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Focused ion beams are indispensable tools in the semiconductor industry because of their ability to image and modify structures at the nanometer length scale. Here, we report on performance predictions of a new type of focused ion beam based on photo-ionization of a laser cooled and compressed atomic beam. Particle tracing simulations are performed to investigate the effects of disorder-induced heating after ionization in a large electric field. They lead to a constraint on this electric field strength which is used as input for an analytical model which predicts the minimum attainable spot size as a function of, amongst others, the flux density of the atomic beam, the temperature of this beam, and the total current. At low currents (I<10 pA), the spot size will be limited by a combination of spherical aberration and brightness, while at higher currents, this is a combination of chromatic aberration and brightness. It is expected that a nanometer size spot is possible at a current of 1 pA. The analytical model was verified with particle tracing simulations of a complete focused ion beam setup. A genetic algorithm was used to find the optimum acceleration electric field as a function of the current. At low currents, the result agrees well with the analytical model, while at higher currents, the spot sizes found are even lower due to effects that are not taken into account in the analytical model. [ABSTRACT FROM AUTHOR]

A purpose-built RF-photogun as external electron injector for a laser wakefield accelerator has been thoroughly tested. Different properties of the RF-photogun have been measured such as energy, energy spread and transverse emittance. The focus of this study is the investigation of the smallest possible focus spot and focus stability at the entrance of the plasma channel. For an electron bunch with 10 pC charge and 3.7 MeV kinetic energy, the energy spread was 0.5% with a shot-to-shot stability of 0.05%. After focusing the bunch by a pulsed solenoid lens at 140 mm from the middle of the lens, the focal spot was 40 μm with a shot-to-shot stability of 5 μm. Higher charge leads to higher energy spread and to a larger spot size, due to space charge effects. All properties were found to be close to design values. Given the limited energy of 3.7 MeV, the properties are sufficient for this gun to serve as injector for one particular version of laser wakefield acceleration, i.e., injection ahead of the laser pulse. These measured electron bunch properties were then used as input parameters for simulations of electron bunch injection in a laser wakefield accelerator. The arrival time jitter was deduced from measurements of the energy fluctuation, in combination with earlier measurements using THz coherent transition radiation, and is around 150 fs in the present setup. The bunch length in the focus, simulated using particle tracking, depends on the accelerated charge and goes from 100 fs at 0.1 pC to 1 ps at 50 pC. When simulating the injection of the 3.7 MeV electron bunch of 10 pC in front of a 25 TW laser pulse with a waist of 30 μm in a plasma with a density of 0.7 × 1024 m-3, the maximum accelerated charge was found to be 1.2 pC with a kinetic energy of ∼900 MeV and an energy spread of ∼5%. The experiments combined with the simulations show the feasibility of external injection and give a prediction of the output parameters that can be expected from a laser wakefield accelerator with external injection of electrons. [ABSTRACT FROM AUTHOR]

The combination of an ultracold ion source based on photoionization of a laser-cooled gas and time-dependent acceleration fields enables precise manipulation of ion beams. We demonstrate reduction in the longitudinal energy spread and transverse (de)focusing of the beam by applying time-dependent acceleration voltages. In addition, we show how time-dependent acceleration fields can be used to control both the sign and strength of the spherical aberrations. The experimental results are in close agreement with detailed charged particle tracking simulations and can be explained in terms of a simple analytical model. [ABSTRACT FROM AUTHOR]

At present, the smallest spot size which can be achieved with state-of-the-art focused ion beam (FIB) technology is mainly limited by the chromatic aberrations associated with the 4.5 eV energy spread of the liquid-metal ion source. Here we numerically investigate the performance of an ultracold ion source which has the potential for generating ion beams which combine high brightness with small energy spread. The source is based on creating very cold ion beams by near-threshold photoionization of a laser-cooled and trapped atomic gas. We present ab initio numerical calculations of the generation of ultracold beams in a realistic acceleration field and including all Coulomb interactions, i.e., both space charge effects and statistical Coulomb effects. These simulations demonstrate that with existing technology reduced brightness values exceeding 105 A m-2 sr-1 V-1 are feasible at an energy spread as low as 0.1 eV. The estimated spot size of the ultracold ion source in a FIB instrument ranges from 10 nm at a current of 100 pA to 0.8 nm at 1 pA. [ABSTRACT FROM AUTHOR]

