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The first loading of gadolinium (Gd) into Super-Kamiokande in 2020 was successful, and the neutron capture efficiency on Gd reached 50\%. To further increase the Gd neutron capture efficiency to 75\%, 26.1 tons of $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ was additionally loaded into Super-Kamiokande (SK) from May 31 to July 4, 2022. As the amount of loaded $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ was doubled compared to the first loading, the capacity of the powder dissolving system was doubled. We also developed new batches of gadolinium sulfate with even further reduced radioactive impurities. In addition, a more efficient screening method was devised and implemented to evaluate these new batches of $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$. Following the second loading, the Gd concentration in SK was measured to be $333.5\pm2.5$ ppm via an Atomic Absorption Spectrometer (AAS). From the mean neutron capture time constant of neutrons from an Am/Be calibration source, the Gd concentration was independently measured to be 332.7 $\pm$ 6.8(sys.) $\pm$ 1.1(stat.) ppm, consistent with the AAS result. Furthermore, during the loading the Gd concentration was monitored continually using the capture time constant of each spallation neutron produced by cosmic-ray muons,and the final neutron capture efficiency was shown to become 1.5 times higher than that of the first loaded phase, as expected., Comment: 34 pages, 13 figures, submitted to Nuclear Inst. and Methods in Physics Research, A

Exquisite sensitivities are a prominent advantage of quantum sensors. Ramsey sequences allow precise measurement of direct current fields, while Hahn-echo-like sequences measure alternating current fields. However, the latter are restrained for use with high-frequency fields (above approximately $1$ kHz) due to finite coherence times, leaving less-sensitive noncoherent methods for the low-frequency range. In this paper, we propose to bridge the gap with a fitting-based algorithm with a frequency-independent sensitivity to coherently measure low-frequency fields. As the algorithm benefits from coherence-based measurements, its demonstration with a single nitrogen-vacancy center gives a sensitivity of $9.4$ nT Hz$^{-0.5}$ for frequencies below about $0.6$ kHz down to near-constant fields. To inspect the potential in various scenarios, we apply the algorithm at a background field of tens of nTs, and we measure low-frequency signals via synchronization., Comment: 12 pages, 5 figures; supp 14 pages, 9 figures

Creation of nitrogen-vacancy (NV) centers at the nanoscale surface region in diamond, while retaining their excellent spin and optical properties, is essential for applications in quantum technology. Here, we demonstrate the extension of the spin-coherence time ($\it{T}$${_2}$), the stabilization of the charge state, and an improvement of the creation yield of NV centers formed by the ion-implantation technique at a depth of $\sim$15 nm in phosphorus-doped n-type diamond. The longest $\it{T}$${_2}$ of about 580 $\mu$s of a shallow NV center approaches the one in bulk diamond limited by the nuclear spins of natural abundant $^{13}$C. The averaged $\it{T}$${_2}$ in n-type diamond is over 1.7 times longer than that in pure non-doped diamond. Moreover, the stabilization of the charge state and the more than twofold improvement of the creation yield are confirmed. The enhancements for the shallow NV centers in an n-type diamond-semiconductor are significant for future integrated quantum devices., Comment: 21 pages, 5 figures, 1 table

Single crystal, nanoscale diamond membranes are highly sought after for a variety of applications including nanophotonics, nanoelectronics and quantum information science. However, so far, the availability of conductive diamond membranes remained an unreachable goal. In this work we present a complete nanofabrication methodology for engineering high aspect ratio, electrically active single crystal diamond membranes. The membranes have large lateral directions, exceeding 500x500 um2 and are only several hundreds of nanometers thick. We further realize vertical single crystal p-n junctions, made from the diamond membranes that exhibit onset voltages of ~ 10V and a current of several mA. Moreover, we deterministically introduce optically active color centers into the membranes, and demonstrate for the first time a single crystal nanoscale diamond LED. The robust and scalable approach to engineer the electrically active single crystal diamond membranes, offers new pathways for advanced nanophotonics, nanoelectronics and optomechanics devices employing diamond.

In recent years, millisecond duration radio signals originating from distant galaxies appear to have been discovered in the so-called Fast Radio Bursts. These signals are dispersed according to a precise physical law and this dispersion is a key observable quantity which, in tandem with a redshift measurement, can be used for fundamental physical investigations. While every fast radio burst has a dispersion measurement, none before now have had a redshift measurement, due to the difficulty in pinpointing their celestial coordinates. Here we present the discovery of a fast radio burst and the identification of a fading radio transient lasting $\sim 6$ days after the event, which we use to identify the host galaxy; we measure the galaxy's redshift to be $z=0.492\pm0.008$. The dispersion measure and redshift, in combination, provide a direct measurement of the cosmic density of ionised baryons in the intergalactic medium of $\Omega_{\mathrm{IGM}}=4.9 \pm 1.3\%$, in agreement with the expectation from WMAP, and including all of the so-called "missing baryons". The $\sim6$-day transient is largely consistent with a short gamma-ray burst radio afterglow, and its existence and timescale do not support progenitor models such as giant pulses from pulsars, and supernovae. This contrasts with the interpretation of another recently discovered fast radio burst, suggesting there are at least two classes of bursts., Comment: Published in Nature, 2016 Feb 25

Nitrogen-vacancy (NV) centers in diamond have attracted significant interest because of their excellent spin and optical characteristics for quantum information and metrology. To take advantage of the characteristics, the precise control of the orientation of the N-V axis in the lattice is essential. Here we show that the orientation of more than 99 % of the NV centers can be aligned along the [111]-axis by CVD homoepitaxial growth on (111)-substrates. We also discuss about mechanisms of the alignment. Our result enables a fourfold improvement in magnetic-field sensitivity and opens new avenues to the optimum design of NV center devices., Comment: 14 pages, 4 figures, To be published in Applied Physics Express

The dynamics of single electron and nuclear spins in a diamond lattice with different 13C nuclear spin concentration is investigated. It is shown that coherent control of up to three individual nuclei in a dense nuclear spin cluster is feasible. The free induction decays of nuclear spin Bell states and single nuclear coherences among 13C nuclear spins are compared and analyzed. Reduction of a free induction decay time T2* and a coherence time T2 upon increase of nuclear spin concentration has been found. For diamond material with depleted concentration of nuclear spin, T2* as long as 30 microseconds and T2 of up to 1.8 ms for the electron spin has been observed. The 13C concentration dependence of T2* is explained by Fermi contact and dipolar interactions with nuclei in the lattice. It has been found that T2 decreases approximately as 1/n, where n is 13C concentration, as expected for an electron spin interacting with a nuclear spin bath., Comment: 4 pages, 4 figures, 1 movie (avi), 1 supplementary material (pdf)