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Spontaneous symmetry breaking (SSB) is crucial to the occurrence of phase transitions. Once a phase transition occurs, a quantum system presents degenerate eigenstates that lack the symmetry of the Hamiltonian. After crossing the critical point, the system is essentially evolved to a quantum superposition of these eigenstates until decoherence sets in. Despite the fundamental importance and potential applications in quantum technologies, such quantum-mechanical SSB phenomena have not been experimentally explored in many-body systems. We here present an experimental demonstration of the SSB process in the Lipkin-Meshkov-Glick model, governed by the competition between the individual driving and intra-qubit interaction. The model is realized in a circuit quantum electrodynamics system, where 6 Xmon qubits are coupled in an all-to-all manner through virtual photon exchange mediated by a resonator. The observed nonclassical correlations among these qubits in the symmetry-breaking region go beyond the conventional description of SSB, shedding new light on phase transitions for quantum many-body systems., Comment: 27 pages, 18 figures

We propose a scheme for measuring topological properties in a two-photon-driven Kerr-nonlinear resonator (KNR) subjected to a single-photon modulation. The topological properties are revealed through the observation of the Berry curvature and hence the first Chern number, as a nonadiabatic response of the physical observable to the change rate of the control parameter of the modulated drive. The parameter manifold, constructed from the system's Hamiltonian that determines its dynamics constrained in the state space spanned by the even and odd cat states as two basis states, is adjusted so that the degeneracy crossing the manifold indicates a topological transition. The scheme, with such continuous variable states in mesoscpic systems, provides a new perspective for exploration of the geometry and the related topology with complex systems.

To account for neutrino oscillations, it is postulated that the neutrino has nonvanishing mass and each flavor eigenstate is formed by three distinct mass eigenstates, whose probability amplitudes interfere with each other during its propagation. However, I find that the energy conservation law requires these mass eigenstates, if they exist, to be entangled with distinct joint energy eigenstates of the other particles produced by the same weak interaction as the neutrino. This entanglement destroys the quantum coherence among the neutrino's mass eigenstates, which is responsible for flavor oscillations under the aforementioned postulation. I reveal that the neutrino oscillations actually originate from virtual excitation of the Z bosonic field diffusing over the space. During the propagation, the neutrino can continually excite and then immediately re-absorb a virtual Z boson. This virtual bosonic excitation produces a backaction on the neutrino, enabling it to oscillate among three flavors. When the neutrino propagates in matter, its behavior is determined by the competition between the coherent flavor transformation and decoherence effect resulting from scatterings.

The environment-induced dissipation of an open system, once thought as a nuisance, can actually lead to emergence of many intriguing phenomena that are absent in an isolated system. Among these, Weyl exceptional rings (WER), extended from point-like singularities, are particularly interesting. Theoretically, a WER was predicted to carry a topological charge with a nonzero Chern number, but it has not been measured so far. We here investigate this topology in a circuit, where the WER is synthesized with a superconducting qubit controllably coupled to a decaying resonator. The high flexibility of the system enables us to characterize its eigenvectors on different manifolds of parameter space. We extract both the quantized Berry phase and Chern number from these eigenvectors. Furthermore, we demonstrate a topological transition triggered by shrinking the size of the manifold$-$a unique feature of the WER., Comment: 16 pages, 10 figures

Spontaneous symmetry breaking (SSB) plays a central role in understanding a large variety of phenomena associated with phase transitions, such as superfluid and superconductivity. So far, the transition from a symmetric vacuum to a macroscopically ordered phase has been substantially explored. The process bridging these two distinct phases is critical to understanding how a classical world emerges from a quantum phase transition, but so far remains unexplored in experiment. We here report an experimental demonstration of such a process with a quantum Rabi model engineered with a superconducting circuit. We move the system from the normal phase to the superradiant phase featuring two symmetry-breaking field components, one of which is observed to emerge as the classical reality. The results demonstrate that the environment-induced decoherence plays a critical role in the SSB., Comment: 13 pages,9 figures

