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Liquid metal and Mxene enable self-healing soft electronics based on double networks of bacterial cellulose hydrogels.
- Source :
-
Carbohydrate Polymers . Feb2023 Part A, Vol. 301, pN.PAG-N.PAG. 1p. - Publication Year :
- 2023
-
Abstract
- Liquid metal (LM) nanodroplets and MXene nanosheets are integrated with sulfonated bacterial nanocellulose (BNC) and acrylic acid (AA). Upon fast sonication, AA polymerization leads to a crosslinked composite hydrogel in which BNC exfoliates Mxene, forming organized conductive pathways. Soft conducting properties are achieved in the presence of colloidally stable core-shell LM nanodroplets. Due to the unique gelation mechanism and the effect of Mxene, the hydrogels spontaneously undergo surface wrinkling, which improves their electrical sensitivity (GF = 8.09). The hydrogels are further shown to display interfacial adhesion to a variety of surfaces, ultra-elasticity (tailorable elongation, from 1000 % to 3200 %), indentation resistance and self-healing capabilities. Such properties are demonstrated in wearable, force mapping, multi-sensing and patternable electroluminescence devices. [Display omitted] • Nanocellulose-supported LM/MXene composite hydrogels are formed by one-step sonication. • The polymer matrix effectively disperses core-shell LM nanodroplets and MXene nanosheets. • The hydrogels display ultra-elasticity, indentation resistance and self-healing properties. • The composite hydrogel is demonstrated for sensing, force mapping and electroluminescence. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 01448617
- Volume :
- 301
- Database :
- Academic Search Index
- Journal :
- Carbohydrate Polymers
- Publication Type :
- Academic Journal
- Accession number :
- 160397402
- Full Text :
- https://doi.org/10.1016/j.carbpol.2022.120330