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High-Quality All-Inorganic Perovskite CsPbBr3 Quantum Dots Emitter Prepared by a Simple Purified Method and Applications of Light-Emitting Diodes.

Authors :
Tien, Ching-Ho
Chen, Lung-Chien
Lee, Kun-Yi
Tseng, Zong-Liang
Dong, Yu-Shen
Lin, Zi-Jun
Source :
Energies (19961073). Sep2019, Vol. 12 Issue 18, p3507. 1p. 4 Diagrams, 1 Chart, 5 Graphs.
Publication Year :
2019

Abstract

High-quality perovskite CsPbBr3 quantum dots (QDs-CsPbBr3) were prepared using the ultrasonic oscillation method, which is simple and provides variable yield according to requirements. The emission spectra over a large portion of the visible spectral region (450–650 nm) of QD-CsPbX3 (X = Cl, Br, and I) have tunable compositions that can be halide exchanged using the halide anion exchange technique and quantum size-effects. A strong peak with high intensity of (200) lattice plane of purified QDs-CsPbBr3 film is obtained, confirming the formation of an orthorhombic perovskite crystal structure of the Pnma space group. The photoluminescence of QDs-CsPbBr3 was characterized using a narrow line-width emission of 20 nm, with high quantum yields of up to 99.2%, and radioactive lifetime increasing to 26 ns. Finally, through the excellent advantages of QDs-CsPbBr3 mentioned above, purified perovskite QDs-CsPbBr3 as an active layer was utilized in perovskite quantum dot light-emitting diodes structure applications. As a result, the perovskite QDs-CsPbBr3 light-emitting diodes (LEDs) exhibits a turn-on voltage of 7 V and a maximum luminance of 5.1 cd/m2. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
19961073
Volume :
12
Issue :
18
Database :
Academic Search Index
Journal :
Energies (19961073)
Publication Type :
Academic Journal
Accession number :
138941974
Full Text :
https://doi.org/10.3390/en12183507