1. Water Induced Ferroelectric Switching: The Crucial Role of Collective Dynamics
- Author
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Aslam, Muhammad Awais, Stankovic, Igor, Murastov, Gennadiy, Carl, Amy, Song, Zehao, Watanabe, Kenji, Taniguchi, Takashi, Lugstein, Alois, Teichert, Christian, Gorbachev, Roman, Rodriguez, Raul David, and Matkovic, Aleksandar
- Subjects
Condensed Matter - Mesoscale and Nanoscale Physics - Abstract
The interaction mechanisms of water with nanoscale geometries remain poorly understood. This study focuses on behaviour of water clusters under varying external electric fields with a particular focus on molecular ferroelectric devices. We employ a two-fold approach, combining experiments with large-scale molecular dynamics simulations on graphene nanoribbon field effect transistors. We show that bilayer graphene nanoribbons provide stable anchoring of water clusters on the oxygenated edges, resulting in a ferroelectric effect. A molecular dynamics model is then used to investigate water cluster behaviour under varying external electric fields. Finally, we show that these nanoribbons exhibit significant and persistent remanent fields that can be employed in ferroelectric heterostructures and neuromorphic circuits.
- Published
- 2023