Influence of mineral dust on changes of 7Be concentrations in air as measured by CTBTO global monitoring system.

Abstract Atmospheric Transport Modelling (ATM) results were combined with 7Be observations collected during the 2009–2015 period by the three radionuclide stations from the International Monitoring System (IMS), located in Mauritania (18.1 N, 15.9 W), Kuwait (29.3 N, 47.9 E) and Panama (9.0 N, 79.5 W), to study the influence of Saharan dust on changes in 7Be surface concentrations. It is demonstrated that for long-range transport (>3000 km), the overall impact of Sahara can be reproduced using a single point source located in the Bodélé depression (17.0 N, 18.0 E). To monitor the arrival time of dust plumes at the IMS stations, a series of 14-day forward simulations with daily releases from the Bodélé, during dusty episodes between 2009 and 2015, were generated. In total 1020 simulations with the output at the surface level (0–150 m) and 420 simulations with the output at 9 vertical layers ranging from the surface up to 10 km, were analysed. In the simulations, the analysed meteorological input data provided by the European Centre for Medium-Range Weather Forecasts (ECMWF) were used. It is demonstrated that an influx of dust at high levels (3–10 km) tends to locally increase surface 7Be concentrations in area under the influence of subsiding dust plume. It is also shown that an influx of dust at lower altitudes (up to 1 km) will have the opposite effect on surface concentrations. In case dust is present in the whole column of atmosphere, its final impact depends on the ratio between its amount in the upper layers (3–10 km) and lower layers (0–1 km). In consequence an increase up to 30% or a decrease up 20% in daily 7Be surface values may be observed during such an episode. On a monthly scale a few episodes related to an increase of 7Be values or its decrease may follow each other. It was estimated that on average the presence of dust leads to the increase of 7Be mean monthly surface values. The largest increase was noted at the station MRP43, of about 4.1 ± 1.3%; and the smallest at the stations KWP40, of about 2.0 ± 1.6% and PAP50, of about 2.0 ± 1.0%, respectively. Highlights • Time series of 7Be collected at 3 IMS stations are analysed over a 7-y period. • Atmospheric Transport Modelling helped explaining 7Be fluctuations at 3 IMS stations. • Vertical profile of 7Be is crucial in explaining the impact of Saharan dust. • Dust from high (low) altitudes increases (decreases) surface 7Be concentrations. • Long-range transport of Saharan dust can be approximated by a single source point. [ABSTRACT FROM AUTHOR]