Critical systems near quantum phase transitions were predicted to be useful for improvement of metrological precision, thanks to their ultra-sensitive response to a tiny variation of the control Hamiltonian. Despite the promising perspective, realization of criticality-enhanced quantum metrology is an experimentally challenging task, mainly owing to the extremely long time needed to encode the signal to some physical quantity of a critical system. We here circumvent this problem by making use of the critical behaviors in the Jaynes-Cummings model, comprising a single qubit and a photonic resonator, to which the signal field is coupled. The information about the field amplitude is encoded in the qubit's excitation number in the dark state, which displays a divergent changing rate at the critical point. The most remarkable feature of this critical sensor is that the performance is insensitive to the leakage to bright eigenstates, caused by decoherence and non-adiabatic effects. We demonstrate such a metrological protocol in a superconducting circuit, where an Xmon qubit, interacting with a resonator, is used as a probe for estimating the amplitude of a microwave field coupled to the resonator. The measured quantum Fisher information exhibits a critical quantum enhancement, confirming the potential of this system for quantum metrology., Comment: 13 pages, 11 figures

Understanding the dynamical behavior of a qubit in a reservoir is critical to applications in quantum technological protocols, ranging from quantum computation to quantum metrology. The effect of the reservoir depends on reservoir's spectral structure, as well as on the qubit-reservoir coupling strength. We here propose a measure for quantifying the non-Markovian effect of a reservoir with a Lorentzian spectrum, based on the maximum qubit-reservoir quantum entanglement that can be extracted. Numerical simulation shows this entanglement exhibits a monotonous behavior in response to the variation of the coupling strength. We confirm the validity of this measure with an experiment, where a superconducting qubit is controllably coupled to a lossy resonator, which acts as a reservoir for the qubit. The experimental results illustrate the maximal extractable entanglement is progressively increased with the strengthening of the non-Markovianity.

Owing to the presence of exceptional points (EPs), non-Hermitian (NH) systems can display intriguing topological phenomena without Hermitian analogs. However, experimental characteristics of exceptional topological invariants have been restricted to second-order EPs (EP2s) in classical or semiclassical systems. We here propose an NH multi-qubit model with higher-order EPs, each of which is underlain by a multifold-degenerate multipartite entangled eigenstate. We implement the three-qubit model by controllably coupling a superconducting qubit to two microwave resonators, one serving as a Hermitian photonic qubit while the other as an NH qubit. We experimentally quantify the topological invariant for an EP3, by mapping out the complex eigenspectra along a loop surrounding this EP3 in the parameter space. The nonclassicality of the realized topology is manifested by the observed quantum correlations in the corresponding eigenstates. Our results extend research of exceptional topology to fully quantum-mechanical models with multi-partite entangled eigenstates. We further demonstrate the non-reciprocal transmission of a single photon, during which the photon is nonlocally shared by three individual elements.

Quantum operations by utilizing the underlying geometric phases produced in physical systems are favoured due to its potential robustness. When a system in a non-degenerate eigenstate undergoes an adiabatically cyclic evolution dominated by its Hamiltonian, it will get a geometric phase, referred to as the Berry Phase. While a non-adiabatically cyclic evolution produces an Aharonov-Anandan geometric phase. The two types of Abelian geometric phases are extended to the non-Abelian cases, where the phase factors become matrix-valued and the transformations associated with different loops are non-commutable. Abelian and non-Abelian (holonomic) operations are prevalent in discrete variable systems, whose limited (say, two) energy levels, form the qubit. While their developments in continuous systems have also been investigated, mainly due to that, bosonic modes (in, such as, cat states) with large Hilbert spaces, provide potential advantages in fault-tolerant quantum computation. Here we propose a feasible scheme to realize non-adiabatic holonomic quantum logic operations in continuous variable systems with cat codes. We construct arbitrary single-qubit (two-qubit) gates with the combination of single- and two-photon drivings applied to a Kerr Parametric Oscillator (KPO) (the coupled KPOs). Our scheme relaxes the requirements of the previously proposed quantum geometric operation strategies in continuous variable systems, providing an effective way for quantum control.

