Search

In continuous-variable quantum computation, identifying key elements that enable a quantum computational advantage is a long-standing issue. Starting from the standard results on the necessity of Wigner negativity, we develop a comprehensive and versatile framework that not only enables the identification of a potential quantum computational advantage, but also allows to pinpoint the contribution of each quantum gate in achieving this objective. As such, it can be straightforwardly applied to current continuous-variables quantum circuits, while also constraining the tolerable amount of losses above which any potential quantum advantage can be ruled out. We use $(s)$-ordered quasiprobability distributions on phase-space to capture the non-classical features in the protocol, and focus our model entirely on the ordering parameter $s$. This allows us to highlight the resourcefulness and robustness to loss of a universal set of unitary gates comprising three distinct Gaussian gates, and a fourth one, the cubic gate, providing important insight on the role of non-Gaussianity., Comment: 16 pages, 5 figures

Photon subtraction can enhance entanglement, which for pure states induces a decrease in the purity of reduced states. In contrast, by analyzing the purities of Gaussian states before and after subtracting a single photon, we prove that the purity of a Gaussian state can also be increased by less than 20%. On the one hand, it reveals that photon subtraction can reduce entanglement, and on the other hand, it reveals that it can achieve a limited amount of Gaussian state purification. Through the analysis of some examples, we demonstrate the inherent mechanism and applicable scope of photon-subtraction-based purification. In a multimode system, we find that photon subtraction can increase entanglement and purify some of the reduced states simultaneously. We thus present purification through the suppression of Gaussian noise as a new application for photon subtraction in continuous-variable quantum information processing., Comment: 7 pages, 3 figures, comments welcome!

Quantum correlations are at the core of the power of quantum information and are necessary to reach a quantum computational advantage. In the context of continuous-variable quantum systems, another necessary ressource for quantum advantages is non-Gaussianity. In this work, we propose a witness, based on previously known relations between metrological power and quantum correlations, to detect a strong form of entanglement that only non-Gaussian states possess and that cannot be undone by passive optical operations, i.e., entanglement in all mode bases. The strength of our witness is two-fold: it only requires measurements in one basis to check entanglement in any arbitrary mode basis; it can be made applicable experimentally using homodyne measurements and without requiring a full tomography of the state., Comment: 16 pages, 12 figures, comments are welcome!

Measurement-induced quantum computation with continuous-variable cluster states utilizes teleportation propagating the states through the cluster accompanied by non-Gaussian measurements and feedforward control. We analyze such propagation of a quantum non-Gaussian state with nonlinear squeezing through a small cluster state and show that when a nonlinear feedforward is involved in the teleportation protocol, higher nonlinear squeezing can be transferred. In a probabilistic regime, the improvement can be manifested even with current experimental resources. Better processing of non-Gaussian states can bring us closer to the necessary interplay between cluster states and non-Gaussianity required by quantum computing., Comment: references added

The problem of resolving point-like light sources not only serves as a benchmark for optical resolution but also holds various practical applications ranging from microscopy to astronomy. In this research, we aim to resolve two thermal sources sharing arbitrary mutual coherence using the spatial mode demultiplexing technique. Our analytical study includes scenarios where the coherence and the emission rate depend on the separation between the sources, and is not limited to the faint sources limit. We consider the fluorescence of two interacting dipoles to demonstrate that the dependence of emission characteristics on the parameter of interest can boost the sensitivity of the estimation and noticeably prolong the duration of information decay.

Entanglement in continuous-variable non-Gaussian states provides irreplaceable advantages in many quantum information tasks. However, the sheer amount of information in such states grows exponentially and makes a full characterization impossible. Here, we develop a neural network that allows us to use correlation patterns to effectively detect continuous-variable entanglement through homodyne detection. Using a recently defined stellar hierarchy to rank the states used for training, our algorithm works not only on any kind of Gaussian state but also on a whole class of experimentally achievable non-Gaussian states, including photon-subtracted states. With the same limited amount of data, our method provides higher accuracy than usual methods to detect entanglement based on maximum-likelihood tomography. Moreover, in order to visualize the effect of the neural network, we employ a dimension reduction algorithm on the patterns. This shows that a clear boundary appears between the entangled states and others after the neural network processing. In addition, these techniques allow us to compare different entanglement witnesses and understand their working. Our findings provide a new approach for experimental detection of continuous-variable quantum correlations without resorting to a full tomography of the state and confirm the exciting potential of neural networks in quantum information processing., Comment: 9 pages (incl. appendix), 6 figures, comments welcome!

