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Monopoles and braids are exotic but elusive aspects of fundamental theories of light and matter. In lattice systems, monopoles of band-structure degeneracies are subject to well-established no-go (doubling) theorems that appear to universally apply in closed Hermitian systems and open non-Hermitian systems alike. However, the non-Abelian braid topology of non-Hermitian multi-band systems provides a remarkable loophole to these constraints. Here we make use of this loophole, and experimentally implement, for the first time, a monopole degeneracy in a non-Hermitian three-band system in the form of a single third-order exceptional point. We explicitly demonstrate the intricate braiding topology and the non-Abelian fusion rules underlying the monopole degeneracy. The experiment is carried out using a new design of single-photon interferometry, enabling eigenstate and spectral resolutions for non-Hermitian multi-band systems with widely tunable parameters. Thus, the union of state-of-the-art experiments, fundamental theory, and everyday concepts such as braids paves the way toward the highly exotic non-Abelian topology unique to non-Hermitian settings., Comment: 11 pages, 7 figures

The Yang-Lee edge singularity was originally studied from the standpoint of mathematical foundations of phase transitions, and its physical demonstration has been of active interest both theoretically and experimentally. However, the presence of an imaginary magnetic field in the Yang-Lee edge singularity has made it challenging to develop a direct observation of the anomalous scaling with negative scaling dimension associated with this critical phenomenon. We experimentally implement an imaginary magnetic field and demonstrate the Yang-Lee edge singularity through a nonunitary evolution governed by a non-Hermitian Hamiltonian in an open quantum system, where a classical system is mapped to a quantum system via the equivalent canonical partition function. In particular, we directly observe the partition function in our experiment using heralded single photons. The nonunitary quantum criticality is identified with the singularity at an exceptional point. We also demonstrate unconventional scaling laws for the finite-temperature dynamics unique to quantum systems., Comment: 11 pages, 9 figures

Dynamic behaviors of a physical system often originate from its spectral properties. In open systems, where the effective non-Hermitian description enables a wealth of spectral structures on the complex plane, the concomitant dynamics is significantly enriched, whereas the identification and comprehension of the underlying connections are challenging. Here we experimentally demonstrate the correspondence between the transient self acceleration of local excitations and the non-Hermitian spectral topology using lossy photonic quantum walks. Focusing first on one-dimensional quantum walks, we show that the measured short-time acceleration of the wave function is proportional to the area enclosed by the eigenspectrum. We then reveal similar correspondence in two-dimension quantum walks, where the self acceleration is proportional to the volume enclosed by the eigenspectrum in the complex parameter space. In both dimensions, the transient self acceleration crosses over to a long-time behavior dominated by a constant flow at the drift velocity. Our results unveil the universal correspondence between spectral topology and transient dynamics, and offer a sensitive probe for phenomena in non-Hermitian systems that originate from spectral geometry., Comment: 12 pages, 6 figures

Exceptional points (EPs) of non-Hermitian (NH) systems have recently attracted increasing attention due to their rich phenomenology and intriguing applications. Compared to the predominantly studied second-order EPs, higher-order EPs have been assumed to play a much less prominent role because they generically require the tuning of more parameters. Here we experimentally simulate two-dimensional topological NH band structures using single-photon interferometry, and observe topologically stable third-order EPs obtained by tuning only two real parameters in the presence of symmetry. In particular, we explore how different symmetries stabilize qualitatively different third-order EPs: the parity-time symmetry leads to a generic cube-root dispersion, while a generalized chiral symmetry implies a square-root dispersion coexisting with a flat band. Additionally, we simulate fourfold degeneracies, composed of the non-defective twofold degeneracies and second-order EPs. Our work reveals the abundant and conceptually richer higher-order EPs protected by symmetries and offers a versatile platform for further research on topological NH systems., Comment: 15 pages, 9 figures