Parametrically driven nonlinear resonators represent a building block for realizing fault-tolerant quantum computation and are useful for critical quantum sensing. From a fundamental viewpoint, the most intriguing feature of such a system is perhaps the critical phenomena, which can occur without interaction with any other quantum system. The non-analytic behaviors of its eigenspectrum have been substantially investigated, but those associated with the ground state wavefunction have largely remained unexplored. Using the quantum ground state geometric tensor as an indicator, we comprehensively establish a phase diagram involving the driving parameter $\varepsilon$ and phase $\phi$. The results reveal that with the increase in $\varepsilon$, the system undergoes a quantum phase transition from the normal to the superradiant phase, with the critical point unaffected by $\phi$. Furthermore, the critical exponent and scaling dimension are obtained by an exact numerical method, which is consistent with previous works. Our numerical results show that the phase transition falls within the universality class of the quantum Rabi model. This work reveals that the quantum metric and Berry curvature display diverging behaviors across the quantum phase transition., Comment: Any comments or suggestions are welcome !

We study the quantum metric in a driven Tavis-Cummings model, comprised of multiple qubits interacting with a quantized photonic field. The parametrical driving of the photonic field breaks the system's U(1) symmetry down to a ${\rm Z}_2$ symmetry, whose spontaneous breaking initiates a superradiant phase transition. We analytically solved the eigenenergies and eigenstates, and numerically simulated the system behaviors near the critical point. The critical behaviors near the superradiant phase transition are characterized by the quantum metric, defined in terms of the response of the quantum state to variation of the control parameter. In addition, a quantum metrological protocol based on the critical behaviors of the quantum metric near the superradiant phase transition is proposed, which enables greatly the achievable measurement precision., Comment: 13 pages, 5 figures

Critical phenomena of quantum systems are useful for enhancement of quantum sensing. However, experimental realizations of criticality enhancement have been confined to very few systems, owing to the stringent requirements, including the thermodynamical or scaling limit, and fine control of interacting quantum susystems or particles. We here propose a simple critical quantum sensing scheme that requires neither of these conditions. The critical system is realized with a single parametrically-driven bosonic mode involving many non-interacting bosons. We calculate the quantum Fisher information, and perform a simulation, which confirms the criticality-enabled enhancement. We further detail the response of one of the quadratures to the variation of the control parameter. The numerical results reveal that its inverted variance exhibits a diverging behavior at the critical point. Based on the presently available control techniques of parametric driving, we expect our scheme can be realized in different systems, e.g., ion traps and superconducting circuits., Comment: 6 pages, 4 figures

Quantum systems that undergo quantum phase transitions exhibit divergent susceptibility and can be exploited as probes to estimate physical parameters. We generalize the dynamic framework for criticality-enhanced quantum sensing by the quantum Rabi model (QRM) to its anisotropic counterpart and derive the correspondingly analytical expressions for the quantum Fisher information (QFI). We find that the contributions of the rotating-wave and counterrotating-wave interaction terms are symmetric at the limit of the infinite ratio of qubit frequency to field frequency, with the QFI reaching a maximum for the isotropic quantum Rabi model. At finite frequency scaling, we analytically derive the inverted variance of higher-order correction and find that it is more affected by the rotating-wave coupling than by the counterrotating-wave coupling.

Quantum sensing improves the accuracy of measurements of relevant parameters by exploiting the unique properties of quantum systems. The divergent susceptibility of physical systems near a critical point for quantum phase transition enables criticality-enhanced quantum sensing. The quantum Rabi model (QRM), composed of a single qubit coupled to a single bosonic field, represents a good candidate for realizing such critical enhancement for its simplicity, but it is experimentally challenging to achieve the ultrastrong qubit-field coupling required to realize the critical phenomena. In this work, we explore an alternative to construct the analog of the QRM for the sensing, exploiting the criticality appearing in the Jaynes-Cummings (JC) model whose bosonic field is parametrically driven, not necessitating the ultrastrong coupling condition thus to some extent relaxing the requirement for the practical implementation., Comment: 8 pages, 4 figures

Although originally predicted in relativistic quantum mechanics, Zitterbewegung can also appear in some classical systems, which leads to the important question of whether Zitterbewegung of Dirac particles is underlain by a more fundamental and universal interference behavior without classical analogs. We here reveal such an interference pattern in phase space, which underlies but goes beyond Zitterbewegung, and whose nonclassicality is manifested by the negativity of the phase space quasiprobability distribution, and the associated pseudospin-momentum entanglement. We confirm this discovery by numerical simulation and an on-chip experiment, where a superconducting qubit and a quantized microwave field respectively emulate the internal and external degrees of freedom of a Dirac particle. The measured quasiprobability negativities agree well with the numerical simulation. Besides being of fundamental importance, the demonstrated nonclassical effects are useful in quantum technology., Comment: 20 pages, 15 figures