Historically, the resolution of optical imaging systems was dictated by diffraction, and the Rayleigh criterion was long considered an unsurpassable limit. In superresolution microscopy, this limit is overcome by manipulating the emission properties of the object. However, in passive imaging, when sources are uncontrolled, reaching sub-Rayleigh resolution remains a challenge. Here, we implement a quantum-metrolgy-inspired approach for estimating the separation between two incoherent sources, achieving a sensitivity five orders of magnitude beyond the Rayleigh limit. Using a spatial mode demultiplexer, we examine scenes with bright and faint sources, through intensity measurements in the Hermite-Gauss basis. Analysing sensitivity and accuracy over an extensive range of separations, we demonstrate the remarkable effectiveness of demultiplexing for sub-Rayleigh separation estimation. These results effectively render the Rayleigh limit obsolete for passive imaging.

Quantum-optimal discrimination between one and two closely separated light sources can be achieved by ideal spatial-mode demultiplexing, simply monitoring whether a photon is detected in a single antisymmetric mode. However, we show that for any, no matter how small, imperfections of the demultiplexer, this simple statistical test becomes practically useless, i.e. as good as flipping a coin. While we identify a class of separation-independent tests with vanishing error probabilities in the limit of large numbers of detected photons, they are generally unreliable beyond that very limit. As a practical alternative, we propose a simple semi-separation-independent test, which provides a method for designing reliable experiments, through arbitrary control over the maximal probability of error., Comment: 5 pages + Supplementary Material

Entanglement and non-Gaussianity are physical resources that are essential for a large number of quantum-optics protocols. Non-Gaussian entanglement is indispensable for quantum-computing advantage and outperforms its Gaussian counterparts in a number of quantum-information protocols. The characterization of non-Gaussian entanglement is a critical matter as it is in general highly demanding in terms of resources. We propose a simple protocol based on the Fisher information for witnessing entanglement in an important class of non-Gaussian entangled states: photon-subtracted states. We demonstrate that our protocol is relevant for the detection of non-Gaussian entanglement generated by multiple photon-subtraction and that it is experimentally feasible through homodyne detection., Comment: We have corrected errors found in Figures 8 and 9 of the previous version and improved the manuscript with an analysis of the entanglement produced by multi-photon subtraction. We have adapted the main text, abstract and title correspondingly. 16 pages, 14 figures

Quantum correlations and Wigner negativity are two important signatures of nonclassicality in continuous-variable quantum systems. In this work, we investigate how both are intertwined in the context of the conditional generation of Wigner negativity. It was previously shown that when Alice and Bob share a Gaussian state, Bob can perform some measurement on his system to create Wigner negativity on Alice's side if and only if there is Gaussian steering from Alice to Bob. In this work, we attempt to generalise these findings to a much broader class of scenarios on which Alice and Bob share a non-Gaussian state. We show that if Alice can initially steer Bob's system with Wigner-positive measurements, Bob can remotely create Wigner negativity in Alice's subsystem. Even though this shows that quantum steering is sufficient, we also show that quantum correlations are in general not necessary for the conditional generation of Wigner negativity., Comment: 16 pages, no figures, comments still welcome

Superresolution is one of the key issues at the crossroads of contemporary quantum optics and metrology. Recently, it was shown that for an idealized case of two balanced sources, spatial mode demultiplexing (SPADE) achieves resolution better than direct imaging even in the presence of measurement crosstalk [Phys. Rev. Lett. 125, 100501 (2020)]. In this work, we consider arbitrarily unbalanced sources and provide a systematic analysis of the impact of crosstalk on the resolution obtained from SPADE. As we dissect, in this generalized scenario, SPADE's effectiveness depends non-trivially on the strength of crosstalk, relative brightness and the separation between the sources. In particular, for any source imbalance, SPADE performs worse than ideal direct imaging in the asymptotic limit of vanishing source separations. Nonetheless, for realistic values of crosstalk strength, SPADE is still the superior method for several orders of magnitude of source separations., Comment: 10 pages, 6 figures

