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We present a design and performance tests of an intense source of cold hydrogen atoms for loading large magnetic traps. Our source is based on a cryogenic dissociator of molecular hydrogen at 0.6 K followed by a series of thermal accommodators at 0.5, 0.2 and 0.13 K with inner surfaces covered by a superfluid helium film. All components are thermally anchored to corresponding stages of a dilution refrigerator. The source provides a continuous flux of 7$\cdot$$10^{13}$ H atoms/s in a temperature range of 130-200 mK. We have successfully used the source for loading a large Ioffe-Pritchard magnetic trap recently built in our laboratory [arXiv:2108.09123 or Rev. Sci. Instr. 93 (2), 023201 (2022)]. Calorimetric measurements of the atomic recombination heat allow reliable determination of the atomic flux and H gas density in the trap. We have tested the performance of the source and loading of H atoms into the trap at various configurations of the trapping field, reducing the magnetic barrier height to 75% and 50% of the nominal value of 0.8 T (0.54 K) as well as at the open configuration of the trap at its lower end, when the atoms are in contact with the trapping cell walls covered by a superfluid helium film. In the latter case, raising the trapping cell temperature to 200-250 mK, the low-field seeking atoms at densities exceeding 10$^{11}$ cm$^{-3}$ can be stored for the time over 1000 s, sufficiently long for experiments on precision spectroscopy of cold H gas.

A low energy particle confined by a horizontal reflective surface and gravity settles in gravitationally bound quantum states. These gravitational quantum states (GQS) were so far only observed with neutrons. However, the existence of GQS is predicted also for atoms. The GRASIAN collaboration pursues the first observation of GQS of atoms, using a cryogenic hydrogen beam. This endeavor is motivated by the higher densities, which can be expected from hydrogen compared to neutrons, the easier access, the fact that GQS were never observed with atoms and the accessibility to hypothetical short range interactions. In addition to enabling gravitational quantum spectroscopy, such a cryogenic hydrogen beam with very low vertical velocity components - a few cm s$^{-1}$, can be used for precision optical and microwave spectroscopy. In this article, we report on our methods developed to reduce background and to detect atoms with a low horizontal velocity, which are needed for such an experiment. Our recent measurement results on the collimation of the hydrogen beam to 2 mm, the reduction of background and improvement of signal-to-noise and finally our first detection of atoms with velocities < 72 m s$^{-1}$ are presented. Furthermore, we show calculations, estimating the feasibility of the planned experiment and simulations which confirm that we can select vertical velocity components in the order of cm s$^{-1}$.

In the search for clues to the matter-antimatter puzzle, experiments with atoms or molecules play a particular role. These systems allow measurements with very high precision, as demonstrated by the unprecedented limits down to $10^{-30}$ e.cm on electron EDM using molecular ions, and relative measurements at the level of $10^{-12}$ in spectroscopy of antihydrogen atoms. Building on these impressive measurements, new experimental directions offer potentials for drastic improvements. We review here some of the new perspectives in those fields and their associated prospects for new physics searches.

We report on an Yb:YAG thin-disk multipass amplifier delivering 50 ns long pulses at a central wavelength of 1030 nm with an energy of 330 mJ at a repetition rate of 100 Hz. The beam quality factor at the maximum energy was measured to be $\text{M}^2 = 1.17$. The small signal gain is 20, and the gain at 330 mJ was measured to be 6.9. The 20-pass amplifier is designed as a concatenation of stable resonator segments in which the beam is alternately Fourier transformed and relay-imaged back to the disk by a 4f-imaging optical scheme stage. The Fourier transform propagation makes the output beam robust against spherical phase front distortions, while the 4f-stage is used to compensate the thermal lens of the thin-disk and to reduce the footprint of the amplifier.

We report on the first production of an antihydrogen beam by charge exchange of 6.1 keV antiprotons with a cloud of positronium in the GBAR experiment at CERN. The antiproton beam was delivered by the AD/ELENA facility. The positronium target was produced from a positron beam itself obtained from an electron linear accelerator. We observe an excess over background indicating antihydrogen production with a significance of 3-4 standard deviations.

We demonstrate an injection-seeded thin-disk Yb:YAG laser at 1030 nm, stabilized by the Pound-Drever-Hall (PDH) method. We modified the PDH scheme to obtain an error signal free from Trojan locking points, which allowed robust re-locking of the laser and reliable long-term operation. The single-frequency pulses have 50 mJ energy (limited to avoid laser-induced damage) with a beam quality of $\text{M}^2$ < 1.1 and an adjustable length of 55-110 ns. Heterodyne measurements confirmed a spectral linewidth of 3.7 MHz. The short pulse build-up time (850 ns) makes this laser suitable for laser spectroscopy of muonic hydrogen, pursued by the CREMA collaboration.