Quantum error correction (QEC) aims to protect logical qubits from noises by utilizing the redundancy of a large Hilbert space, where an error, once it occurs, can be detected and corrected in real time. In most QEC codes, a logical qubit is encoded in some discrete variables, e.g., photon numbers. Such encoding schemes make the codewords orthogonal, so that the encoded quantum information can be unambiguously extracted after processing. Based on such discrete-variable encodings, repetitive QEC demonstrations have been reported on various platforms, but there the lifetime of the encoded logical qubit is still shorter than that of the best available physical qubit in the entire system, which represents a break-even point that needs to be surpassed for any QEC code to be of practical use. Here we demonstrate a QEC procedure with a logical qubit encoded in photon-number states of a microwave cavity, dispersively coupled to an ancilla superconducting qubit. By applying a pulse featuring a tailored frequency comb to the ancilla, we can repetitively extract the error syndrome with high fidelity and perform error correction with feedback control accordingly, thereby exceeding the break-even point by about 16% lifetime enhancement. Our work illustrates the potential of the hardware-efficient discrete-variable QEC codes towards a reliable quantum information processor., Comment: Main text: 8 pages, 3 figures, 1 table; Supplement: 12 pages, 8 figures, 2 tables

Non-Hermitian (NH) extension of quantum-mechanical Hamiltonians represents one of the most significant advancements in physics. During the past two decades, numerous captivating NH phenomena have been revealed and demonstrated, but all of which can appear in both quantum and classical systems. This leads to the fundamental question: what NH signature presents a radical departure from classical physics? The solution of this problem is indispensable for exploring genuine NH quantum mechanics, but remains experimentally untouched so far. Here, we resolve this basic issue by unveiling distinct exceptional entanglement phenomena, exemplified by an entanglement transition, occurring at the exceptional point of NH interacting quantum systems. We illustrate and demonstrate such purely quantum-mechanical NH effects with a naturally dissipative light-matter system, engineered in a circuit quantum electrodynamics architecture. Our results lay the foundation for studies of genuinely quantum-mechanical NH physics, signified by exceptional-point-enabled entanglement behaviors.

The experimental observation of quantum phase transitions predicted by the quantum Rabi model in quantum critical systems is usually challenging due to the lack of signature experimental observables associated with them. Here, we describe a method to identify the dynamical critical phenomenon in the quantum Rabi model consisting of a three-level atom and a cavity at the quantum phase transition. Such a critical phenomenon manifests itself as a sudden change of steady-state output photons in the system driven by two classical fields, when both the atom and the cavity are initially unexcited. The process occurs as the high-frequency pump field is converted into the low-frequency Stokes field and multiple cavity photons in the normal phase, while this conversion cannot occur in the superradiant phase. The sudden change of steady-state output photons is an experimentally accessible measure to probe quantum phase transitions, as it does not require preparing the equilibrium state., Comment: has been published in Communcations Physics as a regular article

Superradiant phase transitions (SPTs) are important for understanding light-matter interactions at the quantum level, and play a central role in criticality-enhanced quantum sensing. So far, SPTs have been observed in driven-dissipative systems, but the emergent light fields did not show any nonclassical characteristic due to the presence of strong dissipation. Here we report an experimental demonstration of the SPT featuring the emergence of a highly nonclassical photonic field, realized with a resonator coupled to a superconducting qubit, implementing the quantum Rabi model. We fully characterize the light-matter state by Wigner matrix tomography. The measured matrix elements exhibit quantum interference intrinsic of a photonic mesoscopic superposition, and reveal light-matter entanglement, Comment: 20 pages, 19 figures, 2 tables

Quantum entanglement between an interfering particle and a detector for acquiring the which-path information plays a central role for enforcing Bohr's complementarity principle. However, the quantitative relation between this entanglement and the fringe visibility remains untouched upon for an initial mixed state. Here we find an equality for quantifying this relation. Our equality characterizes how well the interference pattern can be preserved when an interfering particle, initially carrying a definite amount of coherence, is entangled, to a certain degree, with a which-path detector. This equality provides a connection between entanglement and interference in the unified framework of coherence, revealing the quantitative entanglement-interference complementarity. We experimentally demonstrate this relation with a superconducting circuit, where a resonator serves as a which-path detector for an interfering qubit. The measured fringe visibility of the qubit's Ramsey signal and the qubit-resonator entanglement exhibit a complementary relation, in well agreement with the theoretical prediction., Comment: 19 pages, 9 figures, 1 table