Quantum computers promise to dramatically outperform their classical counterparts. However, the non-classical resources enabling such computational advantages are challenging to pinpoint, as it is not a single resource but the subtle interplay of many that can be held responsible for these potential advantages. In this work, we show that every bosonic quantum computation can be recast into a continuous-variable sampling computation where all computational resources are contained in the input state. Using this reduction, we derive a general classical algorithm for the strong simulation of bosonic computations, whose complexity scales with the non-Gaussian stellar rank of both the input state and the measurement setup. We further study the conditions for an efficient classical simulation of the associated continuous-variable sampling computations and identify an operational notion of non-Gaussian entanglement based on the lack of passive separability, thus clarifying the interplay of bosonic quantum computational resources such as squeezing, non-Gaussianity and entanglement., Comment: Published version, 6+14 pages, 2 figures. Comments are welcome!

We determine analytically the quantum Cram\'er-Rao bound for the estimation of the separation between two point sources in arbitrary Gaussian states. Our analytical expression is valid for arbitrary sources brightness, and it allows to determine how different resources, such as mutual coherence (induced by thermal correlations or displacement) or squeezing affect the scaling of the ultimate resolution limit with the mean number of emitted photons. In practical scenarios, we find coherent states of the sources to achieve quantum optimal resolution., Comment: 5 pages, 3 figures, comments are welcome!

Quantum optical metrology aims to identify ultimate sensitivity bounds for the estimation of parameters encoded into quantum states of the electromagnetic field. In many practical applications, including imaging, microscopy, and remote sensing, the parameter of interest is not only encoded in the quantum state of the field, but also in its spatio-temporal distribution, i.e. in its mode structure. In this mode-encoded parameter estimation setting, we derive an analytical expression for the quantum Fisher information valid for arbitrary multimode Gaussian fields. To illustrate the power of our approach, we apply our results to the estimation of the transverse displacement of a beam and to the temporal separation between two pulses. For these examples, we show how the estimation sensitivity can be enhanced by adding squeezing into specific modes., Comment: 20 pages (14 main + 6 appendices), 3 figures. Sec. 4 rewritten to include a completely new set of examples that were not in v1. Comments are very welcome!

Quantum correlations are at the core of current developments in quantum technologies. Certification protocols of entanglement and steering, suitable for continuous-variable non-Gaussian states are scarce and generally highly demanding from an experimental point of view. We propose a protocol based on Fisher information for witnessing steering in general continuous-variable bipartite states, through homodyne detection. It proves to be relevant for the detection of non-Gaussian steering in scenarios where witnesses based on Gaussian features like the covariance matrix are shown to fail., Comment: 14 pages, 14 figures, comments are welcome!

We analyze the problem of resolving two point-sources in the case of mutually coherent sources with arbitrary quantum statistics, mutual phase, relative and absolute intensity. We use a sensitivity measure based on the method of moments and compare direct imaging with spatial mode demultiplexing, analytically proving the advantage of the latter. We show that the sensitivity of spatial mode demultiplexing saturates the quantum Fisher information, for all known cases, even for non-Gaussian states of the sources.

Sensitivity limits are usually determined using the Cram\'er-Rao bound. Recently this approach has been used to obtain the ultimate resolution limit for the estimation of the separation between two incoherent point sources. However, methods that saturate these resolution limits, usually require the full measurement statistics, which can be challenging to access. In this work, we introduce a simple superresolution protocol to estimate the separation between two thermal sources which relies only on the average value of a single accessible observable. We show how optimal observables for this technique may be constructed for arbitrary thermal sources, and we study their sensitivities when one has access to spatially resolved intensity measurements (direct imaging) and photon counting after spatial mode demultiplexing. For demultiplexing, our method is optimal, i.e. it saturates the quantum Cram\'er-Rao bound. We also investigate the impact of noise on the optimal observables, their measurement sensitivity and on the scaling with the number of detected photons of the smallest resolvable separation. For low signals in the image plane, we demonstrate that our method saturates the Cram\'er-Rao bound even in the presence of noise., Comment: 18 pages, 12 figures, 1 table. Comments are very welcome!