Non-Hermiticity significantly enriches the properties of topological models, leading to exotic features such as the non-Hermitian skin effects and non-Bloch bulk-boundary correspondence that have no counterparts in Hermitian settings. Its impact is particularly illustrating in non-Hermitian quasicrystals where the interplay between non-Hermiticity and quasiperiodicity results in the concurrence of the delocalization-localization transition, the parity-time (PT)-symmetry breaking, and the onset of the non-Hermitian skin effects. Here we experimentally simulate non-Hermitian quasicrystals using photonic quantum walks. Using dynamic observables, we demonstrate that the system can transit from a delocalized, PT-symmetry broken phase that features non-Hermitian skin effects, to a localized, PT-symmetry unbroken phase with no non-Hermitian skin effects. The measured critical point is consistent with the theoretical prediction through a spectral winding number, confirming the topological origin of the phase transition. Our work opens the avenue of investigating the interplay of non-Hermiticity, quasiperiodicity, and spectral topology in open quantum systems., Comment: 10 pages, 7 figures. In the updated version, we add new experimental evidence for the presence of a mobility edge in quantum-walk dynamics

Disorder and non-Hermiticity dramatically impact the topological and localization properties of a quantum system, giving rise to intriguing quantum states of matter. The rich interplay of disorder, non-Hermiticity, and topology is epitomized by the recently proposed non-Hermitian topological Anderson insulator that hosts a plethora of exotic phenomena. Here we experimentally simulate the non-Hermitian topological Anderson insulator using disordered photonic quantum walks, and characterize its localization and topological properties. In particular, we focus on the competition between Anderson localization induced by random disorder, and the non-Hermitian skin effect under which all eigenstates are squeezed toward the boundary. The two distinct localization mechanisms prompt a non-monotonous change in profile of the Lyapunov exponent, which we experimentally reveal through dynamic observables. We then probe the disorder-induced topological phase transitions, and demonstrate their biorthogonal criticality. Our experiment further advances the frontier of synthetic topology in open systems., Comment: 15 pages, 11 figures

Non-Bloch topological invariants preserve the bulk-boundary correspondence in non-Hermitian topological systems, and are a key concept in the contemporary study of non-Hermitian topology. Here we report the dynamic detection of non-Bloch topological invariants in single-photon quantum walks, revealed through the biorthogonal chiral displacement, and crosschecked with the dynamic spin textures in the generalized quasimomentum-time domain following a quantum quench. Both detection schemes are robust against symmetry-preserving disorders, and yield consistent results with theoretical predictions. Our experiments are performed far away from any boundaries, and therefore underline non-Bloch topological invariants as intrinsic properties of the system that persist in the thermodynamic limit. Our work sheds new light on the experimental investigation of non-Hermitian topology., Comment: 14 pages, 11 figures

Non-Hermitian systems with parity-time ($\mathcal{PT}$) symmetry give rise to exceptional points (EPs) with exceptional properties that arise due to the coalescence of eigenvectors. Such systems have been extensively explored in the classical domain, where second or higher order EPs have been proposed or realized. In contrast, quantum information studies of $\mathcal{PT}$-symmetric systems have been confined to systems with a two-dimensional Hilbert space. Here by using a single-photon interferometry setup, we simulate quantum dynamics of a four-dimensional $\mathcal{PT}$-symmetric system across a fourth-order exceptional point. By tracking the coherent, non-unitary evolution of the density matrix of the system in $\mathcal{PT}$-symmetry unbroken and broken regions, we observe the entropy dynamics for both the entire system, and the gain and loss subsystems. Our setup is scalable to the higher-dimensional $\mathcal{PT}$-symmetric systems, and our results point towards the rich dynamics and critical properties., Comment: 7 pages, 5 figures

We experimentally simulate in a photonic setting non-Hermitian (NH) metals characterized by the topological properties of their nodal band structures. Implementing nonunitary time evolution in reciprocal space followed by interferometric measurements, we probe the complex eigenenergies of the corresponding NH Bloch Hamiltonians, and study in detail the topology of their exceptional lines (ELs), the NH counterpart of nodal lines in Hermitian systems. We focus on two distinct types of NH metals: two-dimensional systems with symmetry-protected ELs, and three-dimensional systems possessing symmetry-independent topological ELs in the form of knots. While both types feature open Fermi surfaces, we experimentally observe their distinctions by analyzing the impact of symmetry-breaking perturbations on the topology of ELs., Comment: 14 pages, 14 figures

