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Intra-seasonal variability of smoke aerosol optical depth (AOD) and downwelling solar irradiance at the surface during the 2002 biomass burning season in South America was modeled using the Coupled Chemistry-Aerosol-Tracers Transport model with the Brazilian developments on the Regional Atmospheric Modeling System (CCATT-BRAMS). Measurements of total and fine mode fraction (FMF) AOD from the AErosol RObotic NETwork (AERONET) and solar irradiance at the surface from the Solar Radiation Network (SolRad-NET) were used to evaluate model results. In general, the major features associated with AOD evolution over the southern part of the Amazon basin and cerrado ecosystem are captured by the model. The main discrepancies were found for high aerosol loading events. In the northeastern portion of the Amazon basin the model systematically underestimated total AOD, as expected, since smoke contribution is not dominant as it is in the southern portion and emissions other than smoke were not considered in the simulation. Better agreement was obtained comparing the model results with observed FMF AOD, which pointed out the relevance of coarse mode aerosol emission in that region. Likewise, major discrepancies over cerrado during high AOD events were found to be associated with coarse mode aerosol omission in our model. The issue of high aerosol loading events in the southern part of the Amazon was related to difficulties in predicting the smoke AOD field, which was discussed in the context of emissions shortcomings. The Cuiab'a cerrado site was the only one where the highest quality AERONET data were unavailable for both total and FMF AOD. Thus, lower quality data were used. Root-meansquare error (RMSE) between the model and observed FMF AOD decreased from 0.34 to 0.19 when extreme AOD events (FMF AOD550nm ≥ 1.0) and Cuiab'a were excluded from the analysis. Downward surface solar irradiance comparisons also followed similar trends when extreme AOD were excluded. This highlights the need to improve modelling of the regional smoke plume in order to enhance the accuracy of the radiative energy budget. An aerosol optical model based on the mean intensive properties of smoke from the southern part of the Amazon basin produced a radiative flux perturbation efficiency (RFPE) of -158Wm-2/AOD550nm at noon. This value falls between -154Wm-2/AOD550nm and -187Wm-2/AOD550nm, the range obtained when spatially varying optical models were considered. The 24 h average surface radiative flux perturbation over the biomass burning season varied from -55Wm-2 close to smoke sources in the southern part of the Amazon basin and cerrado to-10Wm-2 in remote regions of the southeast Brazilian coast. [ABSTRACT FROM AUTHOR]

Intra-seasonal variability of smoke aerosol optical depth (AOD) and downwelling solar irradiance at the surface during the 2002 biomass burning season in South America was modeled using the Coupled Chemistry-Aerosol-Tracer Transport model to the Brazilian developments on the Regional Atmospheric Modeling System (CCATT-BRAMS). Measurements of AOD from the AErosol RObotic NETwork (AERONET) and solar irradiance at the surface from the Solar Radiation Network (SolRad-NET) were used to evaluate model results. In general, the major features associated with AOD evolution over the southern part of the Amazon Basin and cerrado ecosystem are captured by the model. The main discrepancies were found for high aerosol loading events. In the northeastern portion of the Amazon Basin the model systematically underestimated AOD. This is likely due to the cloudy nature of the region, preventing accurate detection of the fire spots used in the emission model. Moreover, measured AOD were very often close to background conditions and emissions other than smoke were not considered in the simulation. Therefore, under the background scenario, one would expect the model to underestimate AOD. The issue of high aerosol loading events in the southern part of the Amazon and cerrado is also discussed in the context of emission shortcomings. The Cuiaba cerrado site was the only one where the highest quality AERONET data were unavailable. Thus, lower quality data were used. Root-mean-square-error (RMSE) between the model and observations decreased from 0.48 to 0.17 when extreme AOD events (AOD550nm ≥ 1.0) and Cuiaba were excluded from analysis. Downward surface solar irradiance comparisons also followed similar trends when extremes AOD were excluded. This highlights the need to improve the modelling of the regional smoke plume in order to enhance the accuracy of the radiative energy budget. Aerosol optical model based on the mean intensive properties of smoke from the southern part of the Amazon Basin produced a radiative forcing efficiency (RFE) of -158W m-2/AOD550nm at noon. This value is in between -154 W m-2/AOD550nm and -187W m-2/AOD550nm, the range obtained when spatial varying optical models were considered. The average 24 h surface forcing over the biomass burning season varied from -55Wm-2 close to smoke sources in the southern part of the Amazon Basin and cerrado to -10Wm-2 in remote regions of the Southeast Brazilian coast. [ABSTRACT FROM AUTHOR]