Gaussian states have played on important role in the physics of continuous-variable quantum systems. They are appealing for the experimental ease with which they can be produced, and for their compact and elegant mathematical description. Nevertheless, many proposed quantum technologies require us to go beyond the realm of Gaussian states and introduce non-Gaussian elements. In this Tutorial, we provide a roadmap for the physics of non-Gaussian quantum states. We introduce the phase-space representations as a framework to describe the different properties of quantum states in continuous-variable systems. We then use this framework in various ways to explore the structure of the state space. We explain how non-Gaussian states can be characterised not only through the negative values of their Wigner function, but also via other properties such as quantum non-Gaussianity and the related stellar rank. For multimode systems, we are naturally confronted with the question of how non-Gaussian properties behave with respect to quantum correlations. To answer this question, we first show how non-Gaussian states can be created by performing measurements on a subset of modes in a Gaussian state. Then, we highlight that these measured modes must be correlated via specific quantum correlations to the remainder of the system to create quantum non-Gaussian or Wigner-negative states. On the other hand, non-Gaussian operations are also shown to enhance or even create quantum correlations. Finally, we will demonstrate that Wigner negativity is a requirement to violate Bell inequalities and to achieve a quantum computational advantage. At the end of the Tutorial, we also provide an overview of several experimental realisations of non-Gaussian quantum states in quantum optics and beyond., Comment: Tutorial; 61 pages and 7 Figures

Wigner negativity, as a well-known indicator of nonclassicality, plays an essential role in quantum computing and simulation using continuous-variable systems. Recently, it has been proven that Einstein-Podolsky-Rosen steering is a prerequisite to generate Wigner negativity between two remote modes. Motivated by the demand of real-world quantum network, here we investigate the shareability of generated Wigner negativity in the multipartite scenario from a quantitative perspective. By establishing a monogamy relation akin to the generalized Coffman-Kundu-Wootters inequality, we show that the amount of Wigner negativity cannot be freely distributed among different modes. Moreover, for photon subtraction -- one of the main experimentally realized non-Gaussian operations -- we provide a general method to quantify the remotely generated Wigner negativity. With this method, we find that there is no direct quantitative relation between the Gaussian steerability and the amount of generated Wigner negativity. Our results pave the way for exploiting Wigner negativity as a valuable resource for numerous quantum information protocols based on non-Gaussian scenario.

Multi-particle interference is an essential ingredient for fundamental quantum mechanics phenomena and for quantum information processing to provide a computational advantage, as recently emphasized by Boson Sampling experiments. Hence, developing a reliable and efficient technique to witness its presence is pivotal towards the practical implementation of quantum technologies. Here we experimentally identify genuine many-body quantum interference via a recent efficient protocol, which exploits statistical signatures at the output of a multimode quantum device. We successfully apply the test to validate three-photon experiments in an integrated photonic circuit, providing an extensive analysis on the resources required to perform it. Moreover, drawing upon established techniques of machine learning, we show how such tools help to identify the - a priori unknown - optimal features to witness these signatures. Our results provide evidence on the efficacy and feasibility of the method, paving the way for its adoption in large-scale implementations., Comment: 15 pages, 12 figures

Non-Gaussian states of an optical field are important as a proposed resource in quantum information applications. While conditional preparation is a highly successful approach to preparing such states, their quality is limited by detector non-idealities such as dead time, narrow dynamic range, limited quantum efficiency and dark noise. Mesoscopic photon counters, with peak performance at higher photon number, offer many practical advantages over single-photon level conditioning detectors. Here we propose a novel approach involving displacement of the ancilla field into the regime where mesoscopic detectors can be used. We explore this strategy theoretically and present simulations accounting for experimental non-idealities such as loss and amplification noise, showing that precise photon-number resolution is not necessary to herald highly nonclassical states. We conclude that states with strong Wigner negativity can be prepared at high rates by this technique under experimentally attainable conditions.

Entanglement is an indispensable quantum resource for quantum information technology. In continuous-variable quantum optics, photon subtraction can increase the entanglement between Gaussian states of light, but for mixed states the extent of this entanglement increase is poorly understood. In this work, we use an entanglement measure based the R\'enyi-2 entropy to prove that single-photon subtraction increases bipartite entanglement by no more than log 2. This value coincides with the maximal amount of bipartite entanglement that can be achieved with one photon. The upper bound is valid for all Gaussian input states, regardless of the number of modes and the purity.

