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We demonstrate coherent coupling between excitons in a MoSe2/WSe2 heterostructure, as well as rapid interlayer electron and hole transfer. We visualize the spatial homogeneity of the coupling in the presence of significant sample inhomogeneities.

We demonstrate coherent coupling between excitons in a MoSe2/WSe2 heterostructure, as well as rapid interlayer electron and hole transfer. We visualize the spatial homogeneity of the coupling in the presence of significant sample inhomogeneities.

Transition metal dichalcogenides (TMDs) are regarded as a possible materials platform for quantum information science and related device applications. In TMD monolayers, the dephasing time and inhomogeneity are crucial parameters for any quantum information application. In TMD heterostructures, coupling strength and interlayer exciton lifetimes are also parameters of interest. However, many demonstrations in TMDs can only be realized at specific spots on the sample, presenting a challenge to the scalability of these applications. Here, using multi-dimensional coherent imaging spectroscopy (MDCIS), we shed light on the underlying physics - including dephasing, inhomogeneity, and strain - for a MoSe$_2$ monolayer and identify both promising and unfavorable areas for quantum information applications. We furthermore apply the same technique to a MoSe$_2$/WSe$_2$ heterostructure. Despite the notable presence of strain and dielectric environment changes, coherent and incoherent coupling, as well as interlayer exciton lifetimes are mostly robust across the sample. This uniformity is despite a significantly inhomogeneous interlayer exciton photoluminescence distribution that suggests a bad sample for device applications. This robustness strengthens the case for TMDs as a next-generation materials platform in quantum information science and beyond.

We show that accelerated nonlinear imaging, such as stimulated Raman scattering and pump–probe imaging, is enabled by an order of magnitude reduction of data acquisition time when replacing the exponentially-weighted-moving-average low-pass filter in a lock-in amplifier with a simple-moving-average filter. We show that this simple-moving-average (box) lock-in yields a superior signal-to-noise ratio and suppression of extraneous modulations with short pixel dwell times, if one condition for the relation between the lock-in time constant and modulation frequencies is met. Our results, both theoretical and experimental, indicate that for nonlinear imaging applications, the box lock-in significantly outperforms conventional lock-in detection. These results facilitate the application of ultrafast and nonlinear imaging as a new standard for material characterization.

The basic \emph{entanglement swapping protocol} allows to project two qubits, which have never interacted, onto a maximally entangled state. For deterministic swapping, the key ingredient is the maximal entanglement that was initially contained in two pairs of qubits and the capacity of projecting onto a Bell basis. Thus the basic and deterministic entanglement swapping scheme involves three maximal level of entanglement. In this work we propose probabilistic entanglement swapping processes performed with different amounts of initial entanglement. Besides that we suggest a non Bell measuring-basis, to introduce a third entanglement level in the process. Additionally, we propose the \emph{unambiguous state extraction scheme} as the local mechanism for probabilistically achieving the EPR projection. The combination of these three elements allows us to design four strategies for performing probabilistic entanglement swapping. Surprisingly, we find a twofold entanglement threshold effect related to the concurrence of the measuring-basis. Specifically, the maximal probability of accomplishing a EPR projection becomes a constant for concurrences higher than or equal to threshold entanglement value. Thus, we show that maximal entanglement in the measuring-basis is not required for attaining the EPR projection., Comment: 8 pages, 3 figures