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We demonstrate that chiral response can be achieved in resonant metasurfaces with a monoclinic lattice symmetry (the so-called Bravais oblique lattices) where the mirror symmetry is broken by the lattice asymmetry and also by a substrate, whereas each individual meta-atom remains fully achiral. We describe the underlying physics by introducing a mode chirality parameter as a quantitative measure of the lattice chiral eigenmodes. We confirm experimentally selective linear and nonlinear chiral interaction of resonant silicon metasurfaces with circularly polarized light., Comment: 15 pages, 8 figures, 1 table

Generation of even-order optical harmonics requires noncentrosymmetric structures being conventionally observed in crystals lacking the center of inversion. In centrosymmetric systems, even-order harmonics may arise, e.g., at surfaces but such effects are usually very weak. Here we observe optical harmonics up to 4-th order generated under the normal incidence from centrosymmetric dielectric metasurfaces empowered by resonances. We design silicon metasurfaces supporting optical quasibound states in the continuum and guided-mode resonances, and demonstrate the enhancement of second-harmonic signals by over three orders of magnitude compared to nonresonant thin films. Under the optimal conditions, the brightness of the second harmonic approaches that of the third harmonic, and the 4th-order harmonic becomes detectable.

Distant interactions at arbitrary locations and their dynamic control are fundamentally important for realizing large-scale photonic and quantum circuits. Conventional approaches suffer from short coupling distance, poor controllability, fixed locations and low wavelength uniformity, significantly restricting the scalability of photonic and quantum networks. Here, we exploit the intrinsic advantages of optical bound state in the continuum (BIC) and demonstrate an all-in-one solution for dynamically controllable long-range interactions. BIC metasurface can support a series of finite-sized quasi-BIC microlasers at arbitrary locations. The quasi-BICs microlasers have the same wavelength and are inherently connected through BIC waveguide. Consequently, the coupling distances in experiment increase significantly from subwavelength to tens of micrometers. Such long-range interaction in BIC metasurface enables scaling to two-dimensional architectures and ultrafast control of internal laser actions, e.g., non-Hermitian zero-mode lasing and enhanced optical gain. This research shall facilitate the advancement of scalable and reconfigurable photonic networks., Comment: 12 pages, 4 figures

Dynamic control of circular dichroism in photonic structures is critically important for compact spectrometers, stereoscopic displays, and information processing exploiting multiple degrees of freedom. Metasurfaces can help miniaturize chiral devices but only produce static and limited chiral responses. While external stimuli are able to tune resonances, their modulations are often weak, and reversing continuously the sign of circular dichroism is extremely challenging. Here, we demonstrate dynamically tunable chiral response of resonant metasurfaces supporting chiral bound states in the continuum combining them with phase-change materials. Phase transition between amorphous and crystalline phases allows to control chiral response and vary chirality rapidly from -0.947 to +0.958 backward and forward via chirality continuum. Our demonstrations underpin the rapid development of chiral photonics and its applications., Comment: 14 pages, 4 figures

The rise of the 4H-silicon-carbide-on-insulator (SiCOI) platform marks a promising pathway towards the realization of monolithic quantum photonic networks. However, the challenge of establishing room-temperature entangled registers on these integrated photonics platforms remains unresolved. Herein, we demonstrate the first entangled processor on the SiCOI platform. We show that both deterministic generation of single divacancy electron spins and near-unity spin initialization of a single $^{13}$C nuclear spin can be achieved on SiCOI at room temperature. Besides coherently manipulating the single nuclear spin, a maximally entangled state with a fidelity of 0.89 has been prepared on this CMOS-compatible semiconductor-integrated photonics system. This work establishes the foundation for compact and on-chip solutions within existing defect-based computing and sensing protocols, positioning the SiCOI platform as the most promising candidate for integrated monolithic quantum photonic networks., Comment: 16 pages, 4 figures

Superchiral field is highly important for ultrasensitive detection of chiral objects and has been intensively explored. Despite the progress, the construction of electromagnetic field in achiral nanostructures with giant chirality (C) is fundamentally restricted. Here, we demonstrate a novel approach to construct superchiral field in achiral dielectric metasurfaces. Due to the quantum spin-hall effect, each symmetry-protected bound state in the continuum (BIC) exhibits the ability to support a superchiral field in vicinity of \Gamma point. By merging two BICs with orthogonal polarizations, all the criteria for a superchiral field are satisfied and the dramatic enhancement of chirality becomes more robust. Using typical photonic crystal slabs, we have produced a superchiral field with enhancement factor (C/C_CPL) orders of magnitude higher than state-of-the-art in nanostructures. By further introducing active chiral medium, a chiral mode splitting associated with giant enhancement of circular dichroism (CD) has been formed by the chiral light-matter interaction.