Recent works identified resolution limits for the distance between incoherent point sources. However, it remains unclear how to choose suitable observables and estimators to reach these limits in practical situations. Here, we show how estimators saturating the Cram\'er-Rao bound for the distance between two thermal point sources can be constructed using an optimally designed observable in the presence of practical imperfections, such as misalignment, crosstalk and detector noise., Comment: 6 pages, 4 figures. Comments are welcome

We use complex network theory to study a class of continuous-variable quantum states that present both multipartite entanglement and non-Gaussian statistics. We consider the intermediate scale of several dozens of components at which such systems are already hard to characterize. In particular, the states are built from an initial imprinted cluster state created via Gaussian entangling operations according to a complex network structure. We then engender non-Gaussian statistics via multiple photon subtraction operations acting on a single node. We replicate in the quantum regime some of the models that mimic real-world complex networks in order to test their structural properties under local operations. We then go beyond the already known single-mode effects, by studying the emergent network of photon-number correlations via complex networks measures. We analytically prove that the imprinted network structure defines a vicinity of nodes, at a distance of four steps from the photon-subtracted node, in which the emergent network changes due to photon subtraction. Moreover, our numerical analysis shows that the emergent structure is greatly influenced by the structure of the imprinted network. Indeed, while the mean and the variance of the degree and clustering distribution of the emergent network always increase, the higher moments of the distributions are governed by the specific structure of the imprinted network. Finally, we show that the behaviour of nearest neighbours of the subtraction node depends on how they are connected to each other in the imprinted structure., Comment: 26 pages (incl. appendix), 20 figures

We investigate the ground states of spin models defined on networks that we imprint (e.g. non-complex random networks like Erdos-Renyi or complex networks like Watts-Strogatz, and Barabasi-Albert), and their response to decohering processes which we model with network attacks. We quantify the complexity of these ground states, and their response to the attacks, by calculating distributions of network measures of an emergent network whose link weights are the pairwise mutual information between spins. We focus on attacks which projectively measure spins. We find that the emergent networks in the ground state do not satisfy the usual criteria for complexity, and their average properties are captured well by a single dimensionless parameter in the Hamiltonian. While the response of classical networks to attacks is well-studied, where classical complex networks are known to be more robust to random attacks than random networks, we find counterintuitive results for our quantum networks. We find that the ground states for Hamiltonians defined on different classes of imprinted networks respond similarly to all our attacks, and the attacks rescale the average properties of the emergent network by a constant factor. Mean field theory explains these results for relatively dense networks, but we also find the simple rescaling behavior away from the regime of validity of mean field theory. Our calculations indicate that complex spin networks are not more robust to projective measurement attacks, and presumably also other quantum attacks, than non-complex spin networks, in contrast to the classical case. Understanding the response of the spin networks to decoherence and attacks will have applications in understanding the physics of open quantum systems, and in designing robust complex quantum systems, possibly even a robust quantum Internet in the long run, that is maximally resistant to decoherence., Comment: 22 pages, 10 figures + references + appendix

We derive a theoretical framework for the experimental certification of non-Gaussian features of quantum states using double homodyne detection. We rank experimental non-Gaussian states according to the recently defined stellar hierarchy and we propose practical Wigner negativity witnesses. We simulate various use-cases ranging from fidelity estimation to witnessing Wigner negativity. Moreover, we extend results on the robustness of the stellar hierarchy of non-Gaussian states. Our results illustrate the usefulness of double homodyne detection as a practical measurement scheme for retrieving information about continuous variable quantum states., Comment: 9+9 pages, comments welcome

We develop a general formalism, based on the Wigner function representation of continuous-variable quantum states, to describe the action of an arbitrary conditional operation on a multimode Gaussian state. We apply this formalism to several examples, thus showing its potential as an elegant analytical tool for simulating quantum optics experiments. Furthermore, we also use it to prove that EPR steering is a necessary requirement to remotely prepare a Wigner-negative state., Comment: 12 pages, 3 figures

Multi-plane light conversion allows to perform arbitrary transformations on a finite set of spatial modes with no theoretical restriction to the quality of the transformation. Even though the number of shaped modes is in general small, the number of modes transmitted by a multi-plane light converter (MPLC) is extremely large. In this work, we aim to characterize the transmission properties of a multi-plane light converter inside and, for the first time, outside the design-modes subspace. By numerically reconstructing the transmission matrix of such systems, we individuate new ways to evaluate their efficiency in performing the design transformation. Moreover, we develop an analytical random matrix model that suggests that in the regime of a large number of shaped modes an MPLC behaves like a random scattering medium with limited number of controlled channels., Comment: New version of Fig. 1 and significant rewriting