We study the 1S-3S two-photon transition of hydrogen in a thermal atomic beam, using a homemade cw laser source at 205 nm. The experimental method is described, leading in 2017 to the measurement of the 1S-3S transition frequency in hydrogen atom with a relative uncertainty of $9 \times 10^{-13}$. This result contributes to the "proton puzzle" resolution but is in disagreement with the ones of some others experiments. We have recently improved our setup with the aim of carrying out the same measurement in deuterium. With the improved detection system, we have observed a broadened fluorescence signal, superimposed on the narrow signal studied so far, and due to the stray accumulation of atoms in the vacuum chamber. The possible resulting systematic effect is discussed.

At very low energies, a light neutral particle above a horizontal surface can experience quantum reflection. The quantum reflection holds the particle against gravity and leads to gravitational quantum states (GQS). So far, GQS were only observed with neutrons as pioneered by Nesvizhevsky and his collaborators at ILL. However, the existence of GQS is predicted also for atoms. The GRASIAN-collaboration pursues the first observation and studies of GQS of atomic hydrogen. We propose to use atoms in order to exploit the fact that orders of magnitude larger fluxes compared to those of neutrons are available. Moreover, recently the qBounce collaboration, performing GQS spectroscopy with neutrons, reported a discrepancy between theoretical calculations and experiment which deserves further investigations. For this purpose, we set up a cryogenic hydrogen beam at 6 K. We report on our preliminary results, characterizing the hydrogen beam with pulsed laser ionization diagnostics at 243 nm.

The CREMA collaboration is pursuing a measurement of the ground-state hyperfine splitting (HFS) in muonic hydrogen ($\mu$p) with 1 ppm accuracy by means of pulsed laser spectroscopy. In the proposed experiment, the $\mu$p atom is excited by a laser pulse from the singlet to the triplet hyperfine sub-levels, and is quenched back to the singlet state by an inelastic collision with a H$_2$ molecule. The resulting increase of kinetic energy after this cycle modifies the $\mu$p atom diffusion in the hydrogen gas and the arrival time of the $\mu$p atoms at the target walls. This laser-induced modification of the arrival times is used to expose the atomic transition. In this paper we present the simulation of the $\mu$p diffusion in the H$_2$ gas which is at the core of the experimental scheme. These simulations have been implemented with the Geant4 framework by introducing various low-energy processes including the motion of the H$_2$ molecules, i.e. the effects related with the hydrogen target temperature. The simulations have been used to optimize the hydrogen target parameters (pressure, temperatures and thickness) and to estimate signal and background rates. These rates allow to estimate the maximum time needed to find the resonance and the statistical accuracy of the spectroscopy experiment., Comment: Submission to SciPost

The Pound-Drever-Hall (PDH) technique is a popular method for stabilizing the frequency of a laser to a stable optical resonator or, vice versa, the length of a resonator to the frequency of a stable laser. We propose a refinement of the technique yielding an "infinite" dynamic (capture) range so that a resonator is correctly locked to the seed frequency, even after large perturbations. The stable but off-resonant lock points (also called Trojan operating points), present in conventional PDH error signals, are removed by phase modulating the seed laser at a frequency corresponding to half the free spectral range of the resonator. We verify the robustness of our scheme experimentally by realizing an injection-seeded Yb:YAG thin-disk laser. We also give an analytical formulation of the PDH error signal for arbitrary modulation frequencies and discuss the parameter range for which our PDH locking scheme guarantees correct locking. Our scheme is simple as it does not require additional electronics apart from the standard PDH setup and is particularly suited to realize injection-seeded lasers and injection-seeded optical parametric oscillators., Comment: 8 pages, 11 figures

We present a description of the GBAR positron (e+) trapping apparatus, which consists of a three stage Buffer Gas Trap (BGT) followed by a High Field Penning Trap (HFT), and discuss its performance. The overall goal of the GBAR experiment is to measure the acceleration of the neutral antihydrogen (H) atom in the terrestrial gravitational field by neutralising a positive antihydrogen ion (H+), which has been cooled to a low temperature, and observing the subsequent H annihilation following free fall. To produce one H+ ion, about 10^10 positrons, efficiently converted into positronium (Ps), together with about 10^7 antiprotons (p), are required. The positrons, produced from an electron linac-based system, are accumulated first in the BGT whereafter they are stacked in the ultra-high vacuum HFT, where we have been able to trap 1.4(2) x 10^9 positrons in 1100 seconds.

