constant. Nonetheless, we do find that a scale can be defined, all be it, irrelevant to diffusion, which is the product of the squared band velocity and the density of states., Comment: 9 pages including appendices, 1 figure

Recent photoemission spectroscopy measurements [arXiv:1509.01611] on cuprate superconductors have inferred that over a wide range of doping, the imaginary part of the electron self-energy scales as $\Sigma^{\prime\prime}\sim(\omega^2+\pi^2T^2)^a$ with $a=1$ in the overdoped Fermi-liquid state and $a<0.5$ in the optimal to underdoped regime. We show that this non-Fermi-liquid scaling behavior can naturally be explained by the presence of a scale-invariant state of matter known as unparticles. We evaluate analytically the electron self-energy due to interactions with fermionic unparticles. We find that, in agreement with experiments, the imaginary part of the self-energy scales with respect to temperature and energy as $\Sigma^{\prime\prime}\sim T^{2+2\alpha}$ and $\omega^{2+2\alpha}$, where $\alpha$ is the anomalous dimension of the unparticle propagator. In addition, the calculated occupancy and susceptibility of fermionic unparticles, unlike those of normal fermions, have significant spectral weights even at high energies. This unconventional behavior is attributed to the branch cut in the unparticle propagator which broadens the unparticle spectral function over a wide energy range and non-trivially alters the scattering phase space by enhancing (suppressing) the intrinsic susceptibility at low energies for negative (positive) $\alpha$. Our work presents new evidence suggesting that unparticles might be important low-energy degrees of freedom in strongly coupled systems such as the cuprate superconductors., Comment: 10 pages, 7 figures

Recent AC susceptibility and polar Kerr effect measurements in the skutterudite superconductor PrOs4Sb12 (POS) uncovered the nature of the superconducting double transition from a high temperature, high field, time reversal symmetric phase (or the A phase) to a low temperature, low field, time reversal symmetry broken phase (or the B phase). Starting from a microscopic model, we derive a Ginzburg-Landau expansion relevant to POS that describes this entrance into the time reversal symmetry broken phase along the temperature axis. We also provide a study of the low energy inelastic (Raman) response in both the A and B phases of POS, and seek additional signatures which could help reveal the exact form of the gap functions previously proposed in these phases. By appropriately manipulating the incoming and scattered light geometries, along with additional subtraction procedures and suitable assumptions, we show that one can access the various irreducible representations contained in the point group describing POS. We demonstrate how to use this technique on example order parameters proposed in POS. Depending on whether there exist nodes along the c-axis, we find additional low energy spectral weight within the superconducting gap in the Eg geometry, a feature that could pin point the location of nodes on the Fermi surface., Comment: 14 pages and 10 figures including the Appendix

We study impurity scattering in the normal and d-wave superconducting states of line nodal semimetals and show that, due to additional scattering phase space available for impurities on the surface, the quasiparticle interference pattern acquires an extended character instead of a discrete collection of delta function peaks. Moreover, using the T-matrix formalism, we demonstrate that the conventional behavior of a scalar impurity in a d-wave superconductor breaks down on the surface of a line nodal semimetal in the quasi flat band limit., Comment: 11 pages,7 figures including Supplemental Material

Recent neutron scattering observations by Plumb et al. [1] reveal that the ground state of $FeSc_2S_4$ is magnetic with two distinct Fe environments, instead of a quantum spin liquid as had been previously thought. Starting with the relevant O(N)-symmetric vector model of $FeSc_2S_4$, we study how the discrete ($Z_2$) and continuous rotational symmetries are successively broken, yielding nematic and ordered phases. At high temperatures, we find that the nematic order parameter falls as $T^{-\gamma}$ ($\gamma>0$), and therefore, $FeSc_2S_4$ lacks any distinct nematic ordering temperature. This feature indicates that the three-dimensional diamond lattice of $FeSc_2S_4$ is highly susceptible to the breaking of Ising symmetries, and explains the two distinct Fe environments that is present even at high temperatures, as seen by M\"ossbauer and far infrared optical spectroscopy., Comment: 9 pages with Supplemental Material, 5 figures