In the current quest for efficient and experimentally feasible platforms for implementation of multimode squeezing and entanglement in the continuous variable regime, we underpin and complement our results on the generation of versatile multimode entanglement and cluster states in nonlinear waveguide arrays presented by Barral et al., Phys. Rev. Appl. $\bf{14}$, 044025 (2020). We present detailed derivations of the equations that describe the propagation of light through this system, and then we focus on parameter regimes where these equations can be solved analytically. These analytical solutions build an intuition for the wide landscape of quantum states that are accessible through the activation of pumping, coupling and measurement schemes. Furthermore, we showcase the acquired insights by using one of the identified analytical solutions to exhibit the generation, optimization and scalability of spatial linear cluster states., Comment: 20 pages, 9 figures, v2 closer to the published version. arXiv admin note: substantial text overlap with arXiv:1912.11154

The characterization of quantum features in large Hilbert spaces is a crucial requirement for testing quantum protocols. In the continuous variables encoding, quantum homodyne tomography requires an amount of measurements that increases exponentially with the number of involved modes, which practically makes the protocol intractable even with few modes. Here we introduce a new technique, based on a machine learning protocol with artificial Neural Networks, that allows to directly detect negativity of the Wigner function for multimode quantum states. We test the procedure on a whole class of numerically simulated multimode quantum states for which the Wigner function is known analytically. We demonstrate that the method is fast, accurate and more robust than conventional methods when limited amounts of data are available. Moreover the method is applied to an experimental multimode quantum state, for which an additional test of resilience to losses is carried out.

Multimode entanglement is an essential resource for quantum information in continuous-variable systems. Light-based quantum technologies will arguably not be built upon table-top bulk setups, but will presumably rather resort to integrated optics. Sequential bulk optics-like proposals based on cascaded integrated interferometers are not scalable with the current state-of-the-art low-loss materials used for continuous variables. We analyze the multimode continuous-variable entanglement capabilities of a compact currently-available integrated device without bulk-optics analog: the array of nonlinear waveguides. We theoretically demonstrate that this simple and compact structure, together with a reconfigurable input pump distribution and multimode coherent detection of the output modes, is a versatile entanglement synthesizer in the spatial domain. We exhibit this versatility through analytical and numerically optimized multimode squeezing, entanglement, and cluster state generation in different encodings. Our results re-establish spatial encoding as a contender in the game of continuous-variable quantum information processing., Comment: 17 pages, 5 figures, v4 closer to the published version

Negativity of the Wigner function is seen as a crucial resource for reaching a quantum computational advantage with continuous variable systems. However, these systems, while they allow for the deterministic generation of large entangle states, require an extra element such as photon subtraction to obtain such negativity. Photon subtraction is known to affect modes beyond the one where the photon is subtracted, an effect which is governed by the correlations of the state. In this manuscript, we build upon this effect to remotely prepare states with Wigner-negativity. More specifically, we show that photon subtraction can induce Wigner-negativity in a correlated mode if and only if that correlated mode can perform Einstein-Podolsky-Rosen steering in the mode of subtraction., Comment: 5 pages and 2 figures

This Tutorial will introduce the mathematical framework for describing systems of identical particles, and explain the notion of indistinguishability. We will then focus our attention on dynamical systems of free particles and formally introduce the concept of many-particle interference. Its impact on many-particle transition probabilities is computationally challenging to evaluate, and it becomes rapidly intractable for systems with large numbers of identical particles. Hence, this Tutorial will build up towards alternative, more efficient methods for observing signatures of many-particle interference. A first type of signatures relies on the detection of a highly sensitive -but also highly fragile-processes of total destructive interference that occurs in interferometers with a high degree of symmetry. A second class of signatures is based on the statistical features that arise when we study the typical behaviour of correlations between a small number of the interferometer's output ports. We will ultimately show how these statistical signatures of many-particle interference lead us to a statistical version of the Hong-Ou-Mandel effect., Comment: Tutorial / Pedagogical review; 67 pages, 11 figures