Parity-time (PT)-symmetric Hamiltonians have widespread significance in non-Hermitian physics. A PT-symmetric Hamiltonian can exhibit distinct phases with either real or complex eigenspectrum, while the transition points in between, the so-called exceptional points, give rise to a host of critical behaviors that holds great promise for applications. For spatially periodic non-Hermitian systems, PT symmetries are commonly characterized and observed in line with the Bloch band theory, with exceptional points dwelling in the Brillouin zone. Here, in nonunitary quantum walks of single photons, we uncover a novel family of exceptional points beyond this common wisdom. These "non-Bloch exceptional points" originate from the accumulation of bulk eigenstates near boundaries, known as the non-Hermitian skin effect, and inhabit a generalized Brillouin zone. Our finding opens the avenue toward a generalized PT-symmetry framework, and reveals the intriguing interplay between PT symmetry and non-Hermitian skin effect., Comment: 12 pages, 7 figures

Non-Hermitian descriptions of quantum matter have seen impressive progress recently, with major advances in understanding central aspects such as their topological properties or the physics of exceptional points, the non-Hermitian counterpart of critical points. Here, we use single-photon interferometry to reconstruct the non-Hermitian Kibble-Zurek mechanism and its distinct scaling behavior for exceptional points, by simulating the defect production upon performing slow parameter ramps. Importantly, we are able to realise also higher-order exceptional points, providing experimental access to their theoretically predicted characteristic Kibble-Zurek scaling behaviour. Our work represents a crucial step in increasing the experimental complexity of non-Hermitian quantum time-evolution. It thus also furthers the quest to move the frontier from purely single-particle physics towards increasingly complex settings in the many-body realm., Comment: 8 pages, 6 figures

Quantum machine learning aspires to overcome intractability that currently limits its applicability to practical problems. However, quantum machine learning itself is limited by low effective dimensions achievable in state-of-the-art experiments. Here we demonstrate highly successful classifications of real-life images using photonic qubits, combining a quantum tensor-network representation of hand-written digits and entanglement-based optimization. Specifically, we focus on binary classification for hand-written zeroes and ones, whose features are cast into the tensor-network representation, further reduced by optimization based on entanglement entropy and encoded into two-qubit photonic states. We then demonstrate image classification with a high success rate exceeding 98%, through successive gate operations and projective measurements. Although we work with photons, our approach is amenable to other physical realizations such as nitrogen-vacancy centers, nuclear spins and trapped ions, and our scheme can be scaled to efficient multi-qubit encodings of features in the tensor-product representation, thereby setting the stage for quantum-enhanced multi-class classification., Comment: 10 pages, 7 figures

We demonstrate one-sided device-independent self-testing of any pure entangled two-qubit state based on a fine-grained steering inequality. The maximum violation of a fine-grained steering inequality can be used to witness certain steerable correlations, which certify all pure two-qubit entangled states. Our experimental results identify which particular pure two-qubit entangled state has been self-tested and which measurement operators are used on the untrusted side. Furthermore, we analytically derive the robustness bound of our protocol, enabling our subsequent experimental verification of robustness through state tomography. Finally, we ensure that the requisite no-signalling constraints are maintained in the experiment., Comment: 12 pages, 8 figures, accepted version

Recently, an inequality satisfied by non-contextual hidden-variable models and violated by quantum mechanics for all states of a four-level system has been derived based on information-theoretic distance approach to non-classical correlations. In this work, we experimentally demonstrate violation of this inequality with single photons. Our experiment offers a method to study a distinction between quantum and classical correlations from an information-theoretic perspective., Comment: 6 pages, 4 figures