We present the commissioning of the Fast Annihilation Cryogenic Tracker detector (FACT), installed around the antihydrogen production trap inside the 1 T superconducting magnet of the AE\=gIS experiment. FACT is designed to detect pions originating from the annihilation of antiprotons. Its 794 scintillating fibers operate at 4 K and are read out by silicon photomultipliers (MPPCs) at near room temperature. FACT provides the antiproton/antihydrogen annihilation position information with a few ns timing resolution. We present the hardware and software developments which led to the successful operation of the detector for antihydrogen detection and the results of an antiproton-loss based efficiency assessment. The main background to the antihydrogen signal is that of the positrons impinging onto the positronium conversion target and creating a large amount of gamma rays which produce a sizeable signal in the MPPCs shortly before the antihydrogen signal is expected. We detail the characterization of this background signal and its impact on the antihydrogen detection efficiency.

The CREMA collaboration is pursuing a measurement of the ground-state hyperfine splitting (HFS) in muonic hydrogen ($\mu$p) with 1 ppm accuracy by means of pulsed laser spectroscopy to determine the two-photon-exchange contribution with $2\times10^{-4}$ relative accuracy. In the proposed experiment, the $\mu$p atom undergoes a laser excitation from the singlet hyperfine state to the triplet hyperfine state, {then} is quenched back to the singlet state by an inelastic collision with a H$_2$ molecule. The resulting increase of kinetic energy after the collisional deexcitation is used as a signature of a successful laser transition between hyperfine states. In this paper, we calculate the combined probability that a $\mu$p atom initially in the singlet hyperfine state undergoes a laser excitation to the triplet state followed by a collisional-induced deexcitation back to the singlet state. This combined probability has been computed using the optical Bloch equations including the inelastic and elastic collisions. Omitting the decoherence effects caused by {the laser bandwidth and }collisions would overestimate the transition probability by more than a factor of two in the experimental conditions. Moreover, we also account for Doppler effects and provide the matrix element, the saturation fluence, the elastic and inelastic collision rates for the singlet and triplet states, and the resonance linewidth. This calculation thus quantifies one of the key unknowns of the HFS experiment, leading to a precise definition of the requirements for the laser system and to an optimization of the hydrogen gas target where $\mu$p is formed and the laser spectroscopy will occur., Comment: 21 pages, 4 figures

We describe the design and performance of a large magnetic trap for storing and cooling of atomic hydrogen (H). The trap operates in the vacuum space of a dilution refrigerator at a temperature of 1.5 K. Aiming at a large volume of the trap we implemented the octupole configuration of linear currents (Ioffe bars) for the radial confinement, combined with two axial pinch coils and a 3 T solenoid for the cryogenic H dissociator. The octupole magnet consists of eight race-track segments which are compressed towards each other with magnetic forces. This provides a mechanically stable and robust construction with a possibility of replacement or repair of each segment. A maximum trap depth of 0.54 K (0.8 T) was reached, corresponding to an effective volume of 0.5 liters for hydrogen gas at 50 mK. This is an order of magnitude larger than ever used for trapping atoms.

The electric dipole moment of the electron (eEDM) can be measured with high precision using heavy polar molecules. In this paper, we report on a series of new techniques that have improved the statistical sensitivity of the YbF eEDM experiment. We increase the number of molecules participating in the experiment by an order of magnitude using a carefully designed optical pumping scheme. We also increase the detection efficiency of these molecules by another order of magnitude using an optical cycling scheme. In addition, we show how to destabilise dark states and reduce backgrounds that otherwise limit the efficiency of these techniques. Together, these improvements allow us to demonstrate a statistical sensitivity of $1.8 \times 10^{-28}$ e cm after one day of measurement, which is 1.2 times the shot-noise limit. The techniques presented here are applicable to other high-precision measurements using molecules., Comment: 22 pages, 11 figures

We investigate experimentally the possibility of enhancing the production of $2^3S$ positronium atoms by driving the $1^3S$-$3^3P$ and $3^3P$-$2^3S$ transitions, overcoming the natural branching ratio limitation of spontaneous decay from $3^3P$ to $2^3S$. The decay of $3^3P$ positronium atoms towards the $2^3S$ level has been effciently stimulated by a 1312.2nm broadband IR laser pulse. The dependence of the stimulating transition efficiency on the intensity of the IR pulse has been measured to find the optimal enhancement conditions. A maximum relative increase of $ \times (3.1 \pm 1.0) $ in the $2^3S$ production efficiency, with respect to the case where only spontaneous decay is present, was obtained., Comment: 6 pages, 4 figures