Multimode photon-subtraction provides an experimentally feasible option to construct large non-Gaussian quantum states in continuous-variable quantum optics. The non-Gaussian features of the state can lead towards the more exotic aspects of quantum theory, such as negativity of the Wigner function. However, the pay-off for states with such delicate quantum properties is their sensitivity to decoherence. In this paper, we present a general model that treats the most important source of decoherence in a purely optical setting: losses. We use the framework of open quantum systems and master equations to describe losses in n-photon-subtracted multimode states, where each photon can be subtracted in an arbitrary mode. As a main result, we find that mode-dependent losses and photon-subtraction generally do not commute. In particular, the losses do not only reduce the purity of the state, they also change the modal structure of its non-Gaussian features. We then conduct a detailed study of single-photon subtraction from a multimode Gaussian state, which is a setting that lies within the reach of present-day experiments., Comment: 14 pages, 8 figures

Multi-particle interference is a key resource for quantum information processing, as exemplified by Boson Sampling. Hence, given its fragile nature, an essential desideratum is a solid and reliable framework for its validation. However, while several protocols have been introduced to this end, the approach is still fragmented and fails to build a big picture for future developments. In this work, we propose an operational approach to validation that encompasses and strengthens the state of the art for these protocols. To this end, we consider the Bayesian hypothesis testing and the statistical benchmark as most favorable protocols for small- and large-scale applications, respectively. We numerically investigate their operation with finite sample size, extending previous tests to larger dimensions, and against two adversarial algorithms for classical simulation: the Mean-Field sampler and the Metropolized Independent Sampler. To evidence the actual need for refined validation techniques, we show how the assessment of numerically simulated data depends on the available sample size, as well as on the internal hyper-parameters and other practically relevant constraints. Our analyses provide general insights into the challenge of validation, and can inspire the design of algorithms with a measurable quantum advantage., Comment: 10 pages, 7 figures

Even though Gaussian quantum states of multimode light are promising quantum resources due to their scalability, non-Gaussianity is indispensable for quantum technologies, in particular to reach quantum computational advantage. However, embodying non-Gaussianity in a multimode Gaussian state remains a challenge as controllable non-Gaussian operations are hard to implement in a multimode scenario. Here, we report the first generation of non-Gaussian quantum states of a multimode light field by subtracting a photon in a desired mode from multimode Gaussian states, and observe negativity of the Wigner function. For entangled Gaussian states, we observe that photon subtraction makes non-Gaussianity spread among various entangled modes. In addition to applications in quantum technologies, our results shed new light on non-Gaussian multimode entanglement with particular emphasis on quantum networks.

Graph states are the backbone of measurement-based continuous-variable quantum computation. However, experimental realisations of these states induce Gaussian measurement statistics for the field quadratures, which poses a barrier to obtain a genuine quantum advantage. In this letter, we propose mode-selective photon addition and subtraction as viable and experimentally feasible pathways to introduce non-Gaussian features in such continuous-variable graph states. In particular, we investigate how the non-Gaussian properties spread among the vertices of the graph, which allows us to show the degree of control that is achievable in this approach., Comment: 5 pages, 3 figures

Several distinct classes of unitary mode transformations have been known to exhibit the strict suppression of a large set of transmission events, as a consequence of totally destructive many-particle interference. In another work [Dittel et al., Phys. Rev. Lett. 120, 240404 (2018)] we unite these cases by identifying a general class of unitary matrices which exhibit such interferences. Here, we provide a detailed theoretical analysis that substantially expands on all aspects of this generalisation: We prove the suppression laws put forward in our other paper, establish how they interrelate with forbidden single-particle transitions, show how all suppression laws hitherto known can be retrieved from our general formalism, and discuss striking differences between bosons and fermions. Furthermore, beyond many-particle Fock states on input, we consider arbitrary pure initial states and derive suppression laws which stem from the wave function's permutation symmetry alone. Finally, we identify conditions for totally destructive interference to persist when the involved particles become partially distinguishable., Comment: 16 pages, 4 figures