We present a method for producing sub-100 fs electron bunches that are suitable for single-shot ultrafast electron diffraction experiments in the 100 keV energy range. A combination of analytical estimates and state-of-the-art particle tracking simulations show that it is possible to create 100 keV, 0.1 pC, 30 fs electron bunches with a spot size smaller than 500 μm and a transverse coherence length of 3 nm, using established technologies in a table-top setup. The system operates in the space-charge dominated regime to produce energy-correlated bunches that are recompressed by radio-frequency techniques. With this approach we overcome the Coulomb expansion of the bunch, providing a single-shot, ultrafast electron diffraction source concept. [ABSTRACT FROM AUTHOR]

We report the design of a laser wakefield accelerator (LWA) with external injection by a rf photogun and acceleration by a linear wakefield in a capillary discharge channel. The design process is complex due to the large number of intricately coupled free parameters. To alleviate this problem, we performed front-to-end simulations of the complete system. The tool we used was the general particle-tracking code, extended with a module representing the linear wakefield by a two-dimensional traveling wave with appropriate wavelength and amplitude. Given the limitations of existing technology for the longest discharge plasma wavelength (∼50 μm) and shortest electron bunch length (∼100 μm), we studied the regime in which the wakefield acts as slicer and buncher, while rejecting a large fraction of the injected bunch. The optimized parameters for the injected bunch are 10 pC, 300 fs at 6.7 MeV, to be injected into a 70 mm long channel at a plasma density of 7×1023 m-3. A linear wakefield is generated by a 2 TW laser focused to 30 μm. The simulations predict an accelerated output of 0.6 pC, 10 fs bunches at 90 MeV, with energy spread below 10%. The design is currently being implemented. The design process also led to an important conclusion: output specifications directly comparable to those reported recently from “laser-into-gas jet” experiments are feasible, provided the performance of the rf photogun is considerably enhanced. The paper outlines a photogun design providing such a performance level. [ABSTRACT FROM AUTHOR]

Ultrafast electron diffraction (UED) enables studies of structural dynamics at atomic length and timescales, i.e., 0.1 nm and 0.1 ps, in single-shot mode. At present UED experiments are based on femtosecond laser photoemission from solid state cathodes. These photoemission sources perform excellently, but are not sufficiently bright for single-shot studies of, for example, biomolecular samples. We propose a new type of electron source, based on near-threshold photoionization of a laser-cooled and trapped atomic gas. The electron temperature of these sources can be as low as 10 K, implying an increase in brightness by orders of magnitude. We investigate a setup consisting of an ultracold electron source and standard radio-frequency acceleration techniques by GPT tracking simulations. The simulations use realistic fields and include all pairwise Coulomb interactions. We show that in this setup 120 keV, 0.1 pC electron bunches can be produced with a longitudinal emittance sufficiently small for enabling sub-100 fs bunch lengths at 1% relative energy spread. A transverse root-mean-square normalized emittance of ϵx= 10 nm is obtained, significantly better than from photoemission sources. Correlations in transverse phase-space indicate that the transverse emittance can be improved even further, enabling single-shot studies of biomolecular samples. [ABSTRACT FROM AUTHOR]

The realization of high quality ultrashort pulsed beams requires ultrafast time-dependent electron optics. We present derivations of closed expressions both for the longitudinal and transverse focusing powers of resonant microwave TM010 cavities. The derived expressions are validated by particle tracking simulations using realistic cavity fields. For small field amplitudes, in which case the "weak lens" approximation holds, the focusing powers obtained from simulations are in good agreement with the derived expressions. Furthermore, the required phase and temperature stability for synchronization of electron bunches generated by femtosecond photoemission are discussed., (Copyright © 2012 Elsevier B.V. All rights reserved.)