The canonical Robertson-Schr\"{o}dinger uncertainty relation provides a loose bound for the product of variances of two non-commuting observables. Recently, several tight forward and reverse uncertainty relations have been proved which go beyond the traditional uncertainty relations. Here we experimentally test multifold of state-dependent uncertainty relations for the product as well as the sum of variances of two incompatible observables for photonic qutrits. These uncertainty relations are independent of any optimization and still tighter than the Robertson-Schr\"{o}dinger uncertainty relation and other ones found in current literatures. For the first time, we also test the state-dependent reverse uncertainty relations for the sum of variances of two incompatible observables, which implies another unique feature of preparation uncertainty in quantum mechanics. Our experimental results not only foster insight into a fundamental limitation on preparation uncertainty but also may contribute to the study of upper limit of precession measurements for incompatible observables., Comment: Latex file, 5 pages, 4 Figs

We experimentally realize a nonlinear quantum protocol on single-photon qubits with linear optical elements and appropriate measurements. The quantum nonlinearity is induced by post-selecting the polarization qubit based on a measurement result obtained on the spatial degree of freedom of the single photon which plays the role of a second qubit. Initially, both qubits are prepared in the same quantum state and an appropriate two-qubit unitary transformation entangles them before the measurement on the spatial part. We analyze the result by quantum state tomography on the polarization degree of freedom. We then demonstrate the usefulness of the protocol for quantum state discrimination by iteratively applying it on either one of two slightly different quantum states which rapidly converge to different orthogonal states by the iterative dynamics. Our work opens the door to employ effective quantum nonlinear evolution for quantum information processing., Comment: 6 pages, 3 figures

Bulk-boundary correspondence, a central principle in topological matter relating bulk topological invariants to edge states, breaks down in a generic class of non-Hermitian systems that have so far eluded experimental effort. Here we theoretically predict and experimentally observe non-Hermitian bulk-boundary correspondence, a fundamental generalization of the conventional bulk-boundary correspondence, in discrete-time non-unitary quantum-walk dynamics of single photons. We experimentally demonstrate photon localizations near boundaries even in the absence of topological edge states, thus confirming the non-Hermitian skin effect. Facilitated by our experimental scheme of edge-state reconstruction, we directly measure topological edge states, which match excellently with non-Bloch topological invariants calculated from localized bulk-state wave functions. Our work unequivocally establishes the non-Hermitian bulk-boundary correspondence as a general principle underlying non-Hermitian topological systems, and paves the way for a complete understanding of topological matter in open systems., Comment: 15 pages, 9 figures

Topological edge states arise in parity-time ($\mathcal{PT}$)-symmetric non-unitary quantum dynamics but have so far only been discussed in the $\mathcal{PT}$-symmetry-unbroken regime. Here we report the experimental detection of robust topological edge states in one-dimensional photonic quantum walks with spontaneously broken $\mathcal{PT}$ symmetry, thus establishing the existence of topological phenomena therein. We theoretically prove and experimentally confirm that the global Berry phase in non-unitary quantum-walk dynamics unambiguously defines topological invariants of the system in both the $\mathcal{PT}$-symmetry-unbroken and broken regimes. As topological edge states exist in both $\mathcal{PT}$ unbroken and broken regimes, we reveal that topological phenomena are not driven by $\mathcal{PT}$ symmetry., Comment: 15 pages, 7 figures

Conserved quantities such as energy or the electric charge of a closed system, or the Runge-Lenz vector in Kepler dynamics are determined by its global, local, or accidental symmetries. They were instrumental to advances such as the prediction of neutrinos in the (inverse) beta decay process and the development of self-consistent approximate methods for isolated or thermal many-body systems. In contrast, little is known about conservation laws and their consequences in open systems. Recently, a special class of these systems, called parity-time ($\mathcal{PT}$) symmetric systems, has been intensely explored for their remarkable properties that are absent in their closed counterparts. A complete characterization and observation of conserved quantities in these systems and their consequences is still lacking. Here we present a complete set of conserved observables for a broad class of $\mathcal{PT}$-symmetric Hamiltonians and experimentally demonstrate their properties using single-photon linear optical circuit. By simulating the dynamics of a four-site system across a fourth-order exceptional point, we measure its four conserved quantities and demonstrate their consequences. Our results spell out non-local conservation laws in non-unitary dynamics and provide key elements that will underpin self-consistent analysis of non-Hermitian quantum many-body systems that are forthcoming., Comment: 7 pages, 3 figures