A metasurface hologram combines fine spatial resolution and large viewing angles with a planar form factor and compact size. However, it suffers coherent artifacts originating from electromagnetic cross-talk between closely packed meta-atoms and fabrication defects of nanoscale features. Here, we introduce an efficient method to remove all artifacts by fine-tuning the spatial coherence of illumination. Our method is implemented with a degenerate cavity laser, which allows precise, continuous tuning of spatial coherence over a wide range with little variation in emission spectrum and total power. We find the optimal degree of spatial coherence to remove the coherent artifacts of a meta-hologram while maintaining the image sharpness. This work paves the way to compact and dynamical holographic display free of coherent defects., Comment: Submitted for review

Lead halide perovskites (MAPbX3) have emerged as promising materials for photovoltaic and optoelectronic devices. However, their exceptional nonlinear properties have not been fully exploited in nanophotonics yet. Herein we fabricate MAPbX3 perovskite metasurfaces and explore their internal nonlinear processes. While both of third-order harmonic generation (THG) and three-photon luminescence are generated, the latter one is less affected by the material loss and has been significantly enhanced by a factor of 60. The corresponding simulation reveals that the improvement is caused by the resonant enhancement of incident laser in perovskite metasurface. Interestingly, such kind of resonance-enhanced three-photon luminescence holds true for metasurfaces with a small period number of 4, enabling new applications of perovskite metasurface in high-resolution nonlinear color nanoprinting and optical encoding. The encoded information "NANO" is visible only when the incident laser is on-resonance. The off-resonance pumping and the single-photon excitation just produce a uniform dark or photoluminescence background., Comment: 11 pages,5 figures

Lead halide perovskites (MAPbX3) are known to have high refractive index and controllable bandgap, making them attractive for all-dielectric and tunable metasurfaces. Till now, perovskite metasurfaces have only been used in structural colors. More interesting meta-devices with 2{\pi} phase control are still absent. Here we experimentally demonstrate the MAPbX3 perovskite based metasurfaces with a complete control of phase shift in a reflection mode. By utilizing MAPbBr3 cut-wires as meta-atoms on a ground metal film, we find that the MAPbBr3 perovskite metasurface can produce full phase control from 0 to 2{\pi} and high reflection efficiency simultaneously. Consequently, high-efficiency polarization conversion, anomalous reflection and meta-hologram have been successfully produced. Most interestingly, the bandgap of MAPbX3 perovskite can be post-synthetically and reversibly tuned via anion exchange, providing a new approach to dynamically control of the all-dielectric meta-devices with novel function such as anomalous reflection and hologram et al.

Mode-division multiplexing (MDM) is becoming an enabling technique for large-capacity data communications via encoding the information on orthogonal guiding modes. However, the on-chip routing of a multimode waveguide occupies too large chip area due to the constraints on inter-mode cross talk and mode leakage. Very recently, many efforts have been made to shrink the footprint of individual element like bending and crossing, but the devices still occupy >10x10 um2 footprint for three-mode multiplexed signals and the high-speed signal transmission has not been demonstrated yet. In this work, we demonstrate the first MDM circuits based on digitized meta-structures which have extremely compact footprints. The radius for a three-mode bending is only 3.9 {\mu}m and the footprint of a crossing is only 8x8um2. The 3x100 Gbit/s mode-multiplexed signals are arbitrarily routed through the circuits consists of many sharp bends and compact crossing with a bit error rate under forward error correction limit. This work is a significant step towards the large-scale and dense integration of MDM photonic integrated circuits.

With the rapid evolution of lead halide perovskite solar cells, there are considerable evidences that the mobile ions strongly impact their properties. However, except the activation energy, the other properties of ionic migration are mostly explored with first principle calculations. Here we investigate the migration of halide ion (vacancy) in lead bromide perovskite single crystalline microplates. In contrast to conventional studies with external bias voltages, we introduce built-in potentials into the microplates via low-energy electron beams and study the corresponding ionic migrations. By aligning the potentials along particular crystal planes, the reduction of Pb2+ to Pb0 has been observed at the un-irradiated center of each cell, demonstrating that the migration of halide ion has preferred directions for the first time. Our observations are consistent with the recent theoretical models and shall open up a new route to improve the performances of perovskite solar cells.