Positronium in the $2^3S$ metastable state exhibits a low electrical polarizability and a long lifetime (1140 ns) making it a promising candidate for interferometry experiments with a neutral matter-antimatter system. In the present work, $2^3S$ positronium is produced - in absence of electric field - via spontaneous radiative decay from the $3^3P$ level populated with a 205nm UV laser pulse. Thanks to the short temporal length of the pulse, 1.5 ns full-width at half maximum, different velocity populations of a positronium cloud emitted from a nanochannelled positron/positronium converter were selected by delaying the excitation pulse with respect to the production instant. $ 2^3S $ positronium atoms with velocity tuned between $ 7 \cdot 10^4 $ m/s and $ 10 \cdot 10^4 $ m/s were thus produced. Depending on the selected velocity, a $2^3S$ production effciency ranging from $\sim 0.8 \%$ to $\sim 1.7%$, with respect to the total amount of emitted positronium, was obtained. The observed results give a branching ratio for the $3^3P$-$2^3S$ spontaneous decay of $(9.7 \pm 2.7) \% $. The present velocity selection technique could allow to produce an almost monochromatic beam of $\sim 1 \cdot 10^3 $ $2^3S$ atoms with a velocity spread $ < 10^4 $ m/s and an angular divergence of $\sim$ 50 mrad., Comment: 6 pages, 3 figures, 1 table

Producing positronium (Ps) in the metastable $2^3\text{S}$ state is of interest for various applications in fundamental physics. We report here about an experiment in which Ps atoms are produced in this long-lived state by spontaneous radiative decay of Ps excited to the $3^3\text{P}$ level manifold. The Ps cloud excitation is obtained with a UV laser pulse in an experimental vacuum chamber in presence of guiding magnetic field of 25 mT and an average electric field of 300 V/cm. The indication of the $2^3\text{S}$ state production is obtained from a novel analysis technique of single-shot positronium annihilation lifetime spectra. Its production efficiency relative to the total amount of formed Ps is evaluated by fitting a simple rate equations model to the experimental data and found to be $ (2.1 \pm 1.3) \, \% $.

Experiments with antihydrogen ($\overline{\text{H}}$) for a study of matter--antimatter symmetry and antimatter gravity require ultracold $\overline{\text{H}}$ to reach ultimate precision. A promising path towards anti-atoms much colder than a few kelvin involves the pre-cooling of antiprotons by laser-cooled anions. Due to the weak binding of the valence electron in anions - dominated by polarization and correlation effects - only few candidate systems with suitable transitions exist. We report on a combination of experimental and theoretical studies to fully determine the relevant binding energies, transition rates and branching ratios of the most promising candidate La$^{-}$. Using combined transverse and collinear laser spectroscopy, we determined the resonant frequency of the laser cooling transition to be $\nu = 96.592\,713(91)$ THz and its transition rate to be $A = 4.90(50) \times 10^{4}$ s$^{-1}$. Using a novel high-precision theoretical treatment of La$^-$ we calculated yet unmeasured energy levels, transition rates, branching ratios, and lifetimes to complement experimental information on the laser cooling cycle of La$^-$. The new data establish the suitability of La$^-$ for laser cooling and show that the cooling transition is significantly stronger than suggested by a previous theoretical study., Comment: 5 pages, 4 figures

The characteristics of low energy antiproton annihilations on nuclei (e.g. hadronization and product multiplicities) are not well known, and Monte Carlo simulation packages that use different models provide different descriptions of the annihilation events. In this study, we measured the particle multiplicities resulting from antiproton annihilations on nuclei. The results were compared with predictions obtained using different models in the simulation tools GEANT4 and FLUKA. For this study, we exposed thin targets (Cu, Ag and Au) to a very low energy antiproton beam from CERN's Antiproton Decelerator, exploiting the secondary beamline available in the AEgIS experimental zone. The antiproton annihilation products were detected using emulsion films developed at the Laboratory of High Energy Physics in Bern, where they were analysed at the automatic microscope facility. The fragment multiplicity measured in this study is in good agreement with results obtained with FLUKA simulations for both minimally and heavily ionizing particles.

We propose a scheme for laser cooling of negatively charged molecules. We briefly summarise the requirements for such laser cooling and we identify a number of potential candidates. A detailed computation study with C$\_2^-$, the most studied molecular anion, is carried out. Simulations of 3D laser cooling in a gas phase show that this molecule could be cooled down to below 1 mK in only a few tens of milliseconds, using standard lasers. Sisyphus cooling, where no photo-detachment process is present, as well as Doppler laser cooling of trapped C$\_2^-$, are also simulated. This cooling scheme has an impact on the study of cold molecules, molecular anions, charged particle sources and antimatter physics.