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A novel net channel and N‐doping carbon aerogel (CA) are successfully prepared by an in situ and facile method via polyimide (PI) inducting for lithium–sulfur (Li–S) batteries. The PI‐directing carbon aerogel (PI‐CA) presents a cross‐linked framework, abundant porosity, and a high specific surface area. PI‐CA spheres present effective immobilizing polysulfides and high loading sulfur for a Brunauer–Emmett–Teller (BET) surface area of 2039.4 m2 g−1 and N‐doping via physical and chemical adsorption. The Li–S batteries with PI‐CA as cathode matrix exhibit excellent performance. In particular, the initial specific capacity of 2PI‐CA/S with sulfur content of 73.8 wt% delivers 1338 mAh g−1 and remains at 1102 mAh g−1 after 100 cycles at 0.2 C. The enhanced electrochemical performance mainly benefits from the mesh structure of the composite and the interaction between nitrogen and lithium polysulfide. The theoretical calculation by density functional theory (DFT) further supports the template effect of PI and the anchoring mechanism of polysulfides. [ABSTRACT FROM AUTHOR]

Error correction codes, such as low-density parity check (LDPC) codes, are required to be larger scale to meet the increasing demands for reliable and massive data transmission. However, the construction of such a large-scale decoder will result in high complexity and hinder its silicon implementation. Thanks to the advantages of natural computing in high parallelism and low power, we propose a method to synthesize a uniform molecular LDPC decoder by implementing the belief-propagation algorithm with chemical reaction networks (CRNs). This method enables us to flexibly design the LDPC decoder with arbitrary code length, code rate, and node degrees. Compared with existing methods, our proposal reduces the number of reactions to update the variable nodes by 42.86% and the check nodes by 47.37%. Numerical results are presented to show the feasibility and validity of our proposal.