In this work, we propose a composite pulses scheme by modulating phases to achieve high fidelity population transfer in three-level systems. To circumvent the obstacle that not enough variables are exploited to eliminate the systematic errors in the transition probability, we put forward a cost function to find the optimal value. The cost function is independently constructed either in ensuring an accurate population of the target state, or in suppressing the population of the leakage state, or both of them. The results demonstrate that population transfer is implemented with high fidelity even when existing the deviations in the coupling coefficients. Furthermore, our composite pulses scheme can be extensible to arbitrarily long pulse sequences. As an example, we employ the composite pulses sequence for achieving the three-atom singlet state in an atom-cavity system with ultrahigh fidelity. The final singlet state shows robustness against deviations and is not seriously affected by waveform distortions. Also, the singlet state maintains a high fidelity under the decoherence environment., Comment: 20 pages, 13 figures

Quantum key distribution (QKD) provides an information-theoretically secure method to share keys between legitimate users. To achieve large-scale deployment of QKD, it should be easily scalable and cost-effective. The infrastructure construction of quantum access network (QAN) expands network capacity and the integration between QKD and classical optical communications reduces the cost of channel. Here, we present a practical downstream QAN over a 10 Gbit/s Ethernet passive optical network (10G-EPON), which can support up to 64 users. In the full coexistence scheme using the single feeder fiber structure, the co-propagation of QAN and 10G-EPON signals with 9 dB attenuation is achieved over 21 km fiber, and the secure key rate for each of 16 users reaches 1.5 kbps. In the partial coexistence scheme using the dual feeder fiber structure, the combination of QAN and full-power 10G-EPON signals is achieved over 11 km with a network capacity of 64-user. The practical QAN over the 10G-EPON in our work implements an important step towards the achievement of large-scale QKD infrastructure., Comment: 9 pages, 4 figures. Accepted for publication in Optics Express

We propose a Rydberg molecule dressing scheme to create strong and long-ranged interactions at selective distances. This is achieved through laser coupling ground-state atoms off-resonantly to an attractive molecular curve of two interacting Rydberg atoms. Although dephasing due to Rydberg state decay occurs in all dressing schemes, an advantage of the molecule dressing is that a large ratio of dressed interaction to dephasing rate can be realized at large atomic separations. In an optical lattice or tweezer setting, we show that the strong interaction permits the fast generation of spin squeezing for several tens of dressed atoms. The proposed setting offers a new route to study complex many-body dynamics and to realize quantum information processing with non-convex long-range interactions., Comment: 5 pages, 4 figures. Supplementary Material of 6 pages, 2 figures

Nonreciprocal transmission of optical or microwave signals is indispensable in various applications involving sensitive measurements. In this paper, we study optomechanically induced directional amplification and isolation in a generic setup including two cavities and two mechanical oscillators by exclusively using blue-sideband drive tones. The input and output ports defined by the two cavity modes are coupled through coherent and dissipative paths mediated by the two mechanical resonators, respectively. By choosing appropriate transfer phases and strengths of the driving fields, either a directional amplifier or an isolator can be implemented at low thermal temperature, and both of them show bi-directional nonreciprocity working at two mirrored frequencies. The nonreciprocal device can potentially be demonstrated by opto- and electro-mechanical setups in both optical and microwave domains., Comment: 5 pages, 3 figures

We propose a protocol to realize nonadiabatic geometric quantum computation of small-amplitude Schr\"odinger cat qubits via invariant-based reverse engineering. We consider a system with a two-photon driven Kerr nonlinearity, which provides a pair of dressed even and odd coherent states, i.e., Schr\"odinger cat states for fault-tolerant quantum computations. An additional coherent field is applied to linearly drive a cavity mode, to induce oscillations between dressed cat states. By designing this linear drive with invariant-based reverse engineering, nonadiabatic geometric quantum computation with cat qubits can be implemented. The performance of the protocol is estimated by taking into account the influence of systematic errors, additive white Gaussian noise, and decoherence including photon loss and dephasing. Numerical results demonstrate that our protocol is robust against these negative factors. Therefore, this protocol may provide a feasible method for nonadiabatic geometric quantum computation in bosonic systems., Comment: 13 pages, 8 figures, has been published as a Regular Article in Physical Review Research

