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Homogeneously dispersed HPW/graphene for high efficient catalytic oxidative desulfurization prepared by electrochemical deposition.
- Source :
-
Applied Surface Science . Aug2019, Vol. 484, p917-924. 8p. - Publication Year :
- 2019
-
Abstract
- In this work, reduced graphene oxide (rGO) with homogeneously dispersed phosphotungstate acid (HPW), were directly fabricated by using electrochemical strategy. In this one-pot route, the reduction of graphene oxide (GO) and HPW anchoring on rGO (HPW/rGO) have been achieved simultaneously. This strategy has not toxic reductants used, and meanwhile, produces high-quality rGO with sheet structure. Sheeted rGO could provide more anchor sites for HPW and prohibited HPW agglomeration. The produced HPW/rGO hybrid material performed high activity and durability in oxidative desulfurization (ODS) reaction due to the synergism of HPW and rGO. This work provides a novel sight for preparing high-efficient and stable catalyst for oxidative desulfurization. Unlabelled Image • Reducing graphene oxide and anchoring homogeneously dispersed phosphotungstate acid are achieved simultaneously. • Reduced graphene with paper sheet structure prevent phosphotungstate acid from aggregation. • The enhanced catalytic performance is attributed to good dispersion • This material exhibits good stability. [ABSTRACT FROM AUTHOR]
- Subjects :
- *DESULFURIZATION
*GRAPHENE oxide
*ELECTROLYTIC reduction
*REDUCING agents
*GRAPHENE
Subjects
Details
- Language :
- English
- ISSN :
- 01694332
- Volume :
- 484
- Database :
- Academic Search Index
- Journal :
- Applied Surface Science
- Publication Type :
- Academic Journal
- Accession number :
- 139234654
- Full Text :
- https://doi.org/10.1016/j.apsusc.2019.04.156