In a general, multi-mode scattering setup, we show how the permutation symmetry of a many-particle input state determines those scattering unitaries which exhibit strictly suppressed many-particle transition events. We formulate purely algebraic suppression laws that identify these events and show that the many-particle interference at their origin is robust under weak disorder and imperfect indistinguishability of the interfering particles. Finally, we demonstrate that all suppression laws so far described in the literature are embedded in the general framework that we here introduce., Comment: 6 pages, 2 figures

The addition or subtraction of a photon from a Gaussian state of light is a versatile and experimentally feasible procedure to create non-Gaussian states. In multimode setups, these states manifest a wide range of phenomena when the photon is added or subtracted in a mode-tunable way. In this contribution, we derive the truncated correlations, which are multimode generalisations of cumulants, between quadratures in different modes as statistical signatures of these states. These correlations are then used to obtain the full multimode Wigner function, the properties of which are subsequently studied. In particular we investigate the effect of impurity in the subtraction or addition process, and evaluate its impact on the negativity of the Wigner function. Finally, we elaborate on the generation of inherent entanglement through subtraction or addition of a photon from a pure squeezed vacuum., Comment: 27 pages (incl. appendix), 6 figures

Non-Gaussian operations are essential to exploit the quantum advantages in optical continuous variable quantum information protocols. We focus on mode-selective photon addition and subtraction as experimentally promising processes to create multimode non-Gaussian states. Our approach is based on correlation functions, as is common in quantum statistical mechanics and condensed matter physics, mixed with quantum optics tools. We formulate an analytical expression of the Wigner function after subtraction or addition of a single photon, for arbitrarily many modes. It is used to demonstrate entanglement properties specific to non-Gaussian states, and also leads to a practical and elegant condition for Wigner function negativity. Finally, we analyse the potential of photon addition and subtraction for an experimentally generated multimode Gaussian state.

We present a scattering theory for the efficient transmission of an excitation across a finite network with designed disorder. We show that the presence of randomly positioned networks sites allows to significantly accelerate the excitation transfer processes as compared to a dimer structure, if only the disordered Hamiltonians are constrained to be centrosymmetric, and to exhibit a dominant doublet in their spectrum. We identify the cause of this efficiency enhancement in the constructive interplay between disorder-induced fluctuations of the dominant doublet's splitting and the coupling strength between the input and output sites to the scattering channels. We find that the characteristic strength of these fluctuations together with the channel coupling fully control the transfer efficiency., Comment: 9 pages, 7 figures

We establish a mathematically rigorous, general and quantitative framework to describe currents of non- (or weakly) interacting, indistinguishable particles driven far from equilibrium. We derive tight upper and lower bounds for the achievable fermionic and bosonic steady state current, respectively, which can serve as benchmarks for special cases of interacting many-particle dynamics. For fermionic currents, we identify a symmetry-induced enhancement mechanism in parameter regimes where the coupling between system and reservoirs is weak. This mechanism is broadly applicable provided the inter-particle interaction strength is small as compared to typical exchange interactions.

We show how robust statistical features of a many-particle quantum state's two-point correlations after transmission through a multi-mode random scatterer can be used as a sensitive probe of the injected particles' mutual indistinguishability. This generalises Hong-Ou-Mandel interference as a diagnostic tool for many-particle transmission signals across multi-mode random scatterers. Furthermore, we show how, from such statistical features of the many-particle interference pattern, information can be deduced on the temporal structure of the many-particle input state, by inspection of the many-particle interference with an additional probe particle of tuneable distinguishability.

One of the most pertinent problems in the debate on non-trivial quantum effects in biology concerns natural photosynthesis. Since sunlight is composed of thermal photons, it was argued to be unable to induce quantum coherence in matter, and that quantum mechanics is therefore irrelevant for the dynamical processes following photoabsorption. Our present analysis of a toy ``molecular aggregate" -- composed of two dipole-dipole interacting two-level atoms treated as an open quantum system -- however shows that incoherent excitations indeed can trigger coherent dynamics that persist: We demonstrate that collective decay processes induced by the dipole-dipole interaction create coherent intermolecular transport -- regardless of the coherence properties of the incoming radiation. Our analysis shows that the steady state coherence is mediated by the population imbalance between the molecules and, therefore, {\it increases} with the energy difference between the two-level atoms. Our results establish the importance of collective decay processes in the study of ultrafast photophysics, and especially their potential role to generate stationary coherence in incoherently driven quantum transport., Comment: 10 pages, 3 figures