Integrated optical power splitter is one of the fundamental building blocks in photonic integrated circuits (PIC). Conventional multimode interferometer based power splitter is widely used as it has reasonable footprint and is easy to fabricate. However, it is challenging to realize arbitrary split ratio especially for multi-outputs. In this work, an ultra-compact power splitter with a QR code-like nanostructure is designed by a nonlinear fast search method (FSM). The highly functional structure is composed of a number of freely designed square pixels with the size of 120nm x 120nm which could be either dielectric or air. The lightwaves are scattered by a number of etched squares with optimized locations and the scattered waves superimpose at the outputs with the desired power ratio. We demonstrate 1x2 splitters with 1:1, 1:2, 1:3 split ratios and a 1x3 splitter with the ratio of 1:2:1. The footprint for all the devices is only 3.6umx3.6 um. Well-controlled split ratios are measured for all the cases. The measured transmission efficiencies of all the splitters are close to 80% over 30 nm wavelength range.

Lead halide perovskite based micro- and nano- lasers have been widely studied in past two years. Due to their long carrier diffusion length and high external quantum efficiency, lead halide perovskites have been considered to have bright future in optoelectronic devices, especially in the "green gap" wavelength region. However, the quality (Q) factors of perovskite lasers are unspectacular compared to conventional microdisk lasers. The record value of full width at half maximum (FWHM) at threshold is still around 0.22 nm. Herein we synthesized solution-processed, single-crystalline CH3NH3PbBr3 perovskite microrods and studied their lasing actions. In contrast to entirely pumping a microrod on substrate, we partially excited the microrods that were hanging in the air. Consequently, single-mode or few-mode laser emissions have been successfully obtained from the whispering-gallery like diamond modes, which are confined by total internal reflection within the transverse plane. Owning to the better light confinement and high crystal quality, the FWHM at threshold have been significantly improved. The smallest FWHM at threshold is around 0.1 nm, giving a Q factor over 5000., Comment: 7 pages, 4 figures

Solution-based perovskite nanoparticles have been intensively studied in past few years due to their applications in both photovoltaic and optoelectronic devices. Here, based on the common ground between the solution-based perovskite and random lasers, we have studied the mirrorless lasing actions in self-assembled perovskite nanoparticles. After the synthesis from solution, discrete lasing peaks have been observed from the optically pumped perovskites without any well-defined cavity boundaries. The obtained quality (Q) factors and thresholds of random lasers are around 500 and 60 uJ/cm2, respectively. Both values are comparable to the conventional perovskite microdisk lasers with polygon shaped cavity boundaries. From the corresponding studies on laser spectra and fluorescence microscope images, the lasing actions are considered as random lasers that are generated by strong multiple scattering in random gain media. In additional to conventional single-photon excitation, due to the strong nonlinear effects of perovskites, two-photon pumped random lasers have also been demonstrated for the first time. We believe this research will find its potential applications in low-cost coherent light sources and biomedical detection., Comment: 16 pages, 5 figures

Perovskite based micro- and nano- lasers have attracted considerable research attention in past two years. However, the properties of perovskite devices are mostly fixed once they are synthesized. Here we demonstrate the tailoring of lasing properties of perovskite nanowire lasers via nano-manipulation. By utilizing a tungsten probe, one nanowire has been lifted from the wafer and re-positioned its two ends on two nearby perovskite blocks. Consequently, the conventional Fabry-Perot lasers are completely suppressed and a single laser peak has been observed. The corresponding numerical model reveals that the single-mode lasing operation is formed by the whispering gallery mode in the transverse plane of perovskite nanowire. Our research provides a simple way to tailor the properties of nanowire and it will be essential for the applications of perovskite optoelectronics., Comment: 16 pages, 5 figures

Solution-processed lead halide perovskites have shown very bright future in both solar cells and microlasers. Very recently, the nonlinearity of perovskites started to attract considerable research attention. Second harmonic generation and two-photon absorption have been successfully demonstrated. However, the nonlinearity based perovskite devices such as micro- & nano- lasers are still absent. Here we demonstrate the two-photon pumped nanolasers from perovskite nanowires. The CH3NH3PbBr3 perovskite nanowires were synthesized with one-step solution self-assembly method and dispersed on glass substrate. Under the optical excitation at 800 nm, two-photon pumped lasing actions with periodic peaks have been successfully observed at around 546 nm. The obtained quality (Q) factors of two-photon pumped nanolasers are around 960, and the corresponding thresholds are about 674?J=cm2. Both the Q factors and thresholds are comparable to conventional whispering gallery modes in two-dimensional polygon microplates. Our researches are the first demonstrations of two-photon pumped nanolasers in perovskite nanowires. We believe our finding will significantly expand the application of perovskite in low-cost nonlinear optical devices such as optical limiting, optical switch, and biomedical imaging et al., Comment: 14 pages, 5 figures