Quantum key distribution (QKD) enables secure key exchanges between two remote users. The ultimate goal of secure communication is to establish a global quantum network. The existing field tests suggest that quantum networks are feasible. To achieve a practical quantum network, we need to overcome several challenges, including realising versatile topologies for large scales, simple network maintenance, extendable configuration, and robustness to node failures. To this end, we present a field operation of a quantum metropolitan-area network with 46 nodes and show that all these challenges can be overcome with cutting-edge quantum technologies. In particular, we realise different topological structures and continuously run the network for 31 months, by employing standard equipment for network maintenance with an extendable configuration. We realise QKD pairing and key management with a sophisticated key control center. In this implementation, the final keys have been used for secure communication such as real-time voice telephone, text messaging, and file transmission with one-time pad encryption, which can support 11 pairs of users to make audio calls simultaneously. Combined with inter-city quantum backbone and ground-satellite links, our metropolitan implementation paves the way toward a global quantum network., Comment: 14 pages, 5 figures

We propose a method for the dynamical control in three-level open systems and realize it in the experiment with a superconducting qutrit. Our work demonstrates that in the Markovian environment for a relatively long time (3 us), the systemic populations or coherence can still strictly follow the preset evolution paths. This is the first experiment for precisely controlling the Markovian dynamics of three-level open systems, providing a solid foundation for the future realization of dynamical control in multiple open systems. An instant application of the techniques demonstrated in this experiment is to stabilize the energy of quantum batteries., Comment: 12 pages, 11 figures

Quantum key distribution (QKD) provides information theoretically secures key exchange requiring authentication of the classic data processing channel via pre-sharing of symmetric private keys. In previous studies, the lattice-based post-quantum digital signature algorithm Aigis-Sig, combined with public-key infrastructure (PKI) was used to achieve high-efficiency quantum security authentication of QKD, and its advantages in simplifying the MAN network structure and new user entry were demonstrated. This experiment further integrates the PQC algorithm into the commercial QKD system, the Jinan field metropolitan QKD network comprised of 14 user nodes and 5 optical switching nodes. The feasibility, effectiveness and stability of the post-quantum cryptography (PQC) algorithm and advantages of replacing trusted relays with optical switching brought by PQC authentication large-scale metropolitan area QKD network were verified. QKD with PQC authentication has potential in quantum-secure communications, specifically in metropolitan QKD networks., Comment: 11 pages, 3 figures

In this work, we exploit the idea of composite pulses to achieve robust population inversion in a three-level quantum system. The scheme is based on the modulation of the coupling strength, while the other physical parameters remain unchanged. The composite pulses sequence is designed by vanishing high-order error terms, and can compensate the systematic errors to any desired order. In particular, this scheme keeps a good performance under the disturbance of waveform deformations. This trait ensures that population inversion can be nearly obtained even when the pulse sequence has a short jump delay. As an example, we employ the designed composite pulse sequence to prepare the W state in a robust manner in the superconducting circuits. The numerical results show that the fidelity can still maintain a high level in a decoherence environment., Comment: 19 pages, 9 figures

Quantum key distribution endows people with information-theoretical security in communications. Twin-field quantum key distribution (TF-QKD) has attracted considerable attention because of its outstanding key rates over long distances. Recently, several demonstrations of TF-QKD have been realized. Nevertheless, those experiments are implemented in the laboratory, remaining a critical question about whether the TF-QKD is feasible in real-world circumstances. Here, by adopting the sending-or-not-sending twin-field QKD (SNS-TF-QKD) with the method of actively odd parity pairing (AOPP), we demonstrate a field-test QKD over 428~km deployed commercial fiber and two users are physically separated by about 300~km in a straight line. To this end, we explicitly measure the relevant properties of the deployed fiber and develop a carefully designed system with high stability. The secure key rate we achieved breaks the absolute key rate limit of repeater-less QKD. The result provides a new distance record for the field test of both TF-QKD and all types of fiber-based QKD systems. Our work bridges the gap of QKD between laboratory demonstrations and practical applications, and paves the way for intercity QKD network with high-speed and measurement-device-independent security.