We experimentally simulate non-unitary quantum dynamics using a single-photon interferometric network and study the information flow between a parity-time (PT)-symmetric non-Hermitian system and its environment. We observe oscillations of quantum-state distinguishability and complete information retrieval in the PT-symmetry-unbroken regime. We then characterize in detail critical phenomena of the information flow near the exceptional point separating the PT-unbroken and -broken regimes, and demonstrate power-law behavior in key quantities such as the distinguishability and the recurrence time. We also reveal how the critical phenomena are affected by symmetry and initial conditions. Finally, introducing an ancilla as an environment and probing quantum entanglement between the system and the environment, we confirm that the observed information retrieval is induced by a finite-dimensional entanglement partner in the environment. Our work constitutes the first experimental characterization of critical phenomena in PT-symmetric non-unitary quantum dynamics., Comment: 10 pages, 8 figures, new experimental results added

Topological matter exhibits exotic properties yet phases characterized by large topological invariants are difficult to implement, despite rapid experimental progress. A promising route toward higher topological invariants is via engineered Floquet systems, particularly in photonics, where flexible control holds the potential of extending the study of conventional topological matter to novel regimes. Here we implement a one-dimensional photonic quantum walk to explore large winding numbers. By introducing partial measurements and hence loss into the system, we detect winding numbers of three and four in multi-step non-unitary quantum walks, which agree well with theoretical predictions. Moreover, by probing statistical moments of the walker, we identify locations of topological phase transitions in the system, and reveal the breaking of pseudo-unitary near topological phase boundaries. As the winding numbers are associated with non-unitary time evolution, our investigation enriches understanding of topological phenomena in non-unitary settings., Comment: 15 pages, 12 figures

Topology in quench dynamics gives rise to intriguing dynamic topological phenomena, which are intimately connected to the topology of static Hamiltonians yet challenging to probe experimentally. Here we experimentally detect momentum-time skyrmions in parity-time (PT)-symmetric non-unitary quench dynamics, which are protected by dynamic Chern numbers defined for the emergent momentum-time manifold. Specifically, we experimentally simulate non-unitary quench dynamics of PT-symmetric topological systems using single-photon discrete-time quantum walks, and demonstrate emergence of skyrmions by constructing the time-dependent non-Hermitian density matrix via direct measurements in position space. Our work experimentally reveals the interplay of PT symmetry and quench dynamics in inducing emergent topological structures, and highlights the application of discrete-time quantum walks for the study of dynamic topological phenomena., Comment: 11 pages, 6 figures

Signaled by non-analyticities in the time evolution of physical observables, dynamic quantum phase transitions (DQPTs) emerge in quench dynamics of topological systems and possess an interesting geometric origin captured by dynamic topological order parameters (DTOPs). In this work, we report the experimental study of DQPTs using discrete-time quantum walks of single photons. We simulate quench dynamics between distinct Floquet topological phases using quantum-walk dynamics, and experimentally characterize DQPTs and the underlying DTOPs through interference-based measurements. The versatile photonic quantum-walk platform further allows us to experimentally investigate DQPTs for mixed states and in parity-time-symmetric non-unitary dynamics for the first time. Our experiment directly confirms the relation between DQPTs and DTOPs in quench dynamics of a topological system, and opens up the avenue of simulating emergent topological phenomena using discrete-time quantum-walk dynamics., Comment: 13 pages, 8 figures

We realise a quantum three-level system with photons distributed among three different spatial and polarization modes. Ambiguous measurement of the state of the qutrit are realised by blocking one out for the three modes at any one time. Using these measurements we construct a test of a Leggett-Garg inequality as well as tests of no-signalling-in-time for the measurements. We observe violations of the Leggett-Garg inequality that can not be accounted for in terms of signalling. Moreover, we tailor the qutrit dynamics such that both ambiguous and unambiguous measurements are simultaneously non-signalling, which is an essential step for the justification of the use of ambiguous measurements in Leggett-Garg tests., Comment: 7 pages, 4 figures