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In order to study the unique dynamic behavior of the lithium-ion battery system in the periodic high-rate pulse discharge, a frequency-domain impedance model and a dynamic extraction method of impedance parameters are proposed. Moreover, a 24-kWh lithium battery system is built to carry out the pulse-discharged cycle experiment. The harmonic characteristics in high and low frequency pulse discharge are studied by harmonic analysis method. Besides, the impedance characteristics of the 24-kWh lithium battery system under different state-of-charge and different cycles are analyzed quantitatively. The results show some new characteristics and verify that the proposed frequency-domain impedance model and impedance extraction method are well qualified to analyze the frequency-domain characteristics and dynamic behavior of the periodic pulse-discharged lithium battery system. [ABSTRACT FROM AUTHOR]