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Soft-X-ray ARPES facility at the ADRESS beamline of the SLS: concepts, technical realisation and scientific applications.

Authors :
Strocov, V. N.
Wang, X.
Shi, M.
Kobayashi, M.
Krempasky, J.
Hess, C.
Schmitt, T.
Patthey, L.
Source :
Journal of Synchrotron Radiation. Jan2014, Vol. 21 Issue 1, p32-44. 13p.
Publication Year :
2014

Abstract

Soft-X-ray angle-resolved photoelectron spectroscopy (ARPES) with photon energies around 1 keV combines the momentum space resolution with increasing probing depth. The concepts and technical realisation of the new soft-X-ray ARPES endstation at the ADRESS beamline of SLS are described. The experimental geometry of the endstation is characterized by grazing X-ray incidence on the sample to increase the photoyield and vertical orientation of the measurement plane. The vacuum chambers adopt a radial layout allowing most efficient sample transfer. High accuracy of the angular resolution is ensured by alignment strategies focused on precise matching of the X-ray beam and optical axis of the analyzer. The high photon flux of up to 1013 photons s-1 (0.01% bandwidth)-1 delivered by the beamline combined with the optimized experimental geometry break through the dramatic loss of the valence band photoexcitation cross section at soft-X-ray energies. ARPES images with energy resolution up to a few tens of meV are typically acquired on the time scale of minutes. A few application examples illustrate the power of our advanced soft-X-ray ARPES instrumentation to explore the electronic structure of bulk crystals with resolution in three-dimensional momentum, access buried heterostructures and study elemental composition of the valence states using resonant excitation. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
09090495
Volume :
21
Issue :
1
Database :
Academic Search Index
Journal :
Journal of Synchrotron Radiation
Publication Type :
Academic Journal
Accession number :
108922839
Full Text :
https://doi.org/10.1107/S1600577513019085