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We investigate spin conductance in zigzag graphene nanoribbons and propose a spin injection mechanism based only on graphitic nanostructures. We find that nanoribbons with atomically straight, symmetric edges show zero spin conductance, but nonzero spin Hall conductance. Only nanoribbons with asymmetrically shaped edges give rise to a finite spin conductance and can be used for spin injection into graphene. Furthermore, nanoribbons with rough edges exhibit mesoscopic spin conductance fluctuations with a universal value of $\mathrm{rms} G_\mathrm{s}\approx 0.4 e/4\pi$., Comment: 4 pages, 5 figures, PdfLaTeX, accepted for publication in Physical Review Letters

We combine ab initio density functional theory with transport calculations to provide a microscopic basis for distinguishing between good and poor metal contacts to nanotubes. Comparing Ti and Pd as examples of different contact metals, we trace back the observed superiority of Pd to the nature of the metal-nanotube hybridization. Based on large scale Landauer transport calculations, we suggest that the `optimum' metal-nanotube contact combines a weak hybridization with a large contact length between the metal and the nanotube., Comment: final version, including minor corrections by editor

We show that an electrical shift current is generated when electrons are photoexcited from the valence to conduction bands on a BN nanotube. This photocurrent follows the light pulse envelope and its symmetry is controlled by the atomic structure of the nanotube. We find that the shift current has an intrinsic quantum mechanical signature in which the chiral index of the tube determines the direction of the current along the tube axis. We identify discrete lattice effects in the tangent plane of the tube that lead to an azimuthal component of the shift current. The nanotube shift current can lead to ultrafast opto-electronic and opto-mechanical applications., Comment: 4 pages in RevTeX cotaining 2 epsf color figures

Coherent one photon ($2 \omega$) and two photon ($ \omega$) electronic excitations are studied for graphene sheets and for carbon nanotubes using a long wavelength theory for the low energy electronic states. For graphene sheets we find that coherent superposition of these excitations produces a polar asymmetry in the momentum space distribution of the excited carriers with an angular dependence which depends on the relative polarization and phases of the incident fields. For semiconducting nanotubes we find a similar effect which depends on the square of the semiconducting gap, and we calculate its frequency dependence. We find that the third order nonlinearity which controls the direction of the photocurrent is robust for semiconducting t ubes and vanishes in the continuum theory for conducting tubes. We calculate corrections to these results arising from higher order crystal field effects on the band structure and briefly discuss some applications of the theory., Comment: 12 pages in RevTex, 6 epsf figures

Using a scattering technique based on a parametrized linear combination of atomic orbitals Hamiltonian, we calculate the ballistic quantum conductance of multi-wall carbon nanotubes. We find that inter-wall interactions not only block some of the quantum conductance channels, but also redistribute the current non-uniformly over the individual tubes across the structure. Our results provide a natural explanation for the unexpected integer and non-integer conductance values reported for multi-wall nanotubes in Ref.[S. Frank, P. Poncharal, Z.L. Wang, and W. A. de Heer, Science 280, 1744 (1998)], Comment: 16 pages, 5 figures, submitted to PRL